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121.
We have re-examined the prospects of HOCl as an inert reservoir for atmospheric chlorine in the light of new theoretical calculations and available experimental measurements of its photodissociation cross-sections. The theoretical calculations and most recent laboratory studies imply that the broad maxima 3200 Å observed in two other experimental spectra may not belong to HOCl. On the basis of this implication HOCl could have a long lifetime against photodissociation in the stratosphere, and could, thereby, become a reservoir for atmospheric chlorine comparable to ClONO2 or even HCl. In this capacity HOCl could reduce the predicted ozone destruction due to any given level of total chlorine burden. We have also examined the difficulties in laboratory measurements of the HOCl absorption spectrum with particular emphasis on identifying the impurities which may be present in the experimental system. It appears that specialized new experiments are needed to clearly establish the nature and strength of HOCl absorption in the neighbourhood of 3200 Å. Some refinements in the theoretical calculations also seem desirable. In view of the difficulties involved in the laboratory determination of HOCl photodissociation cross-sections, it is suggested that a search for possible stratospheric HOCl by atmospheric spectroscopists would be worthwhile. 相似文献
122.
The dissociation of N2 by electron impact and by e.u.v. photo-absorption is studied, and it is shown that the forbidden predissociation of the numerous 1Πu and 1Σu+ valence and Rydberg states of N2 in the 11–24eV energy range is the dominant mechanism for N atom production. By measuring the absolute emission cross sections for the e.u.v. singlet bands of N2 and by using the generalized oscillator strength data of Lassettre (1974), it has been possible to construct a detailed model of the total N2 dissociation cross section which is in good agreement with the measurements of Winters (1966) and Niehaus (1967) and provides some insights into the maximum possible yield from dissociative excitation. The total cross section for exciting N2 e.u.v. radiation in the 800Å–1100Å wavelength range has been measured and found to have a value of 3.4 ×10?17 cm2 at 100 eV under optically thin conditions. Although this result implies that large fluxes of e.u.v. photons should be excited in auroral substorms and in the airglow, they are not observed, and we show that this development is a consequence of radiation entrapment and predissociation. The total cross section for dissociating N2 by electron impact is given for optically thin and thick media. And some questions concerning the energy budget of a magnetospheric storm which are raised by these results, are discussed. 相似文献
123.
124.
We have analysed the variations of inclination in 13 satellite orbits as they pass slowly, under the action of air drag, through 15th-order resonance with the geopotential, when successive equatorial crossings are 24° apart and the ground track repeats after 15 rev. The size and form of the change in inclination are determined mainly by the values of the geopotential harmonics of 15th order and odd degree, and (with l = 15, 17, 19, …) in the usual notation. Our analysis gives values of these coefficients up to l = 33 as follows:
l | 109C?l,15 | 109S?l,15 |
15 | ?23.5 ± 0.8 | ?7.7 ± 0.8 |
17 | 6.3 ± 1.5 | 5.6 ± 1.5 |
19 | ?25.1 ± 2.5 | ?7.3 ± 2.3 |
21 | 27.8 ± 3.6 | ?0.7 ± 3.4 |
23 | 17.1 ± 4.1 | 13.9 ± 4.8 |
25 | ?1.1 ± 3.0 | 8.5 ± 4.2 |
27 | 10.0 ± 3.3 | 6.7 ± 2.7 |
29 | ?9.4 ± 3.5 | 0.1 ± 4.7 |
31 | 10.1 ± 5.4 | 3.8 ± 5.6 |
33 | 1.1 ± 5.7 | 3.1 ± 5.8 |