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21.
A crystal-chemical classification of borate structures with emphasis on hydrated borates 总被引:1,自引:0,他引:1
The rules governing formation of hydrated borate polyanions that were proposed by C.L. Christ in 1960 are critically reviewed and new rules added on the basis of recent crystal structure determinations. Principles and classifications previously published by others are also critically reviewed briefly. The fundamental building blocks from which borate polyanions can be constructed are defined on the basis of the number n of boron atoms, and the fully hydrated polyanions are illustrated. Known structures are grouped accordingly, and a shorthand notation using n and symbols Δ = triangle, T = tetrahedron is introduced so that the polyanions can be easily characterized. For example, 3:Δ+2T describes [B3O3(OH)5]2?. Correct structural formulas are assigned borates with known structures whereas borates of unknown structure are grouped separately. 相似文献
22.
The total solar eclipse of February 26, 1979 was monitored at far infrared wavelengths from the NASA Lear Jet Observatory flying at 12.9 km in the eclipse shadow. The resultant eclipse curve for radiation within a bandwidth of 20 cm–1 centered upon 25 cm–1 (400 m) was measured and analysed at an equivalent angular resolution of 1 arc sec over a 100 arc sec region adjacent to the limb to provide information on the intensity distribution of continuum radiation close to this limb. The curve has been compared to predictions derived from models of the solar atmosphere for the specific geometry of this eclipse, and is shown to match most closely that derived from a uniform distribution of radiation across the disk. This is in distinct contrast to the result obtained in the only other comparable experiment, carried out over Africa in 1973 from a supersonic Concorde aircraft, in which an intense but narrow spike of far infrared radiation at the extreme solar limb was inferred from the data. The absence also in the present observations of the significant limb brightening predicted by the HSRA model (in which homogeneity within the source region is assumed) is in substantial agreement with lower resolution results from mountain altitudes. This result is interpreted as further evidence for the presence in the Sun's lower chromosphere of significant inhomogeneity with a scale size of at least 1000 km at this depth. 相似文献
23.
Clark M. Johnson Peter W. Lipman Gerald K. Czamanske 《Contributions to Mineralogy and Petrology》1990,104(1):99-124
Over 200 H, O, Sr, Nd, and Pb isotope analyses, in addition to geologic and petrologic constraints, document the magmatic evolution of the 28.5–19 Ma Latir volcanic field and associated intrusive rocks, which includes multiple stages of crustal assimilation, magma mixing, protracted crystallization, and open- and closed-system evolution in the upper crust. In contrast to data from younger volcanic centers in northern New Mexico, relatively low and restricted primary 18O values (+6.4 to +7.4) rule out assimilation of supracrustal rocks enriched in 18O. Initial 87Sr/86Sr ratios (0.705 to 0.708), 18O values (-2 to-7), and 206Pb/204Pb ratios (17.5 to 18.4) of metaluminous precaldera volcanic rocks and postcaldera plutonic rocks suggest that most Latir rocks were generated by fractional crystallization of substantial volumes of mantle-derived basaltic magma that had near-chondritic Nd isotope ratios, accompanied by assimilation of crustal material in two main stages: 1) assimilation of non-radiogenic lower crust, followed by 2) assimilation of middle and upper crust by inter-mediate-composition magmas that had been contaminated during the first stage. Magmatic evolution in the upper crust peaked with eruption of the peralkaline Amalia Tuff (26 Ma), which evolved from metaluminous parental magmas. A third stage of late, roofward assimilation of Proterozoic rocks in the Amalia Tuff magma is indicated by trends in initial 87Sr/86Sr and 206Pb/204Pb ratios from 0.7057 to 0.7098 and 19.5 to 18.8, respectively, toward the top of the pre-eruptive magma chamber. Highly evolved postcaldera plutons are generally fine grained and are zoned in initial 87Sr/86Sr and 206Pb/204Pb ratios, varying from 0.705 to 0.709 and 17.8 to 18.6, respectively. In contrast, the coarser-grained Cabresto Lake (25 Ma) and Rio Hondo (21 Ma) plutons have relatively homogeneous initial 87Sr/86Sr and 206Pb/204Pb ratios of approximately 0.7053 and 17.94 and 17.55, respectively. 18O values for all the postcaldera plutons overlap those of the precaldera rocks and Amalia Tuff, except for those for two late-stage rhyolite dikes associated with the Rio Hondo pluton that have 18O values of-8.6 and-9.5; these dikes are the only Latir rocks which may be largely crustal melts.Chemical and isotopic data from the Latir field suggest that large fluxes of mantle-derived basaltic magma are necessary for developing and sustaining large-volume volcanic centers. Development of a detailed model suggests that 6–15 km of new crust may have been added beneath the volcanic center; such an addition may result in significant changes in the chemical and Sr and Nd isotopic compositions of the crust, although Pb isotope ratios will remain relatively unchanged. If accompanied by assimilation, crystallization of pooled basaltic magma near the MOHO may produce substantial cumulates beneath the MOHO that generate large changes in the isotopic composition of the upper mantle. The Latir field may be similar to other large-volume, long-lived intracratonal volcanic fields that fundamentally owe their origins to extensive injection of basaltic magma into the lower parts of their magmatic systems. Such fields may overlie areas of significant crustal growth and hybridization. 相似文献
24.
Benton C. Clark 《Icarus》1978,34(3):645-665
Converging lines of evidence suggest that a significant portion of the Martian surface fines may consist of salts and smectite clays. Salts can form stoichiometric hydrates as well as eutectic solutions with depressed freezing points; clays contain bound water of constitution and adsorb significant quantities of water from the vapor phase. The formation of ice may be suppressed by these minerals in some regions on Mars, and their presence in abundance would imply important consequences for atmospheric and geologic processes and the prospects for exobiology. 相似文献
25.
The flow law determined experimentally for solid CO2 establishes that a hypothesis of glacial flow of CO2 at the Martian poles is not physically unrealistic. Compression experiments carried out under 1 atm pressure and constant strain rate demonstrate that the strength of CO2 near its sublimation point is considerably less than the strength of water ice near its melting point. The data fit a power law “creep” equation of the form , where ? is compressive strain rate (sec?1), σ is compressive stress (bars), R is the gas constant in calories per mole, and T is absolute temperature. The exponent of σ of 3.9 contrasts with a value near 3.1 for water ice, and indicates that the strain rate is somewhat more sensitive to stress for CO2 than for water. Likewise, the low activation energy for creep, 12 200 cal mole?1, illustrates that CO2 is not highly sensitive to temperature and is thus likely to flow over a broad range of temperatures below its melting point. Strength values for CO2 are of the order of one-tenth to one-third the strength of ice under equivalent conditions.A plausible glacial model for the Martian polar caps can be constructed and is helpful in explaining the unique character of the polar regions. CO2-rich layers deposited near the pole would have flowed outward laterally to relieve high internal shear stresses. The topography of the polar caps, the uniform layering of the layered deposits, and the general extent of the polar “sediments” could all be explained using this model. Flow of CO2 rather than water ice greatly reduces the problems with Martian glaciation. Nevertheless, problems do remain, in particular the large amounts of CO2 necessary, the need to increase vapor pressure and temperature with depth in the polar deposits, and the lack of good observational evidence of flor features. Within the limits of the present knowledge of surface conditions of Mars, CO2 glaciation appears to be a realistic alternate working hypothesis for the origin of the polar features. 相似文献
26.
The surface compositions of 110 asteroids are analyzed from statistically representative data sets of polarimetry as a function of phase angle, broad-band radiometry near 10 and 20 μm, and visible and near-infrared spectrophotometry. A comparison of albedos and diameters determined by polarimetry and radiometry shows that a modest upward revision of the radiometric albedo scale is needed and that a single law relating the slope of the polarization-phase curve to geometric albedo may not hold for very dark asteroids. We present reliable adopted albedos and diameters for 56 objects. Roughdi ameters for 52 additional objects are obtained from spectrophotometry using a correlation between albedo and color. Corrections for sampling bias permit investigation of asteroid compositions as a function of diameter, orbit, and other parameters.More than 90% of the minor planets fall into two broad compositional groups, defined by several optical parameters, designated by the symbols C and S. Comparisons with meteorite spectral albedo curves suggest that the two groups are compositionally similar to carbonaceous and stony-metallic meteorites, respectively. C-type asteroids predominate in the belt, especially in the outer half. An unusual distribution of compositions is found between 2.77 and 3.0 AU. Many S-type objects have diameters of 100–200 km; C-type objects are much more common at both larger and smaller sizes. Vesta is unique, being apparently the only differentiated asteroid remaining intact in the belt. The largest C-type objects are compositionally distinct from smaller ones and possibly are metamorphosed. We sketch some implications for meteoritics and for the early history of the solar system and point to the need for further systematic sampling of smaller and fainter objects by these three observational techniques. 相似文献
27.
The July 12, 1973, occultation of Europa by Io was observed in 30 wavelength channels in the spectral region λλ3200-11, 000 Å with the 200-inch Hale telescope and a multichannel spectrometer. The data are presented in absolute units above the Earth's atmosphere. The data are analyzed to obtain the spectral reflectivity of seven localized areas on the disk of Europa centered on 324°W longitude. The equatorial material is confirmed to be darker than the eastward-skewed bright north polar cap and a hint is evident that the darker material as well may be somewhat redder than the cap material. 相似文献
28.
Susanne Skora Lukas P. Baumgartner Nancy J. Mahlen Clark M. Johnson Sébastien Pilet Eric Hellebrand 《Contributions to Mineralogy and Petrology》2006,152(6):703-720
Garnets from the Zermatt-Saas Fee eclogites contain narrow central peaks for Lu + Yb + Tm ± Er and at least one additional small peak towards the rim. The REE Sm + Eu + Gd + Tb ± Dy are depleted in the cores but show one prominent peak close to the rim. These patterns cannot be modeled using Rayleigh fractionation accompanied by mineral breakdown reactions. Instead, the patterns are well explained using a transient matrix diffusion model where REE uptake is limited by diffusion in the matrix surrounding the porphyroblast. Observed profiles are well matched if a roughly linear radius growth rate is used. The secondary peaks in the garnet profiles are interpreted to reflect thermally activated diffusion due to temperature increase during prograde metamorphism. The model predicts anomalously low 176Lu/177Hf and 147Sm/144Nd ratios in garnets where growth rates are fast compared to diffusion of the REE, and these results have important implications for Lu–Hf and Sm–Nd geochronology using garnet. 相似文献
29.
Seismic Hazards Assessment for Radioactive Waste Disposal Sites in Regions of Low Seismic Activity 总被引:4,自引:0,他引:4
Clark H. Fenton John Adams Stephen Halchuk 《Geotechnical and Geological Engineering》2006,24(3):579-592
A comparative tectonic quiescence and lack of earthquakes make the stable centres of continents attractive for siting long-term
radioactive waste storage facilities. The low rates of deformation in such regions, however, make it difficult to characterize
their long-term seismotectonic behaviour, leading to uncertain estimates for the very low probability hazard estimates required
by society. In an attempt to overcome the deficiency of both contemporary seismicity and paleoseismic data in central Canada,
we have used earthquake histories from regions with similar seismotectonic characteristics from around the world. Substituting
space for time, we estimate a long-term rate per 106 km2 of 0.004 magnitude ≥6 earthquakes per annum, of which 33–100% might rupture to the surface. 相似文献
30.