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1.
The Solubility of Sulphur in Hydrous Rhyolitic Melts 总被引:1,自引:1,他引:1
Experiments performed at 2 kbar, in the temperature range 8001000°C,with fO2 between NNO2·3 and NNO+2·9 (whereNNO is the nickelnickel oxide buffer), and varying amountsof sulphur added to hydrous metaluminous rhyolite bulk compositions,were used to constrain the solubility of sulphur in rhyolitemelts. The results show that fS2 exerts a dominant control onthe sulphur solubility in hydrous silicate melts and that, dependingon fO2, a rhyolitic melt can reach sulphur contents close to1000 ppm at high fS2. At fO2 below NNO+1, the addition of ironto a sulphur-bearing rhyolite magma produces massive crystallizationof pyrrhotite and does not enhance the sulphur solubility ofthe melt. For a given fO2, the melt-sulphur-content increaseswith fS2. For fixed fO2 and fS2, temperature exerts a positivecontrol on sulphur solubilities, at least for fO2 below NNO+1.The mole fraction of dissolved sulphur exhibits essentiallylinear dependence on fH2S at low fO2 and, although the experimentalevidence is less clear, on fSO2 at high fO2. The minimum insulphur solubility corresponds to the redox range where bothfH2S and fSO2 are approximately equal. A thermodynamic modelof sulphur solubility in hydrous rhyolite melts is derived assumingthat total dissolved sulphur results from the additive effectsof H2S and SO2 dissolution reactions. The model reproduces wellthe minimum of sulphur solubility at around NNO+1, in additionto the variation of the sulphide to sulphate ratio with fO2.A simple empirical model of sulphur solubility in rhyoliticmelts is derived, and shows good correspondence between modeland observations for high-silica rhyolites. KEY WORDS: sulphur; solubility; rhyolite; thermodynamics; fO2; fS2 相似文献
2.
Phase Equilibria of the Lyngdal Granodiorite (Norway): Implications for the Origin of Metaluminous Ferroan Granitoids 总被引:2,自引:0,他引:2
BOGAERTS MICHEL; SCAILLET BRUNO; AUWERA JACQUELINE VANDER 《Journal of Petrology》2006,47(12):2405-2431
The Proterozoic (950 Ma) Lyngdal granodiorite of southern Norwaybelongs to a series of hornblendebiotite metaluminousferroan granitoids (HBG suite) coeval with the post-collisionalRogaland AnorthositeMangeriteCharnockite (AMC)suite. This granitoid massif shares many geochemical characteristicswith rapakivi granitoids, yet granodiorites dominate over granites.To constrain both crystallization (P, T, fO2, H2O in melt) andmagma generation conditions, we performed crystallization experimentson two samples of the Lyngdal granodiorite (with 60 and 65 wt% SiO2) at 42 kbar, mainly at fO2 of NNO (nickelnickeloxide) to NNO + 1, and under fluid-saturated conditions withvarious H2OCO2 ratios for each temperature. Comparisonbetween experimental phase equilibria and the mineral assemblagein the Lyngdal granodiorite indicates that it crystallized between4 and 2 kbar, from a magma with 56 wt % H2O at an fO2of NNO to NNO + 1. These oxidized and wet conditions sharplycontrast with the dry and reduced conditions inferred for thepetrogenesis of the AMC suite and many other rapakivi granitesworldwide. The high liquidus temperature and H2O content ofthe Lyngdal granodiorite imply that it is not a primary magmaproduced by the partial melting of the crust but is derivedby the fractionation of a mafic magma. Lyngdal-type magmas appearto have volcanic equivalents in the geological record. In particular,our results show that oxidized high-silica rhyolites, such asthe Bishop Tuff, could be derived via fractionation of oxidizedintermediate magmas and do not necessarily represent primarycrustal melts. This study underlines the great variability ofcrystallization conditions (from anhydrous to hydrous and reducedto oxidized) and petrogenetic processes among the metaluminousferroan magmas of intermediate compositions (granodiorites,quartz mangerites, quartz latites), suggesting that there isnot a single model to explain these rocks. KEY WORDS: ferroan granitoids; crystallization conditions; experiments; Norway; Sveconorwegian; Bishop Tuff 相似文献
3.
VALENTIN BURKI LOUISE HANSEN OLA FREDIN THORBJØRN A. ANDERSEN ACHIM A. BEYLICH MICHEL JABOYEDOFF EILIV LARSEN JAN‐FREDERIK TØNNESEN 《Boreas: An International Journal of Quaternary Research》2010,39(3):551-566
Burki, V., Hansen, L., Fredin, O., Andersen, T. A., Beylich, A. A., Jaboyedoff, M., Larsen, E. & Tønnesen, J.‐ F. 2009: Little Ice Age advance and retreat sediment budgets for an outlet glacier in western Norway. Boreas, Vol. 39, pp. 551–566. 10.1111/j.1502‐3885.2009.00133.x. ISSN 0300‐9483 Bødalsbreen is an outlet glacier of the Jostedalsbreen Ice Field in western Norway. Nine moraine ridges formed during and after the maximum extent of the Little Ice Age (LIA). The stratigraphy of proglacial sediments in the Bødalen basin inside the LIA moraines is examined, and corresponding sediment volumes are calculated based on georadar surveys and seismic profiling. The total erosion rates (etot) by the glacier are determined for the periods AD 1650–1930 and AD 1930–2005 as 0.8 ± 0.4 mm/yr and 0.7 ± 0.3 mm/yr, respectively. These rates are based on the total amount of sediment delivered to the glacier margin. The values are almost one order of magnitude higher than total erosion rates previously calculated for Norwegian glaciers. This is explained by the large amount of pre‐existing sediment that was recycled by Bødalsbreen. Thus, the total erosion rate must be considered as a composite of eroded bedrock and of removed pre‐existing sediments. The total erosion rate is likely to vary with time owing to a decreasing volume of easily erodible, unconsolidated sediment and till under the glacier. A slight increase in the subglacial bedrock erosion is expected owing to the gradually increasing bedrock surface area exposed to subglacial erosion. 相似文献
4.
MICHEL LAMBOY 《Sedimentology》1993,40(1):53-62
Fabrics of phosphatized calcium carbonate particles in various phosphorites have been studied using scanning electron microscopy coupled with X-ray dispersive microanalysis. Replacement of calcium carbonate by apatite has been observed in bivalve shell fragments and in foraminiferal tests; replacement proceeds at constant volume with excellent preservation of the original microtextures. In some deposits, replacement of carbonate by apatite is the main phosphogenic process. However, in general, the process seems to be far less important than might be believed purely on the basis of thin section observations. In many phosphorites, internal or external apatite moulds of bioclasts are common, including very small particles such as coccoliths in phosphatized chalks. Apatite precipitation was typically followed by carbonate dissolution. Later apatite precipitation within the dissolution voids may produce partial or total phosphate pseudomorphs of the original carbonate grain. In these examples direct replacement of carbonate by phosphate cannot be demonstrated. 相似文献
5.
A. BISCHOFF D. WEBER R. N. CLAYTON T. FAESTERMANN I. A. FRANCHI U. HERPERS K. KNIE G. KORSCHINEK P. W. KUBIK T. K. MAYEDA S. MERCHEL R. MICHEL S. NEUMANN H. PALME C. T. PILLINGER L. SCHULTZ A. S. SEXTON B. SPETTEL A. B. VERCHOVSKY H. W. WEBER G. WECKWERTH D. WOLF 《Meteoritics & planetary science》1998,33(6):1243-1257
Abstract— Lunar meteorite Dar al Gani 262 (DG 262)—found in the Libyan part of the Sahara—is a mature, anorthositic regolith breccia with highland affinities. The origin from the Moon is undoubtedly indicated by its bulk chemical composition; radionuclide concentrations; noble gas, N, and O isotopic compositions; and petrographic features. Dar al Gani 262 is a typical anorthositic highland breccia similar in mineralogy and chemical composition to Queen Alexandra Range (QUE) 93069. About 52 vol% of the studied thin sections of Dar al Gani 262 consist of fine-grained(100 μm) constituents, and 48 vol% is mineral and lithic clasts and impact-melt veins. The most abundant clast types are feldspathic fine-grained to microporphyritic crystalline melt breccias (50.2 vol%; includes recrystallized melt breccias), whereas mafic crystalline melt breccias are extremely rare (1.4 vol%). Granulitic lithologies are 12.8 vol%, intragranularly recrystallized anorthosites and cataclastic anorthosites are 8.8 and 8.2 vol%, respectively, and (devitrified) glasses are 2.7 vol%. Impact-melt veins (5.5 vol% of the whole thin sections) cutting across the entire thin section were probably formed subsequent to the lithification process of the bulk rock at pressures below 20 GPa, because the bulk rock never experienced a higher peak shock pressure. Mafic crystalline melt breccias are very rare in Dar al Gani 262 and are similar in abundance to those in QUE 93069. The extremely low abundance of mafic components and the bulk composition may constrain possible areas of the Moon from which the breccia was derived. The source area of Dar al Gani 262 must be a highland terrain lacking significant mafic impact melts or mare components. On the basis of radionuclide activities, an irradiation position of DG 262 on the Moon at a depth of 55–85 g/cm3and a maximum transit time to Earth <0.15 Ma is suggested. Dar al Gani 262 contains high concentrations of solar-wind-implanted noble gases. The isotopic abundance ratio 40Ar/36Ar < 3 is characteristic of lunar soils. The terrestrial weathering of DG 262 is reflected by the occurrence of fractures filled with calcite and by high concentrations of Ca, Ba, Cs, Br, and As. There is also a large amount of terrestrial C and some N in the sample, which was released at low temperatures during stepped heating. High concentrations of Ni, Co, and Ir indicate a significant meteoritic component in the lunar surface regolith from which DG 262 was derived. 相似文献
6.
Abstract Flood forecasting is of prime importance when it comes to reducing the possible number of lives lost to storm-induced floods. Because rainfall-runoff models are far from being perfect, hydrologists need to continuously update outputs from the rainfall-runoff model they use, in order to adapt to the actual emergency situation. This paper introduces a new updating procedure that can be combined with conceptual rainfall-runoff models for flood forecasting purposes. Conceptual models are highly nonlinear and cannot easily accommodate theoretically optimal methods such as Kalman filtering. Most methods developed so far mainly update the states of the system, i.e. the contents of the reservoirs involved in the rainfall-runoff model. The new parameter updating method proves to be superior to a standard error correction method on four watersheds whose floods can cause damage to the greater Paris area. Moreover, further developments of the approach are possible, especially along the idea of combining parameter updating with assimilation of additional data such as soil moisture data from field measurements and/or from remote sensing. 相似文献
7.
Since the first studies on the glacial formations of the Jura mountains there have been two concepts concerning type of glaciation and ice origin during the Würmian glaciation. Some authors believed that the Jura was totally inundated by ice of Alpine origin, while others believed that the Jura had its own glaciers, originating from a single ice-cap. Several recent studies on both the NW and SE slopes of the range define the problem more accurately. This paper presents a synthesis of the new results from mapping the moraine systems and studying the stratigraphic relationships between Alpine and Jura tills. It is concluded that even the highest level of Alpine glaciers could not lead to a penetration of the Jura. A reconstruction of the extension of the Jura glaciers and their relationship with the Alpine glaciers is given, and we conclude that at the Würmian maximum a local ice-cap was present. 相似文献
8.
TH. STELZNER K. HEIDE A. BISCHOFF D. WEBER P. SCHERER L. SCHULTZ M. HAPPEL W. SCHR
N U. NEUPERT R. MICHEL R. N. CLAYTON T. K. MAYEDA G. BONANI I. HAIDAS S. IVY-OCHS M. SUTER 《Meteoritics & planetary science》1999,34(5):787-794
Abstract— Weathering effects on meteorite finds from the Acfer region were studied by various analytical techniques and in dependence on the depth of sampling. In thin sections of weathered meteorites, weathering effects usually decrease from the outside to the interior of the meteorite. The results of evolved gas analysis indicate that variation in weathering between surface and core is not significant in respect to the formation of Fe-oxyhydroxides. The secondary alteration effects in the noble gases are distributed unevenly throughout the specimens, as seen in the nonsystematic differences observed for the heavy noble gases. Chemical analyses show significant enrichment of Ba and Sr in the outer parts of the weathered samples due to element contamination through aqueous solution. Iron, Ni, and Co are partly flushed from the system as the metal oxidation proceeds. Oxygen isotopes show increases in δ18O and δ17O with increasing terrestrial age. For a set of H3 chondrites, the degree of weathering determined from the water content was correlated with terrestrial ages and is discussed with respect to possible weathering mechanisms. 相似文献
9.
10.
JACQUES CALLEDE JEAN LOUP GUYOT JOSYANE RONCHAIL MICHEL MOLINIER EURIDES DE OLIVEIRA 《水文科学杂志》2013,58(2):321-333
Résumé Effectuées dans le cadre du Projet Hidrologia e geoquímica na Bacia Amazönica (HiBAm), les nouvelles mesures de débit à Obidos ont amélioré la connaissance des caractéristiques hydrologiques de l'Amazone à cette station qui contrâle les plus forts débits du monde. Une nouvelle méthode de correction détermine les débits journaliers avec une précision de ±3.0%. La reconstitution des périodes manquantes, avec les observations faites à Manaus, permet de disposer d'une chronologie de près d'un siècle. Avec cet échantillon commençant en 1902, le module interannuel de l'Amazone à Obidos est de 163 000 m3 s?1, avec un coefficient d'irrégularité extrêmement faible (K3 = 1.28). L'étiage décennal (78 000 m3 s?1) est de même grandeur que la crue centenaire du Congo à Brazzaville. La crue décennale est estimée à 260 000 m3 s?1. Le Bilan hydrologique indique un déficit d'écoulement de 1193 mm, qui peut être assimilé à l'évapotranspiration réelle. En conclusion, l'Amazone est bien le fleuve le plus puissant et le plus régulier de la planète. 相似文献