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121.
Rare earth element (REE) adsorption onto sand from a well characterized aquifer, the Carrizo Sand aquifer of Texas, has been investigated in the laboratory using a batch method. The aim was to improve our understanding of REE adsorption behavior across the REE series and to develop a surface complexation model for the REEs, which can be applied to real aquifer-groundwater systems. Our batch experiments show that REE adsorption onto Carrizo sand increases with increasing atomic number across the REE series. For each REE, adsorption increases with increasing pH, such that when pH >6.0, >98% of each REE is adsorbed onto Carrizo sand for all experimental solutions, including when actual groundwaters from the Carrizo Sand aquifer are used in the experiments. Rare earth element adsorption was not sensitive to ionic strength and total initial REE concentrations in our batch experiments. It is possible that the differences in experimental ionic strength conditions (i.e., 0.002-0.01 M NaCl) chosen were insufficient to affect REE adsorption behavior. However, cation competition (e.g., Ca, Mg, and Zn) did affect REE adsorption onto Carrizo sand, especially for light rare earth elements (LREEs) at low pH. Rare earth element adsorption onto Carrizo sand can be successfully modeled using a generalized two-layer surface complexation model. Our model calculations suggest that REE complexation with strong surface sites of Carrizo sand exceeds the stability of the aqueous complexes LnOH2+, LnSO4+, and LnCO3+, but not that of Ln(CO3)2- or LnPO4o in Carrizo groundwaters. Thus, at low pH (<7.3), where major inorganic ligands did not effectively compete with surface sites for dissolved REEs, free metal ion (Ln3+) adsorption was sufficient to describe REE adsorption behavior. However, at higher pH (>7.3) where solution complexation of the dissolved REEs was strong, REEs were adsorbed not only as free metal ion (Ln3+) but also as aqueous complexes (e.g., as Ln(CO3)2- in Carrizo groundwaters). Because heavy rare earth elements (HREEs) were preferentially adsorbed onto Carrizo sand compared to LREEs, original HREE-enriched fractionation patterns in Carrizo groundwaters from the recharge area flattened along the groundwater flow path in the Carrizo Sand aquifer due to adsorption of free- and solution-complexed REEs. 相似文献
122.
云南沿边境地带生态环境3S监测、 评价与调控研究 总被引:8,自引:0,他引:8
本文利用全球新千年整体生态系统评估的理论,以云南省沿边境地带生态系统变化跨境生态安全为研究对象,探寻并揭示我国陆疆系统的跨境生态系统变化监测、评价和生态安全综合调控的基础理论与信息机理;进而研究基于“3S”云南沿边境地带的生态环境监测、评价与综合调控的方法和关键技术,包括方法和技术体系的建立、指标体系的建立、多尺度效应和尺度转换、数学模型的建立、综合调控模式和决策方案的建立等;在案例研究部分,建立了背景数据库,然后选择大、中、小尺度进行了全区生态环境现状评价,重点河道、典型路段和重点口岸的影响评价和预测预报研究,最后进行了综合调控模式和方案的探讨,并对研究结果进行了动态仿真和虚拟表达研究。 相似文献
123.
Mixing of event and pre‐event water in a shallow Entisol in sloping farmland based on isotopic and hydrometric measurements,SW China
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Water percolation and flow processes in subsurface geologic media play an important role in determining the water source for plants and the transport of contaminants or nutrients, which is essential for water resource management and the development of measures for pollution mitigation. During June 2013, the dynamics of the rainwater, soil water, subsurface flows and groundwater in a shallow Entisol on sloping farmland were monitored using a hydrometric and isotopic approach. The results showed that effective mixing of rainwater and soil water occurred in hours. The rebound phenomenon of δD profiles in soils showed that most isotope‐depleted rainwater largely bypassed the soil matrix when the water saturation in the soil was high. Preferential‐flow, which was the dominant water movement pattern in the vadose zone, occurred through the whole soil profile, and infrequent piston‐flow was mainly found at 20–40 cm in depth. The interflow in the soil layer, composed of 75.2% rainwater, was only generated when the soil profile had been saturated. Underflow in the fractured mudrock was the dominant flow type in this hillslope, and outflow was dominated by base flow (groundwater flow) with a mean contribution of 76.7%. The generation mechanism of underflow was groundwater ridging, which was superimposed upon preferential‐flow composed mainly of rainwater. The quick mixing process of rainwater and soil water and the rapid movement of the mixture through preferential channels in the study soil, which shows a typical bimodal pore size distribution, can explain the prompt release of pre‐event water in subsurface flow. Water sources of subsurface flows at peak discharge could be affected by the antecedent soil water content, rain characteristics and antecedent groundwater levels. Copyright © 2016 John Wiley & Sons, Ltd. 相似文献
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Biostratigraphic and detrital zircon age constraints on the basement of the Himalayan Foreland Basin: Implications for a Proterozoic link to the Lesser Himalaya and cratonic India
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The Himalayan Foreland Basin in the Ganga Valley is key to assessing the pre‐collision relationship between cratonic India and the Himalaya – the world's largest mountain chain. The subsurface Ganga Supergroup, representing the sedimentary basement of the Ganga Valley, has been interpreted as a northern extension of the Proterozoic Vindhyan Supergroup in cratonic India. This interpretation is contentious because the depositional age of the Ganga Supergroup is not resolved: whereas the lower Ganga Supergroup is widely regarded as Proterozoic, the upper Ganga Supergroup has been variously inferred to include Neoproterozoic, lower Palaeozoic, or Cretaceous strata. Here, we integrate biostratigraphic and detrital zircon data from drill cores to show that the entire Ganga Supergroup is likely Proterozoic and can be correlated with Proterozoic successions on the northern Indian craton and in the Lesser Himalaya. This helps redefine the first‐order stratigraphic architecture and indicates broad depositional continuity along the northern Indian margin during the Proterozoic. 相似文献
127.
Landform‐oriented flow‐routing algorithm for the dual‐structure loess terrain based on digital elevation models
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The loess landform in the Loess Plateau of China is with typical dual structure, namely, the upper smooth positive terrain and the lower cliffy negative terrain (P–N terrain for short). Obvious differences in their morphological feature, geomorphological mechanism, and hydrological process could be found in the both areas. Based on the differences, a flow‐routing algorithm that separately addresses the dual‐structure terrain would be necessary to encompass this spatial variation in their hydrological behaviour. This paper proposes a mixed flow‐routing algorithm to address aforementioned problems. First, the loess landform surface is divided into P–N terrains based on digital elevation models. Then, specific catchment area is calculated with the new algorithm to simulate the water flows in both positive and negative terrain areas. The mixed algorithm consists of the multiple flow‐routing algorithm (multiple‐flow direction) for positive areas and the D8 algorithm for negative areas, respectively. The approach is validated in two typical geomorphologic areas with low hills and dense gullies in the northern Shaanxi Loess Plateau. Four indices are used to examine the results, which show that the new algorithm is more suitable for loess terrain in simulating the spatial distribution of water accumulation, as well as in modeling the flow characteristics of the true surface by considering the morphological structures of the terrain. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献
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Tang Xinbao Zhang Qinghao Zhou Yan Ma Depeng 《Geotechnical and Geological Engineering》2021,39(8):5895-5906
Geotechnical and Geological Engineering - Soft and hard rock assemblages and anchor solids have important effects on rock mechanics properties under different inclinations and assemblages, so it is... 相似文献
130.
Variability in the vertical hyporheic water exchange affected by hydraulic conductivity and river morphology at a natural confluent meander bend
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Jinxi Song Guotao Zhang Weize Wang Qi Liu Weiwei Jiang Weiqiang Guo Bin Tang Haifeng Bai Xinyi Dou 《水文研究》2017,31(19):3407-3420
River confluences and their associated tributaries are key morphodynamic nodes that play important roles in controlling hydraulic geometry and hyporheic water exchange in fluvial networks. However, the existing knowledge regarding hyporheic water exchange associated with river confluence morphology is relatively scarce. On January 14 and 15, 2016, the general hydraulic and morphological characteristics of the confluent meander bend (CMB) between the Juehe River and the Haohe River in the southern region of Xi'an City, Shaanxi Province, China, were investigated. The patterns and magnitudes of vertical hyporheic water exchange (VHWE) were estimated based on a one‐dimensional heat steady‐state model, whereas the sediment vertical hydraulic conductivity (Kv) was calculated via in situ permeameter tests. The results demonstrated that 6 hydrodynamic zones and their extensions were observed at the CMB during the test period. These zones were likely controlled by the obtuse junction angle and low momentum flux ratio, influencing the sediment grain size distribution of the CMB. The VHWE patterns at the test site during the test period mostly showed upwelling flow dominated by regional groundwater discharging into the river. The occurrence of longitudinal downwelling and upwelling patterns along the meander bend at the CMB was likely subjected to the comprehensive influences of the local sinuosity of the meander bend and regional groundwater discharge and finally formed regional and local flow paths. Additionally, in dominated upwelling areas, the change in VHWE magnitudes was nearly consistent with that in Kv values, and higher values of both variables generally occurred in erosional zones near the thalweg paths of the CMB, which were mostly made up of sand and gravel. This was potentially caused by the erosional and depositional processes subjected to confluence morphology. Furthermore, lower Kv values observed in downwelling areas at the CMB were attributed to sediment clogging caused by local downwelling flow. The confluence morphology and sediment Kv are thus likely the driving factors that cause local variations in the VHWE of fluvial systems. 相似文献