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271.
D. Szymanowski B. S. Ellis J. F. Wotzlaw Y. Buret A. von Quadt I. Peytcheva I. N. Bindeman O. Bachmann 《Contributions to Mineralogy and Petrology》2016,171(12):106
Understanding the processes of differentiation of the Yellowstone–Snake River Plain (YSRP) rhyolites is typically impeded by the apparent lack of erupted intermediate compositions as well as the complex nature of their shallow interaction with the surrounding crust responsible for their typically low O isotopic ratios. A pair of normal-δ18O rhyolitic eruptions from the Heise eruptive centre in eastern Idaho, the Wolverine Creek Tuff and the Conant Creek Tuff, represent unique magmatic products of the Yellowstone hotspot preserving abundant vestiges of the intermediate differentiation steps leading to rhyolite generation. We address both shallow and deep processes of magma generation and storage in the two units by combining high-precision ID–TIMS U–Pb zircon geochronology, trace element, O and Hf isotopic studies of zircon, and Sr isotopic analyses of individual high-Mg# pyroxenes inherited from lower- to mid-crustal differentiation stages. The zircon geochronology confirms the derivation of both tuffs from the same rhyolitic magma reservoir erupted at 5.5941 ± 0.0097 Ma, preceded by at least 92 ± 14 ky of continuous or intermittent zircon saturation approximating the length of pre-eruptive magma accumulation in the upper crust. Some low-Mg# pyroxenes enclosing zircons predate the eruption by at least 45 ± 27 ky, illustrating the co-crystallisation of major and accessory phases in the near-liquidus rhyolitic melts of the YSRP over a significant period of time. Coeval zircon crystals are isotopically heterogeneous (two populations at εHf ~?5 and ?13), requiring the assembly of isotopically distinct melt pockets directly prior to, or during, the eruption. The primitive Mg# 60–90 pyroxenes are out of isotopic equilibrium with the host rhyolitic melt (87Sr/86Sri = 0.70889), covering a range of 87Sr/86Sri = 0.70705–0.70883 corresponding to ratios typical of the most radiogenic YSRP basalts to the least radiogenic YSRP rhyolites. Together with the low εHf in zircon, the Sr isotopic ratios illustrate limited assimilation dominated by radiogenic Archean crustal source materials incorporated into variably evolved YSRP melts as they progress towards rhyolitic compositions by assimilation–fractional crystallisation. 相似文献
272.
Molybdenum disulfide (MoS2), a layered transition-metal dichalcogenide, has been of special importance to the research community of geochemistry, materials
and environmental chemistry, and geotechnical engineering. Understanding the oxidation behavior and charge-transfer mechanisms
in MoS2 is important to gain better insight into the degradation of this mineral in the environment. In addition, understanding the
insertion of metals into molybdenite and evaluation of charge-transfer mechanism and dynamics is important to utilize these
minerals in technological applications. Furthermore, a detailed investigation of thermal oxidation behavior and metal-insertion
will provide a basis to further explore and model the mechanism of adsorption of metal ions onto geomedia. 相似文献
273.
By examining the second leading mode(EOF2)of the summer rainfall in China during 1958–2001 and associated circulations,the authors found that this prominent mode was a dipole pattern with rainfall decreasing to the north of the Yangtze River and increasing to the south.This reverse relationship of the rainfalls to the north and to the south of the Yangtze River was related with the meridional circulations within East Asia and the neighboring region,excited by SST in the South China Sea-northwestern Pacific.... 相似文献
274.
Particle composition and size distributions in and around a deep-pit swine operation,Ames, IA 总被引:1,自引:0,他引:1
Randal S. Martin Philip J. Silva Kori Moore Mark Erupe Vishal S. Doshi 《Journal of Atmospheric Chemistry》2008,59(2):135-150
The contribution of emissions from agricultural facilities is rapidly becoming a major concern for local and regional air
quality. Characterization of particle properties such as physical size distribution and chemical composition can be valuable
in understanding the processes contributing to emissions and ultimate fate of particulate matter from agricultural facilities.
A measurement campaign was conducted at an Iowa, deep-pit, three-barn swine finishing facility to characterize near-source
ambient particulate matter. Size-specific mass concentrations were determined using minivol samplers, with additional size
distribution information obtain using optical particle counters. Particulate composition was determined via ion chromatographic
analysis of the collected filters. A thermal-CO2 elemental/organic carbon analyzer measured particulate carbon. The chemical composition and size distribution of sub-micron
particles were determined via real-time aerosol mass spectrometry. Primary particulate was not found to be a major emission
from the examined facility, with filter-based impactor samples showing average near-source increases (~15–50 m) in ambient
PM10 of 5.8 ± 2.9 μg m−3 above background levels. PM2.5 also showed contribution attributable to the facility (1.7 ± 1.1 μg m−3). Optical particle counter analysis of the numerical size distributions showed bimodal distributions for both the upwind
and downwind conditions, with maximums around 2.5 μm and below the minimum quantified diameter of 0.3 μm. The distributions
showed increased numbers of coarse particles (PM10) during periods when wind transport came from the barns, but the differences were not statistically significant at the 95%
confidence level. The PM10 aerosols showed statistically increased concentrations of sulfate, nitrate, ammonium, calcium, organic carbon, and elemental
carbon when the samplers were downwind from the pig barns. Organic carbon was the major constituent of the barn-impacted particulate
matter in both sub-micron (54%) and coarse size (20%) ranges. The AMS PM1 chemical speciation showed similar species increases, with the exception of and Ca+2, the latter not quantified by the AMS. 相似文献
275.
Shuoben Bi Shengjie Bi Xuan Chen Han Ji Ying Lu 《Asia-Pacific Journal of Atmospheric Sciences》2018,54(4):611-622
Observed climate data are processed under the assumption that their time series are stationary, as in multi-step temperature and precipitation prediction, which usually leads to low prediction accuracy. If a climate system model is based on a single prediction model, the prediction results contain significant uncertainty. In order to overcome this drawback, this study uses a method that integrates ensemble prediction and a stepwise regression model based on a mean-valued generation function. In addition, it utilizes empirical mode decomposition (EMD), which is a new method of handling time series. First, a non-stationary time series is decomposed into a series of intrinsic mode functions (IMFs), which are stationary and multi-scale. Then, a different prediction model is constructed for each component of the IMF using numerical ensemble prediction combined with stepwise regression analysis. Finally, the results are fit to a linear regression model, and a short-term climate prediction system is established using the Visual Studio development platform. The model is validated using temperature data from February 1957 to 2005 from 88 weather stations in Guangxi, China. The results show that compared to single-model prediction methods, the EMD and ensemble prediction model is more effective for forecasting climate change and abrupt climate shifts when using historical data for multi-step prediction. 相似文献
276.
Aircraft turbulence data from the Autonomous Ocean Sampling Network project were analyzed and compared to the Coupled Ocean–Atmosphere
Response Experiment (COARE) bulk parametrization of turbulent fluxes in an ocean area near the coast of California characterized
by complex atmospheric flow. Turbulent fluxes measured at about 35 m above the sea surface using the eddy-correlation method
were lower than bulk estimates under unstable and stable atmospheric stratification for all but light winds. Neutral turbulent
transfer coefficients were used in this comparison because they remove the effects of mean atmospheric conditions and atmospheric
stability. Spectral analysis suggested that kilometre-scale longitudinal rolls affect significantly turbulence measurements
even near the sea surface, depending on sampling direction. Cross-wind sampling tended to capture all the available turbulent
energy. Vertical soundings showed low boundary-layer depths and high flux divergence near the sea surface in the case of sensible
heat flux but minimal flux divergence for the momentum flux. Cross-wind sampling and flux divergence were found to explain
most of the observed discrepancies between the measured and bulk flux estimates. At low wind speeds the drag coefficient determined
with eddy correlation and an inertial dissipation method after corrections were applied still showed high values compared
to bulk estimates. This discrepancy correlated with the dominance of sea swell, which was a usually observed condition under
low wind speeds. Under stable atmospheric conditions measured sensible heat fluxes, which usually have low values over the
ocean, were possibly affected by measurement errors and deviated significantly from bulk estimates. 相似文献
277.
Trace Metal Solid State Speciation in Aerosols of the Northern Levantine Basin,East Mediterranean 总被引:3,自引:0,他引:3
Mustafa Koçak Nilgun Kubilay Barak Herut Malcolm Nimmo 《Journal of Atmospheric Chemistry》2007,56(3):239-257
An established three stage sequential leach scheme was applied to a series of selected high volume aerosol samples (n = 35) collected from the Turkish Eastern Mediterranean coastline (Erdemli). Samples were selected according to their air
mass back trajectory history to reflect the contrasting mixtures of aerosol material present in the Eastern Mediterranean
marine aerosol. Two populations were adopted, those samples which were classed as “anthropogenic” and those which were “Saharan”
dominated aerosol populations. Applying the three stage leach it was possible to define the proportion for each of the considered
metals (Al, Fe, Cu, Pb, Cd, Zn and Mn) present in the (a) “exchangeable” (b) “carbonate / oxide” and (c) “refractory” phases,
representing novel solid state aerosol speciation data for this marine system. Clear trends were established, conforming with
data from previous studies with mainly crustal derived metals (Al and Fe) being present in the refractory phases (Al > 88%;
Fe > 84%) and those influenced by anthropogenic sources being dominating in the exchangeable phase, although for these metals
the variability was comparatively high (12–64%; 19–85%; 40–100% for Zn, Pb and Cd, respectively). For the majority, greater
exchangeable fractions were present the lower the crustal source contribution to the aerosol population, whereas the “refractory”
fraction exhibited contrasting behaviour. This was illustrated by the novel application of the mixing diagram, presenting
each of the three speciation stages against the corresponding percent anthropogenic contribution to each collected sample.
Zn, Pb and Cd all illustrated progressive decrease in the percent exchangeable with increasing crustal contribution to the
aerosol population. The percent exchangeable was discussed in terms of its use to represent the upper limit of the bioavailable
fraction of metal associated with the aerosol, post deposition. The mixing diagram approach enabled the prediction of the
residual fractions for Cd, Pb and Zn (41 ± 4%; 62 ± 4% and 82 ± 5%, respectively,) in Saharan end-member material. 相似文献
278.
Cultivated land change in the Belt and Road Initiative region 总被引:2,自引:1,他引:2
The Belt and Road Initiative (BRI)–a development strategy proposed by China – provides unprecedented opportunities for multi-dimensional communication and cooperation across Asia, Africa and Europe. In this study, we analyse the spatio-temporal changes in cultivated land in the BRI countries (64 in total) to better understand the land use status of China along with its periphery for targeting specific collaboration. We apply FAO statistics and GlobeLand30 (the world’s finest land cover data at a 30-m resolution), and develop three indicator groups (namely quantity, conversion, and utilization degree) for the analysis. The results show that cultivated land area in the BRI region increased 3.73×104 km2 between 2000 and 2010. The increased cultivated land was mainly found in Central and Eastern Europe and Southeast Asia, while the decreased cultivated land was mostly concentrated in China. Russia ranks first with an increase of 1.59×104 km2 cultivated land area, followed by Hungary (0.66×104 km2) and India (0.57×104 km2). China decreased 1.95×104 km2 cultivated land area, followed by Bangladesh (–0.22×104 km2) and Thailand (–0.22×104 km2). Cultivated land was mainly transferred to/from forest, grassland, artificial surfaces and bare land, and transfer types in different regions have different characteristics: while large amount of cultivated land in China was converted to artificial surfaces, considerable forest was converted to cultivated land in Southeast Asia. The increase of multi-cropping index dominated the region except the Central and Eastern Europe, while the increase of fragmentation index was prevailing in the region except for a few South Asian countries. Our results indicate that the negative consequence of cultivated land loss in China might be underestimated by the domestic- focused studies, as none of its close neighbours experienced such obvious cultivated land losses. Nevertheless, the increased cultivated land area in Southeast Asia and the extensive cultivated land use in Ukraine and Russia imply that the regional food production would be greatly improved if China’ “Go Out policy” would help those countries to intensify their cultivated land use. 相似文献
279.
Ecological compensation for desertification control: A review 总被引:1,自引:1,他引:1
Desertification control is a crucial way to enhancing the ecological conditions of arid and semi-arid regions, and maintaining sustainable development globally. Designing and improving an ecological compensation mechanism for desertification control has great significance related to achieving balance amongst the needs of different economic subjects and the assurance of a sustained and stable supply of desert ecosystem services. In this paper, (1) the theoretical bases of ecological compensation for desertification control were re-analyzed; (2) the research status and challenges of three important topics related to ecological compensation for desertification control were systemically discussed, including compensation standards, ecosystem service supply-consumption process and multi-scale effects, and resource- environment basis and policy orientation; (3) a research framework of ecological compensation for desertification control based on the process of desert ecosystem service supply–flow–consumption was proposed; (4) and finally, seven priority research issues were discussed, which aimed to support ecological compensation policy-making and ecological engineering implementation for desertification control. 相似文献
280.
Longfei Han Youpeng Xu Chaogui Lei Liu Yang Xiaojun Deng Chunsheng Hu Guanglai Xu 《地理学报(英文版)》2016,26(6):694-706
Evolution of river systems under the background of human activities has been a heated topic among geographers and hydrologists. Spatial and temporal variations of river systems during the 1960s–2010s in the Yangtze River Delta (YRD) were investigated based on streams derived from the topographic maps in the 1960s, 1980s and 2010s. A list of indices, drainage density (Dd), water surface ratio (WSR), ratio of area to length of main streams (R), evolution coefficient of tributaries (K) and box dimension (D), were classified into three types (quantitative, structural, and complex indices) and used to quantify the variations of stream structure. Results showed that: (1) quantitative indices (Dd, WSR) presented decreasing trend in the past 50 years, and Dd in Wuchengxiyu, Hangjiahu and Yindongnan have decreased most, about 20%. Structurally, the Qinhuai River basin was characterized by significant upward R, and K value in Hangjiahu went down dramatically by 46.8% during the 1960s–2010s. Decreasing tendency in D was found dominating across the YRD, and decreasing magnitude in Wuchengxiyu and Hangjiahu peaks for 7.8% and 6.5%, respectively in the YRD. (2) Urbanization affected the spatial pattern of river system, and areas with high level of urbanization exhibited least Dd (2.18 km/km2), WSR (6.52%), K (2.64) and D (1.42), compared to moderate and low levels of urbanization. (3) Urbanization also affected the evolution of stream system. In the past 50 years, areas with high level of urbanization showed compelling decreasing tendency in quantitative (27.2% and 19.3%) and complex indices (4.9%) and trend of enlarging of main rivers (4.5% and 7.9% in periods of the 1960s–1980s and the 1980s–2010s). In the recent 30 years, areas with low level of urbanization were detected with significant downward trend in Dd and K. (4) Expanding of urban land, construction of hydraulic engineering and irrigation and water conservancy activities were the main means which degraded the river system in the YRD. 相似文献