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241.
Continuous monitoring of dissolved organic matter (DOM) character and concentration at hourly resolution is rare, despite the importance of analysing organic matter variability at high‐temporal resolution to evaluate river carbon budgeting, river water health by detecting episodic pollution and to determine short‐term variations in chemical and ecological function. The authors report a 2‐week experiment performed on DOM sampled from Bournbrook, Birmingham, UK, an urban river for which spectrophotometric (fluorescence, absorbance), physiochemical (dissolved organic carbon [DOC], electrical conductivity, pH) and isotopic (D/H) parameters have been measured at hourly frequency. Our results show that the river had sub‐daily variations in both organic matter concentration and characteristics. In particular, after relatively high‐magnitude precipitation events, organic carbon concentration increased, with an associated increase in intensity of both humic‐like and tryptophan‐like fluorescence. D/H isotopic ratio demonstrates different hydrological responses to different rainfall events, and organic matter character reflects this difference. Events with precipitation < 2 mm typically yielded isotopically heavy water with relatively hydrophilic DOM and relatively low specific absorbance. Events with precipitation > 2 mm had isotopically lighter water with higher specific absorbance and a decrease in the proportion of microbially derived to humic‐like fluorescence. In our heavily urbanized catchment, we interpret these signals as one where riverine DOM is dominated by storm sewer‐derived ‘old’ organic matter at low‐rainfall amounts and a mixed signal at high‐precipitation amounts where ‘event’ surface runoff‐derived organic matter dominate during storm sewer and combined sewer overflow routed DOM. Copyright © 2009 John Wiley & Sons, Ltd. 相似文献
242.
Roger H. Mitchell Malcolm Alexander Lachlan M. D. Cranswick Ian P. Swainson 《Physics and Chemistry of Minerals》2007,34(10):705-712
The cell dimensions and crystal structures of the fluoroperovskite NaMgF3 (neighborite), synthesized by solid state methods, have been determined by powder neutron diffraction and Rietveld refinement
over the temperature range 300–3.6 K using Pt metal as an internal standard for calibration of the neutron wavelength. These
data show that Pbnm NaMgF3 does not undergo any phase transitions to structures of lower symmetry with decreasing temperature. The cell dimensions and
atomic coordinates together with polyhedron volumes and distortion indices are given for Pbnm NaMgF3 at 25 K intervals from 300 to 3.6 K. Decreases in the a and c cell dimensions reach a saturation point at 50 K, whereas the b dimension becomes saturated at 150 K. The distortion of the structure of Pbnm NaMgF3 from the aristotype cubic
structure is described in terms of the tilting of the MgF6 octahedra according to the tilt scheme a
−
a
−
c
+
. With decreasing temperature the antiphase tilt (a
−) increases from 14.24° to 15.39°, whereas the in-phase tilt (c
+
) remains effectively constant at ∼10.7°. Changes in the tilt angles are insufficient to cause changes in the coordination
sphere of Na that might induce a low temperature phase transition. The structure of Pbnm NaMgF3 is also described in terms of normal mode analysis and displacements of the condensed normal modes are compared with those
of Pbnm KCaF3. 相似文献
243.
Within the ZitácuaroValle de Bravo (ZVB) regionof the central Mexican Volcanic Belt (MVB), three lava serieshave erupted during the Quaternary: (1) high-K2O basaltic andesitesand andesites; (2) medium-K2O basaltic andesites, andesitesand dacites; (3) high-TiO2 basalts and basaltic andesites. Thedominant feature of the first two groups is the lack of plagioclaseaccompanying the various ferromagnesian phenocrysts (olivine,orthopyroxene, augite, and hornblende) in all but the dacites.This absence of plagioclase in the phenocryst assemblages ofthe high-K2O and medium-K2O intermediate lavas is significantbecause it indicates high water contents during the stage ofphenocryst equilibration. In contrast, the high-TiO2 group ischaracterized by phenocrysts of plagioclase and olivine. Thespatial distribution of these three lava series is systematic.The southern section of the ZVB transect, 280330 km fromthe Middle America Trench (MAT), is characterized by high-K2Omelts that are relatively enriched in fluid-mobile elementsand have the highest 87Sr/86Sr ratios. Medium-K2O basaltic andesiteand andesite lavas are present throughout the transect, butthose closest to the MAT are MgO-rich (3·59·4wt %) and have phenocryst assemblages indicative of high magmaticwater contents (3·56·5 wt % water) andrelatively low temperatures (9501000°C). In markedcontrast, the northern section of the ZVB transect (380480km from the MAT) has high-TiO2, high field strength element(HFSE)-enriched magmas that have comparatively dry (< 1·5wt % magmatic water) and hot (11001200°C) phenocrystequilibration conditions. The central section of the ZVB transect(330380 km from the MAT) is a transition zone and producesmoderately light rare earth element (LREE) and large ion lithophileelement (LILE)-enriched, medium-K2O lavas with phenocryst assemblagesindicative of intermediate (1·53·5 wt %)water contents and temperatures. The high-K2O series compositionsare the most enriched in LILE and LREE, with a narrow rangeof radiogenic 87Sr/86Sr from 0·704245 to 0·704507,143Nd/144Nd values ranging from 0·512857 to 0·512927(Nd = 4·275·63), and 208Pb/204Pb valuesfrom 38·248 to 38·442, 207Pb/204Pb values from15·563 to 15·585, and 206Pb/204Pb values from18·598 to 18·688. The medium-K2O series compositionsare only moderately enriched in the LILE and LREE, with a broaderrange of 87Sr/86Sr, but similar 143Nd/144Nd and 208Pb/204Pbvalues to those of the high-K2O series. In contrast, the high-TiO2series compositions have little enrichment in LILE or LREE andinstead are enriched in the HFSE and heavy rare earth elements(HREE). The high-TiO2 lavas are isotopically distinct in theirlower and narrower range of 143Nd/144Nd. The isotopic variationsare believed to reflect the upper mantle magma source regionsas the low content of phenocrysts in most lavas precludes significantupper crustal assimilation or magma mixing, other than thatrepresented by the presence of quartz xenocrysts (< 2 vol.%) with rhyolitic glass inclusions, which are found in manyof these lavas. The systematic spatial variation in compositionof the three lava series is a reflection of the underlying subduction-modifiedmantle and its evolution. KEY WORDS: central Mexico; geochemistry; isotopes; Quaternary volcanism; hydrous lavas 相似文献
244.
245.
246.
The Northwest Africa (NWA) 5790 meteorite: A mesostasis‐rich nakhlite with little or no Martian aqueous alteration 下载免费PDF全文
Tim Tomkinson Martin R. Lee Darren F. Mark Katherine J. Dobson Ian A. Franchi 《Meteoritics & planetary science》2015,50(2):287-304
Northwest Africa (NWA) 5790 is the most recently discovered member of the nakhlite group. Its mineralogy differs from the other nakhlites with a high abundance mesostasis (38.1 ± 3.6 vol%) and scarcity of olivine (4.0 ± 2.2 vol%). Furthermore, zoning of augite phenocrysts, and other petrographic and chemical characteristics suggest that NWA 5790 samples the chilled margin of its parent lava flow/sill. NWA 5790 contains calcite and rare clay minerals that are evidence for its exposure to liquid water. The calcite forms a cement to coatings of dust on the outer surface of the find and extends into the interior of the meteorite within veins. The presence of microbial remains within the coating confirms that the dust and its carbonate cement are terrestrial in origin, consistent with the carbon and oxygen isotope composition of the calcite. The clay minerals are finely crystalline and comprise ~0.003 vol% of the meteorite. δD values of the clay minerals range from ?212 ± 109‰ to ?96 ± 132‰, and cannot be used to distinguish between a terrestrial or Martian origin. As petrographic results are also not definitive, we conclude that secondary minerals produced by Martian groundwaters are at best very rare within NWA 5790. The meteorite has therefore sampled a region of the lava flow/sill with little or no exposure to the aqueous solutions that altered other nakhlites. This isolation could relate to the scarcity of olivine in NWA 5790 because dissolution of olivine in other nakhlites by Martian groundwaters enhanced their porosity and permeability, and provided solutes for secondary minerals. 相似文献
247.
A global baroclinic primitive equation model using the spectral technique has been constructed for short‐ and medium‐range numerical weather prediction. The spectral technique, which is a special case of the Galerkin method, employs spherical harmonic basis functions in the evaluation of all horizontal derivatives. The use of a transform technique allows all the horizontal operations to be performed efficiently and allows physical processes to be evaluated in real space. The model employs a semi‐implicit algorithm for time integration and finite differencing in the vertical. Physical processes include orography, moist convection, large scale precipitation and boundary layer processes. 相似文献
248.
Key limitations of integrated assessment models (IAMs) are their highly stylized and aggregated representation of climate damages and associated economic responses, as well as the omission of specific investments related to climate change adaptation. This paper proposes a framework for modeling climate impacts and adaptation that clarifies the relevant research issues and provides a template for making improvements. We identify five desirable characteristics of an ideal integrated assessment modeling platform, which we elaborate into a conceptual model that distinguishes three different classes of adaptation-related activities. Based on these elements we specify an impacts- and adaptation-centric IAM, whose optimality conditions are used to highlight the types of functional relationships necessary for realistic representations of adaptation-related decisions, the specific mechanisms by which these responses can be incorporated into IAMs, and the ways in which the inclusion of adaptation is likely to affect the simulations’ results. 相似文献
249.
Ian Shennan Sarah Hamilton Caroline Hillier Amanda Hunter Ruth Woodall Sarah Bradley Glenn Milne Anthony Brooks Sophie Bassett 《第四纪科学杂志》2006,21(6):601-613
Observations of relative sea‐level change and local deglaciation in western Scotland provide critical constraints for modelling glacio‐isostatic rebound in northern Britain over the last 18 000 years. The longest records come from Skye, Arisaig and Knapdale with a shorter, Holocene, record from Kintail. Biostratigraphic (diatom, pollen, dinoflagellate, foraminifera and thecamoebian), lithological and radiocarbon analyses provide age and elevation parameters for each sea‐level index point. All four sites reveal relative sea‐level change that is highly non‐monotonic in time as the local vertical component of glacio‐isostatic rebound and eustasy (or global meltwater influx) dominate at different periods. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
250.
S. C. Chapman Ian Smail R. J. Ivison A. W. Blain 《Monthly notices of the Royal Astronomical Society》2002,335(1):L17-L21
Spectroscopic surveys of submillimetre(submm)-selected sources have uncovered optically bright galaxies at z ≲ 1 close to the positions of several submm sources. Naive statistical analyses suggest that these galaxies are associated with the submm emission. However, in some cases, it is difficult to understand this association given the relatively modest redshifts and unprepossessing spectral characteristics of the galaxies. These are in stark contrast to those expected from the massive dust-enshrouded starbursts and AGN thought to power the bulk of the bright submm population. We present new observations of optically bright counterparts to two luminous submm sources, along with a compilation of previously proposed optically bright counterparts with z ≲ 1 . We suggest that the majority of these associations between bright galaxies and submm sources may be as a result of the action of the foreground galaxies as gravitational lenses on the much fainter and more distant submm sources. We discuss the implications of this conclusion for our understanding of the SCUBA population. 相似文献