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31.
32.
Sunil Bharati Richard L. Patience Steve R. Larter Guy Standen Iain J. F. Poplett 《Organic Geochemistry》1995,23(11-12)
The significance and validity of integrating data obtained from a variety of analytical techniques to understand, elucidate and model kerogen's complex chemical structure is reported here using degradative (open and closed system pyrolysis, chemical oxidation), non-degradative (13C CP/MAS NMR) and optical (incident white light and blue light) methods. Seven Cambrian Alum Shale samples, ranging in maturity from immature to post-mature with respect to petroleum generation, were studied and were chosen for their simple geological history, uniform organic matter type and high organic carbon content. The Alum Shale kerogens, which primarily consist of algal organic matter, liberate low molecular weight gaseous and aromatic compounds on pyrolysis and give mostly branched dicarboxylic acids on chemical oxidation. 13C NMR spectroscopy shows that the Alum Shale kerogens are anomalously rich in oxygen-bearing functional groups (such as C = O, ArCO, CHO, CHxO), most of which apparently remain intact within the kerogen macro-molecule (KMM) through the diagenetic and catagenetic stages. Fragments released by different degradative techniques are quantified and the aromaticity (fa), O/C and relative proportions of various carbon types estimated by 13C NMR. A synthesis of these data has allowed us to better understand the chemistry of the Alum Shale kerogen. 相似文献
33.
Summary. Rotational remanent magnetization, RRM, is the magnetization acquired when a sample is rotated during alternating field demagnetization. Although the existence of RRM has been well documented in different laboratories, until now no physical mechanism explaining its origin has been given. We propose that the RRM originates from thermal fluctuations biased by a precessional torque associated with the alternating field. Our theory is consistent with the observation that no directional preference exists in the experimental situation until the sample is rotated relative to the alternating field. Moreover, our theory predicts that the combined sample rotation and precession will produce a RRM that switches direction when the frequency of sample rotation increases from any value below the frequency of the alternating field to any value above that frequency as observed in experiments. Although no precise theory is given for the intensity of RRM, the model presented here can qualitatively explain previous intensity observations. 相似文献
34.
The completeness and the accuracy of the Brest sea level time series dating from 1807 make it suitable for long-term sea level trend studies. New data sets were recently discovered in the form of handwritten tabulations, including several decades of the eighteenth century. Sea level observations have been made in Brest since 1679. This paper presents the historical data sets which have been assembled so far. These data sets span approximately 300 years and together constitute the longest, near-continuous set of sea level information in France. However, an important question arises: Can we relate the past and the present-day records? We partially provide an answer to this question by analysing the documents of several historical libraries with the tidal data using a ‘data archaeology’ approach advocated by Woodworth (Geophys Res Lett 26:1589–1592, 1999b). A second question arises concerning the accuracy of such records. Careful editing was undertaken by examining the residuals between tidal predictions and observations. It proved useful to remove the worst effects of timing errors, in particular the sundial correction to be applied prior to August 1, 1714. A refined correction based on sundial literature [Savoie, La gnomique, Editions Les Belles Lettres, Paris, 2001] is proposed, which eliminates the systematic offsets seen in the discrepancies in timing of the sea level measurements. The tidal analysis has also shown that shallow-water tidal harmonics at Brest causes a systematic difference of 0.023 m between mean sea level (MSL) and mean tide level (MTL). Thus, MTL should not be mixed with the time series of MSL because of this systematic offset. The study of the trends in MTL and MSL however indicates that MTL can be used as a proxy for MSL. Three linear trend periods are distinguished in the Brest MTL time series over the period 1807–2004. Our results support the recent findings of Holgate and Woodworth (Geophys Res Lett) of an enhanced coastal sea level rise during the last decade compared to the global estimations of about 1.8 mm/year over longer periods (Douglas, J Geophys Res 96:6981–6992, 1991). The onset of the relatively large global sea level trends observed in the twentieth century is an important question in the science of climate change. Our findings point out to an ‘inflexion point’ at around 1890, which is remarkably close to that in 1880 found in the Liverpool record by Woodworth (Geophys Res Lett 26:1589–1592, 1999b). 相似文献
35.
Uwe Mikolajewicz Matthias Gröger Ernst Maier-Reimer Guy Schurgers Miren Vizcaíno Arne M. E. Winguth 《Climate Dynamics》2007,28(6):599-633
A new complex earth system model consisting of an atmospheric general circulation model, an ocean general circulation model,
a three-dimensional ice sheet model, a marine biogeochemistry model, and a dynamic vegetation model was used to study the
long-term response to anthropogenic carbon emissions. The prescribed emissions follow estimates of past emissions for the
period 1751–2000 and standard IPCC emission scenarios up to the year 2100. After 2100, an exponential decrease of the emissions
was assumed. For each of the scenarios, a small ensemble of simulations was carried out. The North Atlantic overturning collapsed
in the high emission scenario (A2) simulations. In the low emission scenario (B1), only a temporary weakening of the deep
water formation in the North Atlantic is predicted. The moderate emission scenario (A1B) brings the system close to its bifurcation
point, with three out of five runs leading to a collapsed North Atlantic overturning circulation. The atmospheric moisture
transport predominantly contributes to the collapse of the deep water formation. In the simulations with collapsed deep water
formation in the North Atlantic a substantial cooling over parts of the North Atlantic is simulated. Anthropogenic climate
change substantially reduces the ability of land and ocean to sequester anthropogenic carbon. The simulated effect of a collapse
of the deep water formation in the North Atlantic on the atmospheric CO2 concentration turned out to be relatively small. The volume of the Greenland ice sheet is reduced, but its contribution to
global mean sea level is almost counterbalanced by the growth of the Antarctic ice sheet due to enhanced snowfall. The modifications
of the high latitude freshwater input due to the simulated changes in mass balance of the ice sheet are one order of magnitude
smaller than the changes due to atmospheric moisture transport. After the year 3000, the global mean surface temperature is
predicted to be almost constant due to the compensating effects of decreasing atmospheric CO2 concentrations due to oceanic uptake and delayed response to increasing atmospheric CO2 concentrations before. 相似文献
36.
Guy S. Miller & Scott A. Grossman 《Monthly notices of the Royal Astronomical Society》1998,299(1):139-149
In this paper we investigate the dynamical behaviour of radiation-driven winds, specifically winds that arise when Compton scattering transfers momentum from the radiation field to the gas flow. Such winds occur during strong X-ray bursts from slowly accreting neutron stars, and also may be driven from the inner regions of a black hole or neutron star accretion disc when the mass transfer rate is very high. By linearizing the radiation hydrodynamic equations around steady spherical outflow, we evaluate the time-dependent response of these winds to perturbations introduced at their inner boundaries. We find that although radiation-driven winds are generally stable, they act as mechanical filters that should produce quasi-periodic oscillations or peaked noise in their radiation output when perturbations force them stochastically. This behaviour may underlie the photospheric oscillations observed in some strong Type I X-ray bursts. 相似文献
37.
Jeffrey Neal Guy Schumann Paul Bates Wouter Buytaert Patrick Matgen Florian Pappenberger 《水文研究》2009,23(25):3641-3649
River discharge is currently monitored by a diminishing network of gauges, which provide a spatially incomplete picture of global discharges. This study assimilated water level information derived from a fused satellite Synthetic Aperture Radar (SAR) image and digital terrain model (DTM) with simulations from a coupled hydrological and hydrodynamic model to estimate discharge in an un‐gauged basin scenario. Assimilating water level measurements led to a 79% reduction in ensemble discharge uncertainty over the coupled hydrological hydrodynamic model alone. Measurement bias was evident, but the method still provided a means of improving estimates of discharge for high flows. The study demonstrates the potential of currently available synthetic aperture radar imagery to reduce discharge uncertainty in un‐gauged basins when combined with model simulations in a data assimilation framework, where sufficient topographic data are available. The work is timely because in the near future the launch of satellite radar missions will lead to a significant increase in the volume of data available for space‐borne discharge estimation. Copyright © 2009 John Wiley & Sons, Ltd. 相似文献
38.
This paper presents a procedure for the determination of parameters of non‐local damage models. This is to assure a consistent response of a non‐local damage model, as choice of the internal length and other parameters of the model are varied. Correlations between the internal length and other parameters governing the local constitutive behaviour of the model are addressed and exploited. Focus is put on the relationship between the internal length of the non‐local model and the width of the fracture process zone. Numerical examples are used to demonstrate the rigour of the proposed method. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
39.
Although it is traditionally thought that drainage basins are geometrically similar, we present new results which indicate that the aspect ratio of weakly dissected river basins at large scales (10–103 km2 ) depends on the surface slope: steeper surfaces develop narrower and lengthier basins whereas more gently dipping surfaces develop more equant and wider basins. This relationship is interpreted to be related to the nature of water flow over rough surfaces, with steeper slopes causing less flow convergence and lengthier and narrower basins. We derive an empirical relationship that can be used to infer the slope of a surface on which a river basin acquired its geometry based solely on a measure of its basin form. This relation provides a unique means of inferring the relative chronology of river basin development with respect to surface tilting and therefore provides a direct link between river basin morphology and tectonics. 相似文献
40.
Robert J. MACKE Guy J. CONSOLMAGNO Daniel T. BRITT 《Meteoritics & planetary science》2011,46(12):1842-1862
Abstract– We report physical properties (bulk and grain density, magnetic susceptibility, and porosity) measured using nondestructive and noncontaminating methods for 195 stones from 63 carbonaceous chondrites. Grain densities over the whole population average 3.44 g cm?3, ranging from 2.42 g cm?3 (CI1 Orgueil) to 5.66 g cm?3 (CB Bencubbin). Magnetic susceptibilities (in log units of 10?9 m3 kg?1) averaged log χ = 4.22, ranging from 3.23 (CV3 Axtell) to 5.79 (CB Bencubbin). Porosities averaged 17%, ranging from 0 (for a number of meteorites) to 41% (for one stone of the CO Ornans). Notably, we found significant differences in porosity between the oxidized and reduced CV subgroups, with the porosities of CVo averaging approximately 20% and CVr porosities approximately 4%. Overall, porosities of carbonaceous chondrite falls trend with petrographic type, from type 1 (CI) near 35%, type 2 (CM, CR) averaging 23%, type 3 (CV, CO) 21%, to type 4 (CK and some CO) averaging 15%. There is also a significant decrease in porosity between meteorites of shock stage S1 and those of S2, indicative of shock compression. 相似文献