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21.
Yarrow Axford Camilla S. Andresen John T. Andrews Simon T. Belt Áslaug Geirsdóttir Guillaume Massé Gifford H. Miller Sædís Ólafsdóttir Lindsay L. Vare 《第四纪科学杂志》2011,26(6):645-656
Geochemical, mineralogical and biological indicators preserved in sediments are widely used to reconstruct past climate change, but proxies differ in the degree to which their utility as climate indicators has been validated via laboratory experiments, modern spatial calibrations, or down‐core comparisons with instrumental climate data. Multi‐proxy studies provide another means of evaluating interpretations of proxies. This paper presents a multi‐proxy assessment comparing 19 sub‐centennially resolved late Holocene proxy records, covering the period 300–1900 AD, from seven Icelandic marine and lacustrine core sites. We employ simple statistical comparisons between proxy reconstructions to evaluate their correlations over time and, ultimately, their utility as proxies for regional climate. Proxies examined include oxygen isotopic composition of benthic and planktonic foraminifera, abundance of the sea‐ice biomarker IP25, allochthonous quartz in marine sediments (a proxy for drift ice around Iceland), marine carbonate abundance, total organic carbon concentration, chironomid assemblages, lacustrine biogenic silica and carbon/nitrogen ratios in lake sediments. Most of the examined proxy records, including temperature and sea‐ice proxies, correlate strongly with each other over multi‐centennial timescales, and thus do appear to record changes in regional climate. Copyright © 2011 John Wiley & Sons, Ltd. 相似文献
22.
Sophie Raous Thierry Becquer Jérémie Garnier Éder de Souza Martins Guillaume Echevarria Thibault Sterckeman 《Applied Geochemistry》2010
An understanding of the biogeochemical behaviour of metals in mine spoil materials is a prerequisite to rehabilitate Ni mining sites. The objective of this study was to characterize the fate of metals in different Ni ore spoil materials as influenced by hydrological conditions and fertilisation practices. In tropical ultramafic complexes, the different stages of lateritic weathering lead to two types of ores, and therefore, to two spoil types. They are mainly either a clay-rich saprolite, so-called “garnierite”, enriched in phyllosilicates, or a limonitic material, enriched in Fe oxides. Lysimeter columns were designed to monitor leaching waters through both spoil materials. The garnieritic spoil released higher concentrations of Mg (mean = 2.25 mg L−1), Ni (0.39 mg L−1) and Cr (1.19 mg L−1) than the limonitic spoil (Mg = 0.5 mg L−1; Ni = 0.03 mg L−1 and Cr = 0.25 mg L−1). Chromium was mainly in an anionic form in leaching solutions. As exchangeable pools of Cr(VI) in limonite (980 mg kg−1 of KH2PO4-extractable Cr) are considerable its release in water may still occur in the case of a pH increase. In mixed spoil, metal concentrations were almost as low as in the limonitic one. The effect of mineral-N fertilisation was a strong release of cations (Ni, Mg) into the leachate. Phosphate amendment did not affect the soil solution composition under experimental conditions. 相似文献
23.
Adnand Bitri Jean-Pierre Brun Denis Gapais Florence Cagnard Charles Gumiaux Jean Chantraine Guillaume Martelet Catherine Truffert 《Comptes Rendus Geoscience》2010,342(6):448-452
We present results and interpretation of a 72 km long deep seismic reflection profile acquired across the internal zone of the Hercynian belt of South Brittany. The profile is of excellent quality, most of the crust being highly reflective. The “ARMOR 2 South” profile, is correlated with the “ARMOR 2 North” profile that was published in 2003. Correlation of the main subsurface reflections with surface geological and structural data provides important information about the crustal structure that resulted from thickening during Late Devonian and regional-scale extension during Late Carboniferous. In particular, seismics image shows a very high reflectivity zone, lying flat over more than 40 km at about 10–12 km depth. This zone is interpreted as a major zone of ductile crustal thinning. 相似文献
24.
Towards Stochastic Time-Varying Geological Modeling 总被引:3,自引:1,他引:2
Guillaume Caumon 《Mathematical Geosciences》2010,42(5):555-569
The modeling of subsurface geometry and properties is a key element to understand Earth processes and manage natural hazards
and resources. In this paper, we suggest this field should evolve beyond pure data fitting approaches by integrating geological
concepts to constrain interpretations or test their consistency. This process necessarily calls for adding the time dimension
to 3D modeling, both at the geological and human time scales. Also, instead of striving for one single best model, it is appropriate
to generate several possible subsurface models in order to convey a quantitative sense of uncertainty. Depending on the modeling
objective (e.g., quantification of natural resources, production forecast), this population of models can be ranked. Inverse
theory then provides a framework to validate (or rather invalidate) models which are not compatible with certain types of
observations. We review recent methods to better achieve both stochastic and time-varying geomodeling and advocate that the
application of inversion should rely not only on random field models, but also on geological concepts and parameters. 相似文献
25.
The paper discusses the development of economic techniques for dealing with uncertainties in economic analysis of planting trees to mitigate climatic change. In consideration of uncertainty, time preference and intergenerational equity, the traditional cost-benefit analysis framework is challenged with regard to the discounting/non-discounting of carbon uptake benefits, and because it usually uses a constant and positive discount rate. We investigate the influence of various discounting protocols on the outputs of economic analysis. The idea of using the declining discount rate is also considered. Several numerical examples dealing with the analysis of afforestation for carbon sequestration in Scotland and Ukraine are provided. We show that the choice of discounting protocols have a considerable influence on the results of economic analysis, and therefore, on the decision-making processes related to climate change mitigation strategies. The paper concludes with some innovative insights on accounting for uncertainties and time preference in tackling climate change through forestry, several climate policy implications of dealing with uncertainties, and a brief discussion of what the use of different discounting protocols might imply for decision making. 相似文献
26.
The effect of drawdown on suspended solids and phosphorus export from Columbia Lake,Waterloo, Canada
Mike Shantz Elizabeth Dowsett Emma Canham Guillaume Tavernier Mike Stone Jonathan Price 《水文研究》2004,18(5):865-878
This study examines the effect of drawdown on the timing and magnitude of suspended solids and associated phosphorus export from a 12 ha reservoir located in an urbanized watershed in southern Ontario, Canada. Water level in Columbia Lake was lowered by 1·15 m over a 2‐week period in November 2001. The total phosphorus (TP) concentrations ranged from 63 to 486 µg L?1 in Columbia Lake and 71 to 373 µg L?1 at its outflow. All samples exceeded the Provincial Water Quality Objective of 30 µg TP L?1. Outflow concentrations of suspended solids and TP increased significantly with decreasing lake level and were attributed to the resuspension of cohesive bottom sediments that occurred at a critical threshold lake level (0·65 m below summer level). Suspended solids at the outflow consisted of flocculated cohesive materials with a median diameter (D50) of c. 5 µm. Particulate organic carbon accounted for 8·5% of the suspended solids export by mass. A total mass of 18·5 t of suspended solids and 62·6 kg TP was exported from Columbia Lake, which represents a significant pulse of sediment‐associated P to downstream environments each autumn during drawdown. The downstream impacts of this release can be minimized if the water level in Columbia Lake is lowered no more than 0·5 m below summer levels. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
27.
Guillaume Desbois 《Geochimica et cosmochimica acta》2007,71(21):5233-5243
Hydrogen-deuterium exchange in tourmaline single crystals of elbaite composition from Nepal has been studied at 1 atm and at temperatures between 973 and 1073 K. H/D ratios were determined after each annealing experiment using micro FTIR-spectroscopy. Diffusion coefficients (10−16-10−15 m2 s−1) were determined by fitting the data using a 3D numerical simulation. The rate of diffusion is two to three times faster along the c direction than along directions parallel to the basal plane. The diffusion laws are, respectively:
28.
Southern Brazil has recently been the subject of many major natural hazards from weather and climatic origin, including violent floods in 2016 caused by very heavy rains. It has also experienced episodes of droughts and heat waves in recent years. The state of Paraná, located at the climatic transition zone, has densely populated urban areas, vast cultivation areas, and hydro-electric reservoirs (more than 20), so those extreme events are letting local populations vulnerable to the vagaries of the climate and their impacts on community, infrastructure, and ecosystem. This study analyzes climatic variability and trends of about ten climatic indices (with RClimDex), calculated by using daily thermal data of ten stations spread mainly in two geographic regions of Paraná. The Mann-Kendall and Pettitt tests were applied for trends analysis and determine the presence of breakpoints in the time series (1971–2014). Our results showed that for the various thermal indices, there is a reduction of the cold days on all the stations, indicating a more pronounced increase of the indices based on the maximum temperatures (TX), especially in the north. On the other hand, the indexes based on minimum temperatures (TN) show a more modest and partial increase, varying accordingly to the location of the stations. Regionally, the trends calculated were similar, that is, North region presents a more expressive increase of the indices of heat whereas in the east predominates a reduction. 相似文献
29.
30.
Georges Ona-Nguema Guillaume Morin Yuheng Wang Farid Juillot Giuliana Aquilanti Christian Ruby François Guyot Gordon E. Brown Jr. 《Geochimica et cosmochimica acta》2009,73(5):1359-1446
X-ray Absorption Fine Structure (XAFS) spectroscopy was used in combination with high resolution transmission electron microscopy (HRTEM), electron energy loss spectroscopy (EELS), X-ray energy dispersive spectroscopy (XEDS), X-ray powder diffraction, and Mössbauer spectroscopy to obtain detailed information on arsenic and iron speciation in the products of anaerobic reduction of pure and As(V)- or As(III)-adsorbed lepidocrocite (γ-FeOOH) by Shewanella putrefaciens ATCC 12099. We found that this strain of S. putrefaciens is capable of using Fe(III) in lepidocrocite and As(V) in solution or adsorbed on lepidocrocite surfaces as electron acceptors. Bioreduction of lepidocrocite in the absence of arsenic resulted in the formation of hydroxycarbonate green rust 1 [FeII4FeIII2(OH)12CO3: GR1(CO3)], which completely converted into ferrous-carbonate hydroxide (FeII2(OH)2CO3: FCH) over nine months. This study thus provides the first evidence of bacterial reduction of stoichiometric GR1(CO3) into FCH. Bioreduction of As(III)-adsorbed lepidocrocite also led to the formation of GR1(CO3) prior to formation of FCH, but the presence of As(III) slows down this transformation, leading to the co-occurrence of both phases after 22-month of aging. At the end of this experiment, As(III) was found to be adsorbed on the surfaces of GR1(CO3) and FCH. After five months, bioreduction of As(V)-bearing lepidocrocite led directly to the formation of FCH in association with nanometer-sized particles of a minor As-rich Fe(OH)2 phase, with no evidence for green rust formation. In this five-month experiment, As(V) was fully converted to As(III), which was dominantly sorbed at the surface of the Fe(OH)2 nanoparticles as oligomers binding to the edges of Fe(OH)6 octahedra at the edges of the octahedral layers of Fe(OH)2. These multinuclear As(III) surface complexes are characterized by As-As pairs at a distance of 3.32 ± 0.02 Å and by As-Fe pairs at a distance of 3.50 ± 0.02 Å and represent a new type of As(III) surface complex. Chemical analyses show that the majority of As(III) produced in the experiments with As present is associated with iron-bearing hydroxycarbonate or hydroxide solids, reinforcing the idea that, at least under some circumstances, bacterial reduction can promote As(III) sequestration instead of mobilizing it into solution. 相似文献