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211.
212.
Eric?Rodriguez Kevin?A.?McGuinness Duke?U.?OphoriEmail author 《Environmental Geology》2004,45(5):623-632
An initial assessment of an old manufacturing site with groundwater impacted by trichloroethene (TCE) contamination in the metropolitan New York area showed that the TCE was being removed naturally by reductive dechlorination. However, complete dechlorination was not expected at the site because the process was progressing too slowly under transitional to aerobic conditions at a degradation constant of –0.0013 and a TCE half life of 533 days. A pilot test was conducted at the site in which a carbohydrate substrate (molasses) was injected into the groundwater to create an In-Situ Reactive Zone (IRZ). Post-pilot test groundwater sampling and analysis indicated that an IRZ was created successfully as the total organic carbon (TOC) content and conductivity increased significantly while oxidation-reduction (REDOX) potential and dissolved oxygen (DO) decreased. The created IRZ caused enhanced reductive dechlorination of TCE at the site, found to proceed with a degradation constant of –0.0158 and a TCE half life of 44 days. 相似文献
213.
Joseph A. Shacat William J. Green Eric H. Decarlo Silvia Newell 《Aquatic Geochemistry》2004,10(3-4):325-352
Lake Joyce is one of the least studied lakes of the McMurdo Dry Valleys. Similar to other lakes in this region, Lake Joyce is a closed-basin, permanently ice-covered, meromictic lake. We present here a detailed investigation of major ions, nutrients, and dissolved trace elements for Lake Joyce. Specifically, we investigate the role of iron and manganese oxides and hydrous oxides in trace metal cycling.Lake Joyce is characterized by fresh, oxic waters overlying an anoxic brine, primarily Na–Cl. Surface waters have a maximum nitrate concentration of 26M with a molar dissolved inorganic nitrogen to phosphorus ratio of 477. The supply of nitrogen is attributed to atmospheric deposition, possibly from polar stratospheric clouds. Dissolved phosphorus is scavenged by hydrous iron oxides. The pH is highest (10.15) just beneath the 7-m thick ice cover and decreases to a minimum of 7.29 in the redox transition zone. Dissolved Al exceeds 8M in surface waters, and appears to be controlled by equilibrium with gibbsite. In contrast, concentrations of other trace elements in surface waters are quite low (e.g., 5.4nM Cu, 0.19nM Co, <20pM La). Dissolved Fe, Mn, Ni and Cd were below our detection limits of 13 nM, 1. 8 nM, 4.7 nM and 15pM (respectively) in surface waters. There was a 6-m vertical separation in the onset of Mn and Fe reduction, with dissolved Mn appearing higher in the water column than Fe. Based on thermodynamic calculations, dissolved Mn appears to be controlled by equilibrium with hausmannite (Mn3 O4 ). Co tracks the Mn profile closely, suggesting Co(III) is bound in the lattice of Mn oxides, whereas the Ce profile is similar, yet the Ce anomaly suggests oxidative scavenging of Ce. Release of Cu, Ni, Cd and trivalent REE appears to be controlled by pH-induced desorption from Fe and Mn oxides, although Cu (and perhaps Ni) may be scavenged by organic matter in surface waters. 相似文献
214.
Comprehensive studies of water resources systems require integration of modeling tools and data associated with individual processes. An object-oriented approach is presented here that associates ground water models based upon the analytic element method (AEM) with geographic information system (GIS) geodatabase features using an AEM Model Interface. Each aquifer object contains a prescribed geometry, a mathematical representation in the AEM, and GIS hydrogeologic data. The synergistic understanding inherent in such an approach is illustrated by a study linking local AEM model predictions of water elevation with ground water geodatabase objects. This AEM Model Interface provides a key component in establishing a common object-oriented geodatabase modeling approach linking ground water to a variety of natural and social processes. 相似文献
215.
Springs along the south rim of the Grand Canyon, Arizona, are important ecological and cultural resources in Grand Canyon National Park and are discharge points for regional and local aquifers of the Coconino Plateau. This study evaluated the applicability of electrical resistance (ER) sensors for measuring diffuse, low-stage (<1.0 cm) intermittent and ephemeral flow in the steep, rocky spring-fed tributaries of the south rim. ER sensors were used to conduct a baseline survey of spring flow timing at eight sites in three spring-fed tributaries in Grand Canyon. Sensors were attached to a nearly vertical rock wall at a spring outlet and were installed in alluvial and bedrock channels. Spring flow timing data inferred by the ER sensors were consistent with observations during site visits, with flow events recorded with collocated streamflow gauging stations and with local precipitation gauges. ER sensors were able to distinguish the presence of flow along nearly vertical rock surfaces with flow depths between 0.3 and 1.0 cm. Laboratory experiments confirmed the ability of the sensors to monitor the timing of diffuse flow on impervious surfaces. A comparison of flow patterns along the stream reaches and at springs identified the timing and location of perennial and intermittent flow, and periods of increased evapotranspiration. 相似文献
216.
Francis Joseph Turk Byung-Ju Sohn Hyun-Jong Oh Elizabeth E. Ebert Vincenzo Levizzani Eric A. Smith 《Meteorology and Atmospheric Physics》2009,105(1-2):99-108
In order to properly utilize remotely sensed precipitation estimates in hydrometeorological applications, knowledge of the accuracy of the estimates are needed. However, relatively few ground validation networks operate with the necessary spatial density and time-resolution required for validation of high-resolution precipitation products (HRPP) generated at fine space and time scales (e.g., hourly accumulations produced on a 0.25° spatial scale). In this article, we examine over-land validation statistics for an operationally designed, meteorological satellite-based global rainfall analysis that blends intermittent passive microwave-derived rainfall estimates aboard a variety of low Earth-orbiting satellite platforms with sub-hourly time sampling capabilities of visible and infrared imagers aboard operational geostationary platforms. The validation dataset is comprised of raingauge data collected from the dense, nearly homogeneous, 1-min reporting Automated Weather Station (network of the Korean Meteorological Administration during the June to August 2000 summer monsoon season. The space-time RMS error, mean bias, and correlation matrices were computed using various time windows for the gauge averaging, centered about the satellite observation time. For ±10 min time window, a correlation of 0.6 was achieved at 0.1° spatial scale by averaging more than 3 days; coarsening the spatial scale to 1.8° produced the same correlation by averaging over 1 h. Finer than approximately 24-h and 1° time and space scales, respectively, a rapid decay of the error statistics was obtained by trading-off either spatial or time resolution. Beyond a daily time scale, the blended estimates were nearly unbiased and with an RMS error of no worse than 1 mm day?1. 相似文献
217.
Chung-Lin SHIE Long S. CHIU Robert ADLER Eric NELKIN I-I LIN Pingping XIE Feng-Chin WANG R. CHOKNGAMWONG William OLSON D. Allen CHU 《大气科学进展》2009,26(6):1071-1080
Accurate sea surface flux measurements are crucial for
understanding the global water and energy cycles. The oceanic
evaporation, which is a major component of the global oceanic fresh
water flux, is useful for predicting oceanic circulation and
transport. The global Goddard Satellite-based Surface Turbulent
Fluxes Version-2 (GSSTF2; July 1987--December 2000) dateset that was
officially released in 2001 has been widely used by scientific
community for global energy and water cycle research, and regional
and short period data analyses. We have recently been funded by NASA
to resume processing the GSSTF dataset with an objective of
continually producing a uniform dataset of sea surface turbulent
fluxes, derived from remote sensing data. The dataset is to be
reprocessed and brought up-to-date (GSSTF2b) using improved input
datasets such as a recently upgraded NCEP/DOE sea surface
temperature reanalysis, and an upgraded surface wind and microwave
brightness temperature V6 dataset (Version 6) from the Special
Sensor Microwave Imager (SSM/I) produced by Remote Sensing Systems
(RSS). A second new product (GSSTF3) is further proposed with a
finer temporal (12-h) and spatial (0.25ox0.25o)
resolution. GSSTF2b (July 1987--December 2008) and GSSTF3 (July
1999--December 2009) will be released for the research community to
use by late 2009 and early 2011, respectively. 相似文献
218.
An assessment of the likely benefits of assimilating in situ temperature (T) and salinity (S) observations from repeat glider transects and surface velocity observations from high-frequency radar arrays into an eddy-resolving ocean model is presented. The deployment of new shelf observation platforms around Australia is being undertaken through the Australian Integrated Marine Observing System program. In this study, various options for an observing system along the coast of New South Wales, Australia, are assessed for their benefits to an ocean forecast and reanalysis system. The forecast system considered here uses ensemble optimal interpolation (EnOI) for data assimilation. Using error estimates from the EnOI scheme, estimates of the theoretical analysis errors are calculated for different observing systems that include a range of remotely sensed and in situ observations. The results demonstrate that if HF radar observations are assimilated along with the standard components of the global ocean observing system, the analysis errors are likely to reduce by as much as 80% for velocity and 60% for T, S and sea-level in the vicinity of the observations. Owing to the relatively short along-shore decorrelation length-scales for T and S near the shelf, the glider observations are likely to provide the forecast system with a more modest gain. 相似文献
219.
Transnational linkages and the spillover of environment-efficiency into developing countries 总被引:2,自引:0,他引:2
Arguments about the “positive” influence of growing transnational linkages have typically focused on their role in diffusing environmentally superior innovations which help to raise countries’ environment-efficiency. The present article empirically tests these claims by examining whether developing countries’ linkages with more CO2- and SO2-efficient economies contribute to domestic improvements in CO2- and SO2-efficiency. Our large-N, statistical findings caution against some of the efficiency-oriented optimism voiced by supporters of globalization. Although imports ties with more pollution-efficient countries are found to spillover into improved domestic CO2- and SO2-efficiency, neither transnational linkages via exports, inward foreign direct investment (FDI) nor telephone calls appear to have any influence on domestic pollution-efficiency. 相似文献
220.
Future climate in the Pacific Northwest 总被引:4,自引:2,他引:2
Climate models used in the Intergovernmental Panel on Climate Change (IPCC) Fourth Assessment Report (AR4) on the whole reproduce the observed seasonal cycle and twentieth century warming trend of 0.8°C (1.5°F) in the Pacific Northwest, and point to much greater warming for the next century. These models project increases in annual temperature of, on average, 1.1°C (2.0°F) by the 2020s, 1.8°C (3.2°F) by the 2040s, and 3.0°C (5.3°F) by the 2080s, compared with the average from 1970 to 1999, averaged across all climate models. Rates of warming range from 0.1°C to 0.6°C (0.2°F to 1.0°F) per decade. Projected changes in annual precipitation, averaged over all models, are small (+1% to +2%), but some models project an enhanced seasonal cycle with changes toward wetter autumns and winters and drier summers. Changes in nearshore sea surface temperatures, though smaller than on land, are likely to substantially exceed interannual variability, but coastal upwelling changes little. Rates of twenty-first century sea level rise will depend on poorly known factors like ice sheet instability in Greenland and Antarctica, and could be as low as twentieth century values (20 cm, 8″) or as large as 1.3 m (50″). 相似文献