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241.
242.
A natural datolite CaBSiO4(OH) (Bergen Hill, NJ, USA), before and after gamma-ray irradiation (up to ~70 kGy), has been investigated by single-crystal
and powder electron paramagnetic resonance (EPR) spectroscopy from 10 to 295 K. EPR spectra of gamma-ray-irradiated datolite
show the presence of a boron-associated oxygen hole center (BOHC) and an atomic hydrogen center (H0), both of which grow with increasing radiation dose. The principal g and A(11B) values of the BOHC at 10 K are: g
1 = 2.04817(3), g
2 = 2.01179(2), g
3 = 2.00310(2), A
1 = −0.401(7) mT, A
2 = −0.906(2) mT, A
3 = −0.985(2) mT, with the orientations of the g
1 and A
1 axes approximately along the B–OH bond direction. These experimental results suggest that the BOHC represents hole trapping
on the hydroxyl oxygen atom after the removal of the proton (i.e. a [BO4]0 center): via a reaction O3BOH → O3BO· + H0, where · denotes the unpaired electron. Density functional theory (DFT) calculations (CRYSTAL06, B3PW, all-electron basis
sets, and 1 × 2 × 2 supercell) support the proposed structural model and yield the following 11B hyperfine coupling constants: A
1 = −0.429 mT, A
2 = −0.901 mT, A
3 = −0.954 mT, in excellent agreement with the experimental results. The [BO4]0 center undergoes the onset of thermal decay at ~200°C and is completely annealed out at 375°C but can be restored readily
by gamma-ray irradiation. Isothermal annealing experiments show that the [BO4]0 center exhibits a second-order thermal decay with an activation energy of 0.96 eV. The confirmation of the [BO4]0 center (and its formation from the O3BOH precursor) in datolite has implications for not only understanding of BOHCs in alkali borosilicate glasses but also their
applications to nuclear waste disposal. 相似文献
243.
提出一种引入样本熵(SE)优化的经验小波变换(EWT)结合非局部均值(NLM)滤波的组合自适应降噪方法。该方法使用SE确定全部经验模态分量中低频有效信号界限,叠加其余中高频分量后进行NLM滤波处理,之后重构滤波信号与有效信号为最终降噪信号,从而达到滤除高频噪声的目的。模拟数据与实测数据的实验结果表明,优化的EWT-NLM方法整体优于EMD、EWT方法,RMSE分别降低13.41%/10.63%(实测数据/模拟数据)、7.13%/5.78%,信噪比分别提升22.03%/22.54%、9.72%/7.42%。 相似文献
244.
通过对东海外陆坡–冲绳海槽GSW1孔沉积物孔隙水δ13C、δ18O、δ11B、δ37Cl同位素和Cl-、S O42-、K+、Na+等离子指标的分析,探讨了沉积物早期成岩作用、流体来源、迁移和氧化环境的变化。研究发现,GSW1孔孔隙水溶解无机碳主要来自海水和有机质,SO42-浓度随深度下降比较平缓,Cl-浓度远低于海水,该孔表层沉积物中硫酸盐消耗主要由有机质硫酸盐还原作用(OSR)所控制,甲烷厌氧氧化作用(AOM)发生在4 m以下更深的层位。OSR产生的H2S向上扩散富集并被氧化,是导致GSW1孔110~360 cm处SO 42-浓度未明显下降的主要因素。孔隙水SO42-浓度整体随着深度增加呈减小的趋势,表明GSW1孔沉... 相似文献
245.
Assessment of social vulnerability to natural hazards in the Yangtze River Delta, China 总被引:7,自引:3,他引:4
Yi Ge Wen Dou Zhihui Gu Xin Qian Jinfei Wang Wei Xu Peijun Shi Xiaodong Ming Xin Zhou Yuan Chen 《Stochastic Environmental Research and Risk Assessment (SERRA)》2013,27(8):1899-1908
China is exposed to a wide range of natural hazards, and disaster losses have escalated over the past decade. Owing to the pressure from natural disasters, along with changes in climate, social conditions, and regional environment, assessment of social vulnerability (SV) to natural hazards has become increasingly urgent for risk management and sustainable development in China. This paper presents a new method for quantifying SV based on the projection pursuit cluster (PPC) model. A reference social vulnerability index (SVI) at the county level was created for the Yangtze River Delta area in China for 1995, 2000, 2005, and 2009. The result of social vulnerability assessment was validated using data of actual losses from natural disasters. The primary findings are as follows: (i) In the study area, the major factors that impact SVI are regional per capita GDP and per capita income. (ii) The study area was more vulnerable in 1995 than in later years. SV of the whole region had decreased over the study period. (iii) Most part of Shanghai and the southeast part of Jiangsu Province had been the least vulnerable within the region. From this least vulnerable zone to the periphery of the region, the situation deteriorated. The highest SVI values in all evaluated years were found in the northern, western, or southern tips of the Yangtze River Delta. 相似文献
246.
Spatial and depth variability of streambed vertical hydraulic conductivity under the regional flow regimes
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Jinxi Song Liping Wang Xinyi Dou Fangjian Wang Hongtao Guo Junlong Zhang Guotao Zhang Qi Liu Bo Zhang 《水文研究》2018,32(19):3006-3018
This study investigated the influence of the regional flow on the streambed vertical hydraulic conductivity (Kv) within the hyporheic zone in three stream reaches of the Weihe River in July 2016. The streambed Kv with two connected depths was investigated at each test reach. Based on the sediment characteristics, the three test reaches could be divided into three categories: a sandy streambed without continuous silt and clay layer, a sandy streambed with continuous silt and clay layer, and a silt–clay streambed. The results demonstrate that the streambed Kv mainly decreases with the depth at the sandy streambed (without continuous silt and clay layer) and increases with the depth at the other two test reaches. At the sandy streambed (with continuous silt and clay layer) where streambed Kv mainly decreases with the depth, the regional upward flux can suspend fine particles and enhance the pore spacing, resulting in the elevated Kv in the upper sediment layers. At another sandy streambed, the continuous silt and clay layer is the main factor that influences the vertical distribution of fine particles and streambed Kv. An increase in streambed Kv with the depth at the silt/clay streambed is attributed to the regional downward movement of water within the sediments that may lead to more fine particles deposited in the pores in the upper sediment layers. The streambed Kv is very close to the bank in the sandy streambed without continuous silt and clay layer and the channel centre in the other two test reaches. Differences in grain size distribution of the sediments at each test reach exercise a strong controlling influence on the streambed Kv. This study promotes the understanding of dynamics influencing the interactions between groundwater and surface water and provides guidelines to scientific water resources management for rivers. 相似文献
247.
Roughness scale dependence of the relationship between tracer longitudinal dispersion and Peclet number in variable‐aperture fractures
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The relationship between the longitudinal dispersion (DL) and Peclet number (Pe) is crucial for predicting and simulating tracer through the variable‐aperture fracture. In this study, the roughness of the self‐affine fracture wall was decomposed into primary roughness (relatively large‐scale waviness) and secondary roughness (relatively small‐scale waviness) by a multiscaled wavelet analysis technique. Based on the complete dispersion mechanism (diffusion, macrodispersion, and Taylor dispersion) in the variable‐aperture fracture, three relationships (second‐order, power‐law, and linear relationships) between the DL and Pe were investigated at large and small scales, respectively. Our results showed that the primary roughness mostly controlled the Taylor dispersion mechanism, whereas the secondary roughness was a dominant factor for the macrodispersion mechanism. Increasing the Hurst exponent and removing the secondary roughness led to the decreasing range of Pe where macrodispersion mechanism dominated the solute transport. It was found that estimating the DL from the power‐law relationship based on Taylor dispersion theory resulted in considerable errors, even in the range of Pe where the Taylor dispersion mechanism dominated. The exponent of the power‐law relationship increased as the secondary roughness was removed. Analysing the linear relationship between the DL and Pe revealed that the longitudinal dispersivity αL increased linearly. However, this linear increase became weak as the Taylor dispersion mechanism dominated. In the range of Pe where the macrodispersion mechanism dominated, increasing the Hurst exponent caused the increase of αL and the secondary roughness played a significant role in enhancing the αL. As the Taylor dispersion mechanism dominated, the αL was insensitive to the influence of multiscale roughness in variable‐aperture fractures. 相似文献
248.
The objective of this study is to understand the process of fluid flow in pipe and porous media with different pore structures.High-resolution Magnetic Resonance Imaging(MRI)technique was used to visualize the pore structure and measure fluid flow.The porous media was formed by packed bed of glass beads.Flow measurement was carried out by a modified spin echo sequence.The results show that the velocity distribution in pipe is annular and the linear relation between MRI velocity and actual velocity is found in pipe flow measurement.The flow distribution in porous media is rather heterogeneous,and it is consistent with heterogeneous pore structure.The flow through pores with the high volume flow rate is determined largely by geometrical effects such as pore size and cross-sectional area. 相似文献
249.
社会主义新农村建设中的防雷工作探讨 总被引:3,自引:0,他引:3
根据社会主义新农村建设中防雷工作适应新形势的需要,结合近年来农村发生的几起典型雷击事件,详细总结了农村雷击事故形成的原因,并提出加强新农村建设防雷工作的对策,切实履行气象部门监管职责,将新农村建设的防雷减灾工作落到实处. 相似文献
250.