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71.
The effect of iron on montmorillonite stability. (I) Background and thermodynamic considerations 总被引:1,自引:0,他引:1
It is envisaged that high-level nuclear waste (HLW) will be disposed of in underground repositories. Many proposed repository designs include steel waste canisters and bentonite backfill. Natural analogues and experimental data indicate that the montmorillonite component of the backfill could react with steel corrosion products to produce non-swelling Fe-rich phyllosilicates such as chamosite, berthierine, or Fe-rich smectite. In K-bearing systems, the alteration of montmorillonite to illite/glauconite could also be envisaged. If montmorillonite were altered to non-swelling minerals, the swelling capacity and self-healing properties of the bentonite backfill could be reduced, thereby diminishing backfill performance. The main aim of this paper was to investigate Fe-rich phyllosilicate mineral stability at the canister-backfill interface using thermodynamic modelling. Estimates of thermodynamic properties were made for Fe-rich clay minerals in order to construct approximate phase-relations for end-member/simplified mineral compositions in logarithmic activity space. Logarithmic activity diagrams (for the system Al2O3-FeO-Fe2O3-MgO-Na2O-SiO2-H2O) suggest that if pore waters are supersaturated with respect to magnetite in HLW repositories, Fe(II)-rich saponite is the most likely montmorillonite alteration product (if fO2(g) values are significantly lower than magnetite-hematite equilibrium). Therefore, the alteration of montmorillonite may not be detrimental to nuclear waste repositories that include Fe, as long as the swelling behaviour of the Fe-rich smectite produced is maintained. If fO2(g) exceeds magnetite-hematite equilibrium, and solutions are saturated with respect to magnetite in HLW repositories, berthierine is likely to be more stable than smectite minerals. The alteration of montmorillonite to berthierine could be detrimental to the performance of HLW repositories. 相似文献
72.
Water Self-Softening Processes at Waterfall Sites 总被引:1,自引:0,他引:1
David Dian ZHANG 《《地质学报》英文版》2004,78(5):1154-1161
Many rivers in tropical and subtropical karst regions are supersaturated with respect to CaCO3 and have high water hardness. After flowing through waterfall sites, river water is usually softened, accompanied by tufa formation, which is simply described as a result of water turbulence in fast-flowing water. In this paper, a series of laboratory experiments are designed to simulate the hydrological conditions at waterfall sites. The influences of air-water interface, water flow velocity, aeration and solid-water interface on water softening are compared and evaluated on a quantitative basis. The results show that the enhanced inorganic CO2 outgassing due to sudden hydrological changes occurring at waterfall sites is the principal cause of water softening at waterfall sites. Both air-water interface area and water flow velocity increase as a result of the "aeration effect", "low pressure effect" and "jet-flow effect" at waterfall sites, which greatly accelerates CO2 outgassing and therefore makes natural w 相似文献
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The climate–population relationship has long been conceived. Although the topic has been repeatedly investigated, most of
the related works are Eurocentric or qualitative. Consequently, the relationship between climate and population remains ambiguous.
In this study, fine-grained temperature reconstructions and historical population data sets have been employed to statistically
test a hypothesized relationship between temperature change and population growth (i.e., cooling associated with below average
population growth) in China over the past millennium. The important results were: (1) Long-term temperature change significantly
determined the population growth dynamics of China. However, spatial variation existed, whilst population growth in Central
China was shown to be responsive to both long- and short-term temperature changes; in marginal areas, population growth was
only sensitive to short-term temperature fluctuations. (2) Temporally, the temperature–population relationship was obscured
in some periods, which was attributable to the factors of drought and social buffers. In summary, a temperature–population
relationship was mediated by geographic factors, the aridity threshold, and social factors. Given the upcoming threat posed
by climate change to human societies, this study seeks to improve our knowledge and understanding of the climate–society relationship. 相似文献
75.
Seong-Joong Kim Thomas J. Crowley David J. Erickson Bala Govindasamy Phillip B. Duffy Bang Yong Lee 《Climate Dynamics》2008,31(1):1-16
The climate of the last glacial maximum (LGM) is simulated with a high-resolution atmospheric general circulation model, the
NCAR CCM3 at spectral truncation of T170, corresponding to a grid cell size of roughly 75 km. The purpose of the study is
to assess whether there are significant benefits from the higher resolution simulation compared to the lower resolution simulation
associated with the role of topography. The LGM simulations were forced with modified CLIMAP sea ice distribution and sea
surface temperatures (SST) reduced by 1°C, ice sheet topography, reduced CO2, and 21,000 BP orbital parameters. The high-resolution model captures modern climate reasonably well, in particular the distribution
of heavy precipitation in the tropical Pacific. For the ice age case, surface temperature simulated by the high-resolution
model agrees better with those of proxy estimates than does the low-resolution model. Despite the fact that tropical SSTs
were only 2.1°C less than the control run, there are many lowland tropical land areas 4–6°C colder than present. Comparison
of T170 model results with the best constrained proxy temperature estimates (noble gas concentrations in groundwater) now
yield no significant differences between model and observations. There are also significant upland temperature changes in
the best resolved tropical mountain belt (the Andes). We provisionally attribute this result in part as resulting from decreased
lateral mixing between ocean and land in a model with more model grid cells. A longstanding model-data discrepancy therefore
appears to be resolved without invoking any unusual model physics. The response of the Asian summer monsoon can also be more
clearly linked to local geography in the high-resolution model than in the low-resolution model; this distinction should enable
more confident validation of climate proxy data with the high-resolution model. Elsewhere, an inferred salinity increase in
the subtropical North Atlantic may have significant implications for ocean circulation changes during the LGM. A large part
of the Amazon and Congo Basins are simulated to be substantially drier in the ice age—consistent with many (but not all) paleo
data. These results suggest that there are considerable benefits derived from high-resolution model regarding regional climate
responses, and that observationalists can now compare their results with models that resolve geography at a resolution comparable
to that which the proxy data represent. 相似文献
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79.
Anomalies found when apportioning responsibility for streamflow depletion are examined. The anomalies arise when responsibility is assigned to the two states that contribute to depletion of Beaver Creek in the Republican River Basin in the United States. The apportioning procedure for this basin presumes that the sum of streamflow depletions, computed by comparing simulation model runs with and without groundwater pumping from individual states, approximates the streamflow depletion when both states are pumping. In the case study presented here, this presumed superposition fails dramatically. The stream drying and aquifer-storage depletion, as represented in the simulation model used for allocation, are examined in detail to understand the hydrologic and numerical basis for the severe nonlinear response. Users of apportioning procedures that rely on superposition should be aware of the presence and likely magnitude of nonlinear responses in modeling tools. 相似文献
80.