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71.
Michael Bau Brian Alexander John T Chesley Susan L Brantley 《Geochimica et cosmochimica acta》2004,68(6):1199-1216
To compare relative reaction rates of mineral dissolution in a mineralogically simple groundwater aquifer, we studied the controls on solute concentrations, Sr isotopes, and rare earth element and yttrium (REY) systematics in the Cape Cod aquifer. This aquifer comprises mostly carbonate-free Pleistocene sediments that are about 90% quartz with minor K-feldspar, plagioclase, glauconite, and Fe-oxides. Silica concentrations and pH in the groundwater increase systematically with increasing depth, while Sr isotopic ratios decrease. No clear relationship between 87Sr/86Sr and Sr concentration is observed. At all depths, the 87Sr/86Sr ratio of the groundwater is considerably lower than the Sr isotopic ratio of the bulk sediment or its K-feldspar component, but similar to that of a plagioclase-rich accessory separate obtained from the sediment. The Si-87Sr/86Sr-depth relationships are consistent with dissolution of accessory plagioclase. In addition, solutes such as Sr, Ca, and particularly K show concentration spikes superimposed on their respective general trends. The K-Sr-87Sr/86Sr systematics suggests that accessory glauconite is another major solute source to Cape Cod groundwater. Although the authigenic glauconite in the Cape Cod sediment is rich in Rb, it is low in in-grown radiogenic 87Sr because of its young Pleistocene age. The low 87Sr/86Sr ratios are consistent with equilibration of glauconite with seawater. The impact of glauconite is inferred to vary due to its variable abundance in the sediments. In the Cape Cod groundwater, the variation of REY concentrations with sampling depth resembles that of K and Rb, but differs from that of Ca and Sr. Shale-normalized REY patterns are light REY depleted, show negative Ce anomalies and super-chondritic Y/Ho ratios, but no Eu anomalies. REY input from feldspar, therefore, is insignificant compared to input from a K-Rb-bearing phase, inferred to be glauconite. These results emphasize that interpretation of groundwater chemistry, even in relatively simple aquifers, may be complicated by solute contributions from “exotic” accessory minerals such as glauconite. To detect such peculiarities, groundwater studies should combine the study of elemental concentration and isotopic composition of several solutes that show different geochemical behavior. 相似文献
72.
CSA mine exploits a ‘Cobar-type’ Cu–Pb–Zn±Au±Ag deposit within a cleaved and metamorphosed portion of the Cobar Supergroup, central New South Wales. The deposit comprises systems of ‘lenses’ that encompass veins, disseminations and semi-massive to massive Cu–Pb–Zn ores. The systems and contained lenses truncate bedding, are approximately coplanar with regional cleavage and similarly oriented shear zones and plunge parallel to the elongation lineation. Systems have extreme vertical continuity (>1000 m), short strike length (400 m) and narrow width (100 m), exhibit vertical and lateral ore-type variation and have alteration haloes. Models of ore formation include classical hydrothermalism, structurally controlled remobilisation and polymodal concepts; syntectonic emplacement now holds sway.Fluid inclusions were examined from quartz±sulphide veins adjacent to now-extracted ore, from coexisting quartz–sulphide within ore, and from vughs in barren quartz veins. Lack of early primary inclusions precluded direct determination of fluids associated with D2–D3 ore and vein emplacement. Similarly, decrepitation (by near-isobaric heating) of the two oldest secondary populations precluded direct determination of fluid phases immediately following D2–D3 ore and vein emplacement. Post-decrepitation outflow (late D3 to early post-D3) is recorded by monophase CH4 inclusions. Entrained outflow of deeply circulated meteoric fluid modified the CH4 system; modification is recorded by H2O+CH4 and H2O+(trace CH4) secondary populations and by an H2O+(trace CH4) primary population. The contractional tectonics (D2–D3) of ore emplacement was superseded by relaxational tectonics (D4P) that facilitated meteoric water penetration and return flow.Under D2 prograde metamorphism, entrapment temperatures (Tt) and pressures (Pt) for pre-decrepitation secondary inclusions are estimated as Tt300–330 °C and Pt1.5–2 kbar≈Plith (the lithostatic pressure). Decrepitation accompanied peak metamorphism (T350–380 °C) in mid- to late-D3, while in late-D3 to early post-D3, essentially monophase CH4 secondary inclusions were entrapped at Tt350 °C and Pt=1.5–2 kbar≈Plith. Subsequently, abundant CH4 and entrained meteoric water were entrapped as H2O+CH4 secondaries under slowly decreasing temperature (Tt330–350 °C) and constant pressure (Pt1.5–2 kbar). Finally, with increasingly dominant meteoric outflow, H2O+(trace CH4) populations record decreasing temperatures (Tt>300 to <350 down to 275–300 °C) at pressures of Phydrostatic<Pt (1 kbar) <Plith (1.5 kbar).The populations of inclusions provide insight into fluid types, flow regimes and P–T conditions during parts of the deposit's evolution. They indirectly support the role of basin-derived CH4 fluids in ore formation, but provide no insight into a basement-sourced ore-forming fluid. They fully support post-ore involvement of meteoric water. The poorly constrained entrapment history is believed to span 10 Ma from 395 to 385 Ma. 相似文献
73.
John M. Senko Brian S. Campbell James R. Henriksen Mostafa S. Elshahed Lee R. Krumholz 《Geochimica et cosmochimica acta》2004,68(4):773-780
Barite (BaSO4) deposits generally arise from mixing of soluble barium-containing fluids with sulfate-rich fluids. While the role of biological processes in modulating barium solubility has been shown, no studies have shown that the biological oxidation of sulfide to sulfate leads to barite deposition. Here we present an example of microbially mediated barite deposition in a continental setting. A spring in the Anadarko Basin of southwestern Oklahoma produces water containing abundant barium and sulfide. As emergent water travels down a stream to a nearby creek, sulfate concentration increases from 0.06 mM to 2.2 mM while Ba2+ concentration drops from 0.4 mM to less than 7 μM. Stable isotope analysis, microbial activity studies, and in situ experiments provide evidence that as sulfide-rich water flows down the stream, anaerobic, anoxygenic, phototrophic bacteria play a dominant role in oxidizing sulfide to sulfate. Sulfate then precipitates with Ba2+ producing barite as travertine, cements, crusts, and accumulations on microbial mats. Our studies suggest that phototrophic sulfide oxidation and concomitant sulfur cycling could prove to be important processes regulating the cycling of barium in continental sulfur-containing systems. 相似文献
74.
Models of late-glacial environmental change in coastal areas are commonly based on radiocarbon ages on marine shell and basal lake sediments, both of which may be compromised by reservoir effects. The magnitude of the oceanic reservoir age in the inland waters of the Georgia Basin and Puget Lowland of northwestern North America is inferred from radiocarbon ages on shell-wood pairs in Saanich Inlet and previously published estimates. The weighted mean oceanic reservoir correction in the early and mid Holocene is −720±90 yr, slightly smaller than, but not significantly different from, the modern value. The correction in late-glacial time is −950±50 yr. Valley-head sites yield higher reservoir values (−1200±130 yr) immediately after deglaciation. The magnitude of the gyttja reservoir effect is inferred from pairs of bulk gyttja and plant macrofossil ages from four lakes in the region. Incorporation of old carbon into basal gyttja yields ages from bulk samples that are initially about 600 yr too old. The reservoir age declines to less than 100 yr after the first millennium of lake development. When these corrections are accounted for, dates of deglaciation and late-glacial sea-level change in the study area are pushed forward in time by more than 500 yr. 相似文献
75.
This paper describes a series of tests designed to evaluate the capacity of a personal computer (PC) based statistical curve‐fitting program called MIX to quantify composite populations within multi‐modal particle‐size distributions. Three natural soil samples were analysed by a Coulter Multisizer, and their particle‐size distributions analysed using MIX software to identify the modes, standard deviations and proportions of their composite populations. The particle‐size distributions of the three natural soil samples were then numerically combined in equal proportions using a spreadsheet program to create synthetic particle‐size distributions of known populations. MIX was then tested on the synthetic particle‐size distributions to see if the modes and proportions it identified were similar to those modes and proportions known to characterize the synthetic particle‐size distributions. The main outcome is that MIX can very accurately describe the modal particle size and proportions of the major composite populations within a particle‐size distribution. However MIX has difficulty in identifying small populations (those contributing <10 per cent of a total particle‐size distribution), particularly when they are located in the central sections of particle‐size distributions, overlain by larger populations, or when positioned in the fine tails of distributions. Despite these minor shortcomings, MIX is a valuable tool for the examination and interpretation of particle‐size data. Copyright © 2005 John Wiley & Sons, Ltd. 相似文献
76.
A granitic rock avalanche, one of the largest Quaternary landslides in Arizona outside the Grand Canyon with a volume of approximately 5.25 M m3 and a width a little under 0.5 km, ran 1 km from the eastern McDowell Mountains. With lateral levees and pressure ridges, the rock avalanche deposit displays many features found on classic sturzstroms. Failure occurred along a major joint plane paralleling the slope with a dip of 44°, when a major base level lowering event in the Salt River system would have undermined the base of the failed slope, and probably during a period of more moisture than normally available in the present-day arid climate. Failure at the subsurface weathering front highlights the importance of the dramatic permeability change between grussified regolith and relatively fresh bedrock. Rock varnish microlaminations (VMLs) dating, in concert with other geomorphic evidence, suggests that the rock avalanche deposit is slightly older than 500 ka. The rock vanish results also have important implications for sampling strategies designed to use cosmogenic nuclide to date Quaternary landslide deposits. Discovery of a large landslide in close proximity to the extending urban fringe of metropolitan Phoenix argues for a more careful analysis of landslide hazards in the region, especially where rapid development excavates bedrock at the base of steep mountain slopes and where the subsurface weathering front is near the surface. 相似文献
77.
Late Quaternary alluvial induration has greatly influenced contemporary channel morphology on the anabranching Gilbert River in the monsoon tropics of the Gulf of Carpentaria. The Gilbert, one of a number of rivers in this region, has contributed to an extensive system of coalescing low-gradient and partly indurated riverine plains. Extensive channel sands were deposited by enhanced flow conditions during marine oxygen isotope (OI) Stage 5. Subsequent flow declined, probably associated with increased aridity, however, enhanced runoff recurred again in OI Stages 4–3 (65–50 ka). Aridity then capped these plains with 4–7 m of mud. A widespread network of sandy distributary channels was incised into this muddy surface from sometime after the Last Glacial Maximum (LGM) to the mid Holocene during a fluvial episode more active than the present but less so than those of OI Stages 5 and 3. This network is still partly active but with channel avulsion and abandonment now occurring largely proximal to the main Gilbert flow path.A tropical climate and reactive catchment lithology have enhanced chemical weathering and lithification of alluvium along the river resulting in the formation of small rapids, waterfalls and inset gorges, features characteristic more of bedrock than alluvial systems. Thermoluminescence (TL) and comparative optically stimulated luminescence (OSL) ages of the sediments are presented along with U/Th ages of pedogenic calcrete and Fe/Mn oxyhydroxide/ oxide accumulations. They show that calcrete precipitated during the Late Quaternary at times similar to those that favoured ferricrete formation, possibly because of an alternating wet–dry climate. Intense chemical alteration of the alluvium leading to induration appears to have prevailed for much of the Late Quaternary but, probably due to exceptional dryness, not during the LGM. The result has been restricted channel migration and a reduced capacity for the channel to adjust and accommodate sudden changes in bedload. Consequent avulsions have caused local stream powers to increase by an order of magnitude, inducing knickpoint erosion, local incision and the sudden influx of additional bedload that has triggered further avulsions. The Gilbert River, while less energetic than its Pleistocene ancestors, is clearly an avulsive system, and emphasizes the importance in some tropical rivers of alluvial induration for reinforcing the banks, generating nickpoints, reworking sediment and thereby developing and maintaining an indurated and anabranching river style. 相似文献
78.
79.
Brian McGowran 《中国地质大学学报(英文版)》2005,16(3):200-218
INTRODUCTION Microfossilsaregenerallythemostversatileand “useful”offossilsforbothcorrelationandagedeter minationandpaleoenvironmentalanalysis.Among microfossilstheforaminiferaarepre eminent(Fig. 1).Wefindinthesamesample—beitoutcropor subsurface,onshor… 相似文献
80.
Glacial conditions that contribute to the regeneration of Fountain Glacier proglacial icing,Bylot Island,Canada 下载免费PDF全文
Proglacial icings are one of the most common forms of extrusive ice found in the Canadian Arctic. However, the icing adjacent to Fountain Glacier, Bylot Island, is unique due to its annual cycle of growth and decay, and perennial existence without involving freezing point depression of water due to chemical characteristics. Its regeneration depends on the availability of subglacial water and on the balance between ice accretion and hydro‐thermal erosion. The storage and conduction of the glacial meltwater involved in the accretion of the icing were analyzed by conducting topographic and ground penetrating radar surveys in addition to the modelling of the subglacial drainage network and the thermal characteristics of the glacier base. The reflection power analysis of the geophysical data shows that some areas of the lower ablation zone have a high accumulation of liquid water, particularly beneath the centre part of the glacier along the main supraglacial stream. A dielectric permittivity model of the glacier – sediment interface suggests that a considerable portion of the glacier is warm based; allowing water to flow through unfrozen subglacial sediments towards the proglacial outwash plain. All these glacier‐related characteristics contribute to the annual regeneration of the proglacial icing and allow for portions of the icing to be perennial. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献