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121.
E. M. Chamorro Pérez I. Daniel J.-C. Chervin P. Dumas J. D. Bass T. Inoue 《Physics and Chemistry of Minerals》2006,33(7):502-510
High-pressure synchrotron infrared (IR) absorption spectra were collected between 650 and 4,000 cm−1 at ambient temperature for hydrous Mg-ringwoodite (γ-Mg2SiO4) up to 30 GPa. The main feature in the OH− stretching region is an extremely broad band centred at 3,150 cm−1. The hydrogen bond is strong for most protons and the most probable site for protonation is the tetrahedral edge. With increasing pressure, this band shifts downward while decreasing its integrated intensity until disappearance at a pressure of 25 GPa. Only one band at 2,450 cm−1 and an absorption plateau persist with a maximum wavenumber of 3,800 cm−1. This behaviour is reversible upon pressure release. We interpret this as a second-order phase transition occurring in hydrated Mg-ringwoodite at high pressure (beyond ∼ 25 GPa). This result is compatible with the observation by Kleppe et al. (Phys Chem Miner 29:473–476, 2002a) who suggested the presence of Si–O–Si linkages and/or partial increase in the coordination of Si. Beyond the phase transition, the protons are delocalized and their environment on the ringwoodite structure is probably quite different from that at low pressure. Data obtained in situ at high pressures and temperatures are needed to better understand the effect of protonation on the structure and to better constrain this phase transition. 相似文献
122.
A two-dimensional global climate model is used to assessthe climatic changes associated with the new IPCC SRES emissions scenarios and to determine which kind of changes in total solar irradiance and volcanic perturbations could mask the projected anthropogenic global warming associated to the SRES scenarios. Our results suggest that only extremely unlikely changes in total solar irradiance and/or volcanic eruptions would be able to overcome the simulated anthropogenic global warming over the century. Nevertheless, in the critical interval of the next two decades the externally-driven natural climate variability might possibly confuse the debate about temperature trends and impede detection of the anthropogenic climate change signal. 相似文献
123.
In the cold Canadian environment, humidity measurements can be verydifficult to conduct. In this brief communication, humidity observationstaken by two different sensors at six remote Canadian Arctic locations arecompared. The observations collected by Vaisala HMP35CF sensors displaya strong tendency toward the ice saturation point whereas dew cell instrumentsexhibit significantly lower values of relative humidity with respect to ice (RHi).Humidity data collected by HMP35CF hygrometers are therefore unreliable sincethey are subject to persistent icing that lead them to record values of RHi near 100%, irrespective of the air temperature. The high humidity bias emerges atmeteorological stations mounted with the HMP35CF probes since these instrumentsare usually neither sheltered nor heated, and are not attended to at regular intervals. Thus, great care must be taken in utilizing humidity data recorded by HMP35CF sensors across the network of climate autostations in Canada. 相似文献
124.
In South Africa attempts are being made to address the socio-spatial distortions of the apartheid era through a more equitable
distribution of resources, and the re-drawing of municipal geographical boundaries. However, boundaries are not neutral geographic
lines. Boundary changes are often associated with a redistribution of political power and resources. The aim of this paper
is to analyse the effects of the contemporary territorial and administrative restructuring on urban dynamics in South Africa.
More specifically, the focus is on how the process of territorial restructuring impacted on metropolitan areas as well as
on secondary cities and their hinterlands. Examining and elucidating the manner in which various social, economic and political
forces have manifested themselves in the process of boundary delimitation in a major metropolitan centre as well as adjacent
rural areas is a central theme of this paper. There were considerable contestations over the delimitation of new local government
boundaries. Affluent metro authorities like that in Durban were opposed to the spatial extension of their boundaries because
of the costs of the providing services and infrastructure in the deprived margins. Similarly, there was concern that incorporation
of rural areas will result in increased municipal service charges being imposed on these communities. Tensions were heightened
between urban and rural regions because traditional leaders believed that their territorial jurisdiction and authority were
being undermined. In other parts of the country, the merger of traditionally white and black fragments of secondary cities
often resulted in many black locations continuing to be marginalized. There appears to be neither the political will nor the
economic capacity to upgrade these zones of marginalized urban communities. While the Municipal Demarcation Board was largely
successful in eliminating the political geography of apartheid at a macro- scale, this paper suggests that the greater challenge
for government and policy makers is to reduce the socio-spatial and economic inequalities which appears to be still very high
and perhaps increasing.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
125.
José F. Noguera Lluís Rivero Xavier Font Andrés Navarro Francisco Martínez 《Environmental Geology》2002,41(8):898-905
126.
127.
Florent Domin Roda Bounaceur Gerard Scacchi Paul-Marie Marquaire Daniel Dessort Bernard Pradier Olivier Brevart 《Organic Geochemistry》2002,33(12)
The discovery of crude oils and condensates at ever higher temperatures casts doubt on the validity of the usual geochemical modelling approach, that uses empirical reactions and rate constants. The solution used to account for such a high thermal stability is presently to adjust the rate parameters, but the physical meaning and scientific value of such a strategy can be questioned. We have developed a mechanistic model consisting of 5200 lumped free radical reactions to describe the thermal evolution of a mixture of 52 organic species meant to represent light petroleum. Rate constants used are those available in the literature or estimated using well established thermochemistry-reactivity correlations. Chemical structures included in the model are linear, branched and cyclic hydrocarbons, hydro- and alkyl-aromatics, PAHs, and three heteroatomic compounds. Reactions include cracking and alkylation chains and inhibiting and accelerating reactions from the various reactants. This model has been applied to several mixtures with various proportions of reaction inhibitors and accelerators, and to a composition representing a light mature oil. From the results obtained, we conclude that mature oils will be stable up to 240–260 °C, depending on their composition, and that the thermal cracking of oil to gas is not possible under reasonable basin conditions. The kinetics of petroleum cracking are thus much slower than generally recognized. 相似文献
128.
Boualem Bayou Mohamed El-Messaoud Derder Bernard Henry Hamou Djellit Mohamed Amenna 《Comptes Rendus Geoscience》2002,334(2):81-87
Palaeomagnetic study, carried out in the Moscovian (~305 Ma) formation in the Edjeleh anticline, shows the existence of three magnetisation components. Two of them are probably Cenozoic and Permian remagnetisations. The third component determined by both well defined ChRMs and remagnetisation circles analysis passes the fold test. Because the folding started before or during the Stephano-Autunian, this third component is the primary magnetisation. Its palaeomagnetic pole (28.3°S, 58.9°E), close to other poles from the Saharan platform obtained from neighbouring periods but without palaeomagnetic tests, confirms the age of these last data. To cite this article: B. Bayou et al., C. R. Geoscience 334 (2002) 81–87. 相似文献
129.
Jean‐Jacques Macaire Saïda Bellemlih Christian Di‐Giovanni Patrick De Luca Lionel Visset Jacques Bernard 《地球表面变化过程与地形》2002,27(9):991-1009
In the Négron River catchment area (162 km2), surface‐sediment stores are composed of periglacial calcareous ‘grèze’ (5 × 106 t) and loess (21 × 106 t), and Holocene alluvium (12·6 × 106 t), peat (0·6 × 106 t) and colluvium (18·5 × 106 t). Seventy‐five per cent of the Holocene sediments is stored along the thalwegs. Present net sediment yield, calculated from solid discharge at the Négron outlet, is low (0·6 t km?2 a?1) due to the dominance of carbonate rocks in the catchment. Mean sediment yield during the Holocene period is 7·0 t km?2 a?1 from alluvium stores and 7·6 t km?2 a?1 from colluvium stores. Thus, the gross sediment yield during the Holocene period is about 18·7 t km?2 a?1 and the sediment delivery ratio 3 per cent. The yield considerably varies from one sub‐basin to another (3·9 to 24·5 t km?2 a?1) according to lithology: about 25 per cent and 50 per cent of initial stores of periglacial grèze and loess respectively were reworked during the Holocene period. Sediment yield has increased by a factor of 6 in the last 1000 years, due to the development of agriculture. The very high rate of sediment storage on the slope during that period (88 per cent of the yield) can be accounted for by the formation of cultivation steps (‘rideaux’). It is predicted that the current destruction of these steps will result in a sediment wave reaching the valley floors in the coming decades. Subboreal and Subatlantic sediments and pollen assemblages in the Taligny marsh, where one‐third of the alluvium is stored, show the predominant influence of human activity during these periods in the Négron catchment. Copyright © 2002 John Wiley & Sons, Ltd. 相似文献
130.
—?The aim of our study consists of analyzing potentially non-double-couple seismic events recorded at regional distances. In order to define the nature of the seismic source, a moment tensor inversion is carried out as this method is general enough not to initially constrain the source mechanism. In this paper we present an application to a seismic event induced by a mine collapse which occurred near the town of Halle in Germany. Because of its induced nature, many parameters such as the location and geometry of this seismic source are known. This information allows us to test the influence of inadequate propagation modeling on the moment tensor obtained from the inversion. Green's functions have been computed with the reflectivity method in a flat layered medium, using the European model EurID (Du et? al., 1998; Dufumier et al., 1997). From the inversion of P-wave seismograms recorded by the German Regional Seismic Network will, we obtained a source time function which can be decomposed into two subevents. The first one has a large isotropic part and a deviatoric mechanism with near vertical nodal planes. No volume change is observed for the second subevent, but a deviatoric component opposite of the first one. The addition of S-waves does not change the results of the inversion which are stable. Surface waves were not used because of their poor dispersion curves. Based on the moment tensor obtained from these inversions, the physical process at the source is compatible with a large cavity collapse. 相似文献