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11.
A biostratigraphic study carried out in the Monti d'Ocre area, Abruzzi, Central Apennines, allowed us to recognize Orbitolina (Conicorbitolina) moulladei ‘Strata 5 (1985) 1’, Praealveolina iberica Reichel and Praealveolina simplex Reichel in uppermost Albian–lower Cenomanian shelf-edge deposits of the Fossato Machè succession. These foraminifers have now been found for the first time in the Apennines of central Italy; their finding is quite important from a palaeobiogeographic viewpoint, as it contributes to the improvement of our knowledge on facies distribution in the circum-Mediterranean regions during the Cretaceous Period. In the study area, the coeval Monte Rotondo and Monte Orsello sections also crop out; these are characterized by bauxite deposits and stratigraphic gaps reflecting episodes of emergence on the carbonate platform. The Monte Rotondo and Monte Orsello sections accumulated in a platform back-reef environment; consequently, in this sector of the Monti d'Ocre area, the depositional environment shifted from a back-reef westward and southward to a shelf-edge northward, during the latest Albian–early Cenomanian. Owing to synsedimentary tectonics, the area investigated underwent differential subsidence: westward and southward, wide areas were uplifted and subjected to emergence, karstification and bauxite accumulation, whereas sedimentation continued in a shelf-edge environment in the north-eastern area. 相似文献
12.
Modelling nitrogen and oxygen isotope fractionation during denitrification in a lacustrine redox-transition zone 总被引:1,自引:0,他引:1
Moritz F. Lehmann Peter Reichert Alberto Barbieri 《Geochimica et cosmochimica acta》2003,67(14):2529-2542
The stable isotope composition (δ15N and δ18O) of nitrate was measured during Summer 1999 in the anaerobic hypolimnion of eutrophic Lake Lugano (Switzerland). Denitrification was demonstrated by a progressive nitrate depletion coupled to increasing δ15N and δ18O values for residual nitrate. Maximum δ15N and δ18O values amounted to 27.2 and 15.7‰, respectively.15N and 18O enrichment factors for denitrification (ε) were estimated using a closed-system model and a dynamic diffusion-reaction model. Using the Rayleigh equation (closed-system approach), we obtained ε values of −11.2 and −6.6‰ for nitrogen and oxygen, respectively. The average ε values derived using the diffusion-reaction model were determined to be −20.7 ± 3.8 for nitrogen and −11.0 ± 1.7 for oxygen. Both N and O isotope fractionation appeared to be lower when denitrification rates where high, possibly in association with high organic carbon availability. In addition, variations in the isotope effects may be attributed to the variable importance of sedimentary denitrification having only a small isotope effect on the water column. The combined measurement of N and O isotope ratios in nitrate revealed that coupled nitrification-denitrification in the open-water was of minor importance. This is the first study of nitrogen and oxygen isotope effects associated with microbial denitrification in a natural lake. Moreover, this study confirms the high potential of δ18O of nitrate as a valuable biogeochemical tracer in aquatic systems, complementing nitrate δ15N. 相似文献
13.
Increasing physical oceanographic evidence suggests that a regime shift, which featured increased equatoward surface winds and upwelling in the Eastern Pacific Boundary Current region, occurred following the 1997–1998 El Niño. We expect the signal of this change in biota to be stronger in euphausiids than in pelagic fishes such as Pacific hake (Merluccius productus) because lower trophic levels are more responsive to changes in upwelling and primary production. We used acoustic backscatter data from acoustic surveys in summer 1995, 1998, and 2001 to explore whether significant changes in abundance and distribution of euphausiids and fishes have occurred between 1995 and 2001. Graphical and statistical results show that the density of fish schools and euphausiid patches increased significantly south of Cape Blanco between 1995 and both 1998 and 2001. North of Cape Blanco there was no consistent change in euphausiid abundance, although both fish and euphausiid distributions in 2001 appear to be significantly higher nearshore than in the other years. Pelagic fish abundance distributions appeared more closely linked to El Niño than to regime shifts, with abundance shifted much farther north in 1998, an El Niño year, than in the other years, while 1995 and 2001 fish abundance distributions are similar to each other. The regime shift appears so far to have had a stronger effect on euphausiids than on pelagic fishes. The change in euphausiid abundance and distribution between the survey years was linked, through a conceptual model, to the relative strength of the poleward flowing California undercurrent and equatorward flowing California current and to the distribution and abundance of hake. 相似文献
14.
Barbara A. Cohen Cyrena A. Goodrich Klaus Keil 《Geochimica et cosmochimica acta》2004,68(20):4249-4266
Polymict ureilites DaG 164/165, DaG 319, DaG 665, and EET 83309 are regolith breccias composed mainly of monomict ureilite-like material, but containing ∼2 vol% of feldspathic components. We characterized 171 feldspathic clasts in these meteorites in terms of texture, mineralogy, and mineral compositions. Based on this characterization we identified three populations of clasts, each of which appears to represent a common igneous (generally basaltic) lithology and whose mafic minerals show a normal igneous fractionation trend of near-constant Fe/Mn ratio over a range of Fe/Mg ratios that extend to much higher values than those in monomict ureilites. The melts represented by these populations are unlikely to be impact melts, because the ubiquitous presence of carbon in polymict ureilites (the regolith of the ureilite parent body) implies that impact melts would have crystallized under conditions of carbon redox control and therefore have highly magnesian mafic mineral compositions with constant Mn/Mg ratio. Therefore, these melts appear to be indigenous products of igneous differentiation on the ureilite parent body (UPB), complementary to the olivine-pigeonite residues represented by the majority of monomict ureilites.The most abundant population is characterized by albitic plagioclase in association with pyroxenes, phosphates, ilmenite, silica, and incompatible-element enriched glass. Model calculations suggest that it formed by extensive fractional crystallization of the earliest melt(s) of precursor materials from which the most magnesian (shallowest) olivine-pigeonite ureilites formed. A less abundant population, characterized by labradoritic plagioclase, may have formed from melts complementary to more ferroan olivine-pigeonite ureilites, and derived from deeper in the UPB. The third population, characterized by the presence of olivine and augite, could only have formed from melts produced at greater depths in the UPB than the olivine-pigeonite ureilites. Many other feldspathic clasts cannot be positively associated with any of these three populations, because their mafic mineral compositions exhibit carbon redox control. However, they may be products of early crystallization of basaltic melts produced on the UPB, before carbon was exhausted by reduction.Partial melting on the ureilite parent body was a fractional (or incremental) process. Melts were produced early in UPB history, and most likely extracted rapidly, thus preserving primitive chemical and oxygen isotopic signatures in the residues. 相似文献
15.
16.
Characterizing the properties of dissolved organic matter isolated by XAD and C-18 solid phase extraction and ultrafiltration 总被引:1,自引:0,他引:1
17.
Kelly Addy Arthur Gold Barbara Nowicki James McKenna Mark Stolt Peter Groffman 《Estuaries and Coasts》2005,28(6):896-908
Coastal waters are severely threatened by nitrogen (N) loading from direct groundwater discharge. The subterranean estuary,
the mixing zone of fresh groundwater and sea water in a coastal aquifer, has a high potential to remove substantial N. A network
of piezometers was used to characterize the denitrification capacity and groundwater flow paths in the subterranean estuary
below a Rhode Island fringing salt marsh.15N-enriched nitrate was injected into the subterranean estuary (in situ push-pull method) to evaluate the denitrification capacity
of the saturated zone at multiple depths (125–300 cm) below different zones (upland-marsh transition zone, high marsh, and
low marsh). From the upland to low marsh, the water table became shallower, groundwater dissolved oxygen decreased, and groundwater
pH, soil organic carbon, and total root biomass increased. As groundwater approached the high and low marsh, the hydraulic
gradient increased and deep groundwater upwelled. In the warm season (groundwater temperature >12 °C), elevated groundwater
denitrification capacity within each zone was observed. The warm season low marsh groundwater denitrification capacity was
significantly higher than all other zones and depths. In the cool season (groundwater temperature <10.5 °C), elevated groundwater
denitrification capacity was only found in the low marsh. Additions of dissolved organic carbon did not alter groundwater
denitrification capacity suggesting that an alternative electron donor, possibly transported by tidal inundation from the
root zone, may be limiting. Combining flow paths with denitrification capacity and saturated porewater residence time, we
estimated that as much as 29–60 mg N could be removed from 11 of water flowing through the subterranean estuary below the
low marsh, arguing for the significance of subterranean estuaries in annual watershed scale N budgets. 相似文献
18.
19.
Gerd Rantitsch Reinhard F. Sachsenhofer Christian Hasenhüttl Barbara Russegger Thomas Rainer 《Tectonophysics》2005,411(1-4):57-72
Following Early Cretaceous nappe stacking, the Eastern Alps were affected by late-orogenic extension during the Late Cretaceous. In the eastern segment of this range, a Late Cretaceous detachment separates a very low- to low-grade metamorphic cover (Graz Paleozoic Nappe Complex, GPNC) above a low- to high-grade metamorphic basement. Synchronously, the Kainach Gosau Basin (KGB) collapsed and subsided on top of the section.Metamorphism of organic material within this section has been investigated using vitrinite reflectance data and Raman spectra of extracted carbonaceous material. In the southern part of the GPNC, vitrinite reflectance indicates a decrease in organic maturity towards the stratigraphic youngest unit. The remaining part of the GPNC is characterized by an aureole of elevated vitrinite reflectance values and Raman R2 ratios that parallels the margins of the GPNC. Vitrinite reflectance in the KGB shows a steep coalification gradient and increases significantly towards the western basin margin. The observed stratigraphic trend in the southern GPNC is a result of deep Paleozoic to Early Cretaceous burial. This maturity pattern was overprinted along the margins by advective heat and convective fluids during Late Cretaceous to Paleogene exhumation of basement rocks.During shearing, the fault zone was heated up to ca. 500 °C. This overprint is explained by a two-dimensional thermal model with a ramp-flat fault geometry and a slip rate of 1 to 1.5 cm/year during 5 Ma fault movement. The collapse basin above the detachment subsided in a thermal regime which was characterized by relaxing isotherms. 相似文献
20.
Arsenic mobility in alteration products of sulfide-rich, arsenopyrite-bearing mine wastes, Snow Lake, Manitoba, Canada 总被引:2,自引:0,他引:2
Kristin A. Salzsauler Nikolay V. Sidenko Barbara L. Sherriff 《Applied Geochemistry》2005,20(12):2303-2314
The Arsenopyrite Residue Stockpile (ARS) in Snow Lake, Manitoba contains approximately 250,000 tons of cyanide treated, refractory arsenopyrite ore concentrate. The residue was deposited between 1950 and 1959 in an open waste rock impoundment, and remained exposed until 2000, when the pile was capped with layers of waste rock and clay. During the time when the ARS was exposed to the atmosphere, arsenopyrite, pyrrhotite, pyrite and chalcopyrite were oxidized producing scorodite, jarosite and two generations of amorphous Fe sulfo-arsenates (AISA). These secondary phases attenuated some of the As released to pore water during oxidation in the upper layers of the ARS. The imposition of the cap prevented further oxidation. The secondary As minerals are not stable in the reduced environment that currently dominates the pile. Therefore, As currently is being released into the groundwater. Water in an adjacent monitoring well has concentrations of >20 mg/L total As with relative predominance of As(III). 相似文献