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701.
The photochemical instability of several related pteridines in seawater was investigated by aseptic incubation of solutions at 20–22°C under illumination from cool-white light of intensity 6 kerg cm−2 sec−1, and the chemical changes were spectrophotometrically monitored. All the pteridines showed markedly accelerated degradation from this illumination relative to their behaviour in total darkness.Pterin and lumazine were degraded very slowly with zero-order reaction kinetics, while the other pteridines photolysed rapidly (according to first-order kinetics) with decomposition rates increasing in the order dioxylumazine (2,4,6,7-tetrahydroxypteridine) < leucopterin < isoxanthopterin < xanthopterin < oxylumazine (2,4,6-trihydroxypteridine). Excepting leucopterin and dioxylumazine, the photolysis rates were attributable to the pH of seawater and not its salt content; this was also the case with oxylumazine which required the salt content of seawater for decomposition in darkness. Leucopterin and dioxylumazine (both 6,7-dihydroxylated pteridines) gave evidence of complexation with the major divalent cations (Ca2+, Mg2+) of seawater, by virtue of which their photolytic degradation rates were enhanced to magnitudes obtained in pH-10 buffer without seawater. It is proposed that such complexation produces structural forms of these pteridines analogous to their normal ionic forms at pH 10–12.The photolysis of the 6-hydroxylated pteridines (xanthopterin, oxylumazine) proceeded via intermediate formation of their corresponding 7-hydroxylated derivatives (leucopterin, dioxylumazine). 相似文献
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705.
The importance of the diet as a source of tributyltin (TBT) in Nucella lapillus was studied using [14C]tributyltin chloride. In N. lapillus provided with prelabelled mussels, Mytilus edulis, in labelled water (mean 20·5 ng/litre TBT) the rate of accumulation of total 14C was 2–3 times that in unfed animals. Owing to its degradation in the tissues of both fed and unfed animals, concentrations of [14C]TBT tended to reach a plateau after only 28 days. However, total concentrations of 14C were still increasing after 49 days. Under experimental conditions (15°C, ample food, no disturbance) the diet accounted for about 50% of the body burden of TBT in N. lapillus after 49 days exposure: concentration factors (dry tissue/water) for [14C]TBT in both male and female N. lapillus were similar at about 60 000 in fed and 30 000 in unfed animals. It is concluded that the diet may contribute less than half of the body burden of TBT found in natural populations subjected to life-long exposure. 相似文献
706.
A finite element model is set up and experimental tests are performed to help understand the behavior of a concrete canoe and subsequently optimize its design. First, the performance criteria that must be satisfied to participate at the annual ASCE/Master Builders competition are described. Then, the finite element model and the different loading cases that were studied are presented. Results from these loading cases are discussed and used to optimize the material properties as well as the thickness of the hull and the dimensions of the gunwale and reinforcing ribs. Static and dynamic experimental tests were also conducted to validate the results of the finite element analyses. The results indicate that the main stresses and strains are caused by the static load cases. The additional stresses caused during races are small. 相似文献
707.
M. Tiwari R. Ramesh B. L. K. Somayajulu A. J. T. Jull G. S. Burr 《Geo-Marine Letters》2006,26(1):23-30
Rapid shifts in past climate recorded in polar ice sheets have elicited various explanations relating to either thermohaline
circulation changes by ice-rafting or natural greenhouse gas concentrations modulated by climatic conditions in the tropics.
To compare the tropical paleoclimate record with the polar record, one must choose sediment cores from highly productive ocean
regions. Necessarily, such regions reflect the wind records in the tropics, because high productivity is associated with upwelling
driven by winds. Comparing tropical precipitation records with high-latitude records is, however, a more difficult task because
sediments recording paleoprecipitation usually have low sedimentation rates, and offer coarser resolution relative to polar
ice cores. Here, we present δ
18O data of three planktonic species of Foraminifera (a proxy for precipitation) from such a sediment core, spanning the past
35 ka for the equatorial Indian Ocean, which falls under the southwest monsoon (SWM) realm. Results show that minimum SWM
precipitation occurred at the Last Glacial Maximum, with a subsequent increase at Termination IA. During the Holocene, SWM
precipitation intensified uniformly up to the core top (∼2.2 ka b.p.), as revealed by generally decreasing δ
18O values. Variations in precipitation are consistent with climate changes recorded in polar ice sheets. Although the different resolutions of the two records preclude
a rigorous comparison, abrupt cooling/warming events appear to be accompanied by sudden reduction/enhancement in (SWM) rainfall.
Thus, mechanisms with time scales much shorter than a millennium, such as natural greenhouse warming (e.g., CH4 concentration), controlled by emissions from the tropics, could have played a major role in high-latitude climate change. 相似文献
708.
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710.
Data on the Tsushima Current and its neighboring coastal current are analyzed to examine short-term variability of the currents and storm events due to typhoons. A three current-meter array was deployed in a strong current region of the east Tsushima channel during summer in 1983 and 1984, and other two current-meter arrays in the eastern coastal area of the channel (the Sea of Genkai) in the summer and autumn in 1983. The observations of coastal current show that the kinetic energy of the subtidal current component was larger in summer than in autumn by a factor of about 2. A comparison of the wind stresses and the estimated values of mixed layer depth in the summer and autumn season suggest that this seasonal change is closely associated with that of the mixed layer depth rather than with that of the wind stress. The Tsushima Current was greatly influenced by two storm events: its speed increased by a factor of 2 in one event and decreased to nearly zero in the other. Such a large variation of mean current during the storm was observed only for the Tsushima Current and not for the coastal current, suggesting that the Tsushima Current may temporarily change its regular course as a result of a storm. 相似文献