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1.
Multiple sulfur isotope system is a powerful new tracer for atmospheric, volcanic, and biological influences on sulfur cycles in the anoxic early Earth. Here, we report high-precision quadruple sulfur isotope analyses (32S/33S/34S/36S) of barite, pyrite in barite, and sulfides in related hydrothermal and igneous rocks occurring in the ca. 3.5 Ga Dresser Formation, Western Australia. Our results indicate that observed isotopic variations are mainly controlled by mixing of mass-dependently (MD) and non-mass-dependently fractionated (non-MD) sulfur reservoirs. Based on the quadruple sulfur isotope systematics (δ34S-Δ33S-Δ36S) for these minerals, four end-member sulfur reservoirs have been recognized: (1) non-MD sulfate (δ34S = −5 ± 2‰; Δ33S = −3 ± 1‰); (2) MD sulfate (δ34S = +10 ± 3‰); (3) non-MD sulfur (δ34S > +6‰; Δ33S > +4‰); and (4) igneous MD sulfur (δ34S = Δ33S = 0‰). The first and third components show a clear non-MD signatures, thus probably represent sulfate and sulfur aerosol inputs. The MD sulfate component (2) is enriched in 34S (+10 ± 3‰) and may have originated from microbial and/or abiotic disproportionation of volcanic S or SO2. Our results reconfirm that the Dresser barites contain small amounts of pyrite depleted in 34S by 15-22‰ relative to the host barite. These barite-pyrite pairs exhibit a mass-dependent relationship of δ33S/δ34S with slope less than 0.512, which is consistent with that expected for microbial sulfate reduction and is significantly different from that of equilibrium fractionation (0.515). The barite-pyrite pairs also show up to 1‰ difference in Δ36S values and steep Δ36S/Δ33S slopes, which deviate from the main Archean array (Δ36S/Δ33S = −0.9) and are comparable to isotope effects exhibited by sulfate reducing microbes (Δ36S/Δ33S = −5 to −11). These new lines of evidence support the existence of sulfate reducers at ca. 3.5 Ga, whereas microbial sulfur disproportionation may have been more limited than recently suggested. 相似文献
2.
Masahiro Ueno 《Journal of Oceanography》1990,46(3):125-134
In each of six areas with various horizontal scale from 0.4 to 15.6 nautical miles, many surveys with vertical net hauls are made for sampling fish eggs and larvae. Though values ofC
A are widely spread in each area, the variances
2 and the meanm of catch numbers calculated from each survey follow approximately the relation from a Poisson mixture model (PMM).
相似文献
3.
Takeshi Ohno Tsuyoshi Komiya Yuichiro Ueno Takafumi Hirata Shigenori Maruyama 《Gondwana Research》2008,14(1-2):126
We measured both mass-dependent isotope fractionation of δ88Sr (88Sr/86Sr) and radiogenic isotopic variation of Sr (87Sr/86Sr) for the Neoproterozoic Doushantuo Formation that deposited as a cap carbonate immediately above the Marinoan-related Nantuo Tillite. The δ88Sr and 87Sr/86Sr compositions showed three remarkable characteristics: (1) high radiogenic 87Sr/86Sr values and gradual decrease in the 87Sr/86Sr ratios, (2) anomalously low δ88Sr values at the lower part cap carbonate, and (3) a clear correlation between 87Sr/86Sr and δ88Sr values. These isotopic signatures can be explained by assuming an extreme greenhouse condition after the Marinoan glaciation. Surface seawater, mixed with a large amount of freshwater from continental crusts with high 87Sr/86Sr and lighter δ88Sr ratios, was formed during the extreme global warming after the glacial event. High atmospheric CO2 content caused sudden precipitation of cap carbonate from the surface seawater with high 87Sr/86Sr and lighter δ88Sr ratios. Subsequently, the mixing of the underlying seawater, with unradiogenic Sr isotope compositions and normal δ88Sr ratios, probably caused gradual decrease of the 87Sr/86Sr ratios of the seawater and deposition of carbonate with normal δ88Sr ratios. The combination of 87Sr/86Sr and δ88Sr isotope systematics gives us new insights on the surface evolution after the Snowball Earth. 相似文献
4.
More than 600 specimens of ∼3.5 Ga-old hydrothermal silica dikes from the North Pole area, Pilbara craton, Western Australia, have been studied petrographically. The kerogens in 44 samples have been analyzed isotopically (C and N) and chemically (C, N, and H). The silica dikes are composed mainly of fine-grained silica (modal abundance: >97%) and are classified into two types by minor mineral assemblages: B(black)-type and G(gray)-type. The B-type silica dikes contain kerogen (0.37 to 6.72 mgC/g; average 2.44 mgC/g, n = 21) and disseminated sulfides, dominantly pyrite and Fe-poor sphalerite. In some cases, carbonate and apatite are also present. Their silica-dominated and sulfide-poor mineral assemblages suggest precipitation from low-temperature reducing hydrothermal fluid (likely 100-200°C). On the other hand, the G-type silica dikes are sulfide-free and concentrations of kerogen are relatively low (0.05 to 0.41 mgC/g; average 0.17 mgC/g, n = 13). They typically contain Fe-oxide (mainly hematite) which commonly replaces cubic pyrite and rhombic carbonate. Some G-types occur along secondary quartz veins. These textures indicate that the G-type silica dikes were formed by postdepositional metasomatism (oxidation) of the B-types, and that the B-types probably possess premetasomatic signatures. The δ13C values of kerogen in the B-types are −38.1 to −33.1‰ (average −35.9‰, n = 21), which are ∼4‰ lower than those of the G-types (−34.5 to −30.0‰; average −32.2‰, n = 19), and ∼6‰ lower than bedded chert (−31.2 to −29.4‰; average −30.5‰, n = 4). This indicates the preferential loss of 12C during the metasomatism (estimated fractionation factor: 0.9985). Considering the metasomatic effect on carbon isotopes with probably minor diagenetic and metamorphic overprints, we conclude that the original δ13C values of the kerogen in the silica dikes would have been heterogeneous (∼5‰) and at least some material had initial δ13C values of ≤ −38‰. The inferred 13C-depletions of organic carbon could have been produced by anaerobic chemoautotrophs such as methanogen, but not by aerobic photoautotrophs. This is consistent with the estimated physical and chemical condition of the hydrothermal fluid, which was probably habitable for anaerobic and thermophilic/hyperthermophilic chemoautotrophs. Alternatively, the organic matter may have been possibly produced by abiological reaction such as Fischer-Tropsch Type (FTT) synthesis under the hydrothermal condition. However, the estimated condition is inconsistent with the presence of the effective catalysts for the FTT reaction (i.e., Fe-Ni alloy, magnetite, and hematite). These lines of evidence suggest the possible existence of biosphere in the ∼3.5 Ga sub-seafloor hydrothermal system. 相似文献
5.
A study on the impact of asymmetric components around tropical cyclone center on the accuracy of bogus data and the track forecast 总被引:6,自引:0,他引:6
M. Ueno 《Meteorology and Atmospheric Physics》1995,56(1-2):125-134
Summary The Japan Meteorological Agency (JMA) has used a tropical cyclone bogus insertion procedure to produce correctlypositioned, cyclone-like vortices within the initial analyses and to track the vortices throughout the model forecasts. The TC bogus soundings are constructed from a standard axisymmetric vortices for well developed tropical cyclones based on a few manually-analyzed parameters such as storm position, central pressure and radius of gale force wind. Mainly because of such an axi-symmetric property of JMA TC bogus data, which is likely to remove the steering flow from the central core region of TC, all the JMA models have a noticeable slow-start bias error and also northward drifting blas error in TC movement. In order to investigate the impact of asymmetric wind components on the TC track forecast, an experimental analysis-forecast cycle is conducted using the JMA global spectral model, in which asymmetric components extracted from the first guess fields are added to the axisymmetric TC bogus. It is found from the experiment that both the slow-start bias error and northward bias error can be reduced by introducing the asymmetric components into the TC bogus. Besides the impact study, a statistical verification study of the bogus data was also made against real data such as sonde data and superiority of the preparation method of asymmetric components was proved.With 9 Figures 相似文献
6.
7.
Climatic Change - The objective of this study is to assess the global impact of sea level rise and to evaluate the effectiveness of adaptation. Global areas of inundation due to sea level rise are... 相似文献
8.
The impact of the Alaskan Stream (AS) eddies on the chlorophyll a (chl-a) distribution in the central subarctic North Pacific
was investigated through analysis of chl-a and altimetry data from satellite observations. Altimetry observations provided
the locations of mesoscale eddies in time and space within the maps of chlorophyll distributions. The climatological chl-a
distributions averaged in the area and time showing presence of AS eddies suggested that AS eddies contributed significantly
to the chl-a distribution in the deep-sea region of the subarctic North Pacific. The chl-a distribution was closely related
to the AS eddies regardless of whether the eddy was located in or detached from the AS. A combination of two or three AS eddies
sometimes formed high chl-a concentration belts that injected chlorophyll and coastal nutrient-rich waters southward from
the Aleutian Islands far into the deep-sea region of the subarctic North Pacific. These results indicate that chl-a distribution
in the central subarctic North Pacific was strongly impacted by AS eddies. 相似文献
9.
10.
Taku Tada Yoshinobu Tsuji Masahito Tsukamoto Yoshikazu Ueno Masayuki Kawashima Takashi Egawa Yasuhiro Yamazaki 《Pure and Applied Geophysics》1992,138(2):309-322
We carried out observations of sea-level fluctuations simultaneously at three stations on the coast of Heda Bay, Honshu, Japan, using supersonic-type water level gauges controlled by a personal computer. Analyses of the obtained data showed predominant spectral peaks at periods of 7.6, 2.0 and 1.3 minutes for all three stations. Comparison of the observed data with numerically calculated normal oscillation modes of the bay indicates that these three spectral peaks correspond to the theoretical first, third and seventh normal modes of the basin respectively, judging from the results of cross-spectral analyses. The reason for the absence of the remaining normal modes, especially of the second or the lateral first mode of the basin, is briefly considered. 相似文献
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