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111.
    
This study examines the links between 31P solidstate NMR studies of aluminum phosphate minerals and their crystallographic structures. We found that 31P isotropic chemical shift values, iso, carry little information about mineral structures. There seems to be no relation between the chemical shift anisotropy, =3311 (33>22> 11), and indicies of phosphate-tetrahedra distortion. 31P1H heteronuclear magnetic dipole interactions, on the other hand, carry important information about hydrous phosphate mineral structures, information that should prove to be quite valuable in studies of phosphate adsorbed on mineral surfaces. This interaction can be measured through a variety of qualitative and quantitative experiments. It appears that spin diffusion is so rapid that subtle differences in hydrogen-bonding environments cannot be resolved.  相似文献   
112.
We present a numerical method for solving a class of systems of partial differential equations (PDEs) that arises in modeling environmental processes undergoing advection and biogeochemical reactions. The salient feature of these PDEs is that all partial derivatives appear in linear expressions. As a result, the system can be viewed as a set of ordinary differential equations (ODEs), albeit each one along a different characteristic. The method then consists of alternating between equations and integrating each one step-wise along its own characteristic, thus creating a customized grid on which solutions are computed. Since the solutions of such PDEs are generally smoother along their characteristics, the method offers the potential of using larger time steps while maintaining accuracy and reducing numerical dispersion. The advantages in efficiency and accuracy of the proposed method are demonstrated in two illustrative examples that simulate depth-resolved reactive transport and soil carbon cycling.  相似文献   
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Overwash is a major controlling factor in the morphology of the mixing zone of coastal aquifers. Conceptual models of the mixing zone describe an interface controlled by tidal oscillations, wave run-up, and other factors; however, few describe the influence of large storm events. In August 1993, Hatteras Island, North Carolina, USA, experienced a 3-m storm surge due to Hurricane Emily. Sound-side flooding infiltrated a wellfield, causing a dramatic increase in TDS levels that persisted for more than 3 years. Two-dimensional simulations with SUTRA, the USGS finite-element model, are calibrated to the TDS breakthrough data of this storm to infer model dispersivity values. Simulations using the calibrated dispersivity values, predicted flooding levels, and 54 years of hurricane records to determine the influence of the overwash events suggest that it is rare for the mixing zone to approximate the conceptual morphology. Even during quiescent periods such as between 1965 and 1975, TDS levels do not return to theoretical levels before being elevated by a subsequent storm event. Thus, while tidal oscillations and other factors are important to mixing zone development, basic wind events and more severe storm events may have more influence and lasting effect on the morphology of the mixing zone.  相似文献   
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Lithium isotope and abundance data are reported for Apollo 15 and 17 mare basalts and the LaPaz low‐Ti mare basalt meteorites, along with lithium isotope data for carbonaceous, ordinary, and enstatite chondrites, and chondrules from the Allende CV3 meteorite. Apollo 15 low‐Ti mare basalts have lower Li contents and lower δ7Li (3.8 ± 1.2‰; all uncertainties are 2 standard deviations) than Apollo 17 high‐Ti mare basalts (δ7Li = 5.2 ± 1.2‰), with evolved LaPaz mare basalts having high Li contents, but similar low δ7Li (3.7 ± 0.5‰) to Apollo 15 mare basalts. In low‐Ti mare basalt 15555, the highest concentrations of Li occur in late‐stage tridymite (>20 ppm) and plagioclase (11 ± 3 ppm), with olivine (6.1 ± 3.8 ppm), pyroxene (4.2 ± 1.6 ppm), and ilmenite (0.8 ± 0.7 ppm) having lower Li concentrations. Values of δ7Li in low‐ and high‐Ti mare basalt sources broadly correlate negatively with 18O/16O and positively with 56Fe/54Fe (low‐Ti: δ7Li ≤4‰; δ56Fe ≤0.04‰; δ18O ≥5.7‰; high‐Ti: δ7Li >6‰; δ56Fe >0.18‰; δ18O <5.4‰). Lithium does not appear to have acted as a volatile element during planetary formation, with subequal Li contents in mare basalts compared with terrestrial, martian, or vestan basaltic rocks. Observed Li isotopic fractionations in mare basalts can potentially be explained through large‐degree, high‐temperature igneous differentiation of their source regions. Progressive magma ocean crystallization led to enrichment in Li and δ7Li in late‐stage liquids, probably as a consequence of preferential retention of 7Li and Li in the melt relative to crystallizing solids. Lithium isotopic fractionation has not been observed during extensive differentiation in terrestrial magmatic systems and may only be recognizable during extensive planetary magmatic differentiation under volatile‐poor conditions, as expected for the lunar magma ocean. Our new analyses of chondrites show that they have δ7Li ranging between ?2.5‰ and 4‰. The higher δ7Li in planetary basalts than in the compilation of chondrites (2.1 ± 1.3‰) demonstrates that differentiated planetary basalts are, on average, isotopically heavier than most chondrites.  相似文献   
116.
Observations of the vertical profile of hydrogen fluoride (HF) vapor in the stratosphere and of the vertical column amounts of HF above certain altitudes were made using a variety of spectroscopic instruments in the 1982 and 1983 Balloon Intercomparison Campaigns. Both emission instruments working in the far infrared spectral region and absorption instruments using solar occultation in the 2.5m region were employed. No systematic differences were seen in results from the two spectral regions. A mean profile from 20–45 km is presented, with uncertainties ranging from 20% to 50%. Total columns measured from ground and from 12 km are consistent with the profile if the mixing ratio for HF is small in the tropophere and low stratosphere.  相似文献   
117.
    
Water is a dominant component of volcanic clouds and has fundamental control on very fine particle deposition. Particle size characteristics of distal tephra-fall (100s km from source volcano) have a higher proportion of very fine particles compared to predictions based on single particle settling rates. In this study, sedimentological analyses of fallout from for the 18 August and 16–17 September 1992 eruptions of Crater Peak, Alaska, are combined with satellite observations, and cloud trajectory and microphysics modeling to investigate meteorological influences on particle sedimentation. Total grain size distributions of tephra fallout were reconstructed for both Crater Peak eruptions and indicate a predominance of fine particles < 125 μm. Polymodal analysis of the deposits has identified a particle subpopulation with mode ~ 15–18 μm involved in particle aggregation. Accounting for the magmatic water source only, calculated ice water content of the 3.7 hour old September 1992 Spurr cloud was ~ 4.5 × 10− 2 g m− 3 (based on an estimated cloud thickness of ~ 1000 m from trajectory modeling). Hydrometeor formation on particles in the volcanic cloud and subsequent sublimation may induce a cloud base instability that leads to rapid bulk (en masse) sedimentation of very fine particles through a mammatus-like mechanism.  相似文献   
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William T. Reach 《Icarus》2010,209(2):848-850
Interplanetary dust particles from comets and asteroids pervade the Solar System and become temporarily trapped into orbital resonances with Earth, leading to a circumsolar dust ring. Using the unique vantage point of the Spitzer Space Telescope from its Earth-trailing solar orbit, we have measured for the first time the azimuthal structure of the Earth’s resonant dust ring. There is a relative paucity of particles within 0.1 AU of the Earth, followed by an enhancement in a cloud that is centered 0.2 AU behind Earth with a width of 0.08 AU along the Earth’s orbit. The North ecliptic pole is ∼3% brighter at 8 μm wavelength when viewed from inside the enhancement. The presence of azimuthal asymmetries in debris disks around other stars is considered strong evidence for planets. By measuring the properties of the Earth’s resonant ring, we can provide “ground truth” to models for interactions of planets and debris disks, possibly leading to improved predictions for detectability of life-bearing planets. The low amplitude of the azimuthal asymmetry in the Earth’s circumsolar ring suggests significant contributions to the zodiacal light from particles that are large (>30 μm) or have large orbital eccentricity that makes capture into mean motion resonances inefficient.  相似文献   
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