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111.
112.
Reactive mass transport (RMT) simulation is a powerful numerical tool to advance our understanding of complex geochemical processes and their feedbacks in relevant subsurface systems. Thermodynamic equilibrium defines the baseline for solubility, chemical kinetics, and RMT in general. Efficient RMT simulations can be based on the operator-splitting approach, where the solver of chemical equilibria is called by the mass transport part for each control volume whose composition, temperature, or pressure has changed. Modeling of complex natural systems requires consideration of multiphase–multicomponent geochemical models that include nonideal solutions (aqueous electrolytes, fluids, gases, solid solutions, and melts). Direct Gibbs energy minimization (GEM) methods have numerous advantages for the realistic geochemical modeling of such fluid–rock systems. Substantial improvements and extensions to the revised GEM interior point method algorithm based on Karpov’s convex programming approach are described, as implemented in the GEMS3K C/C+?+ code, which is also the numerical kernel of GEM-Selektor v.3 package (http://gems.web.psi.ch). GEMS3K is presented in the context of the essential criteria of chemical plausibility, robustness of results, mass balance accuracy, numerical stability, speed, and portability to high-performance computing systems. The stand-alone GEMS3K code can treat very complex chemical systems with many nonideal solution phases accurately. It is fast, delivering chemically plausible and accurate results with the same or better mass balance precision as that of conventional speciation codes. GEMS3K is already used in several coupled RMT codes (e.g., OpenGeoSys-GEMS) capable of high-performance computing.  相似文献   
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114.
An analysis of the terrain displacement along a funicular in Switzerland was performed by satellite synthetic aperture radar interferometry using ERS-1/2 data. An initial interferometric point target analysis was performed with images acquired before 1999 and excluding all winter acquisitions with snow cover. The line-of-sight profile of the displacement rate along the funicular shows maximum values of about 1.5 cm/year, with negligible displacements near the lower and upper stations. After the spring of 1999, when displacements of several decimeters occurred because of heavy rainfall, the analysis was continued with single interferograms on the previously identified point targets. With a series of interferograms with large baselines the displacement could be analyzed in 1999 and 2000 along parts of the funicular.  相似文献   
115.
We report results of telescope polarimetric imaging of the Moon with a CCD LineScan Camera at large phase angles, near 88°. This allows measurements of the polarization degree with an absolute accuracy better than 0.3% and detection of features with polarization contrast as small as 0.1%. The measurements are carried out in two spectral bands centered near 0.65 and 0.42 μm. We suggest characterizing the lunar regolith with the parameter a(Pmax)A, where Pmax,A, and a are the degree of maximum polarization, albedo, and the parameter describing the linear regression of the correlation Pmax-A. The parameter bears significant information on the particle characteristic size and packing density of the lunar regolith. We also suggest characterizing the lunar regolith with color-ratio images obtained with a polarization filter at large phase angles. We here consider the color-ratios C||(0.65/0.42 μm) and C(0.65/0.42 μm). Using light scattering model calculations we show that the color-ratio images obtained with a polarization filter at large phase angles suggest a new tool to study the lunar surface. In particular, it turns out that the color-ratios C||(0.65/0.42 μm) and C(0.65/0.42 μm) are sensitive to somewhat different thicknesses of the surfaces of regolith particles. We consider the applicability of the Hubble Space Telescope, the Very Large Telescope (ESO), and a spacecraft on a lunar polar orbit for polarimetric observations of the lunar surface.  相似文献   
116.
The age and origin of alkaline rocks emplaced into the sediments of the rift‐related continental Lusitanian basin were investigated to constrain earliest magmatic activity occurring prior to oceanic plate formation between Iberia and Newfoundland. The U–Pb titanite ages are 146.5 ± 1.6 (2σSTERR), 145.3 ± 1.4 and 142.3 ± 1.0 Ma, and initial Pb isotopic ratios of feldspars lie at 18.418–18.978 for 206Pb/204Pb, at 15.594–15.925 for 207Pb/204Pb and at 37.105–39.216 for 208Pb/204Pb. Initial 87Sr/86Sr ratios measured in the same feldspar fractions lie at 0.705409–0.706462. This episode of magmatic activity lasting for at least 4.2 ± 2.6 Myr most likely marks a phase of maximum lithospheric thinning during which zones of weakness were created to allow deep magmas to reach the surface. Such zones are preferentially re‐activated Palaeozoic faults of the Iberian plate. The isotope data suggest that the dominant volume of alkaline magmas was generated by partial melting of the metasomatized subcontinental Iberian mantle.  相似文献   
117.
Abstract— We performed a comprehensive study of the He, Ne, and Ar isotopic abundances and of the chemical composition of bulk material and components of the H chondrites Dhajala, Bath, Cullison, Grove Mountains 98004, Nadiabondi, Ogi, and Zag, of the L chondrites Grassland, Northwest Africa 055, Pavlograd, and Ladder Creek, of the E chondrite Indarch, and of the C chondrites Hammadah al Hamra 288, Acfer 059, and Allende. We discuss a procedure and necessary assumptions for the partitioning of measured data into cosmogenic, radiogenic, implanted, and indigenous noble gas components. For stone meteorites, we derive a cosmogenic ratio 20Ne/22Ne of 0.80 ± 0.03 and a trapped solar 4He/3He ratio of 3310 ± 130 using our own and literature data. Chondrules and matrix from nine meteorites were analyzed. Data from Dhajala chondrules suggest that some of these may have experienced precompaction irradiation by cosmic rays. The other chondrules and matrix samples yield consistent cosmic‐ray exposure (CRE) ages within experimental errors. Some CRE ages of some of the investigated meteorites fall into clusters typically observed for the respective meteorite groups. Only Bath's CRE age falls on the 7 Ma double‐peak of H chondrites, while Ogi's fits the 22 Ma peak. The studied chondrules contain trapped 20Ne and 36Ar concentrations in the range of 10?6–10?9 cm3 STP/g. In most chondrules, trapped Ar is of type Q (ordinary chondritic Ar), which suggests that this component is indigenous to the chondrule precursor material. The history of the Cullison chondrite is special in several respects: large fractions of both CR‐produced 3He and of radiogenic 4He were lost during or after parent body breakup, in the latter case possibly by solar heating at small perihelion distances. Furthermore, one of the matrix samples contains constituents with a regolith history on the parent body before compaction. It also contains trapped Ne with a 20Ne/22Ne ratio of 15.5 ± 0.5, apparently fractionated solar Ne.  相似文献   
118.
Abstract— Impact glasses, tektites and some related basement rocks were analyzed for F, Cl, Br and I. The tektite and impact glasses show similar abundance patterns within the groups. Muong Nong-type tektites indicate that the halogens have been depleted in the order I > Br > Cl > F in their melt under oxidizing conditions. For Darwin Glass selective volatilization of F from the melt is a major depleting process. Cl, Br and I are lost to a lesser extent.  相似文献   
119.
With help of field data from several alpine lakes and results from culture studies [54] an attempt was made to describe the conditions necessary for the occurrence of the blue-green algaAphanizomenon flosaquae in a lake. Special attention was paid to temperature, phosphorus, nitrogen and light.   相似文献   
120.
The transformational behaviour of Hori's noncanonical perturbation theory (Hori 1971) as well as that of the theory of Krylov-Bogoliubof-Mitropolsky is studied. An integration procedure of the perturbation equations is based on the transformation properties that have been established.  相似文献   
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