Characterization of Asian Dust during ACE-Asia

ACE-Asia was a multi-national collaboration organized to investigate and understand the chemistry, radiative properties, and climatic effects of mineral dust and other aerosol particles in the East Asia/Northwest Pacific region. Studies conducted at the Gosan and Zhenbeitai surface supersites show striking variations in aerosol concentrations and properties that were affected by the occurrence and origins of the Asian dust storms, air mass pathways, and mixing during the transport. Investigations conducted on the R/V Ronald H. Brown (RHB) showed that dust had a pervasive influence on the chemical composition, size distribution, and optical properties of the aerosol. Analyses using an aerosol time-of-flight mass spectrometer on the RHB showed that most of the coarse-particle nitrate and sulfate in post-frontal air was associated with dust, and more remarkably, that competitive or exclusionary processes evidently are involved in the uptake or production of these substances. Studies conducted onboard the NCAR C-130 aircraft showed that coarse-mode dust was less absorbing and less hygroscopic than pollution aerosol and that there was little correlation in light scattering and absorption by the sub- vs. super-micrometer aerosol. Below 2 km, dust was commonly mixed with pollutants, and this had a stronger influence on the optical properties of the submicrometer particles than the coarse-mode dust; at higher altitudes, the dust was less affected by pollution. Single particle analyses of C-130 samples showed that the mixing of black carbon (BC) with dust was common, but only certain types of BC particles were aggregated. Models were used in the planning, execution and interpretative phases of ACE-Asia; and summaries of modeling results are presented to illustrate the progress being made in identifying new dust sources; in depicting the time-varying, three-dimensional structure of dust plumes; and in quantifying the production, transport, and deposition of Asian dust.     

Timing of remanent magnetization acquisition in red beds: A case study from a syn-folding sedimentary basin

We propose to explain the origin of the double trend in seismicity of the Macas swarm in the Subandean Cordillera of Cutucú (Ecuador) and characterize the corresponding active deformation of that region. For that purpose, seismological and geological data have been used, with the deployment of a temporary seismological array, with geological field observations and image processing. We found that some earthquakes are aligned on a well known NNE–SSW trend corresponding to the orientation of the nodal planes of the reverse focal mechanism of the M_w=7.0 1995 Macas earthquake as for its aftershocks. Nevertheless, many smaller events are aligned on an unexpected NNW–SSE trend inside the Cutucú Cordillera. We interpret these two orientations of the Macas swarm as linked to Subandean basement thrusts inherited from the inversion tectonics of a NNE–SSW trending Triassic–Jurassic rift, which has been uplifted and partly extruded in the Cutucú Cordillera. The present partitioning of this part of the Subandean deformation is controlled by pre-existing NNE–SSW to NNW–SSE Triassic–Jurassic normal faults that have been subsequently compressed–transpressed and reactivated into reverse faults. Major boundary faults of the rift were NNE–SSW oriented and correspond now to some main Subandean thrusts as confirms the focal mechanism of the 1995 main shock located on the eastern border (Morona frontal thrust) and the orientation of its aftershocks. In the Cutucú Cordillera, the double orientation of present swarm can be interpreted as the result of accommodation of deformation along NNW–SSE pre-existing faults inside the inverted rift system, linked to the motion of the Morona frontal NNE–SSW thrust.     

The causes of land-use and land-cover change: moving beyond the myths

Common understanding of the causes of land-use and land-cover change is dominated by simplifications which, in turn, underlie many environment-development policies. This article tracks some of the major myths on driving forces of land-cover change and proposes alternative pathways of change that are better supported by case study evidence. Cases reviewed support the conclusion that neither population nor poverty alone constitute the sole and major underlying causes of land-cover change worldwide. Rather, peoples’ responses to economic opportunities, as mediated by institutional factors, drive land-cover changes. Opportunities and constraints for new land uses are created by local as well as national markets and policies. Global forces become the main determinants of land-use change, as they amplify or attenuate local factors.     

Numerical Study On Cloud Lines Over An Urban Street In Tokyo

`Kanpachi Street Cloud (KSC)' is an unusual small-scalecumulus cloud line visible during calm summer conditions over a major street in the Tokyo metropolitanarea. In order to understand the mechanism leading to the formation of this cloud line,numerical simulations have been performed using the Regional Atmospheric Modelling System.The general characteristics of the simulated KSC agree well with observations. On alarge-scale view, the KSC can be characterized as a cumulus cloud line generated at the convergenceline of two sea breezes on the western side of Tokyo Bay, while on the microscale view, it resemblesBenard-type thermal convection modified longitudinally by wind shear.The location of the convergence line leading to the KSCformation coincides withthe Kanpachi street location, although the street itself does notmake any direct effect on the KSC formation. Additional numerical experiments were performed toidentify causes of the KSC formation in accordance with urbanization, by changing anthropogenicheat impact, land-cover and grid resolution.They confirmed that the formation of the KSC requirestwo meteorological processes at the same time:(1) the convergence of two sea breezes – the localsouth-eastern sea breeze from Tokyo Bay andan extended southern sea breeze from thePacific Ocean, respectively; (2) Forcing due to an urban heat island. It is shown that urbanization couldchange the intensity and position of the KSC through enhancement of local upward motions and changesin the near-surface horizontal pressure gradient between urban and sub-urban areas. Further,fine horizontal grid resolution is needed to be able to resolve these local thermal convection issues.     

Role of anthropogenic volatile organic compounds and nitrogen oxides as ozone precursors in the wintertime over East Asia

As an exercise in model sensitivity, the Models-3 Community Multiscale Air Quality (CMAQ) modeling system with meteorological fields from the Regional Atmospheric Modeling System (RAMS) was applied to study the response of photochemical oxidants to systematic increases in anthropogenic volatile organic compounds (VOC) and nitrogen oxides (NO_x) emissions in January 1997 over East Asia. Three simulations-one base case and two sensitivity simulations were carried out. Two sensitivity simulations were performed by assuming a 35% separate increase in anthropogenic VOC and NO_x emissions comparing with the base case. Biogenic VOC emissions were held constant across the sensitivity simulations. To evaluate the model performance, ozone mixing ratios (O₃) from the base case simulation were compared with surface observations at five remote sites in Japan, and it was found that the model reproduces most of the important features in the observations. Monthly average O₃ concentrations in the daytime were examined to gain an understanding of how the increase in anthropogenic emissions affected the overall chemical system for each sensitivity simulation.     

Aeolian dust experiment on climate impact: An overview of Japan–China joint project ADEC

The Aeolian Dust Experiment on Climate Impact (ADEC) was initiated in April 2000 as a joint five-year Japan–China project. The goal was to understand the impact of aeolian dust on climate via radiative forcing (RF). Field experiments and numerical simulations were conducted from the source regions in northwestern China to the downwind region in Japan in order to understand wind erosion processes temporal and spatial distribution of dust during their long-range transportation chemical, physical, and optical properties of dust and the direct effect of radiative forcing due to dust. For this, three intensive observation periods (IOP) were conducted from April 2002 to April 2004.The in situ and network observation results are summarized as follows: (1) In situ observations of the wind erosion process revealed that the vertical profile of moving sand has a clear size dependency with height and saltation flux and that threshold wind velocity is dependent on soil moisture. Results also demonstrated that saltation flux is strongly dependent on the parent soil size distribution of the desert surface. (2) Both lidar observations and model simulations revealed a multiple dust layer in East Asia. A numerical simulation of a chemical transport model, CFORS, illustrated the elevated dust layer from the Taklimakan Desert and the lower dust layer from the Gobi Desert. The global-scale dust model, MASINGAR, also simulated the dust layer in the middle to upper free troposphere in East Asia, which originated from North Africa and the Middle East during a dust storm in March 2003. Raman lidar observations at Tsukuba, Japan, found the ice cloud associated with the dust layer at an altitude of 6 to 9 km. Analysis from lidar and the radio-sonde observation suggested that the Asian dust acted as ice nuclei at the ice-saturated region. These results suggest the importance of dust's climate impact via the indirect effect of radiative forcing due to the activation of dust into ice nuclei. (3) Studies on the aerosol concentration indicated that size distributions of aerosols in downwind regions have bimodal peaks. One peak was in the submicron range and the other in the supermicron range. The main soluble components of the supermicron peak were Na⁺, Ca²⁺, NO₃⁻, and Cl⁻. In the downwind region in Japan, the dust, sea salt, and a mixture of the two were found to be dominant in coarse particles in the mixed boundary layer. (4) Observation of the optical properties of dust by sky-radiometer, particle shoot absorption photometer (PSAP), and Nephelometer indicated that unpolluted dust at source region has a weaker absorption than originally believed.A sensitivity experiment of direct RF by dust indicated that single scattering albedo is the most important of the optical properties of dust and that the sensitivity of instantaneous RF in the shortwave region at the top of the atmosphere to the refractive index strongly depends on surface albedo. A global scale dust model, MASINGAR, was used for evaluation of direct RF due to dust. The results indicated the global mean RF at the top and the bottom of the atmosphere were − 0.46 and − 2.13 W m^− 2 with cloud and were almost half of the RF with cloud-free condition.     

Long-term variations of available solar radiation on seasonal timescales in 1955–2006 at Tartu-Tõravere Meteorological Station, Estonia

The time series of the daily sums of global and direct irradiance recorded at Tartu-Tõravere Meteorological Station site (58°16′N, 26°28′E, 70 m a.s.l.) in 1955–2006 have been analyzed in seasonal timescales. The average daily ratio G/G _clear of available global irradiance to its local climatic clear-sky value in the summer half-year corresponds to 65.5%, while that of the direct irradiance on the horizontal surface I′/I′ _clear was 41% of the climatic clear-sky value. In the case of dry Rayleigh atmosphere as a reference, these ratios are 53.5% and 28%, respectively. The time series of the summer season totals reveal a longer interval of reduced values in 1976–1993 as well as two periods of frequent sunny summers in 1967–1975 and since 1994. The probability density distribution of the summer season totals during the observed period is strongly asymmetric; in spring, however, it is close to the normal distribution. In winter, there is a moderate negative correlation between the G/G _clear and the North Atlantic Oscillation as well as the Arctic Oscillation indices.     

Observation of lake breeze penetration and subsequent development of the thermal internal boundary layer for the Nanticoke II Shoreline Diffusion Experiment

The turbulent structure of the lake breeze penetration and subsequent development of the thermal internal boundary layer (TIBL) was observed using a kytoon-mounted ultrasonic anemometer-thermometer. The lake breeze penetrated with an upward rolling motion associated with the upward flow near the lake breeze front. After the lake breeze front passed, the behaviors of the velocity and temperature at the top of the lake breeze layer were similar to those found in convective boundary layers (CBL). Comparing _gq/_*, _u /w _* and _w /w _* between the present observation of TIBL development after the passage of the lake breeze front and CBL data from the literature, the /_* values showed reasonable agreement; however, _u /w _* and _w /W_* had smaller values in the TIBL than in the CBL at higher altitudes. This is due to the differences in the mean velocity profiles. While the CBL has a uniform velocity profile, the TIBL has a peak at lower elevation due to the lake breeze penetration; the velocity then decreases with height.Present address: The Institute of Behavioral Science, 1-35-7 Yoyogi, Tokyo 151, Japan.     

Numerical modeling of the nocturnal urban boundary layer

A numerical case study with a second-order turbulence closure model is proposed to study the role of urban canopy layer (UCL) for the formation of the nocturnal urban boundary layer (UBL). The turbulent diffusion coefficient was determined from an algebraic stress model. The concept of urban building surface area density is proposed to represent the UCL. Calculated results were also compared with field observation data. The height of the elevated inversion above an urban center was simulated and found to be approximately twice the average building height. The turbulent kinetic energy k, energy dissipation rate , and turbulence intensities u ² and w ² increase rapidly at the upwind edge of the urban area. The Reynolds stress uw displayed a nearly uniform profile inside the UBL, and the vertical sensible heat flux w had a negative value at the inversion base height. This indicates that the downward transport of sensible heat from the inversion base may play an important role in the formation of the nocturnal UBL.