On the interaction between cumulus clouds and the larger-scale environment

This article briefly reviews the published and unpublished work carried out by the author and his colleagues during the past few years on the interaction between cumulus clouds and the larger-scale environment. This work has been directed toward: (a) identifying favorable large-scale environments for generation of an organized meso disturbance and (b) investigating the feedback effect of a cumulus ensemble on the large-scale environment. Feedback includes the redistribution of heat and moisture by cumulus clouds in the large-scale atmosphere once a large number of different sized cumuli have developed. Both cumulus clouds over the continental United States and over the tropical oceans are considered in this article and some differences between them are discussed. A number of unsolved questions which the author feels are of importance are raised.     

High molecular weight organic matter in seawater

The presence and nature of high molecular weight organic matter in seawater was critically reviewed and its biogeochemical cycle was discussed.Organic matter that passes through a filter of 0.5–1 μm pore size is called dissolved and that which does not pass through such a filter is defined as particulate. The size of colloidal particles ranges from 0.001 to 1 μm, and therefore, they are included in the dissolved fraction having high molecular weight.High molecular weight organic matter greater than 100,000 molecular weight was found in the seawater of Tokyo Bay. The values ranged from 0.1 to 1.5 mgC/l, and accounted for 8–45% of the total dissolved organic matter.Decomposition experiments on dissolved organic matter showed that macromolecular organic matter is refractory to bacterial attack. However, macromolecular organic materials tend to aggregate or adsorb on small particles to a sufficient size for precipitation. Organic aggregates thus formed sink to the bottom of the sea and bioelements included in them are removed from water column. High molecular weight organic materials are, therefore, considered to play an important role in transportation and distribution of matter in seawater.In order to elucidate the chemical and biological properties of macromolecular organic matter, concentration and isolation of this material are important, using methods such as adsorption on organic adsorbents or ultrafiltration.     

N2O Production, Nitrification and Denitrification in an Estuarine Sediment

The mechanisms regulating N₂O production in an estuarine sediment (Tama Estuary, Japan) were studied by comparing the change in N₂O production with those in nitrification and denitrification using an experimental continuous-flow sediment–water system with¹⁵N tracer (¹⁵N-NO−3 addition). From Feburary to May, both nitrification and denitrification in the sediment increased (246 to 716 μmol N m⁻² h⁻¹and 214 to 1260 μmol N m⁻² h⁻¹, respectively), while benthic N₂O evolution decreased slightly (1560 to 1250 nmol N m⁻² h⁻¹). Apparent diffusion coefficients of inorganic nitrogen compounds and O₂at the sediment–water interface, calculated from the respective concentration gradients and benthic fluxes, were close to the molecular diffusion coefficients (0·68–2·0 times) in February. However, they increased to 8·8–52 times in May except for that of NO−2, suggesting that the enhanced NO−3 and O₂supply from the overlying water by benthic irrigation likely stimulated nitrification and denitrification. Since the progress of anoxic condition by the rise of temperature from February to May (9 to 16 °C) presumably accelerated N₂O production through nitrification, the observed decrease in sedimentary N₂O production seems to be attributed to the decrease in N₂O production/occurrence of its consumption by denitrification. In addition to the activities of both nitrification and denitrification, the change in N₂O metabolism during denitrification by the balance between total demand of the electron acceptor and supply of NO−3+NO−2 can be an important factor regulating N₂O production in nearshore sediments.     

Experiment and validation of numerical simulation of coupled thermal,hydraulic and mechanical behaviour in the engineered buffer materials

Evaluation of the coupled heat transfer, water flow and stress changes in the engineered clay barrier is an important issue in the performance assessment of the high‐level radioactive waste disposal. To demonstrate the function of the engineered barrier system, the large‐scale experiment is conducted, which is called Big Bentonite facility (BIG‐BEN). The facility consists of an electric heater surrounded by glass beads, carbon steel overpack, buffer material and man‐made rock. The buffer is a mixture of bentonite and sand. The heater is operated at 0·8 kW. Water is injected from the interface between the buffer and the man‐made rocks at the pressure of 0·05 MPa. The duration of the experiment is 20 months. The change in temperature and swelling pressure are continuously monitored and gravimetric water content is measured by sampling. The coupled thermal, hydraulic and mechanical processes are simulated with a finite element code THAMES, which can simulate the fully coupled phenomena in the saturated and unsaturated clay under anisothermal condition. To examine the validity of the code, all the parameters used in the model are evaluated from the other laboratory tests. The simulated results are compared with the measured ones without calibration of the parameter values using the results from the BIG‐BEN experiment. It can be concluded that the changes in temperature and gravimetric water content within the buffer can be simulated reasonably well and that the mechanical effect such as swelling pressure is difficult to realize. Copyright © 2000 John Wiley & Sons, Ltd.     

Temperature scaling pattern dependence on representative concentration pathway emission scenarios A letter

To preserve consistency among developed emission scenarios, the scenarios used in climate modeling, and the climate scenarios available for impact research, the pattern scaling technique is useful technique. The basic assumption of pattern scaling is that the spatial response pattern per 1 K increase in the global mean surface air temperature (SAT) (scaling pattern) is the same among emission scenarios, but this assumption requires further validation. We therefore investigated the dependence of the scaling pattern of the annual mean SAT on GHGs emission scenarios of representative concentration pathways (RCP) and the causes of that dependence using the Model for Interdisciplinary research on Climate 5 developed by Japanese research community. In particular, we focused on the relationships of the dependency with effects of aerosols and Atlantic meridional overturning circulation. We found significant dependencies of the scaling pattern on emission scenarios at middle and high latitudes of the Northern Hemisphere, with differences of >15 % over parts of East Asia, North America, and Europe. Impact researchers should take into account those dependencies that seriously affect their research. The mid-latitude dependence is caused by differences in sulfate aerosol emissions per 1 K increase in the global mean SAT, and the high-latitude dependence is mainly caused by nonlinear responses of sea ice and ocean heat transport to global warming. Long-term trends in land-use and land-cover changes did not significantly affect the scaling pattern of annual mean SAT, but they might have an effect at different timescales.     

Model development and calibration for the coupled thermal,hydraulic and mechanical phenomena of the bentonite

In the international DECOVALEX-THMC project, five research teams study the influence of thermal-hydro-mechanical (THM) coupling on the safety of a hypothetical geological repository for spent fuel. In order to improve the analyses, the teams calibrated their bentonite models with results from laboratory experiments, including swelling pressure tests, water uptake tests, thermally gradient tests, and the CEA mock-up THM experiment. This paper describes the mathematical models used by the teams, and compares the results of their calibrations with the experimental data.     

Emission scenario dependencies in climate change assessments of the hydrological cycle

Anthropogenic global warming will lead to changes in the global hydrological cycle. The uncertainty in precipitation sensitivity per 1 K of global warming across coupled atmosphere-ocean general circulation models (AOGCMs) has been actively examined. On the other hand, the uncertainty in precipitation sensitivity in different emission scenarios of greenhouse gases (GHGs) and aerosols has received little attention. Here we show a robust emission-scenario dependency (ESD); smaller global precipitation sensitivities occur in higher GHG and aerosol emission scenarios. Although previous studies have applied this ESD to the multi-AOGCM mean, our surprising finding is that current AOGCMs all have the common ESD in the same direction. Different aerosol emissions lead to this ESD. The implications of the ESD of precipitation sensitivity extend far beyond climate analyses. As we show, the ESD potentially propagates into considerable biases in impact assessments of the hydrological cycle via a widely used technique, so-called pattern scaling. Since pattern scaling is essential to conducting parallel analyses across climate, impact, adaptation and mitigation scenarios in the next report from the Intergovernmental Panel on Climate Change, more attention should be paid to the ESD of precipitation sensitivity.     

Thermal diffusivity of silica glass at pressures up to 9 GPa

The thermal diffusivity of silica glass was measured at pressures up to 9 GPa and temperatures up to 1200 K. The measurements involve adopting the Ångström method to a cylindrical geometry in a uniaxial split-sphere apparatus. This method can be used to determine thermal diffusivity in samples with dominant conductive heat transfer. The thermal diffusivity of silica glass has a negative first pressure derivative but a positive second pressure derivative. Although the elastic moduli have minima near 3 GPa, the thermal diffusivity does not has minimum up to 9 GPa, which cannot be explained by the model of Kittel (1949). The negative pressure derivative of thermal diffusivity is a feature probably unique in silica glass, and its magnitude should decrease with the addition of Na₂O.     

The population in the background of open clusters: tracer of the Norma-Cygnus arm

We present colour–magnitude diagrams of open clusters, located in the range  112° < l < 252°  , manifesting stellar populations in the background of clusters. Some of the populations are found to be located beyond the Perseus arm and may be the part of the Norma-Cygnus (outer) arm. The outer arm seems to be continued from   l ∼ 120°  to ∼235°. The background populations follow the downward warp of the Galactic plane around   l ∼ 240°  .     

Vertical profiles of nitrous oxide and dissolved oxygen in marine sediments

The whole core squeezing method was used to simultaneously obtain profiles of nitrous oxide (N₂O), nitrogenous nutrients, and dissolved oxygen in sediments of Koaziro Bay, Japan (coastal water), the East China Sea (marginal sea), and the central Pacific Ocean (open ocean). In the spring of Koaziro Bay, subsurface peaks of interstitial N₂O (0.5–3.5 cm depth) were observed, at which concentrations were higher than in the overlying water. This was also true for nitrate (NO₃⁻) and nitrite (NO₂⁻) profiles, suggesting that the transport of oxic overlying water to the depth through faunal burrows induced in situ N₂O production depending on nitrification. In the summer of Koaziro Bay, sediment concentrations of N₂O, NO₃⁻ and NO₂⁻ were lower than in the overlying water. In most East China Sea sediments, both N₂O and NO₃⁻ decreased sharply in the top 0.5–2 cm oxic layer (oxygen: 15–130 μM), which may have indicated N₂O and NO₃⁻ consumption by denitrification at anoxic microsites. N₂O peaks at subsurface depth (0.5–6.5 cm) implied in situ production of N₂O and/or its supply from the overlying water through faunal burrows. However, the occurrence of the latter process was not confirmed by the profiles of other constituents. In the central Pacific Ocean, the accumulation of N₂O and NO₃⁻ in the sediments likely resulted from nitrification. Nitrous oxide fluxes from the sediments, calculated using its gradient at the sediment–water interface and the molecular diffusion coefficient, were −45 to 6.9 nmolN m⁻² h⁻¹ in Koaziro Bay in the spring, −29 to −21 nmolN m⁻² h⁻¹ in the summer, −46 to 37 nmolN m⁻² h⁻¹ in the East China Sea, 0.17 to 0.23 nmolN m⁻² h⁻¹ in the equatorial Pacific, and <±0.2 nmolN m⁻² h⁻¹ in the subtropical North Pacific, respectively.