影响气体和粒子干沉积的敏感因子分析

建立了一个模拟气体和气溶胶粒子在各种不同条件下干沉积的数学模式，用以研究了影响气体和粒子干沉积的敏感因子，从而进一步揭示物质干沉积和特征和规律，结果表明：下垫面的性质，气体本身与沉积表面的溶混性和表面的潮温程度是影响气体干沉积的重要因子；对粒子干沉积起主导作用的有粒子直径，平均风速、大气稳定状况和沉积表面的粗糙度。     

Impact of Tropospheric Ozone on Summer Climate in China

The spatial distribution, radiative forcing, and climatic effects of tropospheric ozone in China during summer were investigated by using the regional climate model RegCM4. The results revealed that the tropospheric ozone column concentration was high in East China, Central China, North China, and the Sichuan basin during summer. The increase in tropospheric ozone levels since the industrialization era produced clear-sky shortwave and clear-sky longwave radiative forcing of 0.18 and 0.71 W m^–2, respectively, which increased the average surface air temperature by 0.06 K and the average precipitation by 0.22 mm day^–1 over eastern China during summer. In addition, tropospheric ozone increased the land–sea thermal contrast, leading to an enhancement of East Asian summer monsoon circulation over southern China and a weakening over northern China. The notable increase in surface air temperature in northwestern China, East China, and North China could be attributed to the absorption of longwave radiation by ozone, negative cloud amount anomaly, and corresponding positive shortwave radiation anomaly. There was a substantial increase in precipitation in the middle and lower reaches of the Yangtze River. It was related to the enhanced upward motion and the increased water vapor brought by strengthened southerly winds in the lower troposphere.     

Investigation on the direct radiative effect of fossil fuel black-carbon aerosol over China

In China, due to lack of countrywide monitoring and coarse emission inventory of black carbon (BC) in early years, there are large uncertainties as to the estimations of its loading, direct radiative forcing (DRF) and climate response. Here, we apply an up-to-date emission inventory of BC in 2006 to investigate its loading, optical depth (AOD) at 550?nm and DRF using the coupled Regional Climate Chemistry Modeling System (RegCCMS). A state of the art air quality model (WRF/Chem) is also used to access surface BC concentration. Simulated surface concentrations of BC from these two models were compared with observations, while the AOD was compared with the results both from the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model and from satellite and ground-based simulations. Results show that RegCCMS presented similar patterns and levels of annual mean-surface BC concentration to those of WRF/Chem. The regional distributions and monthly variations of RegCCMS BC were reproduced well in comparison to observations. Simulated pattern of AODs are consistent to but lower than those from satellite (Omi-0.25°) and AERONET simulations. Annual mean DRFs mainly distribute in the area with high BC loadings, with regional mean of 0.75?W?m^?C2 and predicted global mean of 0.343?W?m^?C2. In general, the results are about 0.4?C5 times for regional column burden, about 2 times as high for regional mean DRFs, about 1.3?C1.8 times for global mean DRFs and about 3?C4 times for AOD at 550?nm as compared to those in previous studies in China. These increasing DRFs of BC imply that its warming effect and climate response should be stronger and the DRF of total aerosols should be weaker (less negative).     

Study on conventional atmospheric dispersion models in china, america and canada

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2009年秋季南京地区一次持续性灰霾天气过程研究

2009年10月14—27日,南京地区发生了一次持续性的灰霾天气过程。利用气象观测资料和污染物浓度监测资料,结合焚烧点监测、后向气流轨迹模拟,分析了颗粒物和气态污染物的浓度演变特征、气象要素特征及产生持续灰霾天气的可能原因。研究表明,该次过程中绝大部分时间能见度低于10 km,空气污染指数最大时达到195。地面PM2.5质量浓度有显著增长,在26日达到最大值为0.782 mg/m3。NO2质量浓度日均值在24日和27日超过了环境空气质量二级标准,其含量分别为0.094和0.099 mg/m3,对应NOx质量浓度分别为0.105和0.108 mg/m3。SO2质量浓度在22日达到峰值,最大值为0.161 mg/m3,平均值为0.083 mg/m3,低于环境空气质量二级标准。分析显示:近半个月内南京地区天气形势稳定,处于持续温度偏高、干燥无雨的状态,非常有利于灰霾天气的发生。卫星监测发现24、25、26日江淮之间中部均有火点,其中24日有50个着火点,25日增加为85个,26日减少为38个,表明有秸秆焚烧现象存在。从后向气流轨迹分析来看,在秸秆焚烧最为严重的3 d内,南京地区主要受到来自东到东北方向气流的影响,有利于秸秆焚烧形成的污染物经气流输送影响南京,造成严重灰霾天气。     

不同云滴数浓度参数化方案对硝酸盐气溶胶 第一间接效应影响的比较研究

在区域气候化学模式系统（RegCCMS）中,分别采用Hegg、Hansen、Ghan、Jones等4种云滴数浓度参数化方案,模拟研究了2003年10月硝酸盐气溶胶的浓度分布和第一间接气候效应,并对不同方案进行比较。结果表明,不同方案模拟的硝酸盐气溶胶分布大体上一致,主要集中在河南、山东、河北、四川等地,地面浓度最大值达18 μg/m3。Hegg、Hansen、Ghan、Jones等 4种云滴数浓度参数化方案计算得到的由硝酸盐气溶胶所造成的第一间接辐射强迫全国平均值分别为-148、-205、-161和-140 W/m2。4种方案模拟的硝酸盐气溶胶间接效应都表现为近地面气温下降,降水减少,其中Hansen方案的间接效应最强,Ghan、Hegg方案次之,Jones方案最弱。     

臭氧变化及其气候效应的研究进展

综述了近２０年来臭氧变化的规律和机制及其气候效应等领域的研究进展,指出对流层臭氧（主要在北半球）增加、平流层臭氧减少和臭氧总量减少是全球臭氧的变化趋势,原因主要是人类活动导致的ＮＯｘ、ＮＭＨＣ、ＣＯ、ＣＨ４等对流层臭氧前体物的增加和ＮＯｘ、Ｈ２Ｏ、Ｎ２Ｏ、ＣＦＣｓ等平流层臭氧损耗物质的增加。臭氧变化引起的气候效应表现在对流层臭氧的增加将带来地表和低层大气的升温,平流层臭氧的减少则可能导致地表和低层大气的升温或降温。将全球或区域气候模式和大气化学模式进行完全耦合来研究臭氧变化的气候效应是一种十分有效的手段,具有广阔的应用前景。