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81.
Moore Emerson Skinner Meixner Arens & Jernigan 《Monthly notices of the Royal Astronomical Society》1998,299(4):1209-1214
We present arcsec-resolution images at 8.2, 10.0 and 11.3 μm of the unusual young object WL 16 in Ophiuchus, which has an extended envelope of fluorescing hydrocarbon molecules. To the limit of achieved sensitivity, the faint 10.0-μm continuum has a surface-brightness distribution that is not distinguishable from those at 8.2 and 11.3 μm, where the luminosity is known to be dominated by the polycyclic aromatic hydrocarbon (PAH) emission features. We conclude that the 10-μm continuum either arises from non-equilibrium heating of small dust grains that are well mixed with the hydrocarbons or is quasi-continuous emission from the PAH particles themselves, rather than thermal equilibrium emission from macroscopic dust grains, and that there is no significant silicate absorption variation across the source. The extended hydrocarbon emission may trace a flattened, equatorial distribution of circumstellar material or arise in bipolar lobes. The former case is slightly favoured, based on currently available data, and would imply that WL 16 is a relatively evolved Herbig Ae star, the equatorial plane of which has been almost cleared of normal dust, leaving only fluorescing hydrocarbons and larger coagulated particles as a possibly transient fossil of the original circumstellar disc. 相似文献
82.
Dhanpat Rai R.G. Strickert D.A. Moore R.J. Serne 《Geochimica et cosmochimica acta》1981,45(11):2257-2265
Americium-241 concentrations in solutions contacting contaminated sediments for up to 2 yr were measured as a function of pH. Steady-state concentrations were reached within a few days. The solubility-limited Am concentration was found to decrease approximately 10-fold with one unit increase in pH. The log equilibrium constant for the solubility of Am(soil) solid was found to be ?4.12. The predictions based upon thermodynamic data suggest that Am(aq complex)+ is likely to be Am(OH)2+. Although the chemical formula of Am(soil) was not determined, it does not appear to be Am(OH)3(a).Published data on sorption coefficients of Am by different rocks, soils, and minerals were critically evaluated. Final Am solution concentrations calculated from the sorption coefficients of a variety of earth materials with several solutions agreed well with the concentrations predicted from the solubility of Am(soil) solid, indicating that the sorption coefficient data are controlled by Am precipitation. 相似文献
83.
Willard S. Moore Kenneth W. Bruland Jacqueline Michel 《Earth and Planetary Science Letters》1981,53(3):391-399
Samples from the MANOP Santa Barbara Basin sediment trap intercomparison were analyzed for the isotopes of uranium, thorium, radium, lead, and polonium. All of the traps showed approximately the same compositions and isotopic ratios, indicating that they trapped similar materials. The234Th flux via falling particles was very close to the flux predicted from the production and scavenging rates of234Th from the water column. The210Pb content of the trapped particles and the surface sediments were the same, however, the measured flux of210Pb was seven times greater than the predicted flux. Predicted and measured fluxes of228Th and210Po were similarly out of balance. To explain this apparent inconsistency, we suggest (as others have done) that the Santa Barbara Basin is an area where scavenging from the water column is intensified and where sediments deposited initially on the margins may be physically remobilized on a short time scale. These two effects increase the apparent area from which the basin derives the longer-lived isotopes but does not increase significantly the supply of the short-lived234Th. 相似文献
84.
Emergent Pleistocene sea level indicators in the northern Bahamas include: a bioerosional notch at +5.3 to 5.9 m; sea caves, notches, and marine terraces at about +4.3 m; and lithified coral rubble and reef deposits between 0 and 3 m. Thorium 230 dates of the fossil corals, which were deposited as these features were being produced, span the age range from 100 to 145 thousand years BP with a majority falling between 115 and 130 thousand years BP. The notch at about +5.6 m is interpreted to be the product of a sea level stand 125 thousand years BP, while the features at +4.3 m are believed to be formed sometime later as sea level fell from the higher position. Part of the age span is inherent in the dating technique and possible sample alteration. Another cause of the spread may be mixing of corals of different ages into a single deposit. 相似文献
85.
R.M. Moore J.D. Burton P.J.LeB. Williams M.L. Young 《Geochimica et cosmochimica acta》1979,43(6):919-926
Fractionation by ultra-filtration of the dissolved organic material (DOM) in the River Beaulieu, with typical concentrations of dissolved organic carbon (DOC) of 7–8 mg C/l, showed it to be mainly in the nominal molecular weight range of 103–105, with 16–23% of the total DOC in the fraction > 105. The molecular weight distribution of DOM in the more alkaline River Test (average DOC, 2 mg C/l) was similar. In the River Beaulieu water, containing 136–314 βg Fe/l in ‘dissolved’ forms, 90% or more of this Fe was in the nominal molecular weight fraction > 105. Experiments showed that DOM of nominal molecular weight <105 could stabilize Fe(III) in ‘dissolved’ forms. The concentrations of ‘dissolved’ Fe in the river water probably reflect the presence of colloidal Fe stabilized by organic material and this process may influence the apparent molecular weight of the DOM. Dissolved. Mn (100–136 βg/l) in the River Beaulieu was mainly in true solution, probably as Mn(II), with some 30% in forms of molecular weight greater than ca 104.During mi xing in the Beaulieu Estuary, DOC and dissolved Mn behave essentially conservatively. This contrasts with the removal of a large fraction of the dissolved Fe (Holliday and LISS, 1976, Est. Coastal Mar. Sci. 4, 349–353). Concentrations of lattice-held Fe and Mn in suspended particulate material were essentially uniform in the estuary, at 3.2 and 0.012%, respectively, whereas the non-lattice held fractions decreased markedly with increase in salinity. For Mn the decrease was linear and could be most simply accounted for by the physical mixing of riverborne and marine participates, although the possibility that some desorption occurs is not excluded. The non-linear decrease in the concentration of non-lattice held Fe in particulates reflected the more complex situation in which physical mixing is accompanied by removal of material from the ‘dissolved’ fraction. 相似文献
86.
David F. Reid Willard S. Moore William M. Sackett 《Earth and Planetary Science Letters》1979,43(2):227-236
The Mn-fiber technique for extracting radium from seawater has proved useful for studying the marine geochemistry of228Ra. In the Gulf of Mexico, this technique was used to measure the surface and near-surface distribution of226Ra and228Ra. The observed surface distribution of228Ra, and particularly the radium activity ratio (228/226) can be explained by known circulation patterns, or, when local surface currents are not well understood, may provide insight into their general characteristics.The radium activity ratio has increased from 0.5 in 1968 to 0.7 in 1973 in the surface Gulf of Mexico. This observed increase cannot be attributed to known anthropogenic or natural source perturbations within the Caribbean Sea-Gulf of Mexico system. Possible causes include a change in the residence time for near-surface water, or variations in the relative dominance of the two sources for water entering the eastern Caribbean; the North Equatorial Current and the Guiana Current.The temporal distribution of228Ra is unstable and naturally variable over a time period less than or equal to five years in the Gulf of Mexico and by extrapolation, the Caribbean Sea. Therefore, its usefulness in calculations of eddy diffusion coefficients for these regions is greatly diminished. 相似文献
87.
Willard S. Moore Herbert W. Feely Yuan-Hui Li 《Earth and Planetary Science Letters》1980,49(2):329-340
Measurements of the228Ra/226Ra activity ratio in the waters of the Greenland, Norwegian and Labrador Seas and Baffin Bay reveal strong horizontal gradients in the surface waters. The coastal waters are dominated by228Ra injection from nearshore sediments. There is an inverse correlation between the228Ra/226Ra activity ratio and salinity in the 30–36‰ salinity range. Vertical profiles indicate that the228Ra/226Ra activity ratio is also strongly coupled toσθ except for some regions where228Ra is being injected into higher density water as these isopycnals intersect coastal areas. We use these measurements in the area of formation of North Atlantic Deep Water to estimate that this water mass forms with a228Ra/226Ra activity ratio of 0.10. 相似文献
88.
Concentrations of dissolved226Ra in Winyah Bay, South Carolina, and in the adjacent Atlantic Ocean are augmented by the desorption of radium from sediments in the low-salinity area of the estuary and diffusion from bottom sediments. Desorption of226Ra is reflected by lower concentrations in suspended sediments from higher-salinity regions of the estuary. Bottom sediments from the high-salinity region have lower226Ra/230Th activity ratios than those from the low-salinity end.The shape of the dissolved226Ra vs. salinity profile is influenced by the river discharge. During average-discharge conditions, desorption of226Ra from suspended and bottom sediments increases the dissolved226Ra concentrations by a factor of 3.5 as the water passes through Winyah Bay. High river discharge produces an initial increase of dissolved226Ra by a factor of 2 to 3 and apparently reflects only desorption from suspended sediments. By driving the salt wedge down the estuary and reducing the zone of contact of salt water with bottom sediments, the high-flow conditions sharply reduce the flux of226Ra from bottom sediments. 相似文献
89.
Willard S. Moore Walter E. Dean S. Krishnaswami D.V. Borole 《Earth and Planetary Science Letters》1980,46(2):191-200
226Ra is used to document the growth histories of six manganese nodules from Oneida Lake, New York. Detailed sectioning and analysis reveal that there are discontinuous gradients in226Ra content in these samples. These gradients result from periods of rapid growth (>1 mm/100 years) separated by periods of no growth of erosion. Although the226Ra “age” of the nodules approximates the age of Oneida Lake, the nodules are not sediment-covered because they occur only in areas of the lake where fine-grained sediments are not accumulating. 相似文献
90.
Bioassay of a No. 2 fuel oil dispersion with shrimp in a continuous flow system using measured waterborne oil as the indicator of oil concentrations reveals a treatment more definable than those previously described in terms of volume ratios and produces lower lethal concentrations. Shrimp 96-h LC50 was 0.8 mg/l in this study as compared to values from 1.5 to 50 mg/l reported for other methods. Mean concentrations in tests do not give significant differences in concentration with respect to day of the test or spatial distribution in the exposure tanks. 相似文献