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71.
Francesco Di Benedetto Ilaria Bencistà Francesco D’Acapito Silvia Frizzera Andrea Caneschi Massimo Innocenti Alessandro Lavacchi Giordano Montegrossi Werner Oberhauser Maurizio Romanelli Herbert Dittrich Luca A. Pardi Gerold Tippelt Georg Amthauer 《Physics and Chemistry of Minerals》2016,43(8):535-544
The successful synthesis of nanoparticles of Fe-bearing kuramite, (Cu,Fe)3SnS4, is reported in this study. Nanocrystalline powders were obtained through a mild, environmentally friendly and scalable solvothermal approach, in a single run. The sample was the object of a multidisciplinary investigation, including X-ray diffraction and absorption, scanning electron microscopy and microanalysis, electron paramagnetic resonance, diffuse reflectance and Mössbauer spectroscopy as well as SQUID magnetometry. The nanoparticles consist of pure Fe-bearing kuramite, exhibiting tetragonal structure. The valence state of the metal cations was assessed to be Cu+, Sn4+ and Fe3+. The material presents a band gap value of 1.6 eV, which is fully compatible with solar cell applications. The uptake of Fe by nanokuramite opens a compositional field where the physical properties can be tuned. We thus foster the application of Fe-bearing nanokuramite for photovoltaics and energy storage purposes. 相似文献
72.
73.
José?D.?CarriquiryEmail author Pablo?Jorgensen Julio?A.?Villaescusa Silvia?E.?Ibarra-Obando 《Estuaries and Coasts》2016,39(2):451-461
Nutrient sources of San Quintin Bay, a coastal lagoon affected by coastal upwelling off Baja California (Mexico), were traced using generalized additive (mixed) models (GAMM) to the stable nitrogen isotopic composition, C:N and N content of two co-occurring macrophytes (the macroalgae Ulva spp. and the seagrass Zostera marina). The geochemical tracers followed a spatial trend that partly responded to the long-term nutrient gradient from the ocean towards the interior of the bay. N content in Z. marina and Ulva spp. decreased linearly (while C:N increased) towards the middle section of the bay to concentration levels that indicate potential N limitation for growth. Concurrently midway into the bay (6–9 km), the δ15N of both macrophytes showed a gradual enrichment in 15N reflecting progressive denitrification. The spatial pattern of δ15N and the decrease in C:N of the macrophytes towards the innermost section of the bay indicated an additional nonoceanic source of dissolved nitrogen in this zone. The similarity of the δ15N pattern of Z. marina and Ulva spp. implies that their δ15N composition is mainly controlled by the availability of N, in spite of the physiological differences between taxa. A better fit of GAMM to N content and C:N was obtained for Z. marina than for Ulva spp. indicating that the former delineate more steadily and smoothly the influence of upwelling along the spatial gradient. Nonetheless, Ulva spp. may be analyzed in combination with Z. marina to characterize the environmental conditions at the time of sampling. 相似文献
74.
The effectiveness of high-resolution LiDAR data combined with PSInSAR data in landslide study 总被引:1,自引:0,他引:1
Andrea Ciampalini Federico Raspini William Frodella Federica Bardi Silvia Bianchini Sandro Moretti 《Landslides》2016,13(2):399-410
The spatial resolution of digital elevation models (DEMs) is an important factor for reliable landslide studies. Multi-interferometric techniques such as persistent scatterer interferometric synthetic aperture radar (PSInSAR) are used to evaluate the landslide state of activity and its ground deformation velocity, which is commonly measured along the satellite line of sight (LOS). In order to compare velocities measured by different satellites in different periods, their values can be projected along the steepest slope direction, which is the most probable direction of real movement. In order to achieve this result, DEM-derived products are needed. In this paper, the effectiveness of different DEM resolutions was evaluated in order to project ground deformation velocities measured by means of PSInSAR technique in two different case studies in the Messina Province (Sicily, southern Italy): San Fratello and Giampilieri. Three DEMs were used: (i) a 20-m resolution DEM of the Italian Military Geographic Institute (IGM), (ii) a 2-m resolution DEM derived from airborne laser scanning (ALS) light detection and ranging (LiDAR) data for the San Fratello 2010 landslide, and (iii) a 1-m resolution DEM derived from ALS LiDAR data for the area of Giampilieri. The evaluation of the applied method effectiveness was performed by comparing the DEMs elevation with those of each single permanent scatterer (PS) and projecting the measured velocities along the steepest slope direction. Results highlight that the higher DEM resolution is more suitable for this type of analysis; in particular, the PS located nearby the watershed divides is affected by geometrical problems when their velocities are projected along the steepest slope. 相似文献
75.
Daniel Karthe Ole Behrmann Verena Blättel Dennis Elsässer Christian Heese Matthias Hügle Frank Hufert Andreas Kunze Reinhard Niessner Johannes Ho Buren Scharaw Matthias Spoo Andreas Tiehm Gerald Urban Silvia Vosseler Thomas Westerhoff Gregory Dame Michael Seidel 《Environmental Earth Sciences》2016,75(23):1481
The state-of-the-art monitoring of drinking water hygiene is based on the cultivation and enumeration of indicator bacteria. Despite its proven reliability, this approach has the disadvantages of being (a) relatively slow and (b) limited to a small number of indicator bacteria. Ideally, alternative methods would be less time-consuming while providing information about a larger set of hygienically relevant microorganisms including viruses. In this paper, we present insights into the design of a modular concentration and detection system for bacteria, bacteriophages and viruses. Following further validation, this or similar techniques have the potential to extend and speed up the monitoring of raw and drinking water hygiene in the future. The system consists of different modules for the concentration of microorganisms, an amplification and detection unit that includes a module for the differentiation between live and dead microorganisms, and an automated system for decision support and self-diagnosis. The ongoing testing under controlled laboratory conditions and real-life conditions in the water supply industry yields further system improvements. Moreover, the increased sensitivity and broader range of microbiological parameters emphasize the need for a reconsideration of the currently used criteria for the assessment of (drinking) water hygiene. 相似文献
76.
77.
Fossi MC Casini S Marsili L Ancora S Mori G Neri G Romeo T Ausili A 《Marine environmental research》2004,58(2-5):425-429
In this project we investigated the ecotoxicological effects of endocrine disrupters in a four-year survey of the Mediterranean population of swordfish (Xiphias gladius). In the Mediterranean environment, top predators, such as swordfish, accumulate high concentrations of polyhalogenated aromatic hydrocarbons (PHAHs) and toxic metals, potentially incurring high toxicological risk. The effects of organochlorines and trace elements (Hg, Cd and Pb) in 192 swordfish specimens, caught in the Strait of Messina, Sicily, Italy, were investigated using vitellogenin (Vtg), zona radiata proteins (Zrp) and CYP1A (BPMO, EROD) activities. Vtg and Zrp were found to be dramatically induced in some adult male specimens, suggesting that this species is highly exposed to estrogens in the Mediterranean Sea. A role of organochlorines in this induction phenomenon is suggested by the statistically significant correlations between Zrp in plasma and PCB concentrations in muscle (p<0.032) and Vtg in plasma and PCB concentrations in liver (p<0.034) of male specimens. Levels of trace elements in liver were in the following ranges: Hg 1-22, Cd 1-28 and Pb 0-1.6 ppm d.w. These data indicate potential reproductive alterations in large pelagic fish and suggest the need for continuous monitoring to avoid reductions in the population of this fish species of high commercial and ecological interest. 相似文献
78.
Jan Sverre Laberg Martyn S. Stoker K.I. Torbjrn Dahlgren Henk de Haas Haflidi Haflidason Berit O. Hjelstuen Tove Nielsen Pat M. Shannon Tore O. Vorren Tjeerd C.E. van Weering Silvia Ceramicola 《Marine and Petroleum Geology》2005,22(9-10):1069
Based on studies of sediment accumulations deposited from-and erode by-alongslope flowing ocean currents on the European continental margin from Porcupine (Ireland) to Lofoten (Norway), the evolution of the Cenozoic paleocirculation was reconstructed as part of the STRATAGEM project. There is evidence of ocean current-controlled erosion and deposition in the Rockall Trough, in the Faeroe-Shetland Channel and on the Vøring Plateau since the late Eocene, although the circulation pattern remains ambiguous. The late Palaeogene flow in the Rockall Trough was almost probably driven by southerly-derived Tethyan Outflow Water. The extent and strength of any northerly-derived flow is uncertain. From the early Neogene (early-mid-Miocene), there was a massive regional expansion of contourite drift development both in the North Atlantic and in the Norwegian-Greenland Sea. This was most probably related to the development of the Faroe Conduit, the opening of the Fram Strait and the general subsidence of the Greenland-Scotland Ridge. These may have combined to cause a considerable acceleration in the exchange and overflow of deep waters between the Arctic and Atlantic Oceans. An early late Neogene (late early Pliocene) regional erosional event has been ascribed to a vigorous pulse of bottom-current activity, most probably the result of a global reorganisation of ocean currents associated with the closure of the Central American Seaway. During the late Neogene, contourites and sediment drifts developed in deep-water basins, between units of glacigenic sediments as well as infill of several paleo-slide scars. These sediments were derived from areas of bottom-current erosion as well as from the development of Plio-Pleistocene prograding sediment wedges, incorporating the extensive sediment supply derived from shelf-wide ice sheets. Presently a profound winnowing prevails along the shelf and upper slope due to the inflowing currents of Atlantic water. Depocentres of sediments derived from the winnowing are located (locally) in lower slope embayments and in slide scars. 相似文献
79.
M. Cristina Fossi Silvia Casini Letizia Marsili Stefania Ancora Gabriele Mori Giovanni Neri Teresa Romeo Antonella Ausili 《Marine environmental research》2004,58(2-5):425
In this project we investigated the ecotoxicological effects of endocrine disrupters in a four-year survey of the Mediterranean population of swordfish (Xiphias gladius). In the Mediterranean environment, top predators, such as swordfish, accumulate high concentrations of polyhalogenated aromatic hydrocarbons (PHAHs) and toxic metals, potentially incurring high toxicological risk. The effects of organochlorines and trace elements (Hg, Cd and Pb) in 192 swordfish specimens, caught in the Strait of Messina, Sicily, Italy, were investigated using vitellogenin (Vtg), zona radiata proteins (Zrp) and CYP1A (BPMO, EROD) activities. Vtg and Zrp were found to be dramatically induced in some adult male specimens, suggesting that this species is highly exposed to estrogens in the Mediterranean Sea. A role of organochlorines in this induction phenomenon is suggested by the statistically significant correlations between Zrp in plasma and PCB concentrations in muscle (p<0.032) and Vtg in plasma and PCB concentrations in liver (p<0.034) of male specimens. Levels of trace elements in liver were in the following ranges: Hg 1–22, Cd 1–28 and Pb 0–1.6 ppm d.w. These data indicate potential reproductive alterations in large pelagic fish and suggest the need for continuous monitoring to avoid reductions in the population of this fish species of high commercial and ecological interest. 相似文献
80.
Bogdan Wszolek Konrad Rudnicki Silvia Masi Paolo De Bernardis Antonio Salvi 《Astrophysics and Space Science》1989,152(1):29-34
We used theIRAS All Sky Maps in order to search for infrared emission in the direction of the Okroy Cloud (R.A.=12h50m, =22°). An enhancement of 100 m diffuse emission is evident in such a region, with an anomalous value of the ratioI
v (100 m)/A
v
; hydrogen 21 cm emission is also present with low radial speed, thus suggesting that the cloud could be a satellite of our Galaxy. 相似文献