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Characteristics and genesis of maghemite in Chinese loess and paleosols: Mechanism for magnetic susceptibility enhancement in paleosols 总被引:4,自引:0,他引:4
Tianhu Chen Huifang Xu Qiaoqin Xie Jun Chen Junfeng Ji Huayu Lu 《Earth and Planetary Science Letters》2005,240(3-4):790-802
Morphological characteristics and microstructures of magnetic minerals extracted from Chinese loess and paleosols were investigated using powder X-ray diffraction (XRD) and high-resolution transmission electron microscopy (HRTEM). Our results indicate that maghemite in loess–paleosol sequences was transformed from magnetite through oxidation of magnetite. Maghemite transformed from eolian magnetite during chemical weathering has low-angle grain boundaries among maghemite nano-crystals. Some nano-crystalline maghemites with nanoporous texture resulted from microbe-induced precipitation of magnetite or transformation of poorly crystalline ferric Fe (oxy)hydroxides in presence of Fe-reducing bacteria. Aggregates of euhedral maghemite nano-crystals were transformed from magnetite magnetosomes. Both microbe-induced nanoporous magnetite and microbe-produced magnetite magnetosomes are directly related to microbial activities and pedogenesis of the paleosols. It is proposed that the formation of nano-crystalline maghemite with superparamagnetic property in paleosol results in the enhancement of magnetic susceptibility, although the total amount (weight percent) of magnetic minerals in both paleosol and loess units is similar. Our results also show that nano-crystalline and nanoporous magnetite grains prefer to transform into maghemite in semi-arid soil environments instead of hematite, although hematite is a thermodynamically stable phase. This result also indicates that a decrease in crystal size will increase stability of maghemite. It is also inferred that surface energy of maghemite is lower than that of hematite. 相似文献
196.
Wenkai Lu 《Geophysical Prospecting》2005,53(1):149-158
This paper presents a new algorithm for estimating non‐minimum‐phase seismic wavelets by using the second‐ and higher‐order statistics (HOS) of the wavelets. In contrast to many, if not most, of the HOS‐based methods, the proposed method does not need to assume that subsurface seismic reflectivity is a non‐Gaussian, statistically independent and identically distributed random process. The amplitude and phase spectra of the wavelets are estimated, respectively, using the second‐order statistics (SOS) and third‐order moment (TOM) of the wavelets, which will, in turn, be derived from the HOS of the seismic traces. In our approach, the wavelets can be ‘calculated’ from seismic traces efficiently; no optimization or inversion is necessarily required. Very good results have been obtained by applying this method to both synthetic and real‐field data sets. 相似文献
197.
南半球对流层气候年代际变化及其与太阳活动的联系 总被引:7,自引:0,他引:7
通过南半球对流层温度场谱分析和逐次滤波分析发现,南半球对流层大气温度场半个多世纪以来呈现明显的持续升温趋势,升温幅度由低层到高层逐步增加,其中地面层1 000 hPa年升温率为0.013℃/a,对流层中部500 hPa年升温率为0.019℃/ a,对流层上部300 hPa年升温率为0.036℃/ a;滤除南半球大气温度场的趋势变化,发现南半球大气温度场从地面层直至对流层顶广泛盛行着十分显著的与太阳磁场磁性22年周期变化相一致的变化周期。太阳磁场磁性周期变化趋势略有超前,分析认为,这是南半球对流层大气气候系统对太阳磁场周期性变化的响应。进一步分析还发现,南半球从地面层1 000 hPa到对流层顶,再到平流层中部10 hPa各层次大气温度变化22年周期分量振荡位相基本一致,周期振幅由低层到高层迅速增大,说明太阳磁场变化对对流层高层比低层影响大,对平流层影响更大。其中地面层1 000 hPa温度场的22年变化周期是在滤除趋势变化和11年周期之后才显现出来的,所以太阳磁场磁性周期变化对地面层气候的影响较小并且经常处于被掩盖状态;南半球地面层1 000 hPa温度场滤除趋势变化之后显示出十分显著的与太阳活动11年周期相一致的变化周期,分析认为,这是南半球对流层大气气候系统对太阳活动11周期性变化的响应。对流层上层300 hPa温度场滤除趋势变化和22年周期之后也显示出11年变化周期,而对流层中部500 hPa则无此周期反应,说明太阳活动11年周期对地面层1 000 hPa大气气候影响最明显,对流层中上层影响较弱。 相似文献
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利用我国北极黄河站所在地,德国Koldwey站1994—2003年的逐时常规气象资料,对北极苔原Ny lesund地区短期气候特征进行了初步分析。结果表明,由于受北大西洋暖流的影响,该地是北极同纬度温度最高的地区。岛上气候温暖湿润,即使在隆冬季节,日平均气温都可以升至0℃以上。全年平均风力较小,以东南(SE)风居多。该地区平均增温速度为0. 68℃/10a,是北极增温较快的地区之一。与同期我国北冰洋浮冰区考察数据相比较,Ny lesund气候更温暖湿润,风速要小得多。在Ny lesund地区,美国国家环境预测中心/美国国家大气研究中心(NCEP/NCAR)的近地面气温的再分析结果,与Koldwey站实测常规地面资料相比,在冬季基本一致,而在夏季则差异较大。 相似文献
200.
Element mobility during pyrite weathering: implications for acid and heavy metal pollution at mining-impacted sites 总被引:1,自引:0,他引:1
Long Lu Rucheng Wang Fanrong Chen Jiyue Xue Peihua Zhang Jianjun Lu 《Environmental Geology》2005,49(1):82-89
Based on back scattered electron images and electron micro-probe analysis results, four alteration layers, including a transition layer, a reticulated ferric oxide layer, a nubby ferric oxide layer and a cellular ferric oxide layer, were identified in the naturally weathering products of pyrite. These layers represent a progressive alteration sequence of pyrite under weathering conditions. The cellular ferric oxide layer correlates with the strongest weathering phase and results from the dissolution of nubby ferric oxide by acidic porewater. Leaching coefficient was introduced to better express the response of element mobility to the degree of pyrite weathering. Its variation shows that the mobility of S, Co and Bi is stronger than As, Cu and Zn. Sulfur in pyrite is oxidized to sulfuric acid and sulfate that are basically released into to porewater, and heavy metals Co and Bi are evidently released by acid dissolution. As, Cu and Zn are enriched in ferric oxide by adsorption and by co-precipitation, but they would re-release to the environment via desorption or dissolution when porewater pH becomes low enough. Consequently, Co, Bi, As, Cu and Zn may pose a substantial impact on water quality. Considering that metal mobility and its concentration in mine waste are two important factors influencing heavy metal pollution at mining-impacted sites, Bi and Co are more important pollutants in this case. 相似文献