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11.
Heinz Lettau 《Boundary-Layer Meteorology》1990,50(1-4):1-9
The official report on this first comprehensive field experiment in boundary-layer meteorology was published 1957 in two volumes, edited by Lettau and Davidson (hereafter L&D). The official report is supplemented in this paper by relevant pre-history developments and a discussion of some selected post-history interpretations and follow-up experiments. 相似文献
12.
Grain boundaries influence many physical and chemical properties of crystalline materials. Here, we perform molecular dynamics simulations to study the structure of a series of [100] symmetric tilt grain boundaries in Mg2SiO4 forsterite. The present results show that grain boundary energies depend significantly on misorientation angle. For small misorientation angles (up to 22°), grain boundary structures consist of an array of partial edge dislocations with Burgers vector $\frac{1}{2}[001]$ associated with stacking faults and their energies can be readily fit with a model which adds the Peach-Koehler equation to the Read-Shockley dislocation model for grain boundaries. The core radius of partial dislocations and the spacing between the partials derived from grain boundary energies show that the transition from low- to high-angle grain boundaries occurs for a misorientation angle between 22° and 32°. For high misorientation angles (32.1° and 60.8°), the cores of dislocations overlap and form repeated structural units. Finally, we use a low energy atomic configuration obtained by molecular dynamics for the misorientation of 12.18° as input to simulate a high-resolution transmission electron microscopy (HRTEM) image. The simulated image is in good agreement with an observed HRTEM image, which indicates the power of the present approach to predict realistic atomic structures of grain boundaries in complex silicates. 相似文献
13.
Simulation of DNAPL infiltration and spreading behaviour in the saturated zone at varying flow velocities and alternating subsurface geometries 总被引:3,自引:1,他引:2
Katharina Erning Sibylle Grandel Andreas Dahmke Dirk Schäfer 《Environmental Earth Sciences》2012,65(4):1119-1131
The influence of varying groundwater flow velocities on DNAPL infiltration and spreading behaviour was investigated by multiphase
modelling using TMVOC and PetraSim. The multiphase models were calibrated by results of previously conducted laboratory experiments
for the complete spatio-temporal range of the experiments. The small scale 2D scenario modelling was applied to qualify and
quantify changes in position, architecture, geometry and dissolution of a TCE body in a fully saturated homogeneous sandy
medium. The applied flow velocities ranging from 0.05 up to 40.00 m/day exhibited that the DNAPL TCE is affected even at the
lowest flow velocity in its position, its size and its architecture. Additionally, several impermeable lenses with simple
geometry were assumed in the model, to investigate the influence of stratified subsoil. In the experimental set-ups, the DNAPL
body reacts more sensitive to the applied groundwater flow velocities than to the geometrical set-up of the scenarios. A possible
consequence can be the transportation and displacement of a DNAPL pool due to natural or anthropogenic induced high groundwater
flow velocities, as by Pump and Treat facilities, complicating site investigation process and planning of remediation activities. 相似文献
14.
Perception of landslides risk and responsibility: a case study in eastern Styria, Austria 总被引:2,自引:2,他引:0
This paper presents a case study about the perception of landslide risk. Following a major set of landslides in the eastern part of Austria in June 2009, we surveyed local experts, residents who had suffered losses from the landslides, and others living in the affected communities. Overall, the risk perception was significantly higher among those who had been personally affected by a landslide, had knowledge of the geology in the study region, had been affected by another natural hazard, or spent a lot of time outdoors and in touch with nature. Non-experts viewed natural factors as the main causes for the occurrence of landslides, while experts viewed anthropogenic factors as more important. Likewise, non-experts placed a greater emphasis on hard measures (such as retaining walls) to reduce the risk, whereas the experts tended to focus on better information and land-use planning. In terms of responsibility for mitigative actions, a majority of inhabitants believed that public authorities should undertake most of the costs, whereby those who had personal experience with landslides were more likely to favor the government paying for it. 相似文献
15.
Stable carbon isotope distribution of particulate organic matter in the ocean: a model study 总被引:4,自引:0,他引:4
Matthias Hofmann Dieter A. Wolf-Gladrow Taro Takahashi Steward C. Sutherland Katharina D. Six Ernst Maier-Reimer 《Marine Chemistry》2000,72(2-4)
The stable carbon isotopic composition of particulate organic matter in the ocean, δ13CPOC, shows characteristic spatial variations with high values in low latitudes and low values in high latitudes. The lowest δ13CPOC values (−32‰ to −35‰) have been reported in the Southern Ocean, whereas in arctic and subarctic regions δ13CPOC values do not drop below −27‰. This interhemispheric asymmetry is still unexplained. Global gradients in δ13CPOC are much greater than in δ13CDIC, suggesting that variations in isotopic fractionation during organic matter production are primarily responsible for the observed range in δ13CPOC. Understanding the factors that control isotope variability is a prerequisite when applying δ13CPOC to the study of marine carbon biogeochemistry. The present model study attempts to reproduce the δ13CPOC distribution pattern in the ocean. The three-dimensional (3D) Hamburg Model of the Oceanic Carbon Cycle version 3.1 (HAMOCC3.1) was combined with two different parametrizations of the biological fractionation of stable carbon isotopes. In the first parametrization, it is assumed that the isotopic fractionation between CO2 in seawater and the organic material produced by algae, P, is a function of the ambient CO2 concentration. The two parameters of this function are derived from observations and are not based on an assumption of any specific mechanism. Thus, this parametrization is purely empirical. The second parametrization is based on fractionation models for microalgae. It is supported by several laboratory experiments. Here the fractionation, P, depends on the CO2 concentration in seawater and on the (instantaneous) growth rates, μi, of the phytoplankton. In the Atlantic Ocean, where most field data are available, both parametrizations reproduce the latitudinal variability of the mean δ13CPOC distribution. The interhemispheric asymmetry of δ13CPOC can mostly be attributed to the interhemispheric asymmetry of CO2 concentration in the water. However, the strong seasonal variations of δ13CPOC as reported by several authors, can only be explained by a growth rate-dependent fractionation, which reflects variations in the cellular carbon demand. 相似文献
16.
Katharina Marquardt Elena Petrishcheva Rainer Abart Emmanuel Gardés Richard Wirth Ralf Dohmen Hans-Werner Becker Wilhelm Heinrich 《Physics and Chemistry of Minerals》2010,37(10):751-760
In this study, we address volume diffusion of ytterbium in yttrium aluminum garnet (YAG) using thin-film single crystal diffusion
couples. We employ analytical transmission electron microscopy (ATEM) as a tool for combined microstructural and microchemical
analysis and compare the results to Rutherford backscattering (RBS) analysis. Given the high spatial resolution of the method,
we focus on microstructural changes of the thin-film diffusant source during the diffusion anneal. We evaluate the potential
influence of the associated changes in its transport properties on the evolution of concentration profiles in the single crystal
substrate. This approach allows us to test the reliability of determination of volume diffusion coefficients from thin-film
diffusion experiments. We found that for the chosen experimental setting, the influence of thin-film re-crystallization is
small when compared with the experimental uncertainty and good estimates for the volume diffusion coefficients of Yb in YAG
can be obtained using standard assumptions. Both Yb-concentration profiles analyzed with ATEM and with RBS give similar results.
At 1,450°C and 1 bar, we infer log D
Yb (m2/s) values of −19.37 ± 0.07 (TEM) and −19.84 ± 0.02 (RBS). Although the change in thin-film transport properties associated
with successive crystallization during the diffusion anneal does not play a major role for our experimental setup, this effect
cannot generally be ignored. 相似文献
17.
Alfred Ngomanda Katharina Neumann Astrid Schweizer Jean Maley 《Quaternary Research》2009,71(3):307-318
The third millennium BP crisis of the central African rainforest is not sufficiently understood. The low resolution of most pollen profiles and a large plateau of the calibration curve aggravate the exact dating of the event, and its causal climatic parameters are debated. We present a high-resolution pollen profile from the swamp site Nyabessan in the southern Cameroonian rainforest, covering the period 3100-2300 cal yr BP. Between 3100 and 2500 cal yr BP, the climate was favourable for a regional evergreen forest with Caesalpiniaceae and Lophira and a local Raphia swamp forest. Around 2500/2400 cal yr BP, a significant decrease of mature forest and swamp forest taxa and an increase of pioneers indicate that the rain forest was seriously disturbed and replaced by secondary formations. The dominance of Trema orientalis, a pioneer well adapted to seasonal desiccation, points to a much more accentuated seasonality after 2500 cal yr BP, which seems to be linked to a southwards shift of the ITCZ during the northern hemisphere winter months. We propose that the rain forest crisis between 2500 and 2200 cal BP created favourable conditions for farming and paved the way for a major expansion of Bantu speaking populations. 相似文献
18.
Katharina?Marquardt Elena?Petrishcheva Emmanuel?Gardés Richard?Wirth Rainer?Abart Wilhelm?Heinrich 《Contributions to Mineralogy and Petrology》2011,162(4):739-749
Yb-Y inter-diffusion along a single grain boundary of a synthetic yttrium aluminium garnet (YAG) bicrystal has been studied
using analytical transmission electron microscopy (ATEM). To investigate the diffusion, a thin-film containing Yb as the diffusant
was deposited perpendicular to the bicrystal grain boundary by pulsed laser deposition (PLD). Structural properties and their
change with time in both the diffusant source and the grain boundary are reported. The diffusion profiles are incorporated
in a numerical diffusion model, which is applied to determine the grain boundary diffusion coefficient, D
gb
, at 1.723 K it is equal to 3 × 10−15 m2/s. We find that grain boundary diffusion is 4.85 orders of magnitude faster than volume diffusion, which was determined from
the same diffusion experiment. This result is discussed in the context of special versus general grain boundaries. Finally,
we successfully tested the capability of synchrotron-based nano-X-ray fluorescence analysis to map micro-chemical patterns
in two dimensions with sub-micrometre resolution. 相似文献
19.
Katharina Dulias Kathleen R. Stoof-Leichsenring Luidmila A. Pestryakova Ulrike Herzschuh 《Journal of Paleolimnology》2017,57(1):51-66
The Arctic treeline ecotone is characterised by a steep vegetation gradient from arctic tundra to northern taiga forests, which is thought to influence the water chemistry of thermokarst lakes in this region. Environmentally sensitive diatoms respond to such ecological changes in terms of variation in diatom diversity and richness, which so far has only been documented by microscopic surveys. We applied next-generation sequencing to analyse the diatom composition of lake sediment DNA extracted from 32 lakes across the treeline in the Khatanga region, Siberia, using a short fragment of the rbcL chloroplast gene as a genetic barcode. We compared diatom richness and diversity obtained from the genetic approach with diatom counts from traditional microscopic analysis. Both datasets were employed to investigate diversity and relationships with environmental variables, using ordination methods. After effective filtering of the raw data, the two methods gave similar results for diatom richness and composition at the genus level (DNA 12 taxa; morphology 19 taxa), even though there was a much higher absolute number of sequences obtained per genetic sample (median 50,278), compared with microscopic counts (median 426). Dissolved organic carbon explained the highest percentage of variance in both datasets (14.2 % DNA; 18.7 % morphology), reflecting the compositional turnover of diatom assemblages along the tundra-taiga transition. Differences between the two approaches are mostly a consequence of the filtering process of genetic data and limitations of genetic references in the database, which restricted the determination of genetically identified sequence types to the genus level. The morphological approach, however, allowed identifications mostly to species level, which permits better ecological interpretation of the diatom data. Nevertheless, because of a rapidly increasing reference database, the genetic approach with sediment DNA will, in the future, enable reliable investigations of diatom composition from lake sediments that will have potential applications in both paleoecology and environmental monitoring. 相似文献
20.
Dissolved and particulate organic matter (DOM and POM) distribution, lignin phenol signatures, bulk elemental compositions, fluorescence indices and microbial plankton (algae, bacteria, viruses) in a temperate river floodplain system were monitored from January to November 2003. We aimed to elucidate the sources and compositions of allochthonous and autochthonous organic matter (OM) in the main channel and a representative backwater in relation to the hydrological regime. Additionally, bacterial secondary production was measured to evaluate the impact of organic carbon source on heterotrophic prokaryotic productivity. OM properties in the backwater tended to diverge from those in the main channel during phases without surface water connectivity; this was likely enhanced due to the exceptionally low river discharge in 2003. The terrestrial OM in this river floodplain system was largely derived from angiosperm leaves and grasses, as indicated by the lignin phenol composition. The lignin signatures exhibited significant seasonal changes, comparable to the seasonality of plankton-derived material. Microbially-derived material contributed significantly to POM and DOM, especially during periods of low discharge. High rates of bacterial secondary production (up to 135 μg C L(-1) d(-1)) followed algal blooms and suggested that autochthonous OM significantly supported heterotrophic microbial productivity. 相似文献