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121.
Three experimental techniques – ion exchange, liquid–liquid extraction with competitive ligand exchange, and solid-phase extraction with competitive ligand exchange (CLE–SPE) – were evaluated as methods for determining conditional stability constants (K) for the binding of mercury (Hg2+) to dissolved organic matter (DOM). To determine the utility of a given method to measure stability constants at environmentally relevant experimental conditions, experimental results should meet three criteria: (1) the data must be experimentally valid, in that they were acquired under conditions that meet all the requirements of the experimental method, (2) the Hg:DOM ratio should be determined and it should fall within levels that are consistent with environmental conditions, and (3) the stability constants must fall within the detection window of the method. The ion exchange method was found to be limited by its detection window, which constrains the method to stability constants with log K values less than about 14. The liquid–liquid extraction method was found to be complicated by the ability of Hg–DOM complexes to partition into the organic phase. The CLE–SPE method was found to be the most suitable of these methods for the measurement of Hg–DOM stability constants. Stability constants for DOM isolates measured using the CLE–SPE method at environmentally relevant Hg:DOM ratios were log K = 25–30 (M−1). These values are consistent with the strong Hg2+ binding expected for reduced S-containing binding sites. 相似文献
122.
Lucinid bivalves dominate the infauna of tropical seagrass sediments. While the effect of seagrass on lucinids has been studied,
the reverse effect has largely been ignored. Lucinids can alter porewater chemistry (i.e., increase porewater nutrients by
suspension feeding and decrease porewater sulfides by oxygen introduction and bacterial oxidation), which can potentially
change seagrass productivity and growth morphology. To observe correlations between porewater chemistry and lucinid presence,
a field survey and laboratory microcosm experiment were conducted. Survey sampling sites with lucinids had significantly lower
sulfide and higher ammonium concentrations than sampling sites without lucinids. There was no difference in phosphate concentration
among sampling sites. Both lucinid species used in the microcosm experiment (Ctena orbiculata andLucinesca nassula) significantly lowered sulfide concentrations in the sediment porewater. Microcosm and field survey results were incorporated
into a sulfide budget. In seagrass sediments, lucinids remove 2–16% of the total sulfide produced. Sulfide is a major stressor
to both plants and animals in Florida Bay sediments; this removal may be important to maintaining seagrass productivity and
health. Oxygen introduction into sediments byC. orbiculata was estimated in a dye experiment.C. orbiculata were added to small tubes containing sieved mud and incubated in a bath of seawater with a Rhodamine WT. Rhodamine WT accumulation
in the sediment was measured. A first order estimate showed that oxygen introduction can account for less than 5% ofC. orbiculata sulfide removal. 相似文献
123.
Carole Cordier Martial Caroff Thierry Juteau Corinne Fleutelot Christophe Hmond Marion Drouin Joseph Cotten Claire Bollinger 《Lithos》2007,99(3-4):289-311
The present study is based on a set of lavas and crosscutting dikes collected by dives along detailed vertical transects on the northern flank of the western part of the Blanco Transform Fault, Northeast Pacific. The studied area consists of a small basin, the Western Blanco Depression (WBD), extending from the southern end of the Juan de Fuca ridge to a pseudofault trace 60 km eastward. The Northern Scarp of the WBD comprises a volcanic unit overlying a sheeted-dike complex. Major and trace element data, coupled with Sr–Nd isotope ratios, reveal a two-component mantle source, composed by an isotopically depleted matrix variably veined by more enriched material. One chemical group (NS2), indistinguishable from the other Northern Scarp samples on the basis of trace element data, has an unusually depleted isotopic composition typical of a nearly pure mantle end-member. Some cogenetic samples of the Northern Scarp have been used to constrain the differentiation modalities. Anorthite and MgO content profiles in plagioclase xenocrysts and phenocrysts reveal (i) the existence of H2O-bearing evolved melts in the mushy zones and (ii) the occurrence of mixing process between these melts and anhydrous mafic liquids. The hydration is supported by other petrographic features such as high magmatic fO2 values, calculated from Fe–Ti oxide pairs, and the presence of pyroxene inclusions in plagioclase phenocrysts. Mixing, consistent with the existence of Ni-rich ferrobasalts, is interpreted to be the consequence of the reservoir refilling by mafic liquids (Mg# = 70). These petrological and geochemical evidences are combined with the evolution of Mg# with depth to suggest a periodic open-system magma chamber evolution beneath the southern end of the Juan de Fuca ridge. 相似文献
124.
北阿尔金巴什考供-斯米尔布拉克花岗杂岩特征及锆石SHRIMP U-Pb定年 总被引:6,自引:0,他引:6
北阿尔金巴什考供-斯米尔布拉克杂岩体位于巴什考供盆地北缘, 呈东西向展布, 宽约 2~6 km, 长约30 km, 出露面积约140 km2. 主要由灰黑色石英闪长岩、灰白色花岗岩、粉红色花岗岩和花岗伟晶岩组成. 围岩为前寒武系片岩、变质泥岩及变质凝灰岩. 岩石地球化学特征表明, 石英闪长岩属钙碱性系列, 具有Ⅰ型花岗岩的属性; 而粉红色和灰白色花岗岩属高钾钙碱性系列, 具有S型花岗岩的属性. 锆石SHRIMP定年结果表明, 石英闪长岩的年龄为(481.6±5.6) Ma, 而灰白色花岗岩和粉红色花岗岩的年龄在误差范围内基本一致, 分别为(437.0±3.0)~(433.1±3.4) Ma 和(443±11)~(434.6±1.6) Ma. 结合区域地质特征, 认为石英闪长岩可能形成于洋壳俯冲环境, 而灰白色和粉红色花岗岩可能形成于碰撞后环境. 相似文献
125.
In this paper, we formulate a finite element procedure for approximating the coupled fluid and mechanics in Biot’s consolidation
model of poroelasticity. Here, we approximate the pressure by a mixed finite element method and the displacements by a Galerkin
method. Theoretical convergence error estimates are derived in a discrete-in-time setting. Of particular interest is the case
when the lowest-order Raviart–Thomas approximating space or cell-centered finite differences are used in the mixed formulation
and continuous piecewise linear approximations are used for displacements. This approach appears to be the one most frequently
applied to existing reservoir engineering simulators. 相似文献
126.
In this paper, we formulate a finite element procedure for approximating the coupled fluid and mechanics in Biot’s consolidation
model of poroelasticity. Here, we approximate the pressure by a mixed finite element method and the displacements by a Galerkin
method. Theoretical convergence error estimates are derived in a continuous in-time setting for a strictly positive constrained
specific storage coefficient. Of particular interest is the case when the lowest-order Raviart–Thomas approximating space
or cell-centered finite differences are used in the mixed formulation, and continuous piecewise linear approximations are
used for displacements. This approach appears to be the one most frequently applied to existing reservoir engineering simulators. 相似文献
127.
Wusi Yue Marc B. Parlange Charles Meneveau Weihong Zhu René van Hout Joseph Katz 《Boundary-Layer Meteorology》2007,124(2):183-203
Turbulent flow in a corn canopy is simulated using large-eddy simulation (LES) with a Lagrangian dynamic Smagorinsky model.
A new numerical representation of plant canopies is presented that resolves approximately the local structure of plants and
takes into account their spatial arrangement. As a validation, computational results are compared with experimental data from
recent field particle image velocimetry (PIV) measurements and two previous experimental campaigns. Numerical simulation using
the traditional modelling method to represent the canopy (field-scale approach) is also conducted as a comparison to the plant-scale
approach. The combination of temporal PIV data, LES and spatial PIV data allows us to couple a wide range of relevant turbulence
scales. There is good agreement between experimental data and numerical predictions using the plant-scale approach in terms
of various turbulence statistics. Within the canopy, the plant-scale approach also allows the capture of more details than
the field-scale approach, including instantaneous gusts that penetrate deep inside the canopy. 相似文献
128.
Particle image velocimetry (PIV) data obtained in a wind-tunnel model of a canopy boundary layer is used to examine the characteristics
of mean flow and turbulence. The vector spacing varies between 1.7 and 2.5 times the Kolmogorov scales. Conditional sampling
based on quadrants, i.e. based on the signs of velocity fluctuations, reveals fundamental differences in flow structure, especially
between sweep and ejection events, which dominate the flow. During sweeps, the downward flow generates a narrow, highly turbulent,
shear layer containing multiple small-scale vortices just below canopy height. During ejections, the upward flow expands this
shear layer and the associated small-scale flow structures to a broad region located above the canopy. Consequently, during
sweeps the turbulent kinetic energy (TKE), Reynolds stresses, as well as production and dissipation rates, have distinct narrow
peaks just below canopy height, whereas during ejections these variables have broad maxima well above the canopy. Three methods
to estimate the dissipation rate are compared, including spectral fits, measured subgrid-scale (SGS) energy fluxes at different
scales, and direct measurements of slightly underresolved instantaneous velocity gradients. The SGS energy flux is 40–60%
of the gradient-based (direct) estimates for filter sizes inside the inertial range, while decreasing with scale, as expected,
within the dissipation range. The spectral fits are within 5–30% of the direct estimates. The spectral fits exceed the direct
estimates near canopy height, but are lower well above and below canopy height. The dissipation rate below canopy height increases
with velocity magnitude, i.e. it has the highest values during sweep and quadrant 1 events, and is significantly lower during
ejection and quadrant 3 events. Well above the canopy, ejections are the most dissipative. Turbulent transport during sweep
events acts as a source below the narrow shear layer within the canopy and as a sink above it. Transport during ejection events
is a source only well above the canopy. The residual term in the TKE transport equation, representing mostly the effect of
pressure–velocity correlations, is substantial only within the canopy, and is dominated by sweeps. 相似文献
129.
Falconer David A. Jordan Stuart D. Brosius Jeffrey W. Davila Joseph M. Thomas Roger J. Andreatta Vicenzo Hara Hirohisa 《Solar physics》1998,180(1-2):179-191
We investigate the possibility that strong EUV lines observed with the Goddard Solar EUV Rocket Telescope and Spectrograph (SERTS) provide good proxies for estimating the total coronal flux over shorter wavelength ranges. We use coordinated SERTS and Yohkoh observations to obtain both polynomial and power-law fits relating the broad-band soft X-ray fluxes to the intensities of Fexvi 335 Ú and 361 Ú, Fexv 284 Ú and 417 Ú, and Mgix 368 Ú measured with SERTS. We found that the power-law fits best cover the full range of solar conditions from quiet Sun through active region, though not surprisingly the cooler Mgix 368 Ú line proves to be a poor proxy. The quadratic polynomial fits yield fair agreement over a large range for all but the Mgix line. However, the linear fits fail conspicuously when extrapolated into the quiet-Sun regime. The implications of this work for the Heii 304 Ú line formation problem are also briefly considered. 相似文献
130.
Joseph R. Oppong 《The Professional geographer》1998,50(4):437-448
Ten years after the human immuno-deficiency virus (HIV) was first reported in Ghana, it continues to spread throughout the country following patterns that are rare in other African countries. HIV is seen in twice as many females as males, more frequently in rural than urban regions, and regions with high rates of polygamy have significantly lower rates. The evidence presented in this paper shows that HIV diffusion patterns probably reflect the spatial distribution and social networks of vulnerable social groups. While information-based campaigns are still necessary in the fight against HIV/AIDS, they fail to enable or empower vulnerable people to protect themselves against infection. 相似文献