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371.
Surface and gravity-cored sediments were collected from the Kaoping coastal area off southwestern Taiwan to determine particle size, organic carbon, trace metal concentration and enrichment factor (EF), 210Pb dating, and 206Pb/207Pb ratio for determining present and historical metal pollution. Surface distributions of trace metals ranged from 0.02 to 0.13 mg/kg for Cd (EF: 0.16-1.65), from 35 to 189 mg/kg for Cr (EF: 0.85-2.92), from 25 to 64 mg/kg for Ni (EF: 0.53-2.38), from 10 to 32 mg/kg for Pb (EF: 1.20-4.94), and from 29 to 129 mg/kg for Zn (EF: 1.18-3.50). Trace metal concentrations correlate closely with distributions of mud (<63 microm) and organic carbon which accumulate largely around river mouths and within the Kaoping Canyon. With the exception of Cd, Cr and Ni in certain areas with rather coarse sediments, metals were generally elevated above the baseline levels over the studied area. Metals were also relatively enriched in areas with high contents of mud and organic carbon. Sedimentation rates derived from the excess 210Pb data in core sediments sampled from the canyon illustrate metal pollution beginning around 1970 that is corresponding to the booming time of economic growth in Taiwan. Meanwhile, the status of Pb pollution in core sediments is verified by an inversed correlation between 206Pb/207Pb ratios and Pb concentrations. Anthropogenic Pb and other metals in the studied area were apparently derived primarily from the Kaoping River and accumulated around the river mouth and within the Kaoping Canyon. The Kaoping Canyon appears to act as a major sink for river borne trace metals. 相似文献
372.
New evidence for covalent coupling of peptides to humic acids based on 2D NMR spectroscopy: A means for preservation 总被引:1,自引:0,他引:1
Pang-Hung Hsu 《Geochimica et cosmochimica acta》2005,69(18):4521-4533
Nitrogen immobilization in soils and sediments involving the preservation of peptides is an important yet not well-understood process. Several hypotheses have been proposed for the preservation of peptides in these systems; however, to date, there is no direct molecular-level evidence for any one of several hypotheses. In this study, a synthesized peptide with 15N-labeled amino acid residues was utilized to examine the mechanism by which humic substances from a peat might chemically interact with peptides to induce preservation. Two-dimensional 15N-1H HSQC NMR experiments were performed to evaluate the bonding and nonbonding interactions between 15N-labeled peptide and an Everglades peat humic acid. The observed changes in cross peaks provide the first direct spectroscopic evidence for what we believe to be covalent binding between these substances. Noncovalent interactions between the 15N-labeled peptides and humic acid molecules are also observed in the spectra. Quinone structures in humic acids are suggested to be the important reactive groups, based on reaction of the labeled peptide with a model quinone which shows similar nitrogen-proton correlated peak patterns as is observed in the HSQC NMR spectra of humic acids reacted with the peptide. The Michael reaction with quinone structures is proposed, and this type of reaction provides a mechanism that is consistent with previous observation for the chemistry of sedimentary nitrogen species. 相似文献
373.
Albert S. Chen Ming-Hsi Hsu Wei-Hsien Teng Chen-Jia Huang Sen-Hae Yeh Wan-Yu Lien 《Natural Hazards》2006,37(1-2):107-132
The structural measure was the major solution for flood defense in Taiwan. However, the measure is always limited to the design
standard and cannot prevent the damages when floods exceed certain scale. Therefore, non-structural measures for flood mitigation
are the indispensable complements to structural solutions. The study introduces the establishment of inundation potential
database that provides required information for the non-structural measures in Taiwan. The database was built by numerical
simulations, based on different rainfall scenarios, and has been applied by the local governments of Taiwan for land use managements,
flood warning systems, emergency responses, and flood insurance programs to reduce the flood damages and impacts. 相似文献
374.
Covalent and non-covalent interaction of proteinaceous materials in soils and sediments has been suggested as an important mechanism for immobilizing nitrogen in numerous types of environments. In a previous study (Hsu P.-H., Hatcher, P.G., 2005. New evidence for covalent coupling of peptides to humic acids based on 2D NMR spectroscopy: A means for preservation. Geochimica et Cosmochimica Acta 69, 4521–4533), we provided molecular evidence for covalent, as well as non-covalent, bonding between 15N-labeled peptides and humic acid molecules using the 2D HSQC (heteronuclear single quantum coherence) NMR technique. In this report, we examine the influence of aromaticity and aliphaticity of peptides and humic materials on these covalent and non-covalent interactions. We use 2D NMR techniques to evaluate bonding interactions of 15N labeled peptides, having different aromatic and aliphatic properties, with three humic acids that vary in degree of aromaticity. The peptide containing primarily aromatic amino acid residues is observed to form covalent and non-covalent bonds with mainly aromatic-rich humic acids. The peptide composed of aliphatic amino acid residues shows, on the other hand, only bonding interactions with aliphatic-rich humic acids. These observations provide the first direct molecular evidence that aliphatic functional groups are involved in bonding with proteinaceous materials. The process may play an important role in sequestration of proteinaceous materials in sedimentary systems such as marine systems where the humic materials are mainly aliphatic in nature. 相似文献
375.
In August 2009,Typhoon Morakot brought a large amount of rainfall with both high intensity and long duration to a vast area of Taiwan.Unfortunately,this resulted in a catastrophic landslide in Hsiaolin Village,Taiwan.Meanwhile,large amounts of landslides were formed in the Jiaopu Stream watershed near the southeast part of the Hsiaolin Village.The Hsiaolin Village access road(Provincial Highway No.21 and Bridge No.8) was completely destroyed by the landslide and consequent debris flow.The major scope of this study is to apply a debris flow model to simulate the disaster caused by the debris flow that occurred in the Jiaopu Stream during Typhoon Morakot.According to the interviews with local residents,this study applied the destruction time of Bridge No.8 and Chen's house to verify the numerical debris flow model.By the spatial rainfall distributions information,the numerical simulations of the debris flow are conducted in two stages.In the first stage(before the landslide-dam failure),the elevation of the debris flow and the corresponding potential damages toward residential properties were investigated.In the second stage(after the landslidedam failure),comparisons of simulation results between the longitudinal and cross profiles of the Jiaopu Stream were performed using topographic maps and satellite imagery.In summary,applications of the adopted numerical debris flow model have shown positive impact on supporting better understanding of the occurrence and movement of debris flow processes. 相似文献
376.
377.
Climate Dynamics - Seasonal cycle of China summer precipitation has significant impacts on its subseasonal predictability; yet current understanding of seasonal evolution of the intraseasonal... 相似文献
378.
由于全球变暖,极地地区的气候经历了明显的变暖放大.在本项研究中,我们根据CMIP6模式的三种变暖情景(SSP1-2,6,SSP2-4.5和SSP5-8.5)下,极地放大变化对各个反馈机制(包括普朗克,温度递减率,云,水蒸气,反照率反馈,CO2强迫,海洋热吸收和大气热传输)的响应进行了分析.结果表明,通过用“辐射核”方法... 相似文献
379.
S. A. Hsu 《Boundary-Layer Meteorology》1992,60(4):397-402
The Offshore and Coastal Dispersion (OCD) model proposed and evaluated by Hanna et al. (1985) requires the Monin-Obukhov length to compute the stability class. Both wind shear and heat flux are needed for this computation; since these parameters are not normally observed, the stability length has been converted into a nomogram which consists of routinely measured wind speed and air-sea temperature difference. An analysis of the vertical turbulence intensity as a function of the stability length demonstrates that under neutral conditions, the stability scheme used in the OCD model is reasonable. 相似文献
380.
S. A. Hsu 《Boundary-Layer Meteorology》1983,25(4):417-421
Estimates of the latent heat flux at the air-sea interface made by the profile method are compared to estimates by a wind-wave interaction (WWI) method that takes into account both wind and wave characteristics. A data set that consisted of profile measurements (six levels) of wind, temperature, and humidity over the Arabian Sea was used to compare the methods, and the agreement is good. It is shown that this WWI method can be used to compute the shear velocity, and then the results can be applied in the computation of latent heat flux. The parameters used in the WWI method are wind speed and direction, air temperature and humidity, sea-surface temperature, and significant wave height and period. All these data may be obtained from standard ship observations. 相似文献