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HIDEKAZU MATSUEDA HISAYUKI YOSHIKAWA INOUE MASAO ISHII 《Tellus. Series B, Chemical and physical meteorology》2002,54(1):1-21
Abstract The spatial and temporal variations of atmospheric CO2 at 8–13 km from April 1993 to April 1999 were observed by measuring CO2 mixing ratios in samples collected biweekly from a commercial airliner between Australia and Japan. The CO2 growth rate showed a considerable interannual variation, with a maximum of about 3 ppm yr−1 during late 1997. This variation is related to the El Niño/Southern Oscillation (ENSO) events. A year-to-year change related to the ENSO events was also found in the latitudinal distribution pattern of the CO2 annual mean between 30°N and 30°S. The averaged CO2 seasonal cycle in the Northern Hemisphere gradually decayed toward the equator, and a relatively complicated variation with a double seasonal maximum appeared in the Southern Hemisphere. A significant yearly change of the seasonal cycle pattern was observed in the Southern Hemisphere. The impact of a tropical biomass-burning injection on the upper tropospheric CO2 was estimated on the basis of the CO data from the same airliner observation. 相似文献
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We studied calcite and rhodochrosite from exploratory drill cores (TH‐4 and TH‐6) near the Toyoha deposit, southwestern Hokkaido, Japan, from the aspect of stable isotope geochemistry, together with measuring the homogenization temperatures of fluid inclusions. The alteration observed in the drill cores is classified into four zones: ore mineralized zone, mixed‐layer minerals zone, kaolin minerals zone, and propylitic zone. Calcite is widespread in all the zones except for the kaolin minerals zone. The occurrence of rhodochrosite is restricted in the ore mineralized zone associated with Fe, Mn‐rich chlorite and sulfides, the mineral assemblage of which is basically equivalent to that in the Toyoha veins. The measured δ18OSMOW and δ13CPDB values of calcite scatter in the relatively narrow ranges from ?2 to 5‰ and from ?9 to ?5‰, respectively; those of rhodochrosite from 3 to 9‰ and from ?9 to ?5‰, excluding some data with large deviations. The variation of the isotopic compositions with temperature and depth could be explained by a mixing process between a heated surface meteoric water (100°C δ18O =?12‰, δ13C =?10‰) and a deep high temperature water (300°C, δ18O =?5‰, δ13C =?4‰). Boiling was less effective in isotopic fractionation than that of mixing. The plots of δ18O and δ13C indicate that the carbonates precipitated from H2CO3‐dominated fluids under the conditions of pH = 6–7 and T = 200–300°C. The sequential precipitation from calcite to rhodochrosite in a vein brought about the disequilibrium isotopic fractionation between the two minerals. The hydrothermal fluids circulated during the precipitation of carbonates in TH‐4 and TH‐6 are similar in origin to the ore‐forming fluids pertaining to the formation of veins in the Toyoha deposit. 相似文献
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SHOICHI TAGUCHI HIDEKAZU MATSUEDA HISAYUKI Y. INOUE YOUSUKE SAWA 《Tellus. Series B, Chemical and physical meteorology》2002,54(1):22-40
High concentrations of carbon monoxide (CO) were observed in October 1997 at the upper troposphere of the western tropical Pacific. Transport from the potential sources of CO due to biomass burnings in the tropics was investigated by using a global chemical transport model (CTM) driven by assimilated meteorological data provided from European Centre for Medium-Range Weather Forecasts (ECMWF). A CTM evaluation simulation using water vapor showed that the amount of vertical transport of moisture by large-scale flow was consistent with the precipitation predicted at the convective zone. A series of CTM simulations using 10-day emission periods of an artificial material with lifetime of 60 days indicated that vertical lifting of surface air at the Indonesian archipelago occurred in the concentrated convections west of Sumatra Island. No evidence was found that CO from the Amazon region or Africa significantly contributed to high concentrations in the western tropical Pacific. Transport formed a large-scale anvil below the tropopause by rapid vertical transport and by divergence flow. The average time required for the transport from Kalimantan and Sumatra Island to the point of high CO concentration was about 15 days. High concentrations at an altitude of 10 km in the Southern Hemisphere were transported by large-scale subsidence from the upper tropospheric maximum, which was presumably produced from the sources at Kalimantan and Sumatra Island. Estimated emissions of CO in September and October from Kalimantan and Sumatra were substantially larger than the previous estimates. Omission of chemical reaction was a possible problem for the overestimate, but not significant. The possible problems in the transport were incorrect CTM transport due to insufficient horizontal (2.5×2.5°) and vertical resolution of the CTM, and to inaccuracy in the wind fields at the upper part of the troposphere and a divergent flow pattern in the upper part of the troposphere. 相似文献
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基于相似系数和R/S分析方法的 闽台产业同构性 总被引:3,自引:0,他引:3
产业同构化可能造成区域间产业升级优化和彼此合作发展的瓶颈。选取闽台为研究对象,从三次产业、制造业和第三产业内部结构三个方面着手,应用相似系数指标,分别从静态与动态的角度分析闽台产业同构的现状与变化,并在此基础上,依据分形理论中的R/S分析方法,预测两地产业同构化的未来发展趋势。结果显示,闽台产业同构现象显著,如果在原有条件下继续发展,未来三次产业同构化程度将继续加大,制造业相似性总体上将呈现波动加强态势,第三产业结构同构化程度继续缓慢减小。然而闽台产业同构具有其内在必然性,相似的资源禀赋、日益接近的经济发展水平以及日益紧密的经济联系对产业同构的形成产生了正面影响;同时,产业同构也揭示了闽台产业分工已经由垂直分工向水平分工方向发展。因此宏观层面的产业同构未必给闽台未来经济合作产生明显的负面影响。 相似文献
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Numericalanalysisoftheinteractionofsoil┐structureunderearthquakeloadingGEN-DEZHANG1)(章根德)SHU-CHENGNING2)(宁书成)1)InstituteofMe... 相似文献