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41.
A new particulate Mn-Fe-P-shuttle at the redoxcline of anoxic basins   总被引:1,自引:0,他引:1  
Pelagic redoxclines of anoxic basins and deeps form the suboxic transition between oxygenated surface and anoxic or even sulfidic bottom waters. Intense element cycling, favoured by elevated microbial activity, causes steep gradients of physico-chemical parameters, nutrients and redox-sensitive trace metals. This study presents a conceptual model for authigenic particle formation at pelagic redoxclines, which is based on the tight coupling of Mn, Fe, and P cycles. Besides the well-known occurrence of Mn-oxides, textural (SEM-EDX) and geochemical (ICP-OES, ICP-MS) analyses of particles from the redoxclines of the Black Sea and the Baltic Sea (Gotland Basin, Landsort Deep) evidence the existence of earlier postulated Fe-oxyhydroxo-phosphates and emphasize mixed phases consisting of Mn-oxides and Fe-oxyhydroxo-phosphates as a new solid species. Most of the analyzed particles are star-shaped, of about 5 μm in size, and occur as single particles or aggregates without any morphological differences between Mn-oxides, Fe-oxyhydroxo-phosphates, and mixed phases. Throughout the redoxcline, these minerals show a general succession with maximum abundance of Mn-oxides above the redoxcline followed by mixed phases and almost pure Fe-phosphates within and below the redoxcline, respectively. Molar Fe/P ratios of single particles argue against the formation of known pure Fe-phosphates like vivianite or strengite at the lower end of the redox transition zone, but are consistent with recent experimental findings for colloidal P-bearing hydrous ferric oxides. Moreover, morphological similarities suggest the formation of irregular Fe-oxyhydroxo coatings due to oxidation of upward diffusing Fe2+ by oxygen and stepwise replacement of Mn(IV) by Fe(III) on sinking MnOx particles followed by immediate adsorption or even co-precipitation of phosphate. Batch-type experiments using biogenic MnOx particles demonstrate the efficient potential of Fe2+ oxidation by sinking MnOx particles. When entering sulfidic waters MnOx particles are progressively reduced leading to an increasing relative abundance of Fe- and P-rich particles. In deeper parts of the water column these particles are also reductively dissolved, thereby releasing Fe2+ and phosphate to the water column. This Mn-Fe-P-shuttle likely affects phosphate transport throughout the water column and thus impacts primary production at least over longer time scales. Furthermore, the particulate Mn-Fe-P-shuttle must have played an important role for the cycling of P and certain trace metals in ancient ocean basins, e.g., during certain periods of Cretaceous black shale formation and should be considered in future mass balances and modeling approaches dealing with oxic/anoxic interfaces of aquatic ecosystems.  相似文献   
42.
Lacustrine sediments have been widely used to investigate past climatic and environmental changes on millennial to seasonal time scales. Sedimentary archives of lakes in mountainous regions may also record non-climatic events such as earthquakes. We argue herein that a set of 64 annual laminae couplets reconciles a stratigraphically inconsistent accelerator mass spectrometry (AMS) 14C chronology in a ~4-m-long sediment core from Lake Mengda, in the north-eastern Tibetan Plateau. The laminations suggest the lake was formed by a large landslide, triggered by the 1927 Gulang earthquake (M = 8.0). The lake sediment sequence can be separated into three units based on lithologic, sedimentary, and isotopic characteristics. Starting from the bottom of the sequence, these are: (1) unweathered, coarse, sandy valley-floor deposits or landslide debris that pre-date the lake, (2) landslide-induced, fine-grained soil or reworked landslide debris with a high organic content, and (3) lacustrine sediments with low organic content and laminations. These annual laminations provide a high-resolution record of anthropogenic and environmental changes during the twentieth century, recording enhanced sediment input associated with two phases of construction activities. The high mean sedimentation rates of up to 4.8 mm year?1 underscore the potential for reconstructing such distinct sediment pulses in remote, forested, and seemingly undisturbed mountain catchments.  相似文献   
43.
Concerns related to climate change have resulted in an increasing interest in the importance of hydrological events such as droughts in affecting biogeochemical responses of watersheds. The effects of an unusually dry summer in 2002 had a marked impact on the biogeochemistry of three watersheds in the north‐eastern USA. Chemical, isotopic and hydrological responses with particular emphasis on S dynamics were evaluated for Archer Creek (New York), Sleepers River (Vermont) and Cone Pond (New Hampshire) watersheds. From 1 August to 14 September 2002, all three watersheds had very low precipitation (48 to 69 mm) resulting in either very low or no discharge (mean 0·015, 0·15 and 0·000 mm day?1 for Archer Creek, Sleepers River and Cone Pond, respectively). From 15 September to 31 October 2002, there was a substantial increase in precipitation totals (212, 246 and 198 mm, respectively) with increased discharge. Archer Creek was characterized by a large range of SO42? concentrations (152 to 389 µeq L?1, mean = 273 µeq L?1) and also exhibited the greatest range in δ34S values of SO42? (?1·4 to 8·8 ‰ ). Sleepers River's SO42? concentrations ranged from 136 to 243 µeq L?1 (mean = 167 µeq L?1) and δ34S values of SO42? ranged from 4·0 to 9·0 ‰ . Cone Pond's SO42? concentrations (126–187 µeq L?1, mean = 154 µeq L?1) and δ34S values (2·4 to 4·3 ‰ ) had the smallest ranges of the three watersheds. The range and mean of δ18O‐SO42? values for Archer Creek and Cone Pond were similar (3·0 to 8·9 ‰ , mean = 4·5 ‰ ; 3·9 to 6·3 ‰ , mean = 4·9 ‰ ; respectively) while δ18O‐SO42? values for Sleepers River covered a larger range with a lower mean (1·2 to 10·0 ‰ , mean = 2·5). The difference in Sleepers River chemical and isotopic responses was attributed to weathering reactions contributing SO42?. For Archer Creek wetland areas containing previously reduced S compounds that were reoxidized to SO42? probably provided a substantial source of S. Cone Pond had limited internal S sources and less chemical or isotopic response to storms. Differences among the three watersheds in S biogeochemical responses during these storm events were attributed to differences in S mineral weathering contributions, hydrological pathways and landscape features. Further evaluations of differences and similarities in biogeochemical and hydrological responses among watersheds are needed to predict the impacts of climate change. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   
44.
We present intermediate-resolution HST /STIS spectra of a high-velocity interstellar cloud ( v LSR=+80 km s−1) towards DI 1388, a young star in the Magellanic Bridge located between the Small and Large Magellanic Clouds. The STIS data have a signal-to-noise ratio (S/N) of 20–45 and a spectral resolution of about 6.5 km s−1 (FWHM). The high-velocity cloud absorption is observed in the lines of C  ii , O  i , Si  ii , Si  iii , Si  iv and S  iii . Limits can be placed on the amount of S  ii and Fe  ii absorption that is present. An analysis of the relative abundances derived from the observed species, particularly C  ii and O  i , suggests that this high-velocity gas is warm ( T k∼103–104 K) and predominantly ionized. This hypothesis is supported by the presence of absorption produced by highly ionized species, such as Si  iv . This sightline also intercepts two other high-velocity clouds that produce weak absorption features at v LSR=+113 and +130 km s−1 in the STIS spectra.  相似文献   
45.
Cosmological perturbations on a F-R-W background are considered in a modified de Donder gauge. To guarantee the energy-momentum conservation for the perturbations in the de Donder gauge a compatibility condition is obtained. Finally we present the basic equations for the propagation of spherically symmetric perturbations. These equations are the basis for investigating the influence of cosmological epoches on the growing of density contrasts.  相似文献   
46.
Exploratory synthetic spectra were computed for carbon-rich long-period variables. We used dynamic model atmospheres of Höfner &; Dorfi (1997) and calculated partial pressures, absorption- and scattering coefficients as input for the spectral synthesis code of Jørgensen et al. (1992). First ISO SWS-observations of the carbon-Mira T Dra are compared with our synthetic spectra.  相似文献   
47.
48.
Three successive Mesozoic neptunian dyke generations and related unconformities suggest recurrent extensional fracturing and periods of relative sea-level rise along the NW Trento Plateau margin in the Southern Alps, Italy. The first neptunian dyke generation was induced by NNW–SSE directed extension of Early Jurassic skeletal oolitic periplatform deposits generating micritic early Middle Liassic neptunian dykes with orthogonal orientation. The second generation of neptunian dykes was possibly caused by marginal extension at the drowned platform edge penetrating Late Jurassic, red pelagic limestones with a pelagic matrix of Albian/Cenomanian age and nearly orthogonal fracture orientation. The third generation of neptunian dykes occurred after a prolonged period of submarine exposure and erosion (Aptian/Albian to Late Maastrichtian) during the rapid burial of the submarine Trento Plateau margin relief. The Late Maastrichtian neptunian dykes were caused by extension of Early to Middle Jurassic oolitic periplatform limestones along steep (inclination > 10°) submarine slopes. Generally successive neptunian dyke generations along drowned carbonate platform margins could be caused by repeated extensional brittle fracturing of lithified periplatform deposits and the filling of micritic matrix derived from overlying pelagic sediment sequences under substantial hydrostatic pressure. This would suggest that recurrent extensional fracturing is continuously recorded by neptunian dyke formation which could be used to indicate extensional tectonic activity at a foundering deep-marine carbonate platform edge.  相似文献   
49.
Morphological changes in coastal areas, especially in river estuaries, are of high interest in many parts of the world. Satellite data from both optical and radar sensors can help to monitor and investigate these changes. Data from both kinds of sensors being available for up to 30 years now, allow examinations over large timescales, while high resolution sensors developed within the last decade allow increased accuracy. So the creation of digital elevation models (DEMs) of, for example, the wadden sea from a series of satellite images is already possible. ENVISAT, successfully launched on March 1, 2002, continues the line of higher resolution synthetic aperture radar (SAR) imaging sensors with its ASAR instrument and now also allows several polarization modes for better separation of land and water areas. This article gives an overview of sensors and algorithms for waterline determination as well as several applications. Both optical and SAR images are considered. Applications include morphodynamic monitoring studies and DEM generation.
Andreas NiedermeierEmail:
  相似文献   
50.
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