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11.
Trace elements contamination of agricultural soils affected by sulphide exploitation (Iberian Pyrite Belt,Sw Spain) 总被引:1,自引:0,他引:1
Agricultural soils of the Riotinto mining area (Iberian Pyrite Belt) have been studied to assess the degree of pollution by
trace elements as a consequence of the extraction and treatment of sulphides. Fifteen soil samples were collected and analysed
by ICP-OES and INAA for 51 elements. Chemical analyses showed an As–Cu–Pb–Zn association related with the mineralisation of
the Iberian Pyrite Belt. Concentrations were 19–994 mg kg−1 for As, 41–4,890 mg kg−1 for Pb, 95–897 mg kg−1 for Zn and of 27–1,160 mg kg−1 for Cu. Most of the samples displayed concentrations of these elements higher than the 90th percentile of the corresponding
geological dominium, which suggests an anthropogenic input besides the bedrock influence. Samples collected from sediments
were more contaminated than leptosols because they were polluted by leachates or by mining spills coming from the waste rock
piles. The weathering of the bedrock is responsible for high concentrations in Co, Cr and Ni, but an anthropogenic input,
such as wind-blown dust, seems to be indicative of the high content of As, Cu, Pb and Zn in leptosols. The metal partitioning
patterns show that most trace elements are associated with Fe amorphous oxy-hydroxides, or take part of the residual fraction.
According to the results obtained, the following mobility sequence is proposed for major and minor elements: Mn, Pb, Cd, > Zn,
Cu > Ni > As > Fe > Cr. The high mobility of Pb, Cu and Zn involve an environmental risk in this area, even in soils where
the concentrations are not so high. 相似文献
12.
J. L. Simón M. A. Soriano L. E. Arlegui J. Gracia C. L. Liesa A. Pocoví 《Environmental Geology》2008,53(5):1057-1065
Space and time variations of alluvial karst subsidence in the central Ebro Basin are analysed in trenches (paleodolines),
aerial photographs (historical dolines) and field surveys (present-day active dolines). The measured subsidence rates, as
well as a comparison between densities of paleodolines computed in randomly selected scan-lines and density of active dolines
computed in maps, suggest that present-day subsidence in favourable areas is more intense than that of Pleistocene times.
According to diachronic maps drawn from (a) different aerial photographs taken after 1946 and (b) field surveys on deformations
in urbanized areas, subsidence behaved as a nearly steady process while the whole area was used for agriculture. In contrast,
rapid changes (through periods of several tens of years) have occurred in urbanized areas, in which dolines expand their boundaries
through small marginal collapses, shifting sharply their sinking centres to neighbouring sites. These rapid changes do not
have an equivalent in observed paleodolines. 相似文献
13.
Quick-look assessments to identify optimal CO2 EOR storage sites 总被引:1,自引:0,他引:1
Vanessa Núñez-López Mark H. Holtz Derek J. Wood William A. Ambrose Susan D. Hovorka 《Environmental Geology》2008,54(8):1695-1706
A newly developed, multistage quick-look methodology allows for the efficient screening of an unmanageably large number of
reservoirs to generate a workable set of sites that closely match the requirements for optimal CO2 enhanced oil recovery (EOR) storage. The objective of the study is to quickly identify miscible CO2 EOR candidates in areas that contain thousands of reservoirs and to estimate additional oil recovery and sequestration capacities
of selected top options through dimensionless modeling and reservoir characterization. Quick-look assessments indicate that
the CO2 EOR resource potential along the US Gulf Coast is 4.7 billion barrels, and CO2 sequestration capacity is 2.6 billion metric tons. In the first stage, oil reservoirs are screened and ranked in terms of
technical and practical feasibility for miscible CO2 EOR. The second stage provides quick estimates of CO2 EOR potential and sequestration capacities. In the third stage, a dimensionless group model is applied to a selected set
of sites to improve the estimates of oil recovery and storage potential using appropriate inputs for rock and fluid properties,
disregarding reservoir architecture and sweep design. The fourth stage validates and refines the results by simulating flow
in a model that describes the internal architecture and fluid distribution in the reservoir. The stated approach both saves
time and allows more resources to be applied to the best candidate sites. 相似文献
14.
The Cu–Co–Ni Texeo mine has been the most important source of Cu in NW Spain since Roman times and now, approximately 40,000 m3 of wastes from mine and metallurgical operations, containing average concentrations of 9,263 mg kg−1 Cu, 1,100 mg kg−1 As, 549 mg kg−1 Co, and 840 mg kg−1 Ni, remain on-site. Since the cessation of the activity, the abandoned works, facilities and waste piles have been posing
a threat to the environment, derived from the release of toxic elements. In order to assess the potential environmental pollution
caused by the mining operations, a sequential sampling strategy was undertaken in wastes, soil, surface and groundwater, and
sediments. First, screening field tools were used to identify hotspots, before defining formal sampling strategies; so, in
the areas where anomalies were detected in a first sampling stage, a second detailed sampling campaign was undertaken. Metal
concentrations in the soils are highly above the local background, reaching up to 9,921 mg kg−1 Cu, 1,373 mg kg−1 As, 685 mg kg−1 Co, and 1,040 mg kg−1 Ni, among others. Copper concentrations downstream of the mine works reach values up to 1,869 μg l−1 and 240 mg kg−1 in surface water and stream sediments, respectively. Computer-based risk assessment for the site gives a carcinogenic risk
associated with the presence of As in surface waters and soils, and a health risk for long exposures; so, trigger levels of
these elements are high enough to warrant further investigation. 相似文献
15.
Vittorio Zanon Fátima Viveiros Catarina Silva Ana Rita Hipólito Teresa Ferreira 《Natural Hazards》2008,45(1):19-31
A detailed study was carried out on a piece of land that had been struck by lightning during the violent rainstorm that raged
over the Island of S?o Miguel (Azores Archipelago) in late October 2006. Temperature and gas measurements (CO2, CO, H2S and CH4) were performed in four study trenches, dug in an area of ∼3 m2, where an underground fire had been initiated by the impact with a lightning stroke, followed by the emission of a column
of gases and smoke. The soil under study was originally a well-pedogenized about 80 cm thick bed, made of volcanic clayey
to silty tephra fallouts and contained 5.5–9.7% of organic matter. The underground fire was monitored for one week and revealed a peak release of
404 ppm CO and 3.4% CO2 originating from a horizon located about 45 cm under the soil surface. Measurements of temperature, performed one week after
the impact, indicated a maximum value of 326°C inside the soil, while 516.5°C were measured on the surface of a lava block
interred about 20 cm under the surface. Subsequently, a stratigraphic and sedimentologic study proved the role of the grain-size
of the soil and of the organic matter content of the different horizons of the impact area, in determining the ratio between
anoxic/oxidised combustion conditions and in the progress of the process itself. It was also noticed that combustion was not
total all over in the soil bed and that the process had slightly migrated toward SW during the observation period. The combustion
process went on for about ten days, in spite of several other violent rainstorms, until it was artificially extinguished through
the excavations made to obtain study trenches. This particular circumstance evidenced the potential natural hazard represented
by this kind of atmospheric event, especially in a land where the volcanic nature of the soil may easily mislead inexperienced
observers and, consequently, delay proper action. 相似文献
16.
Rain-induced debris and mudflow triggering factors assessment in the Santiago cordilleran foothills,Central Chile 总被引:1,自引:1,他引:0
Debris and mudflows are some of the main geological hazards in the mountain foothills of the Chilean capital city of Santiago.
There, the risk of flows triggered in the basins of ravines that drain the range into the city increases with time due to
the city growth. A multivariate statistical study based on the logistic regression method is presented. The model provides
equations that allow the computation of combined meteorological triggering factors associated with a probability of rain-induced
flow occurrence. Daily rainfall, accumulated rainfall and the snowfall level, traditionally considered as the relevant factors,
are analysed for a 25-year period. The results show a strong relevance of the rainfall on the day of the flow event over the
other factors. However, the relatively low probabilities returned for some real flow events suggest that the model does not
capture all the significant variables and the problem is more complex than as it has been traditionally assumed, and further
investigations are needed to develop predictive models of flow triggering. 相似文献
17.
M. Mejías J. Garcia-Orellana J. L. Plata M. Marina E. Garcia-Solsona B. Ballesteros P. Masqué J. López C. Fernández-Arrojo 《Environmental Geology》2008,54(3):521-536
A methodology for the characterization of deep carbonate aquifers has been developed and applied to El Maestrazgo Jurassic
aquifer in Castellón, Spain. Characterization of these aquifer formations, located at more than 300 m deep, consisted of a
previous phase of compilation, analysis and synthesis of the existing information about the area, followed by a coordinated
combination of different speciality studies: geology, stratigraphy, structural analysis, hydrogeology, hydrochemistry, geophysics
and remote sensing. Geological studies included geological mapping, definition of stratigraphical units and facies and structural
analysis. The aim of the hydrogeology study was to define aquifer formations, recharge area, aquifer points inventory and
groundwater flow directions for the establishment of piezometric and water quality observation nets. Special techniques were
applied, like thermal infrared aerial images and the evaluation of submarine groundwater discharge by means of natural radium
isotopes. Hydrochemical techniques, including majority elements characterization and stable isotopes (18O, 2H and 3H) determination, allowed classifying hydrochemical facies and establishing a renewal pattern for water within the system.
Geophysics was useful in determining the aquifer geometry, the features of the basement and the petrophysical characteristics
of the geological formations. Preliminary results show an important tectonic complexity and the possibilities for groundwater
uses in the area of study. 相似文献
18.
The Cambrian-Vendian groundwater body plays an important role in drinking water supply of capital Tallinn and other settlements
in northern Estonia. Water quality in this deep-seated confined groundwater body is influenced by the intrusion of present-day
seawater and pumping-induced upward migration of deeper saline groundwater. The aim of this study is to evaluate the threshold
values applying the methodology worked out within the EU 6th FP project “Background criteria for the identification of groundwater
thresholds (BRIDGE)” and to compare the results with the values proposed by local authorities. A database containing 250 monitoring
points was completed and used for the calculation of natural background levels (as the 90 and 97.7 percentile) in groundwater.
The calculation of threshold values is based on natural background levels and reference values. In case of Cambrian-Vendian
groundwater body the receptor is drinking water, thus limit values set by Estonian drinking water standard were used as reference
values. The threshold values proposed by local authorities are more or less the same as calculated by BRIDGE methodology.
Exceptionally different values are derived in case of chloride and ammonium. 相似文献
19.
Summary Using the results of spherical harmonic analyses of the geomagnetic field for some fourteen different epochs, includingGauss' first analysis for epoch 1835, and theErman-Petersen analysis for epoch 1829, the strength and axes of geomagnetic multipoles have been computed. In particular, a dipole from the three first order spherical harmonic coefficients, a quadrupole from five second order coefficients, and an octupole from seven third order coefficients. The axes of the quadrupole and octupole have moved quite rapidly when compared with movements of the dipole axis, and show a general movement westwards. Although the strength of the dipole has generally diminished, the strengths of the quadrupole and octupole have generally increased.On leave National University of La Plata, Argentina 相似文献
20.
Leaños-Castañeda O Gold-Bouchot G Van Der Kraak G Lister A Ceja-Moreno V Simá-Alvarez R 《Marine environmental research》2004,58(2-5):337-342
The objective of this study was to determine if tamoxifen or an aromatase inhibitor (4-hydroxyandrostenedione; 4-OHA) affected plasma concentrations of o,p' -DDT and its metabolites, o,p'-DDD and o,p'-DDE, in mature tilapia. Male and female tilapia were injected 6 times intraperitoneally with o,p'-DDT (40 mg/kg) alone or in combination with 4-OHA (2 mg/kg) over a 12 day period. An additional group of male fish was injected with tamoxifen (5 mg/kg) plus o,p'-DDT. At the end of the treatment period, plasma samples were extracted and analyzed by GC/ECD. Females injected only with o,p'-DDT had significantly higher levels of o,p'-DDT compared with males. Interestingly, females and males treated concomitantly with o,p'-DDT and 4-OHA or tamoxifen had significantly lower concentrations of plasma o,p'-DDT (about 50%) compared with fish treated with only o,p'-DDT. These initial results suggest that an interaction between endocrine-active compounds occurs in vivo in tilapia and may involve alterations in metabolism of o,p'-DDT. 相似文献