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131.
Surface complexation modeling of Cu(II) adsorption on mixtures of hydrous ferric oxide and kaolinite
Tracy J Lund Carla M Koretsky Christopher J Landry Melinda S Schaller Soumya Das 《Geochemical transactions》2008,9(1):9
Background
The application of surface complexation models (SCMs) to natural sediments and soils is hindered by a lack of consistent models and data for large suites of metals and minerals of interest. Furthermore, the surface complexation approach has mostly been developed and tested for single solid systems. Few studies have extended the SCM approach to systems containing multiple solids. 相似文献132.
Many Gulf of Mexico estuaries have low ratios of water volume to bottom surface area, and benthic processes in these systems
likely have a major influence on system structure and function. The purpose of this study was to determine the spatiotemporal
distribution of biomass and community composition of subtidal benthic microalgal (BMA) communities in Galveston Bay, TX, USA,
compare BMA community composition and biomass to phytoplankton in overlying waters, and estimate the potential contribution
of BMA to the trophodynamics in this shallow, turbid, subtropical estuary. The estimates of BMA biomass (mean = 4.21 mg Chl
a m−2) for Galveston Bay were within the range of the reported values for similar Gulf of Mexico estuaries. BMA biomass in the
central part of the bay was essentially homogeneous, whereas biomass at the seaward and upper bay ends of the transect were
significantly lower. Peridinin, fucoxanthin, and alloxanthin were the three carotenoids with the highest concentrations, with
fucoxanthin having the highest mean concentration (1.82 mg m−2). The seaward and landward ends of the transect differed from the central region of the bay with respect to the relative
abundances of chlorophytes, cyanobacteria, and photosynthetic bacteria. Benthic microalgal community composition also showed
a gradual shift over time due to changes in the relative abundances of photosynthetic bacteria, cryptophytes, dinoflagellates,
and cyanobacteria. Major changes in community composition occurred in the spring months (March to April). On an areal basis,
BMA biomass in Galveston Bay occurred at minor concentrations (16.5%) relative to phytoplankton. Furthermore, the concentrations
of carotenoid pigments for phytoplankton and BMA (fucoxanthin, alloxanthin, and zeaxanthin) were correlated (r = 0.48 to 0.61), suggesting a close linkage between microalgae in the water column and sediments. The contribution of BMA
to the primary productivity of the deeper waters (>2 m) of Galveston Bay is probably very small in comparison to shallower
waters along the bay margins. The significant similarities in the community composition of phytoplankton and BMA illustrate
the potential importance of deposition and resuspension processes in this turbid, shallow estuary. 相似文献
133.
Macrofaunal Spatial Patterns in Relationship to Environmental Variables in the Richibucto Estuary,New Brunswick,Canada 总被引:1,自引:0,他引:1
Estuarine macrobenthos respond to a variety of environmental gradients such as sediment type and salinity, and organic enrichment.
A relatively new influence, organic loading from suspended bivalve culture, has the potential to alter this response. A study
on soft-bottom macrobenthic communities was carried out in the Richibucto estuary (46°40′N, 64°50′W), New Brunswick, Canada,
with samples collected from 18 stations in late September and early October 2006. The site consisted of a large tidal channel
originating upstream in a small river. The channel was punctuated by bag culture of oysters along its length. A total of 88
species were recorded. The mean values of abundance, species richness, and diversity (H′) of macrofauna were 11,199 ind. m−2 (ranged from 4,371 to 19,930 ind. m−2), 23.4 species grab−1 and 3.29 grab−1, respectively. In general species richness and H′ increased from the upper estuary to the estuarine mouth. Multivariate analyses clearly exhibited the spatial distribution
in community structure, which coincided with the locations along the estuary (the upper, the lower and the mouth), as well
as inside and outside the channel. Species richness and diversity H′ showed strong positive correlations with salinity (21.2–25.2 ppt), and abundance was positively correlated with water depth
(1.0–4.5 m). Abundance and species richness were negatively correlated with both of silt–clay fraction (3.3–24.8%) and sorting
(σI). Species richness was also negatively correlated with organic content (1.9–12.7%). The BIO-ENV analyses identified silt–clay
fraction, σI and salinity as the major environmental variable combination influencing the macrofaunal patterns, and silt–clay fraction
as the single best-correlated variable. 相似文献
134.
135.
Florencia Botto Agustina Mendez-Casariego Macarena Valiñas Oscar Iribarne 《Estuaries and Coasts》2008,31(1):134-143
We show that, as previously described, there are conflicts between areas used by people and shorebirds. However, we propose
that burrowing organisms add complexity to the shorebird–human interaction that should be taken into account for management
and conservation. This is because SW Atlantic mudflats are dominated by high densities (up to 60 crabs m−2) of a strong bioturbator, the burrowing crab Neohelice granulata (=Chasmagnathus granulatus). These crabs affect the habitat use and foraging performance of shorebird species. The two-banded plover Charadrius falklandicus feed more in burrow areas whereas the yellowlegs Tringa spp. and the white-rumped sandpiper Calidris fuscicollis tend to avoid burrow areas. We evaluated the effect of human recreational activities on shorebirds, taking into account shorebird–crab
interaction, during shorebird migratory periods (November to April) of 2001, 2002, and 2003. This study was performed at the
Mar Chiquita coastal lagoon (37° 40′ S, Argentina). Results showed that people only rarely used the extensive soft bottom
intertidals dominated by burrowing assemblages of N. granulata because the soft sediments make walking difficult. Therefore, human impact is reduced for the two-banded plover. However,
for several migratory shorebirds that also avoid burrow areas, these areas act as suboptimal alternative areas when human
impact is important in their preferred habitats. When human activity is low, shorebirds remain foraging in the area but they
decrease their feeding intakes. The extensions of burrow areas differ among estuaries and are likely to generate between-estuaries
differences as stopover sites for shorebirds. Also, other species that form large burrowing assemblages can have a similar
impact on shorebird–human interactions. 相似文献
136.
We developed light requirements for eelgrass in the Pacific Northwest, USA, to evaluate the effects of short- and long-term
reductions in irradiance reaching eelgrass, especially related to turbidity and overwater structures. Photosynthesis-irradiance
experiments and depth distribution field studies indicated that eelgrass productivity was maximum at a photosynthetic photon
flux density (PPFD) of about 350–550 μmol quanta m−2 s−1. Winter plants had approximately threefold greater net apparent primary productivity rate at the same irradiance as summer
plants. Growth studies using artificial shading as well as field monitoring of light and eelgrass growth indicated that long-term
survival required at least 3 mol quanta m−2 day−1 on average during spring and summer (i.e., May-September), and that growth was saturated above about 7 mol quanta m−2 day−1. We conclude that non-light-limited growth of eelgrass in the Pacific Northwest requires an average of at least 7 mol quanta
m−2 day−1 during spring and summer and that long-term survival requires a minimum average of 3 mol quanta m−2 day−1. 相似文献
137.
Dynamic data integration for structural modeling: model screening approach using a distance-based model parameterization 总被引:2,自引:0,他引:2
This paper proposes a novel history-matching method where reservoir structure is inverted from dynamic fluid flow response.
The proposed workflow consists of searching for models that match production history from a large set of prior structural
model realizations. This prior set represents the reservoir structural uncertainty because of interpretation uncertainty on
seismic sections. To make such a search effective, we introduce a parameter space defined with a “similarity distance” for
accommodating this large set of realizations. The inverse solutions are found using a stochastic search method. Realistic
reservoir examples are presented to prove the applicability of the proposed method. 相似文献
138.
Analyses of 72 samples from Upper Panjhara basin in the northern part of Deccan Plateau, India, indicate that geochemical
incongruity of groundwater is largely a function of mineral composition of the basaltic lithology. Higher proportion of alkaline
earth elements to total cations and HCO3>Cl + SO4 reflect weathering of primary silicates as chief source of ions. Inputs of Cl, SO4, and NO3 are related to rainfall and localized anthropogenic factors. Groundwater from recharge area representing Ca + Mg–HCO3 type progressively evolves to Ca + Na–HCO3 and Na–Ca–HCO3 class along flow direction replicates the role of cation exchange and precipitation processes. While the post-monsoon chemistry
is controlled by silicate mineral dissolution + cation exchange reactions, pre-monsoon variability is attributable chiefly
to precipitation reactions + anthropogenic factors. Positive correlations between Mg vs HCO3 and Ca + Mg vs HCO3 supports selective dissolution of olivine and pyroxene as dominant process in post-monsoon followed by dissolution of plagioclase
feldspar and secondary carbonates. The pre-monsoon data however, points toward the dissolution of plagioclase and precipitation
of CaCO3 supported by improved correlation coefficients between Na + Ca vs HCO3 and negative correlation of Ca vs HCO3, respectively. It is proposed that the eccentricity in the composition of groundwater from the Panjhara basin is a function
of selective dissolution of olivine > pyroxene followed by plagioclase feldspar.
The data suggest siallitization (L < R and R
k) as dominant mechanism of chemical weathering of basalts, stimulating monosiallitic (kaolinite) and bisiallitic (montmorillonite)
products. The chemical denudation rates for Panjhara basin worked out separately for the ground and surface water component
range from 6.98 to 36.65 tons/km2/yr, respectively. The values of the CO2 consumption rates range between 0.18 × 106 mol//km2/yr (groundwater) and 0.9 × 106 mol/km2/yr (surface water), which indicates that the groundwater forms a considerable fraction of CO2 consumption, an inference, that is, not taken into contemplation in most of the studies. 相似文献
139.
A multi-lithology diffusive stratigraphic model is considered, which simulates at large scales in space and time the infill
of sedimentary basins governed by the interaction between tectonics displacements, eustatic variations, sediment supply, and
sediment transport laws. The model accounts for the mass conservation of each sediment lithology resulting in a mixed parabolic,
hyperbolic system of partial differential equations (PDEs) for the lithology concentrations and the sediment thickness. It
also takes into account a limit on the rock alteration velocity modeled as a unilaterality constraint. To obtain a robust,
fast, and accurate simulation, fully and semi-implicit finite volume discre tization schemes are derived for which the existence
of stable solutions is proved. Then, the set of nonlinear equations is solved using a Newton algorithm adapted to the unilaterality
constraint, and preconditioning strategies are defined for the solution of the linear system at each Newton iteration. They
are based on an algebraic approximate decoupling of the sediment thickness and the concentration variables as well as on a
proper preconditioning of each variable. These algorithms are studied and compared in terms of robustness, scalability, and
efficiency on two real basin test cases. 相似文献
140.
Environmental tracers as indicators of karst conduits in groundwater in South Dakota,USA 总被引:3,自引:1,他引:2
Environmental tracers sampled from the carbonate Madison aquifer on the eastern flank of the Black Hills, South Dakota, USA indicated the approximate locations of four major karst conduits. Contamination issues are a major concern because these conduits are characterized by direct connections to sinking streams, high groundwater velocities, and proximity to public water supplies. Objectives of the study were to estimate approximate conduit locations and assess possible anthropogenic influences associated with conduits. Anomalies of young groundwater based on chlorofluorocarbons (CFCs), tritium, and electrical conductivity (EC) indicated fast moving, focused flow and thus the likely presence of conduits. δ18O was useful for determining sources of recharge for each conduit, and nitrate was a useful tracer for assessing flow paths for anthropogenic influences. Two of the four conduits terminate at or near a large spring complex. CFC apparent ages ranged from 15 years near conduits to >50 years in other areas. Nitrate-N concentrations >0.4 mg/L in groundwater were associated with each of the four conduits compared with concentrations ranging from <0.1 to 0.4 mg/L in other areas. These higher nitrate-N concentrations probably do not result from sinking streams but rather from other areas of infiltration. 相似文献