The shale gas boom in the United States spurred a shift in electricity generation from coal to natural gas. Natural gas combined cycle units emit half of the CO2 to produce the same energy as a coal unit; therefore, the market trend is credited for a reduction in GHG emissions from the US power sector. However, methane that escapes the natural gas supply chain may undercut these relative climate benefits. In 2016, Canada, the United States and Mexico pledged to reduce methane emissions from the oil and natural gas sector 40–45% from 2012 levels by 2025. This article reviews the science-policy landscape of methane measurement and mitigation relevant for meeting this pledge, including changes in US policy following the 2016 presidential election. Considerable policy incoherence exists in all three countries. Reliable inventories remain elusive; despite government and private sector research efforts, the magnitude of methane emissions remains in dispute. Meanwhile, mitigation efforts vary significantly. A framework that integrates science and policy would enable actors to more effectively inform, leverage and pursue advances in methane measurement and mitigation. The framework is applied to North America, but could apply to other geographic contexts.
Key policy insights
The oil and gas sector’s contribution to atmospheric methane concentrations is becoming an increasingly prominent issue in climate policy.
Efforts to measure and control fugitive methane emissions do not presently proceed within a coherent framework that integrates science and policy.
In 2016, the governments of Canada, Mexico and the United States pledged to reduce methane emissions from the oil and natural gas sector 40–45% from 2012 levels by 2025.
The 2016 presidential election in the United States has halted American progress at the federal level, suggesting a heavier reliance on industry and subnational efforts in that country.
Collectively or individually, the countries, individual agencies, or private stakeholders could use the proposed North American Methane Reduction framework to direct research, enhance monitoring and evaluate mitigation efforts, and improve the chances that continental methane reduction targets will be achieved.
Bio-physical glider measurements from a unique process-oriented experiment in the Eastern Alboran Sea (AlborEx) allowed us to observe the distribution of the deep chlorophyll maximum (DCM) across an intense density front, with a resolution (~ 400 m) suitable for investigating sub-mesoscale dynamics. This front, at the interface between Atlantic and Mediterranean waters, had a sharp density gradient (Δρ ~ 1 kg/m3 in ~ 10 km) and showed imprints of (sub-)mesoscale phenomena on tracer distributions. Specifically, the chlorophyll-a concentration within the DCM showed a disrupted pattern along isopycnal surfaces, with patches bearing a relationship to the stratification (buoyancy frequency) at depths between 30 and 60 m. In order to estimate the primary production (PP) rate within the chlorophyll patches observed at the sub-surface, we applied the Morel and Andrè (J Geophys Res 96:685–698 1991) bio-optical model using the photosynthetic active radiation (PAR) from Argo profiles collected simultaneously with glider data. The highest production was located concurrently with domed isopycnals on the fresh side of the front, suggestive that (sub-)mesoscale upwelling is carrying phytoplankton patches from less to more illuminated levels, with a contemporaneous delivering of nutrients. Integrated estimations of PP (1.3 g C m?2d?1) along the glider path are two to four times larger than the estimations obtained from satellite-based algorithms, i.e., derived from the 8-day composite fields extracted over the glider trip path. Despite the differences in spatial and temporal sampling between instruments, the differences in PP estimations are mainly due to the inability of the satellite to measure DCM patches responsible for the high production. The deepest (depth > 60 m) chlorophyll patches are almost unproductive and probably transported passively (subducted) from upper productive layers. Finally, the relationship between primary production and oxygen is also investigated. The logarithm of the primary production in the DCM interior (chlorophyll (Chl) > 0.5 mg/m3) shows a linear negative relationship with the apparent oxygen utilization, confirming that high chlorophyll patches are productive. The slope of this relationship is different for Atlantic, mixed interface waters and Mediterranean waters, suggesting the presence of differences in planktonic communities (whether physiological, population, or community level should be object of further investigation) on the different sides of the front. In addition, the ratio of optical backscatter to Chl is high within the intermediate (mixed) waters, which is suggestive of large phytoplankton cells, and lower within the core of the Atlantic and Mediterranean waters. These observations highlight the relevance of fronts in triggering primary production at DCM level and shaping the characteristic patchiness of the pelagic domain. This gains further relevance considering the inadequacy of optical satellite sensors to observe DCM concentrations at such fine scales. 相似文献
CO2 emissions to the atmosphere were studied in a fertilized sandy agricultural soil with and without a catch crop sown into the main crop. The catch crop was grown primarily with the purpose to decrease N-leaching but this study also wanted to find out if the catch crop could have an effect in a climate change perspective. Plots with catch crop showed decreased CO2 emissions from the soil. Since previous results have shown that catch crops effectively decrease N-leaching we recommend growing catch crops as an effective measure for helping both the climate and the eutrophication issue. Seasonal variations in CO2 emissions were pronounced with maximum emissions from the fertilized agricultural soil in June and from an adjacent unmanaged grassland in August. From the plot with catch crop emissions decreased in July and August but somewhat increased later in the autumn. Fertilized agricultural soil showed a within-soil CO2 sink after harvest, i.e. within-soil CO2 uptake. Availability of NH4+ or NO3- in the soil seems to influence the within-soil CO2 sink, with NH4+ enforcing the sink while the same amount of NO3- instead increased CO2 emissions. 相似文献
Boron and Li isotopes have been tested as environmental tracers of treated sewage injected into a sandy aquifer (Shafdan reclamation project, Israel). During a 38 days injection test in a newly dug injection well, a conservative artificial tracer (Br−) was monitored together with δ11B and δ7Li in the injectate, in the unsaturated soil zone (porous cup) and an observation well in the aquifer. In spite of B and Li concentrations in the injectate close to background values, significant shifts of the isotope signatures could be observed over the duration of the injection test. Boron isotope ratios show a breakthrough curve delayed with respect to Br− breakthrough due to some reversible sorption on the aquifer material. No isotope fractionation was observed in the unsaturated or the saturated zone so that B isotopes can be considered as conservative in the investigated part of the aquifer system. Lithium isotopes are strongly fractionated, probably due to sorption processes. Lithium concentrations point to a Li sink in the system, δ7Li values vary strongly with a tendency of 7Li depletion in the liquid phase over the duration of the experiment. This is opposite to the expected preferential sorption of 6Li onto clay minerals. Boron isotopes reveals a valuable tracer of artificial recharge of freshwaters derived from treated sewage, both for short term tracer tests and for long-term monitoring of artificial recharge, even if in aquifers with higher clay contents, sorption-linked isotope fractionation cannot be excluded. More data are needed on Li isotope fractionation in natural groundwater systems to assess the potential of this tracer as monitoring tool. 相似文献
Climate change in contrasting river basins: adaptation strategies for water, food and environment. Edited by J Aerts and P Droogers. Published in 2004 by CABI Publishing, 288 p., hardcover. ISBN: 0–85199–835–6. Price: US$100 (orders: services@dadirect.com.au). Australian water bugs. Their biology and identification (Hemiptera‐Heteroptera, Gerromorpha &; Nepomorpha). By Nils M Andersen? and Tom A Weir. Published in 2004 by CSIRO Publishing/Apollo Books, P.O. Box 1139, Collingwood, VIC 3066, Australia. 344 p., hardcover. ISBN: 0–643–090517. Price: AU$135.00 (orders: publishing.sales@csiro.au). The Lakes Handbook. Volume I: Limnology and Limnetic Ecology. Volume II: Lake restoration and rehabilitation. Edited by Patrick O'Sullivan and Colin Reynolds. Published by Blackwell Publishing Ltd., 109 Cowley Road, Oxford OX4 1JF, United Kingdom (http//www.blackwellpublishing.com). Volume I (published in 2003) 712 p., hardcover. ISBN: 0632047976. Price: £125. Volume II (published in 2004) 568 p., hardcover. ISBN: 063204795X. Price: £125. 相似文献
The precise application of risk assessment can lead to different conclusions about risk depending on how species are grouped in the assessment. We compared the use of different risk assessment methods for three different classes of pesticide, the herbicide diuron, the fungicide chlorothalonil, and the insecticide permethrin for marine and estuarine species. Permethrin was the most toxic pesticide to marine and estuarine crustaceans. Diuron was the most toxic pesticide to algae, and chlorothalonil was most toxic to early life stages of molluscs and other invertebrates. Toxicity data (96 h LC50/EC50 values) were analyzed using a probability distribution on the ranked toxicity values and 10th centile values were calculated based on different groups of species and for all species combined. Our results indicate that an assessment of risk based on smaller taxonomic groups can be informative, especially for pesticides of less specific modes of action such as chlorothalonil. 相似文献