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231.
We present near-IR spectra of solid CO2 in H2O and CH3OH, and find they are significantly different from that of pure solid CO2. Peaks not present in either pure H2O or pure CO2 spectra become evident when the two are mixed. First, the putative theoretically forbidden CO2 (2ν3) overtone near 2.134 μm (4685 cm−1), that is absent from our spectrum of pure solid CO2, is prominent in the spectra of H2O/CO2=5 and 25 mixtures. Second, a 2.74-μm (3650 cm−1) dangling OH feature of H2O (and a potentially related peak at 1.89 μm) appear in the spectra of CO2-H2O ice mixtures, but are probably not diagnostic of the presence of CO2. Other CO2 peaks display shifts in position and increased width because of intermolecular interactions with H2O. Warming causes some peak positions and profiles in the spectrum of a H2O/CO2=5 mixture to take on the appearance of pure CO2. Absolute strengths for absorptions of CO2 in solid H2O are estimated. Similar results are observed for CO2 in solid CH3OH. Since the CO2 (2ν3) overtone near 2.134 μm (4685 cm−1) is not present in pure CO2 but prominent in mixtures, it may be a good observational (spectral) indicator of whether solid CO2 is a pure material or intimately mixed with other molecules. These observations may be applicable to Mars polar caps as well as outer Solar System bodies. 相似文献
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Ricardo Génova-Santos José Alberto Rubiño-Martín Rafael Rebolo † Kieran Cleary ‡ Rod D. Davies Richard J. Davis Clive Dickinson § Nelson Falcón ‡‡ Keith Grainge Carlos M. Gutiérrez Michael P. Hobson Michael E. Jones ¶ Rüdiger Kneissl Katy Lancaster Carmen P. Padilla-Torres Richard D. E. Saunders Paul F. Scott Angela C. Taylor ¶ Robert A. Watson †† 《Monthly notices of the Royal Astronomical Society》2005,363(1):79-92
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Scott A. Sandford 《Meteoritics & planetary science》1993,28(4):579-585
Abstract— The mid-infrared (4000–450 cm?1; 2.5–22.2 μm) transmission spectra of seven Antarctic ureilites and 10 Antarctic H-5 ordinary chondrites are presented. The ureilite spectra show a number of absorption bands, the strongest of which is a wide, complex feature centered near 1000 cm?1 (10 μm) due to Si-O stretching vibrations in silicates. The profiles and positions of the substructure in this feature indicate that Mg-rich olivines and pyroxenes are the main silicates responsible. The relative abundances of these two minerals, as inferred from the spectra, show substantial variation from meteorite to meteorite, but generally indicate olivine is the most abundant (olivine:pyroxene = 60:40 to 95:5). Both the predominance of olivine and the variable olivine-to-pyroxene ratio are consistent with the known composition and heterogeneity of ureilites. The H-5 ordinary chondrites spanned a range of weathering classes and were used to provide a means of addressing the extent to which the ureilite spectra may have been altered by weathering processes. It was found that, while weathering of these meteorites produces some weak bands due to the formation of small amounts of carbonates and hydrates, the profile of the main silicate feature has been little affected by Antarctic exposure in the meteorites studied here. The mid-infrared ureilite spectra provide an additional means of testing potential asteroidal parent bodies for the ureilites. At present, the best candidates include the subset of S-type asteroids having low albedos and weak absorption features in the near infrared. 相似文献
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Abstract— The western flank of the Haughton impact structure was imaged with a reflection profile generating 9.8 km of subsurface information. Ten reflecting horizons were recognized and have been correlated via a sonic log with the Paleozoic limestone/dolomite rock sequences. The seismic section is dominated by a dense and complex compound fault system with variable attitudes. These steeply dipping faults penetrated the sedimentary rocks but showed no recognizable extension into the crystalline basement. According to the seismically recognized fracture zones of the western margin, the structure is significantly larger than previously estimated. Reconstruction of the crater on the basis of the seismic information and existing scaling relationships reveals a structure with an apparent diameter of 23.9 km, and an excavated cavity of 10.3 km width and 1.97 km depth. The estimated diameters of the transient crater and the central uplift are 12 km and 11 km respectively. The morphologically distinct ring zones do not have seismically recognizable subsurface signatures. The underlying crystalline basement rocks did not exhibit seismically mappable impact-related zones of disturbance. In the central interior region, coherent reflection signals are virtually absent. Valuable information for this area was provided by a 10.26 km long refraction profile that indicated nearly uniform velocities (~5000 m/s) to a considerable depth. Major lateral variations in the velocity field across the structure were not detected. 相似文献
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Robert A. Watson Pedro Carreira Kieran Cleary Rod D. Davies Richard J. Davis Clive Dickinson Keith Grainge † Carlos M. Gutiérrez Michael P. Hobson Michael E. Jones Rüdiger Kneissl Anthony Lasenby Klaus Maisinger Guy G. Pooley Rafael Rebolo José Alberto Rubiño-Martin ‡ Ben Rusholme § Richard D. E. Saunders Richard Savage Paul F. Scott Ane Slosar Pedro J. Sosa Molina Angela C. Taylor David Titterington Elizabeth Waldram Althea Wilkinson 《Monthly notices of the Royal Astronomical Society》2003,341(4):1057-1065