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11.
12.
Justus E. E. van Beusekom Sabine Diel-Christiansen 《International Journal of Earth Sciences》2009,98(2):269-280
Phytoplankton plays a dominant role in shelf biogeochemistry by producing the major part of organic matter. Part of the organic
matter will reach the sediment where diagenetic processes like denitrification, apatite formation or burial will remove nutrients
from the biogeochemical cycle. In this article current knowledge on the decadal plankton variability in the North Sea is summarized
and possible implications of these changes for the biogeochemistry of the North Sea are discussed. Most of the observed interdecadal
dynamics seem to be linked to large-scale oceanographic and atmospheric processes. Prominent changes in the North Sea ecosystem
have taken place around 1979 and 1988. In general, the phytoplankton color (CPRS indicator of phytoplankton biomass) reached
minimum values during the end of the 1970s and has increased especially since the mid 1980s. Changes with a similar timing
have been identified in many time series from the North Sea through the entire ecosystem and are sometimes referred to as
regime shifts. It is suggested that the impact of global change on the local biogeochemistry is largely driven by the phyto-
and zooplankton dynamics during spring and early summer. At that time the extent of zooplankton–phytoplankton interaction
either allows that a large part of the new production is settling to the sediment, or that a significant part of the new production
including the fixed nutrients is kept within the pelagic system. The origin of the extent of the phytoplankton–zooplankton
interaction in spring is probably set in the previous autumn and winter. In coastal areas, both large-scale atmospheric and
oceanographic changes as well as anthropogenic factors influence the long-term dynamics. Due to eutrophication, local primary
production nowadays still is up to five times higher than during pre-industrial conditions, despite a decreasing trend. Recently,
introduced species have strengthened the filter feeder component of coastal ecosystems. Especially in shallow coastal seas
like the Wadden Sea, this will enhance particle retention, shift organic matter degradation to the benthic compartment and
enhance nutrient removal from the biogeochemical cycle by denitrification or apatite formation. 相似文献
13.
Over the past few years, OSL and TCN datings of glacial material from High Asia have come into fashion. To this day, however,
these techniques do not permit safe calibration. The intensity of the cosmic ray flux is being modulated by the solar and
terrestrial magnetic fields and their secular fluctuations in the past. So far, these variations cannot be converted into
the respective local TCN production rates for High Asia. We have reason to believe that the ages that are being calculated
despite these uncertainties are generally overestimated. This assessment is supported by conventional radiocarbon dates and
above all by the glacial chronology developed independently on the basis of the Quaternary geological method. The strongly
emerging evidence for a much more extensive LGM glaciation of High Asia is, however, either being ignored or rejected by many
authors, solely on the basis of the above-mentioned uncalibrated datings. This self-conceit based on the “dating fallacy”,
as we call it, should be avoided since it goes decidedly against the standards of the scientific method established in Quaternary
geology and makes a fundamental scientific discussion impossible. 相似文献
14.
15.
Behavior of arsenic and antimony in the surface freshwater reaches of a highly turbid estuary, the Gironde Estuary, France 总被引:1,自引:0,他引:1
Matthieu Masson Jrg Schfer Grard Blanc Aymeric Dabrin Sabine Castelle Gilbert Lavaux 《Applied Geochemistry》2009,24(9):1747-1756
This study reports on the behavior of two redox-sensitive elements, As and Sb, along the turbidity gradient in the freshwater reaches of the turbid Gironde Estuary. During a 17-month survey, surface water and suspended particulate matter (SPM) were sampled monthly at six sites representing both fluvial branches of the Gironde Estuary. Additionally, two longitudinal high resolution profiles were sampled along the fluvial estuary of the Garonne Branch during two contrasted seasons, i.e. with and without the presence of the maximum turbidity zone (MTZ). Seasonal variability and spatial distribution of dissolved (<0.2 μm; <0.02 μm) and particulate As, Sb and Fe were measured and combined with SPM data to understand metalloid behavior in the estuarine freshwater turbidity gradient.At the two main fluvial entries of the Gironde Estuary, dissolved As and Sb concentrations showed strong (by a factor of 2–4) seasonal variations, that were only partly controlled by discharge-related dilution. Seasonal addition of dissolved As and Sb was attributed to the degradation of particulate As and Sb carrier phases in bottom sediment and/or in the adjacent aquifers, rather than release from SPM. In the surface freshwater reaches of the Gironde Estuary, Sb behaved conservatively under all hydrological conditions. In contrast, As was strongly reactive in the presence of the MTZ, with opposite behaviors in the two fluvial branches of the estuary: in the Garonne Branch As was removed from the dissolved phase, whereas in the Dordogne Branch As was added. Redistribution of As between the dissolved and the particulate phases along the turbidity gradient in estuarine freshwater only affected the <0.02 μm fraction, as the 0.02–0.2 μm fraction remained constant (300 ng L−1 in September 2005). Accordingly, As removal seemed to be decoupled from concomitant “colloidal” (0.02–0.2 μm) Fe flocculation in the turbidity gradient. The contrasting behavior of dissolved As in the fluvial estuaries of the Garonne and Dordogne Branches was attributed to sorption processes during equilibration of river-borne dissolved As with estuarine SPM forming the MTZ. This equilibrium, described by a distinct distribution coefficient Kd(As) 11,000 L kg−1 in the MTZ, resulted in either As release (desorption; Dordogne Branch) or removal (adsorption; Garonne Branch) in the respective fluvial estuaries. A mixing experiment under controlled laboratory conditions tended to support that equilibration between the dissolved phase and MTZ particles may induce both As release and removal in the estuarine freshwater reaches, with As distribution evolving towards a distinct Kd value for increasing SPM concentrations. The long-term survey allowed estimating annual (2004) dissolved fluxes of As and, for the first time Sb, at the main fluvial entries of the Gironde Estuary at 30.7 t a−1 and 3.2 t a−1 (Garonne River) and at 8.0 t a−1 and 2.3 t a−1 (Dordogne River), respectively. 相似文献
16.
Patrick Drupp Eric Heinen De Carlo Fred T. Mackenzie Paul Bienfang Christopher L. Sabine 《Aquatic Geochemistry》2011,17(4-5):473-498
The marine shelf areas in subtropical and tropical regions represent only 35% of the total shelf areas globally, but receive a disproportionately large amount of water (65%) and sediment (58%) discharges that enter such environments. Small rivers and/or streams that drain the mountainous areas in these climatic zones deliver the majority of the sediment and nutrient inputs to these narrow shelf environments; such inputs often occur as discrete, episodic introductions associated with storm events. To gain insight into the linked biogeochemical behavior of subtropical/tropical mountainous watershed-coastal ocean ecosystems, this work describes the use of a buoy system to monitor autonomously water quality responses to land-derived nutrient inputs and physical forcing associated with local storm events in the coastal ocean of southern Kaneohe Bay, Oahu, Hawaii, USA. The data represent 2.5 years of near-real time observations at a fixed station, collected concurrently with spatially distributed synoptic sampling over larger sections of Kaneohe Bay. Storm events cause most of the fluvial nutrient, particulate, and dissolved organic carbon inputs to Kaneohe Bay. Nutrient loadings from direct rainfall and/or terrestrial runoff produce an immediate increase in the N:P ratio of bay waters up to values of 48 and drive phytoplankton biomass growth. Rapid uptake of such nutrient subsidies by phytoplankton causes rapid declines of N levels, return to N-limited conditions, and subsequent decline of phytoplankton biomass over timescales ranging from a few days to several weeks, depending on conditions and proximity to the sources of runoff. The enhanced productivity may promote the drawing down of pCO2 and lowering of surface water column carbonate saturation states, and in some events, a temporary shift from N to P limitation. The productivity-driven CO2 drawdown may temporarily lead to air-to-sea transfer of atmospheric CO2 in a system that is on an annual basis a source of CO2 to the atmosphere due to calcification and perhaps heterotrophy. Storms may also strongly affect proximal coastal zone pCO2 and hence carbonate saturation state due to river runoff flushing out high pCO2 soil and ground waters. Mixing of the CO2-charged water with seawater causes a salting out effect that releases CO2 to the atmosphere. Many subtropical and tropical systems throughout the Pacific region are similar to Kaneohe Bay, and our work provides an important indication of the variability and range of CO2 dynamics that are likely to exist elsewhere. Such variability must be taken into account in any analysis of the direction and magnitude of the air?Csea CO2 exchange for the integrated coastal ocean, proximal and distal. It cannot be overemphasized that this research illustrates several examples of how high frequency sampling by a moored autonomous system can provide details about ecosystem responses to stochastic atmospheric forcing that are commonly missed by traditional synoptic observational approaches. Finally, the work exemplifies the utility of combining synoptic sampling and real-time autonomous observations to elucidate the biogeochemical and physical responses of coastal subtropical/tropical coral reef ecosystems to climatic perturbations. 相似文献
17.
18.
S. Bauer H. Class M. Ebert V. Feeser H. G?tze A. Holzheid O. Kolditz Sabine Rosenbaum W. Rabbel D. Sch?fer A. Dahmke 《Environmental Earth Sciences》2012,67(2):351-367
Capture and geological sequestration of CO2 from large industrial sources is considered a measure for reducing anthropogenic emissions of CO2 and thus mitigating climate change. One of the main storage options proposed are deep saline formations, as they provide the largest potential storage capacities among the geologic options. A thorough assessment of this type of storage site therefore is required. The CO2-MoPa project aims at contributing to the dimensioning of CO2 storage projects and to evaluating monitoring methods for CO2 injection by an integrated approach. For this, virtual, but realistic test sites are designed geometrically and fully parameterized. Numerical process models are developed and then used to simulate the effects of a CO2 injection into the virtual test sites. Because the parameterization of the virtual sites is known completely, investigation as well as monitoring methods can be closely examined and evaluated by comparing the virtual monitoring result with the simulation. To this end, the monitoring or investigation method is also simulated, and the (virtual) measurements are recorded and evaluated like real data. Application to a synthetic site typical for the north German basin showed that pressure response has to be evaluated taking into account the layered structure of the storage system. Microgravimetric measurements are found to be promising for detecting the CO2 phase distribution. A combination of seismic and geoelectric measurements can be used to constrain the CO2 phase distribution for the anticline system used in the synthetic site. 相似文献
19.
Daniel Bernard Jamal El Khattabi Emilie Lefevre Hani Serhal Sabine Bastin-Lacherez Isam Shahrour 《Environmental Geology》2008,53(5):1129-1138
In the north of France, high registers of nickel are sometimes recorded within the chalk aquifer. In a confined context, the
presence of pyrite in the covering clays or in the marcasite nodules encrusted in the clay may constitute a natural source
of trace metals. With an objective of sanitary control, the limits of chemical contents regulating the quality of water destined
for human consumption have been lowered by the European Framework Directive in the field of water policy (2000/60/EC). As
a result, nickel limits have been reduced from 50 to 20 μg/l. The analyses, carried out on three water catchment fields in
our area of study, were centred on variable parameters (Eh, O2(d), pH, Conductivity, T°), major elements (SO4, NO3) and metals (Fe, Ni, Mn, Co). The acquired data enabled us to identify from one hand, the conditions which are presented
within the site, special thanks to the evolution of nitrate and iron contents and on the other hand, the natural origin (geological)
of nickel for two of the three sites studied based essentially on the evaluation of the Nickel/Cobalt ratio. Thus, on the
first site, the evolution of nickel content and nitrate content showed the influence of the phenomenon of denitrification
on the re-mobilisation of the nickel. Whereas on the second site, a high variation of total iron content and oxygen dissolved
in solution highlighted a particular phenomenon of oxidation of the pyrite through molecular oxygen. Finally, the correlation
with the sulphates clearly showed behaviour of the nickel, once released, that was entirely dependent on the phenomenon of
adsorption on the iron and manganese hydroxides. 相似文献
20.
Hydrological interactions between surface water and groundwater (GW) can be described using hydrochemical and biological methods. Surface water–groundwater interactions and their effects on groundwater invertebrate communities were studied in the Nakdong River floodplain in South Korea. Furthermore, the GW-Fauna-Index, a promising new index for assessing the strength of surface-water influence on groundwater, was tested. The influence of surface water on groundwater decreased with increasing depth and distance from the river. While hydrochemistry prevailingly reflected the origin of the waters in the study area (i.e. whether alluvial or from adjacent rock), faunal communities seemed to display an affinity to surface-water intrusion. Fauna reacted quickly to changes in hydrology, and temporal changes in faunal community structure were significantly linked to the hydrological situation in the floodplain. The metazoan faunal community and the GW-Fauna-Index allow a distinction between surface and subsurface waters with varying degrees of exchange. The results indicate that hydrological conditions are reflected by faunal assemblages on a high spatiotemporal resolution, and that surface-water intrusion can be estimated using the GW-Fauna-Index. 相似文献