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201.
A three-dimensional two-phase flow model is coupled to a non-linear reactive transport model to study the efficacy of potassium permanganate treatment on dense, non-aqueous phase liquid (DNAPL) source removal in porous media. A linear relationship between the soil permeability (k) and concentration of manganese dioxide precipitate ([MnO2(s)]), k = ko + Srind [MnO2(s)], is utilized to simulate nodal permeability reductions due to precipitate formation. Using published experimental column studies, an Srind = −5.5 × 10−16 m2 L/mg was determined for trichloroethylene (TCE) DNAPL. This Srind was then applied to treatment simulations on three-dimensional TCE DNAPL source zones comprising either DNAPL at residual saturations, or DNAPL at pooled saturations. 相似文献
202.
203.
Hydroxyl and Peroxy Radical Chemistry in a Rural Area of Central Pennsylvania: Observations and Model Comparisons 总被引:2,自引:0,他引:2
Xinrong?RenEmail author William?H.?Brune Christopher?A.?Cantrell Gavin?D.?Edwards Terry?Shirley Andrew?R.?Metcalf Robert?L.?Lesher 《Journal of Atmospheric Chemistry》2005,52(3):231-257
Atmospheric hydroxyl (OH), hydroperoxy (HO2), total peroxy (HO2 and organic peroxy radicals, RO2) mixing ratios and OH reactivity (first order OH loss rate) were measured at a rural site in central Pennsylvania during
May and June 2002. OH and HO2 mixing ratios were measured with laser induced fluorescence (LIF); HO2
+ RO2 mixing ratios were measured with chemical ionization mass spectrometry (CIMS). The daytime maximum mixing ratios were up
to 0.6 parts per trillion by volume (pptv) for OH, 30 pptv for HO2, and 45 pptv for HO2 + RO2. A parameterized RACM (Regional Atmospheric Chemistry Mechanism) box model was used to predict steady state OH, HO2 and HO2 + RO2 concentrations by constraining the model to the measured OH reactivity and previously measured volatile organic compound
(VOC) distributions. The averaged model calculations are generally in good agreement with the observations. For OH, the model
matched the observations for day and night, with an average observed-to-modeled ratio of 0.80. In previous studies such as
PROPHET98, nighttime NO was near 0 pptv and observed nighttime OH was significantly larger than modeled OH. In this study,
nighttime observed and modeled OH agree to within measurement and model uncertainties because the main source of the nighttime
OH was the reaction HO2 + NO → OH + NO2, with the NO being continually emitted from the surrounding fertilized corn field. The observed-to-modeled ratio for HO2 is 1.0 on average, although daytime HO2 is underpredicted by a factor of 1.2 and nighttime HO2 is over-predicted by a factor of ∼2. The average measured and modeled HO2 + RO2 agree well during daytime, but the modeled value is about twice the measured value during nighttime. While measured HO2 + RO2 values agree with modeled values for NO mixing ratios less than a few parts per billion by volume (ppbv), it increases substantially
above the expected value for NO greater than a few ppbv. This observation of the higher-than-expected HO2 + RO2 with the CIMS technique confirms the observed increase of HO2 above expected values at higher NO mixing ratios in HO2 measurements with the LIF technique. The maximum instantaneous O3 production rate calculated from HO2 and RO2 reactions with NO was as high as 10–15 ppb h−1 at midday; the total daily O3 production varied from 13 to 113 ppbv d−1 and was 48 ppbv d−1 on average during this campaign. 相似文献
204.
Matthew Colless Gavin Dalton Steve Maddox Will Sutherland Peder Norberg Shaun Cole Joss Bland-Hawthorn Terry Bridges Russell Cannon Chris Collins Warrick Couch Nicholas Cross Kathryn Deeley Roberto De Propris Simon P. Driver George Efstathiou Richard S. Ellis Carlos S. Frenk Karl Glazebrook Carole Jackson Ofer Lahav Ian Lewis Stuart Lumsden Darren Madgwick John A. Peacock Bruce A. Peterson Ian Price Mark Seaborne Keith Taylor 《Monthly notices of the Royal Astronomical Society》2001,328(4):1039-1063
205.
Shaun Cole Will J. Percival John A. Peacock Peder Norberg Carlton M. Baugh Carlos S. Frenk Ivan Baldry Joss Bland-Hawthorn Terry Bridges Russell Cannon Matthew Colless Chris Collins Warrick Couch Nicholas J. G. Cross Gavin Dalton Vincent R. Eke Roberto De Propris Simon P. Driver George Efstathiou Richard S. Ellis Karl Glazebrook Carole Jackson Adrian Jenkins Ofer Lahav Ian Lewis Stuart Lumsden Steve Maddox Darren Madgwick Bruce A. Peterson Will Sutherland Keith Taylor 《Monthly notices of the Royal Astronomical Society》2005,362(2):505-534
206.
Theory and management of tropical fisheries. Edited by D. Pauly and G. I. Murphy. Proceedings of the ICLARM/CSIRO Workshop on the Theory and Management of Tropical Multispecies Stocks. 12–21 January 1981, Cronulla, Australia. 1982. 360 p. $US21.50 surface; hardbound. Animals of the estuary shore : illustrated guide and ecology. By Malcolm B. Jones, 1983. University of Canterbury publication No. 32. 162p., 140 figures, 11 keys. ISBN 0900–392–32–0 (soft cover, spiral bound). Price NZ$7.50. Numerical ecology. By L. Legendre and P. Legendre, 1983. Elsevier Scientific Publishing Company, Amsterdam. $US83.00. The control of oil pollution (revised edition). Edited by J Wardley‐Smith. Graham & Trot‐man Limited, London. 1983. 285 p., 98 figures, 17 tables. ISBN 0.86010 3382. £19.00/$US35.00. Physical oceanography in Australia. Edited by J. Imberger. Reprinted from the Australian Journal of Marine and Freshwater Research, Volume 34, 1–230, 1983. CSIRO, Melbourne 1983. 相似文献