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631.
Stability of biomass-derived black carbon in soils 总被引:16,自引:0,他引:16
Biqing Liang Dawit Solomon Janice E. Thies Flavio J. Luizão Eduardo G. Neves 《Geochimica et cosmochimica acta》2008,72(24):6069-6078
Black carbon (BC) may play an important role in the global C budget, due to its potential to act as a significant sink of atmospheric CO2. In order to fully evaluate the influence of BC on the global C cycle, an understanding of the stability of BC is required. The biochemical stability of BC was assessed in a chronosequence of high-BC-containing Anthrosols from the central Amazon, Brazil, using a range of spectroscopic and biological methods. Results revealed that the Anthrosols had 61-80% lower (P < 0.05) CO2 evolution per unit C over 532 days compared to their respective adjacent soils with low BC contents. No significant (P > 0.05) difference in CO2 respiration per unit C was observed between Anthrosols with contrasting ages of BC (600-8700 years BP) and soil textures (0.3-36% clay). Similarly, the molecular composition of the core regions of micrometer-sized BC particles quantified by synchrotron-based Near-Edge X-ray Fine Structure (NEXAFS) spectroscopy coupled to Scanning Transmission X-ray Microscopy (STXM) remained similar regardless of their ages and closely resembled the spectral characteristics of fresh BC. BC decomposed extremely slowly to an extent that it was not possible to detect chemical changes between youngest and oldest samples, as also confirmed by X-ray Photoelectron Spectroscopy (XPS). Deconvolution of NEXAFS spectra revealed greater oxidation on the surfaces of BC particles with little penetration into the core of the particles. The similar C mineralization between different BC-rich soils regardless of soil texture underpins the importance of chemical recalcitrance for the stability of BC, in contrast to adjacent soils which showed the highest mineralization in the sandiest soil. However, the BC-rich Anthrosols had higher proportions (72-90%) of C in the more stable organo-mineral fraction than BC-poor adjacent soils (2-70%), suggesting some degree of physical stabilization. 相似文献
632.
F. A. Temporim Ricardo Ivan Ferreirae da Trindade Marcos Egydio-Silva Tiago Valim Angelo Eric Tohver Caroline Cibele Soares Lucas Pequeno Gouvêa Julio Cesar Mendes Silvia Regina Medeiros Antônio Carlos Pedrosa-Soares Gabriel Gomes Silva 《地学学报》2023,35(1):23-31
Featuring 3 000-km-long large and hot orogen, the Mantiqueira Province provides a rare opportunity to study the process of gravitational collapse at mid to deep crustal levels. Distinct but contemporary (~500 Ma) post-collisional intrusions show structures and anisotropy of magnetic susceptibility (AMS) fabrics related to their emplacements, recording different flow patterns. In southern deep-seated intrusions, ellipsoidal-shaped roots with gabbroic-to-hybrid cores surrounded by granitic rocks show concentric patterns of AMS fabrics that cut across the NE-trending regional foliation. In contrast, northern intrusions, exposed as the upper sections of batholith-size bodies of coarse-grained granite emplaced at the shallow to mid-crust, show general NS-trending magnetic fabrics roughly parallel to strike of the orogen and the regional foliation of host rocks. These contrasting magnetic patterns from shallow to deeper crust suggest vertical magma migration from the overthickened orogenic core to be emplaced across its thinner stretched flanks during the gravitational collapse of the orogenic edifice. 相似文献
633.
Al-Qadami Ebrahim Hamid Hussein Mustaffa Zahiraniza Shah Syed Muzzamil Hussain Matínez-Gomariz Eduardo Yusof Khamaruzaman Wan 《Natural Hazards》2022,110(1):325-348
Natural Hazards - Vehicles can be easily swept away by floodwaters once the flow velocity and depth reach certain critical limits, with probabilities toward fatality reported to be nearly 50%.... 相似文献