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181.
The behavior of ammonium, NH4+, in aqueous systems was studied based on Raman spectroscopic experiments to 600 °C and about 1.3 GPa. Spectra obtained at ambient conditions revealed a strong reduction of the dynamic three-dimensional network of water with addition of ammonium chloride, particularly at small solute concentrations. The differential scattering cross section of the ν1-NH4+ Raman band in these solutions was found to be similar to that of salammoniac.The Raman band of silica monomers at ∼780 cm−1 was present in all spectra of the fluid at high temperatures in hydrothermal diamond-anvil cell experiments with H2O ± NH4Cl and quartz or the assemblage quartz + kyanite + K-feldspar ± muscovite/tobelite. However, these spectra indicated that dissolved silica is less polymerized in ammonium chloride solutions than in comparable experiments with water. Quantification based on the normalized integrated intensity of the H4SiO40 band showed that the silica solubility in experiments with H2O + NH4Cl was significantly lower than that in equimolal NaCl solutions. This suggests that ammonium causes a stronger decrease in the activity of water in chloridic solutions than sodium.The Raman spectra of the fluid also showed that a significant fraction of ammonium was converted to ammonia, NH3, in all experiments at temperatures above 300 °C. This indicates a shift towards acidic conditions for experiments without a buffering mineral assemblage. The estimated pH of the fluid was ∼2 at 600 °C, 0.26 GPa, 6.6 m initial NH4Cl, based on the ratio of the integrated ν1-NH3 and ν1-NH4+ intensities and the HCl0 dissociation constant. The NH3/NH4+ ratio increased with temperature and decreased with pressure. This implies that more ammonium should be retained in K-bearing minerals coexisting with chloridic fluids upon high-P low-T metamorphism. At 500 °C, 0.73 GPa, ammonium partitions preferentially into the fluid, as constrained from infrared spectroscopy on the muscovite and from mass balance.The conversion of K-feldspar to muscovite proceeded much faster in experiments with NH4Cl solutions than in comparable experiments with water. This is interpreted as being caused by enhancement of the rate-limiting alumina solubility, suggesting complexation of Al with NH4. Nucleation and growth of mica at the expense of K-feldspar and NH4+/K+ exchange between fluid and K-feldspar occurred simultaneously, but incorporation of NH4+ into K-feldspar was distinctly faster than K-feldspar consumption. 相似文献
182.
Barbara Suski Gilles Brocard Christine Authemayou Beatriz Consenza Muralles Christian Teyssier Klaus Holliger 《Tectonophysics》2010,480(1-4):88-98
The Polochic and Motagua faults define the active plate boundary between the North American and Caribbean plates in central Guatemala. A splay of the Polochic Fault traverses the rapidly growing city of San Miguel Uspantán that is periodically affected by destructive earthquakes. This fault splay was located using a 2D electrical resistivity tomography (ERT) survey that also characterized the fault damage zone and evaluated the thickness and nature of recent deposits upon which most of the city is built. ERT images show the fault as a ~50 m wide, near-vertical low-resistivity anomaly, bounded within a few meters by high resistivity anomalies. Forward modeling reproduces the key aspects of the observed electrical resistivity data with remarkable fidelity thus defining the overall location, geometry, and internal structure of the fault zone as well as the affected lithologies. Our results indicate that the city is constructed on a ~20 m thick surficial layer consisting of poorly consolidated, highly porous, water-logged pumice. This soft layer is likely to amplify seismic waves and to liquefy upon moderate to strong ground shaking. The electrical conductivity as well as the major element chemistry of the groundwater provides evidence to suggest that the local aquifer might, at least in part, be fed by water rising along the fault. Therefore, the potential threat posed by this fault splay may not be limited to its seismic activity per se, but could be compounded its potential propensity to enhance seismic site effects by injecting water into the soft surficial sediments. The results of this study provide the basis for a rigorous analysis of seismic hazard and sustainable development of San Miguel Uspantán and illustrate the potential of ERT surveying for paleoseismic studies. 相似文献
183.
A compilation of phytoplankton species abundance data from the spring bloom along the northern Norwegian coast and in the
Barents Sea shows that the quantitatively most important species are the prymnesiophyte Phaeocystis pouchetii and the common cold water to temperate diatoms Chaetoceros socialis, Skeletonema costatum sensu lato, Fragilariopsis oceanica, Thalassiosira spp., Chaetoceros furcellatus, Chaetoceros compressus, Chaetoceros debilis and Bacterosira bathyomphala. The relative abundance of diatoms and Phaeocystis varied highly and apparently stochastically between years. P. pouchetii occurred during all stages of the spring bloom and sometimes completely dominated the phytoplankton community. Along the
Norwegian coast, the importance of P. pouchetii increased northwards. The species composition in coastal fjords at 70° N is surprisingly similar to that of shelf waters
in the Barents Sea (up to 80° N). An exception is S. costatum sensu lato which was seldom observed in Arctic waters. Small flagellates (<10 μm) other than dinoflagellates and P. pouchetii are also important among the Barents Sea spring phytoplankton. Associations of species seem rigid over time and are dominated
by C. socialis and P. pouchetii in northern waters. Biogeographical categories of spring bloom species in relation to environmental conditions are discussed. 相似文献
184.
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186.
Worldwide, the ammonoid genus Prolobites is only known from a few localities, and from these fossil beds almost all of the specimens are adults as shown by the presence
of a terminal growth stage. This is in marked contrast to the co-occurring ammonoid genera such as Sporadoceras, Prionoceras, and Platyclymenia. Size distribution of specimens of Prolobites from three studied localities show that, unlike in the co-occurring ammonoid species, most of the material belongs to adult
individuals. The morphometric analysis of Prolobites delphinus (Sandberger & Sandberger 1851) demonstrates the intraspecific variability including variants with elliptical coiling and that dimorphism is not detectable.
The Prolobites material shows close resemblance to spawning populations of Recent coleoids such as the squid Todarodes filippovae Adam
1975. Possible mass spawning events are discussed in the context of the size distribution and limited geographic range of Prolobites. Finally, the potential fecundity and brooding behaviour of Prolobites is hypothesized using the examples of post spawning egg care in Recent coleoids. 相似文献
187.
Christian Götze András Jung Ines Merbach Rainer Wennrich Cornelia Gläßer 《Central European Journal of Geosciences》2010,2(2):132-137
Floodplain ecosystems are affected by flood dynamics, nutrient supply as well as anthropogenic activities. Heavy metal pollution poses a serious environmental challenge. Pollution transfer from the soil to vegetation is still present at the central location of Elbe River, Germany. The goal of this study was to assess and separate the current heavy metal contamination of the floodplain ecosystem, using spectrometric field and laboratory measurements. A standardized pot experiment with floodplain vegetation in differently contaminated soils provided the basis for the measurements. The dominant plant types of the floodplains are: Urtica dioica, Phalaris arundinacea and Alopecurus pratensis, these were also chemically analysed. Various vegetation indices and methods were used to estimate the red edge position, to normalise the spectral curve of the vegetation and to investigate the potential of different methods for separating plant stress in floodplain vegetation. The main task was to compare spectral bands during phenological phases to find a method to detect heavy metal stress in plants. A multi-level algorithm for the curve parameterisation was developed. Chemo-analytical and ecophysiological parameters of plants were considered in the results and correlated with spectral data. The results of this study show the influence of heavy metals on the spectral characteristics of the focal plants. The developed method (depth CR1730) showed significant relationship between the plants and the contamination. 相似文献
188.
Anne-Cathrin Wölfl Chai Heng Lim H. Christian Hass Sebastian Lindhorst Gabriela Tosonotto Karsten Alexander Lettmann Gerhard Kuhn Jörg-Olaf Wolff Doris Abele 《Geo-Marine Letters》2014,34(5):435-446
Marine habitats worldwide are increasingly pressurized by climate change, especially along the Antarctic Peninsula. Well-studied areas in front of rapidly retreating tidewater glaciers like Potter Cove are representative for similar coastal environments and, therefore, shed light on habitat formation and development on not only a local but also regional scale. The objective of this study was to provide insights into habitat distribution in Potter Cove, King George Island, Antarctica, and to evaluate the associated environmental processes. Furthermore, an assessment concerning the future development of the habitats is provided. To describe the seafloor habitats in Potter Cove, an acoustic seabed discrimination system (RoxAnn) was used in combination with underwater video images and sediment samples. Due to the absence of wave and current measurements in the study area, bed shear stress estimates served to delineate zones prone to sediment erosion. On the basis of the investigations, two habitat classes were identified in Potter Cove, namely soft-sediment and stone habitats that, besides influences from sediment supply and coastal morphology, are controlled by sediment erosion. A future expansion of the stone habitat is predicted if recent environmental change trends continue. Possible implications for the Potter Cove environment, and other coastal ecosystems under similar pressure, include changes in biomass and species composition. 相似文献
189.
In most multiple-point simulation algorithms, all statistical features are provided by one or several training images (TI) that serve as a substitute for a random field model. However, because in practice the TI is always of finite size, the stochastic nature of multiple-point simulation is questionable. This issue is addressed by considering the case of a sequential simulation algorithm applied to a binary TI that is a genuine realization of an underlying random field. At each step, the algorithm uses templates containing the current target point as well as all previously simulated points. The simulation is validated by checking that all statistical features of the random field (supported by the simulation domain) are retrieved as an average over a large number of outcomes. The results are as follows. It is demonstrated that multiple-point simulation performs well whenever the TI is a complete (infinitely large) realization of a stationary, ergodic random field. As soon as the TI is restricted to a limited domain, the statistical features cannot be obtained exactly, but integral range techniques make it possible to predict how much the TI should be extended to approximate them up to a prespecified precision. Moreover, one can take advantage of extending the TI to reduce the number of disruptions in the execution of the algorithm, which arise when no conditioning template can be found in the TI. 相似文献
190.
Nicolas Hawie Remy Deschamps Fadi H. Nader Christian Gorini Carla Müller Delphine Desmares Ahmed Hoteit Didier Granjeon Lucien Montadert François Baudin 《Arabian Journal of Geosciences》2014,7(4):1323-1349
This paper presents an updated review of the Upper Mesozoic and Cenozoic sedimentological and stratigraphic evolution of the Levant margin with a focus on the northern Lebanon. Facies and microfacies analysis of outcrop sections and onshore well cores (i.e., Kousba and Chekka) supported by nannofossil and planktonic foraminifers biostratigraphy, allowed to constrain the depositional environments prevailing in the Turonian to Late Miocene. The “Senonian” (a historical term used to define the Coniacian to Maastrichtian) source rock interval was subdivided into four sub-units with related outer-shelfal facies: (1) Upper Santonian, (2) Lower, (3) Upper Campanian, and (4) Lower Maastrichtian. This Upper Cretaceous rock unit marks the major drowning of the former Turonian rudist platform. This paper confirms the Late Lutetian to Late Burdigalian hiatus, which appears to be a direct consequence of major geodynamic events affecting the Levant region (i.e., the continued collision of Afro-Arabia with Eurasia), potentially enhanced by regressional cycles (e.g., Rupelian lowstand). The distribution of Late Burdigalian–Serravallian rhodalgal banks identified in northern Lebanon was controlled by pre-existing structures inherited from the pulsating onshore deformation. Reef barriers facies occur around the Qalhat anticline, separating an eastern, restricted back-reef setting from a western, coastal to open marine one. The acme of Mount Lebanon’s uplift and exposure is dated back to the Middle–Late Miocene; it led to important erosion of carbonates that were subsequently deposited in paleo-topographic lows. The Late Cretaceous to Cenozoic facies variations and hiatuses show that the northern Lebanon was in a higher structural position compared to the south since at least the Late Cretaceous. 相似文献