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981.
E. J. Palin M. T. Dove S. A. T. Redfern C. I. Saniz-Díaz W. T. Lee 《Physics and Chemistry of Minerals》2003,30(5):293-304
As part of a wider study of the nature and origins of cation order–disorder in micas, a variety of computational techniques
have been used to investigate the nature of tetrahedral and octahedral ordering in phengite, K2
[6](Al3Mg)[4](Si7Al)O20(OH)4. Values of the atomic exchange interaction parameters J
n
used to model the energies of order–disorder were calculated. Both tetrahedral Al–Si and octahedral Al–Mg ordering were studied
and hence three types of interaction parameter were necessary: for T–T, O–O and T–O interactions (where T denotes tetrahedral
sites and O denotes octahedral sites). Values for the T–T and O–O interactions were taken from results on other systems, whilst
we calculated new values for the T–O interactions. We have demonstrated that modelling the octahedral and tetrahedral sheets
alone and independently produces different results from modelling a whole T–O–T layer, hence justifying the inclusion of the
T–O interactions. Simulations of a whole T–O–T layer of phengite indicated the presence of short-range order, but no long-range
order was observed.
Received: 8 August 2002 / Accepted: 14 February 2003
Acknowledgements The authors are grateful to EPSRC (EJP) and the Royal Society (CIS) for financial support. Monte Carlo simulations were performed
on the Mineral Physics Group's Beowulf cluster and the University of Cambridge's High Performance Computing Facility. 相似文献
982.
S. K. Deb M. H. Manghnani K. Ross R. A. Livingston P. J. M. Monteiro 《Physics and Chemistry of Minerals》2003,30(1):31-38
A Raman scattering and X-ray diffraction study of the thermal decomposition of a naturally occurring, ettringite-group crystal
is presented. Raman spectra, recorded with increasing temperature, indicate that the thermal decomposition begins at ≈55 °C,
accompanied by dehydration of water molecules from the mineral. This is in contrast to previous studies that reported higher
temperature breakdown of ettringite. The dehydration is completed by 175 °C and this results in total collapse of the crystalline
structure and the material becomes amorphous. The Raman scattering results are supported by X-ray diffraction results obtained
at increasing temperatures.
Received: 9 July 2001 / Accepted: 14 August 2002 相似文献
983.
Serpentinization of abyssal peridotites from the MARK area, Mid-Atlantic Ridge: sulfur geochemistry and reaction modeling 总被引:1,自引:0,他引:1
The opaque mineralogy and the contents and isotope compositions of sulfur in serpentinized peridotites from the MARK (Mid-Atlantic Ridge, Kane Fracture Zone) area were examined to understand the conditions of serpentinization and evaluate this process as a sink for seawater sulfur. The serpentinites contain a sulfur-rich secondary mineral assemblage and have high sulfur contents (up to 1 wt.%) and elevated δ34Ssulfide (3.7 to 12.7‰). Geochemical reaction modeling indicates that seawater-peridotite interaction at 300 to 400°C alone cannot account for both the high sulfur contents and high δ34Ssulfide. These require a multistage reaction with leaching of sulfide from subjacent gabbro during higher temperature (∼400°C) reactions with seawater and subsequent deposition of sulfide during serpentinization of peridotite at ∼300°C. Serpentinization produces highly reducing conditions and significant amounts of H2 and results in the partial reduction of seawater carbonate to methane. The latter is documented by formation of carbonate veins enriched in 13C (up to 4.5‰) at temperatures above 250°C. Although different processes produce variable sulfur isotope effects in other oceanic serpentinites, sulfur is consistently added to abyssal peridotites during serpentinization. Data for serpentinites drilled and dredged from oceanic crust and from ophiolites indicate that oceanic peridotites are a sink for up to 0.4 to 6.0 × 1012 g seawater S yr−1. This is comparable to sulfur exchange that occurs in hydrothermal systems in mafic oceanic crust at midocean ridges and on ridge flanks and amounts to 2 to 30% of the riverine sulfate source and sedimentary sulfide sink in the oceans. The high concentrations and modified isotope compositions of sulfur in serpentinites could be important for mantle metasomatism during subduction of crust generated at slow spreading rates. 相似文献
984.
In this paper, we present a brief review of the thermodynamic equilibrium of binary solid solution-aqueous solution (SS-AS) systems and derive an expression that allows us to evaluate the supersaturation or undersaturation of a given aqueous solution with respect to the whole range of solid compositions: the δ(x) function. Such an expression is based on the two conditions that define the SS-AS thermodynamic equilibrium. The derivation of the new supersaturation function, δ(x), was made by considering in detail the compositional relationships between solid and aqueous phases. To represent the new formulation on Lippmann diagrams, we have defined a new thermodynamic concept: the “actual activity.” In addition, we show how our supersaturation function behaves for both ideal and subregular solid solutions. The behaviour and applicability of both the δ(x) function and a previous supersaturation function, β(x), defined by Prieto et al. (1993), is discussed. 相似文献
985.
986.
In the present study, an attempt has been made to delineate and characterize the different geomorphic units of Tundiya river
catchment in a part of Lower Maharahstra Metamorphic Plateau, north-eastern part of Nagpur district, Maharashtra. The drainage,
contour and delineated geological units have been overlaid on IRS-ID LISS III satellite imagery (bands 2,3 and 4) in EASI/PACE
analysis system to delineate and characterize different geomorphological units and analysis of their processes based on the
field observations. The study area is basically of metamorphic in origin with different geological formations and is influenced
by the various fluvio-morphological processes. Based on the satellite data analysis, the distinct geomorphological units viz.,
table top summits, structural hills, subdued plateau, linear ridges, shallow, moderate and deeply buried foot slopes, shallow
valley fills and deep valley fills have been delineated and characterized. The information generated from satellite data in
the form of vector layers has been used in GIS to generate geological and geomorphological maps of the study area. The present
study demonstrates that IRS-ID LISS-III data in conjunction with geology, drainage and contour parameters to enable detailed
evaluation of different geomorphological units and analysis of their processes based on the field observations. The delineated
geomorphological units can be utilized for evaluation and management of natural resources and geo-environment on sustainable
basis at river catchment level. 相似文献
987.
The paper discusses the land damage assessment and change detection analysis with reference to a mineral bearing zone in Manjhi,
Manuni and Churan valleys. The area is located in environmentally sensitive and fragile region of Himalaya and constitutes
of nearly 400 small-scale mines of slate, which were operative since last one hundred years and are stopped by court of law
since 1995 on account of environment deterioration. The status of land degradation has been studied using IRS-1B satellite
data of 1988,1992 and 1995. The geo-coded data on 1:50,000 scale has been interpreted and an increase in land degradation
status was noticed. Finally, the management strategy for arresting the further land damage in a broader perspective is suggested. 相似文献
988.
Permeshwar S. Chauhan Mahesh C. Porwal Lalit Sharma Jay Devs.negi 《Journal of the Indian Society of Remote Sensing》2003,31(3):211-218
The review of study site have revealed the change in vegetation cover of Sal Dense to Sal Medium and Sal Open in 6 forest
Mosaics owing to biotic and abiotic conditions prevailing in the specific areas. Analysis carried out using thematic map derived
from aerial photograph of 1976 and satellite data of IRS 1C LISS III False Colour Composite (FCC) of March 1999 revealed the
cause for change in forest density classes. Deforestation, encroachment and agriculture have been identified as the underlying
causes, which have affected some specific locations to a marked extent. There has been a progressive and remarkable change
among vegetation classes from 1976 to 1999. It is evident from forest type and density map that Sal density has significantly
reduced from Sal Dense 65.61 % in 1976 to Sal Dense 11.12% in the year 1999 followed by Sal Open 11.18 % and Sal Medium 18.24
%. The overall change has been estimated to be 42.11% of the total forested area. 相似文献
989.
The Himalayas has one of the largest concentrations of glaciers outside the Polar Regions. Various reports suggest that significant number of mountain glaciers is shrinking due to climatic variations. Monitoring of these glaciers is important to assess future availability of water resources in the Himalayan region. However, Himalayan glaciers are normally difficult to monitor due to the rugged, mountainous terrain. Therefore, images of Indian Remote Sensing Satellite were used to monitor glaciers in the Baspa basin. Investigations have shown the presence of 30 glaciers in the basin, with areal extent of 167 km2. Out of these, 19 glaciers, with areal extent of 140 km2 were selected to estimate retreat. Investigation suggests that almost all glaciers are retreating in the study basin and overall 19% deglaciation has been observed from 1962 to 2001. In general, altitude distribution appears to have significant influence on glacial retreat. Glaciers located around 5000 m altitude range are showing 24% loss as compared to 14% by glaciers located in altitude range higher than 5400 m. In addition, mean altitude of glacier terminus is shifted upward by 88 m, i.e. from 4482 to 4570 m in last 39 years. The glacial volumes were estimated using regression relationship between area and depth. The investigations have suggested that 19.10 km3 of glacial water stored in the 19 glaciers in 1962, has been reduced to 14.71 km3 in 2001, respectively, an overall loss of 23 percent in a period between 1962 and 2001. These investigations suggest that all glaciers in the Baspa Basin are reducing and in long term, such reducing trend can create scarcity of water in the region. 相似文献
990.
A. Chakraborty H. C. Upadhyaya O. P. Sharma S. K. Deb 《Meteorology and Atmospheric Physics》2003,83(3-4):221-236
Summary ?A newly developed ocean general circulation model has been tested and verified with some idealized experiments. Generally
two types of idealized experiments have been done here. First types are called as “symmetric experiments” and second types
are called as “transport experiments”. The first types of experiment help to correct the model core and any deficiency from
boundary conditions. The second types of experiment are the type of validation experiment. In both the experiments there are
no continents, so in the first type of experiments where symmetric forcings are provided one can expect that model should
maintain the symmetric nature. In the second type of experiments one can expect that model should respond correctly to the
wind forcings, if no wind curl is present in the wind forcing there will be no circulation in the extratropics and if there
is no wind the equator there will be no circulation. The model reproduces the possible envisaged results of these experiments
and gives the confidence for performing the realistic integration.
Received February 20, 2002; accepted July 7, 2002
Published online: February 20, 2003 相似文献