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1.
Distribution of dissolved species and suspended particulate copper in an intertidal ecosystem affected by copper mine tailings in Northern Chile 总被引:1,自引:0,他引:1
The coastline near Chañaral in Northern Chile is one of the most highly Cu-contaminated zones in the world due to discharges from mining activities for more than 60 years. The speciation of Cu has been studied to determine the importance of organic complexation in highly contaminated areas, and to assess the likely physiological impacts of Cu on marine organisms. Dissolved Cu concentrations of up to 500 nM were measured, completely saturating organic ligands and leading to free Cu2+ concentrations in excess of 10− 8 M. These values are higher than those reported in any other marine environment, and because they occur over an extensive area, provide a unique opportunity to study the effects of Cu on marine ecosystems and to see how Cu behaves when its speciation is predominantly inorganic. We found strong gradients in free Cu2+ between Chañaral and adjacent areas with lower Cu, where speciation is dominated by organic complexation. There is also a significant increase in the partitioning of Cu onto suspended particles in the contaminated areas, consistent with previous studies that showed that organic ligands stabilize Cu in the dissolved phase, whilst “excess” Cu is rapidly scavenged. Those high dissolved Cu concentrations persist in spite of solid phase partitioning and advective processes along this open-ocean coastline, suggesting that Cu inputs into the system are still very large. Measurements were made using anodic stripping voltammetry with a thin mercury film coated with Nafion, which previous workers have shown can mitigate ambiguity in the data arising from inadvertent reduction of organic complexes. Our findings suggest that this is a useful methodology for contaminated systems. 相似文献
2.
Claudia Wienberg Dierk Hebbeln Hiske G. Fink Furu Mienis Boris Dorschel Agostina Vertino Matthias Lpez Correa Andr Freiwald 《Deep Sea Research Part I: Oceanographic Research Papers》2009,56(10):1873-1893
This paper presents the first compilation of information on the spatial distribution of scleractinian cold-water corals in the Gulf of Cádiz based on literature research and own observations (video footage, sediment samples). Scleractinian cold-water corals are widely distributed along the Spanish and Moroccan margins in the Gulf of Cádiz, where they are mainly associated with mud volcanoes, diapiric ridges, steep fault escarpments, and coral mounds. Dendrophyllia cornigera, Dendrophyllia alternata, Eguchipsammia cornucopia, Madrepora oculata and Lophelia pertusa are the most abundant reef-forming species. Today, they are almost solely present as isolated patches of fossil coral and coral rubble. The absence of living scleractinian corals is likely related to a reduced food supply caused by low productivity and diminished tidal effects. In contrast, during the past 48 kyr scleractinian corals were abundant in the Gulf of Cádiz, although their occurrence demonstrates no relationship with main climatic or oceanographic changes. Nevertheless, there exists a conspicuous relationship when the main species are considered separately. Dendrophylliids are associated with periods of relatively stable and warm conditions. The occurrence of L. pertusa mainly clusters within the last glacial when bottom current strength in the Gulf of Cádiz was enhanced and long-term stable conditions existed in terms of temperature. Madrepora oculata shows a higher tolerance to abrupt environmental changes. 相似文献
3.
4.
High concentrations of N and P in biosolids are one of the strongest appeals for their agronomic use. However, it is essential
to understand the fate of N in soils treated with biosolids for both plant nutrition and managing the environmental risk of
NO
3
−
-N leaching. This work aims to evaluate the risk of nitrate leaching from a sandy Podosol soil and from a clay Ferrosol soil,
each one amended at the range 0.5–8.0 dry Mg/ha rates of freshly tertiary sewage sludge, composted sludge, limed sludge, heating-dried
sludge and solar-irradiated sludge. Results showed that for similar biosolids application rates NO
3
−
-N accumulated up to 3 times as much in the Ferrosol than in Podosol soil. However, there was a fixed 20% NO
3
−
-N loss from the 20 cm amended-Ferrosol topsoil, whilst the N-nitrified expected to leach down from 20 cm amended-Podosol
topsoil layer ranged from 42% to 76% of the accumulated NO
3
−
-N, depending on the biosolid type. After all, NO
3
−
-N expected to leach from Podosol soil ranged from 0.6 (heating-dried sludge) to 3.9 times (limed sludge) relative to Ferrosol
soil at similar biosolid application rates. Nevertheless, the risk of NO
3
−
-N groundwater contamination caused by biosolids applied at 0.5−8.0 dry Mg/ha rates could be considered very low.
Published in Russian in Vodnye Resursy, 2006, Vol. 33, No. 4, pp. 492–503. 相似文献
5.
Juliano Kuchle Claiton Marlon dos Santos Scherer Christian Correa Born Renata dos Santos Alvarenga Felipe Adegas 《Journal of South American Earth Sciences》2011,31(4):358-371
The Dom João Stage comprises an interval with variable thickness between 100 and 1200 m, composed of fluvial, eolian and lacustrine deposits of Late Jurassic age, based mainly on the lacustrine ostracod fauna (although the top deposits may extend into the Early Cretaceous). These deposits comprise the so-called Afro-Brazilian Depression, initially characterized as containing the Brotas Group of the Recôncavo Basin (which includes the Aliança and the Sergi Formations) and subsequently extended into the Tucano, Jatobá, Camamu, Almada, Sergipe, Alagoas and Araripe Basins in northeastern Brazil, encompassing the study area of this paper. The large occurrence area of the Dom João Stage gives rise to discussions about the depositional connectivity between the basins, and the real extension of sedimentation. In the first studies of this stratigraphic interval, the Dom João Stage was strictly associated with the rift phase, as an initial stage (decades of 1960–70), but subsequent analyses considered the Dom João as an intracratonic basin or pre-rift phase – without any relation to the active mechanics of a tectonic syn-rift phase (decades of 1980–2000). The present work developed an evolutionary stratigraphic and tectonic model, based on the characterization of depositional sequences, internal flooding surfaces, depositional systems arrangement and paleoflow directions. Several outcrops on the onshore basins were used to build composite sections of each basin, comprising facies, architectural elements, depositional systems, stratigraphic and lithostratigraphic frameworks, and paleocurrents. In addition to that, over a hundred onshore and offshore exploration wells were used (only 21 of which are showed) to map the depositional sequences and generate correlation sections. These show the characteristics and relations of the Dom João Stage in each studied basin, and they were also extended to the Gabon Basin. The results indicate that there were two main phases during the Dom João Stage, in which distinctive sedimentary environments were developed, reflecting depositional system arrangements, paleoflow directions were diverse, and continuous or compartmented basins were developed. 相似文献
6.
A. Correa‐Metrio S. Lozano‐García S. Xelhuantzi‐López S. Sosa‐Nájera S. E. Metcalfe 《第四纪科学杂志》2012,27(5):509-518
The late glacial and the transition towards the Holocene marked a period of significant environmental change at a global scale. In western Central Mexico, few records span beyond the Holocene, and little is known about Pleistocene climatic and environmental variability. Here we report on the pollen record of a composite sequence made of three cores that cover the last 50 ka (thousands of calibrated radiocarbon years before present) in the Zacapu Basin, western Central Mexico (~1970 m asl). The conjunction of modern pollen rain from the area with the composite fossil pollen sequence from cores Cantabria, Cantabria 1 and CEMCA Point‐1 provided a detailed history of the vegetation of the area. Recognition of modern environmental patterns through individual modern pollen taxa proved difficult, but multivariate analysis separated different vegetation types. No‐modern‐analog communities relative to the modern vegetation cover of the area were evident, especially during periods of drought. Apparently, summer precipitation was significant before 40 ka and after the deglaciation. However, this moisture source declined from ~40 to 10 ka because tradewinds from the Gulf of Mexico were blocked by the eastern mountains of Central Mexico as a result of lower temperatures. By contrast, westerly and northerly winds were enhanced by maximum ice cover from ~19 to 17 ka, providing abundant winter precipitation and therefore preventing extreme drought in the area. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
7.
A sediment quality triad (SQT) assessment was made of the impact of copper mine tailings disposal on littoral meiofaunal assemblages in the Atacama region of northern Chile. This situation is unusual in that the disposal is direct into the high-energy coastal system and not via a river estuary or other low-energy environment. This situation also allows for the examination of the impact of copper mine tailings in the absence of confounding effects from other pollutants. The three components of the SQT were: 1. an analysis of the bioavailable metals in both the sedimentary porewater and the adjacent seawater, 2. a microcosm bioassay of both sediments and seawaters using meiofaunal assemblages, and 3. quantitative field samples of the meiofaunal assemblages. Twelve study sites with varying degrees of impact were used, including three reference sites. The study identified that both the meiofaunal assemblage densities and taxa diversities decrease with increasing levels of bioavailable copper, that the Foraminifera and Harpacticoida are sensitive to copper, and that otoplanid Turbellaria are often characteristic of impacted sites; tailings also have both chemical and physical impacts on the environment. In some cases the physical impact of tailings is more important in excluding some organisms e.g. the interstitial polychaete, Saccocirrus sonomacus, from a site than is their chemical impact. 相似文献
8.
Alicia Correa Boris F Ochoa-Tocachi Christian Birkel Ana Ochoa-Sánchez Charles Zogheib Carolina Tovar Wouter Buytaert 《水文研究》2020,34(24):4609-4627
Páramos, a neotropical alpine grassland-peatland biome of the northern Andes and Central America, play an essential role in regional and global cycles of water, carbon, and nutrients. They act as water towers, delivering water and ecosystem services from the high mountains down to the Pacific, Caribbean, and Amazon regions. Páramos are also widely recognized as a biodiversity and climate change hot spots, yet they are threatened by anthropogenic activities and environmental changes. Despite their importance for water security and carbon storage, and their vulnerability to human activities, only three decades ago, páramos were severely understudied. Increasing awareness of the need for hydrological evidence to guide sustainable management of páramos prompted action for generating data and for filling long-standing knowledge gaps. This has led to a remarkably successful increase in scientific knowledge, induced by a strong interaction between the scientific, policy, and (local) management communities. A combination of well-established and innovative approaches has been applied to data collection, processing, and analysis. In this review, we provide a short overview of the historical development of research and state of knowledge of the hydrometeorology, flux dynamics, anthropogenic impacts, and the influence of extreme events in páramos. We then present emerging technologies for hydrology and water resources research and management applied to páramos. We discuss how converging science and policy efforts have leveraged traditional and new observational techniques to generate an evidence base that can support the sustainable management of páramos. We conclude that this co-evolution of science and policy was able to successfully cover different spatial and temporal scales. Lastly, we outline future research directions to showcase how sustainable long-term data collection can foster the responsible conservation of páramos water towers. 相似文献
9.
Jorge Ramón Alicia Correa Edison Timbe Giovanny M. Mosquera Enma Mora Patricio Crespo 《水文研究》2021,35(6):e14209
Hydrogeochemical based mixing models have been successfully used to investigate the composition and source identification of streamflow. The applicability of these models is limited due to the high costs associated with data collection and the hydrogeochemical analysis of water samples. Fortunately, a variety of mixing models exist, requiting different amount of data as input, and in data scarce regions it is likely that preference will be given to models with the lowest requirement of input data. An unanswered question is if models with high or low input requirement are equally accurate. To this end, the performance of two mixing models with different input requirement, the mixing model analysis (MMA) and the end-member mixing analysis (EMMA), were verified on a tropical montane headwater catchment (21.7 km2) in the Ecuadorian Andes. Nineteen hydrogeochemical tracers were measured on water samples collected weekly during 3 years in streamflow and eight potential water sources or end-members (precipitation, lake water, soil water from different horizons and springs). Results based on 6 conservative tracers, revealed that EMMA (using all tracers) and MMA (using pair-combinations out of the 6 conservative ones), identified the same end-members: rainfall, soil water and spring water., as well as, similar contribution fractions to streamflow from rainfall 21.9% and 21.4%, soil water 52.7% and 52.3%, and spring water 26.1% and 28.7%, respectively. Our findings show that a hydrogeochemical mixing model requiring a few tracers can provide similar outcomes than models demanding more tracers as input data. This underlines the value of a preliminary detailed hydrogeochemical characterization as basis to derive the most cost-efficient monitoring strategy. 相似文献
10.
Noelia?Liliana?AlchaparEmail author Claudia?Cotrim?Pezzuto Erica?Norma?Correa Lucila?Chebel Labaki 《Theoretical and Applied Climatology》2017,130(1-2):35-50
This paper describes different ways of reducing urban air temperature and their results in two cities: Campinas, Brazil—a warm temperate climate with a dry winter and hot summer (Cwa), and Mendoza, Argentina—a desert climate with cold steppe (BWk). A high-resolution microclimate modeling system—ENVI-met 3.1—was used to evaluate the thermal performance of an urban canyon in each city. A total of 18 scenarios were simulated including changes in the surface albedo, vegetation percentage, and the H/W aspect ratio of the urban canyons. These results revealed the same trend in behavior for each of the combinations of strategies evaluated in both cities. Nevertheless, these strategies produce a greater temperature reduction in the warm temperate climate (Cwa). Increasing the vegetation percentage reduces air temperatures and mean radiant temperatures in all scenarios. In addition, there is a greater decrease of urban temperature with the vegetation increase when the H/W aspect ratio is lower. Also, applying low albedo on vertical surfaces and high albedo on horizontal surfaces is successful in reducing air temperatures without raising the mean radiant temperature. The best combination of strategies—60 % of vegetation, low albedos on walls and high albedos on pavements and roofs, and 1.5 H/W—could reduce air temperatures up to 6.4 °C in Campinas and 3.5 °C in Mendoza. 相似文献