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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
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本文综述了活动星系核 ,特别是blazar天体的研究现状 ,对blazar天体的多波段与多波段能谱特性研究进行了较为详细的评述。主要的研究工作包括以下内容 :(一 )γ噪blazar天体的短时标光变研究 ,通过对 1 6个γ噪blazar天体 (其中包括全部已证认和观测到VHEγ射线爆发的可能甚高能γ射线源 )自 1 998年的光学观测及光变分析研究表明 ,短时标光变 (小时量级 )是GeVγ噪blazar天体的普遍特性 ,光变幅度通常可达 0 .6mag/h ,对PKS 1 51 0 -0 89类星体的观测发现在一个小时内对象变暗 2个星等 ,对如此激烈的光变变暗目前的理论还不能很好的解释 ,但它同样反映了辐射区域的内部结构 ;而对TBLs的监测表明 ,其光学波段的短时标光变没有其他对象激烈 ,出现的频度和振幅变化都较小 ;(二 )在研究γ噪blazar天体光变时 ,研究了寄主星系对光变的影响 ,得到了 1ES 2 3 44 + 51 4的光变与PSF的FWHM的关联 ,表明随着大气视宁度的下降 (即FWHM变大 ) ,对象变暗 ,即由于寄主星系的影响从而导致假光变的产生 ;(三 )引进两个多波段复合谱指数 ,αxox=αox-αx 及αoro=αor-αo。对样本的统计研究表明 ,RBLs是能谱特性界于XBLs和OVVs之间的一类中间态 ,所得结果支持了Sambrunaetal.( 1 996)大样本多波段能谱分布特性的统计研 相似文献
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Three continuous marine fish cell lines of FG (i. e., Hounder Gill) from flounder (Paralichthys olivaceus) gill, SPH (i. e. , Sea Perch Heart) from sea perch (Lateolabrax japonicus) heart and RSBF (i.e., Red Sea Bream Fin) from red sea bream (Pagrosomus major) fin, were characterized by lactate dehydrogenase (LDH) isozyme and morphological analysis. The LDH isozyme patterns of these three cell lines and their corresponding tissues of origin were investigated and compared. The results showed: (1) No difference was found in the LDH isozyme patterns of FG and flounder gill tissue. However, the LDH isozyme patterns of SPH and RSBF were significantly different from their corresponding tissues of origin; (2) LDH isozyme patterns of FG, SPH and RSBF were markedly different from each other and could serve as genetic markers for species identification and detection of cross contamination. Morphological change analysis of these three cell lines in comparison to their original tissues indicated that FG cells still appeared epithelioid without morphological transformation. However, morphological changes were found in SPH and RSBF compared to their original tissues. Therefore, the cellular morphology was still plastic in the relatively stable culture conditions, and it was possible that change of LDH patterns wasrelated to morphological changes of fish cells in vitro. 相似文献
4.
本文叙述南天区 5GHzVLBI普查中新发现的视超光速射电源 ,0 4 2 0— 0 1 4,1 334—1 2 7和 2 345— 1 67,这些结果尚待进一步的观测加以证实 相似文献
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利用野外资料、地震资料、煤田钻孔资料以及古生物资料,对松辽盆地外围探区敦化盆地的代表性地层划分方案进行了梳理,通过敦化盆地与周缘盆地之间的对比和分析,得出下列认识:(1)明确了珲春组的时代为始新世—渐新世;(2)指出白垩系上统龙井组地层在敦化盆地内可能是不存在的;(3)将原帽儿山组上段和下段分别划归泉水村组和长财组;(4)认为大砬子组、泉水村组、长财组和屯田营组在敦化盆地内是存在的,并通过盆间岩性地层和古生物地层对比指出大砬子组的时代可能为早白垩世阿普特期(Aptian)—阿尔布期(Albian),长财组时代可能为早白垩世贝利阿斯期—阿普特期;(5)对敦化盆地内几个地方地层名称的使用进行了修正;(6)建立了敦化盆地内目前可供参考使用的地层序列。 相似文献
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根据2005年4~5月在黄海和长江口海域进行的春季底拖网调查,应用稳定同位素方法研究了黄海中南部鯷鱼(Engraulis japonicus)及其可能摄食饵料的碳氮稳定同位素比值,结果表明:(1)黄海中南部鯷鱼的食物组成为不同粒径的浮游动物、太平洋磷虾(Euphausia pacifuca)和仔稚鱼,其中以粒径为500-900μm的浮游动物为主,贡献比例占61%~84%;仔稚鱼贡献比例占16%~21%,较传统胃含物方法分析的结果小;(2)黄海中部海域鯷鱼的碳氮稳定同位素比值平均值较南部海域高,原因可能与各海域的能量来源不同或存在微食物环有关,也可能与不同海域鯷鱼的能量转换途径不一样,即与食物链长短不一有关. 相似文献
10.
Parthenogenesis in Laminaria and Alaria has been observed by Yabu, Nakaharaet al. and Fang et al. After we had made some preliminary progress in the study ofthe haploid phases of Laminaria japonica, similar study was started in 1974 on anotherspecies of brown algae, i. e., Undaria pinnatifida Sur. Some interesting results of such astudy on Undaria are summarized here. I. MATERIAL AND METHODS The material used in the experiments was mature sporophyte of Undaria collectedfrom the lower tide regions at Qingdao. The methods used in collecting Undaria zoo- 相似文献