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1.
为研究广州市湖泊水体中的防腐剂及其毒性,在广州市选择15个湖泊采集水样,采用液液萃取-气质联用法对湖泊水体中的对羟基苯甲酸甲酯、对羟基苯甲酸乙酯等5种防腐剂进行浓度检测和毒性分析.结果表明:广州市区内15个湖泊水体中均检出防腐剂,但其浓度略低于国外天然水体中的浓度,溶解相的防腐剂平均浓度为5.06 ng/L,颗粒相的平均浓度为0.78 ng/L;广州市区的湖泊水体中溶解相浓度最高的防腐剂为对羟基苯甲酸丁酯,占总量的30.45%,对羟基苯甲酸苯甲酯所占比例最小,占6.71%;以防腐剂对发光细菌光强的抑制强弱来表征其毒性的大小,对羟基苯甲酸苯甲酯的毒性最强,对广州市湖泊水体环境的影响最大.  相似文献   

2.
2006年4月在武汉月湖采集了8个样点的水样和表层沉积物样品,采用气-质联用技术分析了样品中25种半挥发性有机污染物(SVOCs)的含量,探讨月湖受有机物污染的程度.水样中25种半挥发性有机污染物总浓度为564.04-1209.41ng/L,平均值为965.64ng/L.沉积物中总浓度为8500.26-23347.20ng/g(DW),平均值为14832.04ng/g(DW).邻苯二甲酸酯类物质是月湖的主要污染物,其中,邻苯二甲酸乙基己基酯和邻苯二甲酸二丁酯含量最高.多环芳烃、硝基甲苯、异佛尔酮等均有不同程度检出,靠近以前的排污口的样点浓度最高.沉积物中25种半挥发性有机污染物的含量大约是水体中含量的15倍,具有潜在生态风险.  相似文献   

3.
万宏滨  周娟  罗端  杨浩  黄昌春  黄涛 《湖泊科学》2020,32(6):1632-1645
为明确长江中游地区湖泊沉积物中多环芳烃(PAHs)的分布特征、来源及其生态风险,于2018年7月采集了该地区12个湖泊的表层沉积物样品.采用气相色谱-质谱联用仪(GC-MS)测定了沉积物中16种PAHs的含量.结果表明:12个湖泊沉积物中均检测出16种优控PAHs,PAHs的总含量在572.7~1766.2 ng/g (dw)之间(均值为976.5±285.0 ng/g (dw)).武汉市东湖沉积物中PAHs含量最高,达到1634.8±111.4 ng/g (dw).与国内外其他地区湖泊沉积物相比,长江中游地区湖泊沉积物中PAHs含量高于国内偏远地区的抚仙湖、青海湖及博斯腾湖,低于东部地区的巢湖、太湖及美国经济工业发达地区的湖泊.根据单体PAH的聚类分析结果,12个湖泊可以分成3种类型,类型1主要以低环为主,占比为64.04%±7.02%,类型2低环和中高环分布相对平均,分别为50.76%±5.17%和49.24%±5.17%,类型3低、中、高环分布相对平均,占比分别为35.35%±3.56%、26.17%±0.45%和38.48%±3.84%.综合该区域PAHs的分布特征及异构体比值法与主成分分析法的结果表明,类型1湖泊沉积物中PAHs主要来源为煤炭、木材等生物质的燃烧源;类型2和类型3湖泊沉积物中PAHs主要来源为煤炭、木材等生物质的低温燃烧以及机动车等燃烧汽油、柴油的尾气排放和工业炼焦等化石燃料的高温燃烧源.沉积物中PAHs与总有机碳(TOC)之间显著的相关性表明,沉积物中TOC含量是影响长江中游湖泊沉积物中PAHs归趋分布的主要因素.长江中游流域湖泊沉积物中PAHs的RQNCs值均小于800,且RQMPCs值大于1的风险商值法生态风险评价结果表明,长江中游流域湖泊表层沉积物中PAHs整体呈中等风险水平.  相似文献   

4.
为了解白洋淀表层沉积物中有机氯农药(OCPs)和多氯联苯(PCBs)的污染情况,采用改进的GC-μECD方法对白洋淀11处沉积物进行了20种OCPs和全部209种PCB单体的定量检测和分析.结果显示:白洋淀11个沉积物样品共检出10种OCPs和24种PCBs,∑OCPs和∑PCBs的含量范围分别为1.22~52.45 ng/g(DW)和nd~37.61 ng/g,在国内处于中等水平; OCPs组成中以HCHs和Dieldrin(狄氏剂)为主,分别占到∑OCPs的39.9%和31.5%,其中7个采样点的HCHs以林丹输入为主,4个采样点以工业六六六污染为主.DDTs检出率较低,来源主要为历史残留;检出的PCB单体以低氯联苯为主,其中一氯、二氯和三氯联苯占∑PCBs的64.73%;采用沉积物质量标准法进行生态风险评估,结果表明白洋淀地区沉积物中p,p'-DDD和∑PCBs生态风险较低,Dieldrin生态风险尚需关注,γ-HCH生态风险较高,不容忽视.  相似文献   

5.
回顾了有关长江中下游地区湖泊水、生物、沉积物中营养盐的迁移、转化、循环和交换等研究工作进展.典型湖泊的研究结果显示,历史上长江中下游地区湖泊的营养本底的确较高,处于中营养和富营养状态;人类活动在最近几十年中加快了这些湖泊的富营养化进程.长江中下游地区湖泊的治理不仅要重视外源污染的削减,也要重视湖泊内源污染的控制.长江中下游地区的浅水湖泊沉积物中,一般只有30%以下的磷是以较活跃的藻类易利用态存在的,表层沉积物通过吸附-解吸等交换作用对浅水湖泊水体中磷的浓度有较大的影响.长江中下游浅水湖泊沉积物中的营养盐释放主要有静态和动态二种释放方式.前者是基于化学平衡条件下的水土界面扩散作用.决定其释放量大小的主要因子是孔隙水与上覆水之间的营养盐浓度差.后者是基于水动力扰动对水土界面物理破坏条件下的底泥悬浮释放作用.二种释放模式在浅水水体中都存在.无论是静态或动态,水土界面的氧化还原环境,铁、锰、铝等元素含量,都对释放有影响.动态释放能在短期内大大提高水体颗粒态营养盐的浓度.在动态释放的初期,将有效增加水体可溶性营养盐,但是如果沉积物中铁、铝等金属元素较丰富,水体中的溶解性营养盐将由于吸附等作用而沉淀至湖底,因此,这样的湖泊往往具有较强的自我净化能力.长江中下游地区绝大多数湖泊都属于这种类型的湖泊.用底泥疏浚方法来控制湖泊内源污染的方法只适用湖泊面积较小、还原环境强烈,或者沉积物中铁、锰含量较低、水体去除可溶性营养盐的能力较弱的水体.此外,长江中下游地区的浅水湖泊生态系统对富营养化也具有强烈的反馈作用.水华暴发期间蓝藻的暴发性生长能通过改变水体的pH而引发沉积物中磷释放数量的大幅增加,大量释放的营养盐反过来又会促使蓝藻的大量生长,从而加剧水华的暴发.研究显示污染相对较重的水域水体中营养盐的含量高,微生物的生物量及生产力也高,碱性磷酸酶的活性也高,水体营养盐的循环也就更快.这反过来又促使微生物生产力增加,营养盐循环更快,加剧富营养化的危害.今后的工作应该重点围绕生物参与下营养盐的迁移转化等方面开展工作.  相似文献   

6.
运用金汞齐-冷原子荧光光谱法(CVAFS)和气相色谱技术(GC),对贵州省草海不同水文季节(枯水期和丰水期)表层水中汞的各种赋存形态,包括总汞(HgT)、溶解态汞(HgD)、活性汞(HgR)、颗粒态汞(HgP)、总甲基汞(MeHgT)、溶解态甲基汞(MeHgD)和颗粒态甲基汞(MeHgP)以及沉积物间隙水剖面中的溶解态总汞和甲基汞含量进行了测定.结果显示:草海表层水体总汞浓度为1.7-9.0ng/L,活性汞浓度为0.06-1.4ng/L,总甲基汞浓度为0.11-0.67ng/L.沉积物间隙水中溶解态汞浓度为8.6-39.6ng/L,溶解态甲基汞浓度为0.11-4.9ng/L.实验数据表明,草海湖水以溶解态汞为主,其占总汞的比例为枯水期87%,丰水期51%,溶解态汞与总汞呈显著相关(丰水期P<0.01;枯水期P<0.05),颗粒态汞与总汞也呈显著相关(丰水期P<0.01;枯水期P<0.05).溶解态甲基汞与总甲基汞呈显著相关(丰水期P<0.01;枯水期P<0.05),表明溶解态甲基汞控制总甲基汞的分布.沉积物间隙水溶解态汞与溶解态甲基汞浓度明显高于上覆水体,表明沉积物为草海湖水中汞的一个重要来源.  相似文献   

7.
分析了河北西大洋水库沉积物中16种多环芳烃的含量及分布状况,并对其来源和生态风险进行了分析和评估.结果表明,表层沉积物多环芳烃总含量范围在422.36 - 1052.90 ng/g之间,且由库区上游到坝前逐渐升高.水库剖面沉积物中多环芳烃总含量在388.81 - 1205.56 ng,/g之间,自底层20 cm到表层多...  相似文献   

8.
轮叶黑藻(Hydrilla verticillata)是我国浅水湖泊常见的沉水植物,经常用于湖泊生态修复工程.然而在生态修复中后期,轮叶黑藻又往往会过度繁殖,影响其他湖泊功能的发挥.镧改性膨润土(锁磷剂)可以有效地降低沉积物中生物可利用磷含量,近年来被用于控制湖泊沉积物磷释放,其对轮叶黑藻生长和形态的影响还有待阐明.本研究在2种不同上覆水营养盐浓度条件下,设置添加和不添加锁磷剂2种处理,探究沉积物添加锁磷剂对轮叶黑藻生长及形态特征的影响.结果表明:1)沉积物添加锁磷剂之后,铁锰结合态磷、有机磷、铝结合态磷等生物可利用磷浓度显著降低,而生物不可用磷,如钙结合态磷浓度显著升高; 2)沉积物添加锁磷剂显著降低了轮叶黑藻的生物量和生长率.添加锁磷剂的处理组植物的株高、地上部分生物量均明显低于无锁磷剂组;相反,添加锁磷剂显著增加了植物的根长和地下部分生物量,进而提高了植物的根冠比; 3)锁磷剂对轮叶黑藻生长的影响程度与水体营养盐浓度有关,在低营养盐浓度水体中锁磷剂对植物生长和形态特征的影响更为显著.本研究表明,锁磷剂的添加能降低沉积物中生物可利用磷浓度,抑制轮叶黑藻的生长,同时这种影响程度与在水体营养盐浓度有关.  相似文献   

9.
博斯腾湖沉积物中有机氯农药的分布特征及生态风险评价   总被引:3,自引:0,他引:3  
对新疆博斯腾湖表层沉积物中有机氯农药进行分析,探讨其分布特征及来源,并对其生态风险进行评价.结果表明,沉积物中总有机氯农药的含量为2.15-16.80ng/g,其中氯丹和滴滴涕的含量较高,分别为0.12-12.08 mg/g、0.42-5.13ng/g·博斯腾湖总有机氯农药的含量从入湖口到湖心呈现出下降的趋势,说明其污...  相似文献   

10.
δ13C和δ15N指示不同生态类型湖泊无机氮及有机质来源   总被引:2,自引:0,他引:2  
为了探讨不同生态类型湖泊(天然湖泊、城市湖泊)中无机氮和有机质来源,分别采集湖泊中水体、表层沉积物、水生植物、底栖动物进行碳、氮同位素特征分析.结果表明:蚌湖水体δ15N-NH4均值为-1.8‰±1.0‰,δ15N-NO3-均值为-0.5‰±1.7‰,说明蚌湖水体氮表现为雨水和农业肥料氮污染;象湖δ15 N-NH4+均值为6.8‰±8.6‰,其中养殖废水和管道排污口δ15N-NH4+值分别为13.5‰和25.4‰,表现出污水氮同位素特征,象湖δ15 N-NO3-均值为-2.9‰±4.2‰,是氨的硝化作用引起的氮同位素分馏所致.蚌湖表层沉积物、水生植物δ15N差别不大,分别为6.6‰±0.3‰、7.1‰±0.7‰,水生植物δ13C均值为-27.5‰±0.3‰,比沉积物δ13C偏负3‰.有机C/N为9.4±0.5,比沉积物C/N明显偏高6,反映水生植物是蚌湖有机质的主要来源.象湖表层沉积物δ15N、δ13C及有机C/N分布范围大,δ15N在3.6‰~8.3‰之间,均值为5.9‰±1.6‰,δ13C在-27.1‰~-24.7‰之间,均值为-26.0‰±1.0‰,有机C/N在2.6 ~10.8之间,均值为6.2±2.7,表明城市湖泊沉积有机质来源复杂.2个湖泊蚌类δ15N组成与各自湖泊表层沉积物δ15N组成相对应.  相似文献   

11.
持久性有机污染物(POPs)在环境中分布广泛且持久存在并具有高生物富集性,通常具有致癌、致畸、致突变等危害.湖泊是POPs的主要环境归宿之一,湖泊中的POPs可被水生生物富集并通过食物网传递,对生态系统及人体健康构成极大的危害.中国是POPs生产及使用大国,也是世界上湖泊较多的国家之一.湖泊生物尤其是水产品是中国人饮食中的重要组成部分,因此POPs在中国湖泊生物体中的富集对当地的生态系统和人体健康存在很大的潜在危害.本文通过收集、分析1997年—2017年7月公开发表的中国湖泊生物体POPs数据,发现中国湖泊生物中POPs富集研究主要集中在东部平原湖区,青藏高原及云贵高原湖区有少量研究;不同POPs在不同湖区湖泊生物中富集的含量存在较大差异,DDTs和HCHs在各湖区生物中普遍检出且存在明显差异,东部平原湖区生物体内多氯联苯、多溴联苯醚含量高于其他湖区生物体内含量,其他POPs在湖泊生物体内的富集研究相对较少且主要集中在东部湖泊.中国湖泊生物中DDTs、HCHs、多环芳烃、多氯联苯、多溴联苯醚、多氯苯并二英和多氯苯并呋喃、全氟化合物、全氟辛酸、有机锡及六溴环十二烷脂肪归一化后的平均含量分别为454.56±653.40、153.57±435.99、2849.49±3092.52、118.40±20.28、18.40±20.28、17.43±19.43、147.17±192.93、1542.18±1347.64、11380.75±5316.75和2.19±1.92 ng/g.POPs在中国湖泊生物体内的含量水平与生物所处营养级、脂肪含量和年龄呈正相关,但并非完全一致,还受到生活习性、生物物种与结构、生存环境及生物量等多种因素的影响;生物不同组织对POPs的富集能力有较大差异,内脏器官对POPs的富集能力明显高于肌肉组织.  相似文献   

12.
白洋淀是雄安新区的核心生态功能区.为探究白洋淀不同植物群落区表层沉积物碳(C)氮(N)磷(P)化学计量特征,采集了96组表层沉积物样品开展对比分析.研究表明:白洋淀湿地表层沉积物总有机碳(TOC)含量均值为39.64 g/kg,范围为14.4~ 136.82 g/kg,总氮(TN)和总磷(TP)均值分别为2.62和0....  相似文献   

13.
The evolutions of diatom floras and the total phosphorous (TP) concentrations in the historical period were reconstructed for two lakes, Longgan and Taibai in the middle Yangtze River,based on high resolutional fossil diatom study from two sediment cores and an established regional diatom-TP transfer function. The TP concentration in Longgan Lake changed slightly in the range of 36-62 μg/L and kept its middle trophic level in the past 200 years. The changes of diatom assemblages reflect a macrophyte-dominated history of the lake. During the nineteenth century, the lake TP concentration increased comparatively, corresponding to the increase in abundance of benthic diatoms. The progressive increase of epiphytic diatoms since the onset of the twentieth century indicates the development of aquatic plants, coinciding with the twice drops of water TP level. The TP concentration in Taibai Lake kept a stable status about 50 μg/L before 1953 AD, while diatoms dominated by facultative planktonic Aulacoseira granulata shifted quickly to epiphytic diatom species, indicating a rapid expansion of aquatic vegetation. During 1953-1970 AD, the coverage of aquatic plants decreased greatly inferred by the low abundance of epiphytic diatoms as well as declined planktonic types, and the reconstructed TP concentration shows an obvious rising trend firstly, suggesting the beginning of the lake eutrophication. The lake was in the eutrophic condition after 1970, coinciding with the successive increase of planktonic diatoms. The comparison of the two lakes suggests the internal adjustment and purification function of aquatic plants for nutrients in water. The discrepancy of TP trends in the two lakes after 1960 reflects two different patterns of lake environmental response to human disturbance. Sediments in Taibai Lake clearly recorded the process of lake ecological transformation from the macrophyte-dominated stage to the algae-dominated stage. The limits of TP concentration (68-118 μg/L) in the transitional state can be considered as the critical value between the two stable ecosystems. Further work will be necessary to provide more evidence from the sediments in more eutrophic lakes for the primary inference. The reconstructive TP level and the inference of aquatic plants from fossil diatoms in different lakes, as well as their comparison provide a scientific basis for ecological restoration of eutrophic lakes in research regions.  相似文献   

14.
The evolutions of diatom floras and the total phosphorous (TP) concentrations in the historical period were reconstructed for two lakes, Longgan and Taibai in the middle Yangtze River, based on high resolutional fossil diatom study from two sediment cores and an established regional diatom-TP transfer function. The TP concentration in Longgan Lake changed slightly in the range of 36–62 μg/L and kept its middle trophic level in the past 200 years. The changes of diatom assemblages reflect a macrophyte-dominated history of the lake. During the nineteenth century, the lake TP concentration increased comparatively, corresponding to the increase in abundance of benthic diatoms. The progressive increase of epiphytic diatoms since the onset of the twentieth century indicates the development of aquatic plants, coinciding with the twice drops of water TP level. The TP concentration in Taibai Lake kept a stable status about 50 μg/L before 1953 AD, while diatoms dominated by facultative planktonic Aulacoseira granulata shifted quickly to epiphytic diatom species, indicating a rapid expansion of aquatic vegetation. During 1953–1970 AD, the coverage of aquatic plants decreased greatly inferred by the low abundance of epiphytic diatoms as well as declined planktonic types, and the reconstructed TP concentration shows an obvious rising trend firstly, suggesting the beginning of the lake eutrophication. The lake was in the eutrophic condition after 1970, coinciding with the successive increase of planktonic diatoms. The comparison of the two lakes suggests the internal adjustment and purification function of aquatic plants for nutrients in water. The discrepancy of TP trends in the two lakes after 1960 reflects two different patterns of lake environmental response to human disturbance. Sediments in Taibai Lake clearly recorded the process of lake ecological transformation from the macrophyte-dominated stage to the algae-dominated stage. The limits of TP concentration (68–118 μg/L) in the transitional state can be considered as the critical value between the two stable ecosystems. Further work will be necessary to provide more evidence from the sediments in more eutrophic lakes for the primary inference. The reconstructive TP level and the inference of aquatic plants from fossil diatoms in different lakes, as well as their comparison provide a scientific basis for ecological restoration of eutrophic lakes in research regions.  相似文献   

15.
Hydrologic regime plays an important role in maintaining aquatic ecosystem structures and biogeochemical processes of endorheic salt lakes. Due to joint influences of regional climate change, runoff regulation and water withdrawal, ecological water deficiency has been increasingly prominent in endorheic salt lakes in Northwest China, especially in the Inner Mongolian Plateau. Previous studies mainly focused on establishing and applying methods to determine ecological water levels of lakes, while much less attention was paid to a more important problem – how such water levels could be reached under changed watershed hydrological processes. Solutions of this gap were explored in this study using the Dalinuoer Lake as an example. This lake is a typical endorheic salt lake located in the Inner Mongolian Plateau. It is a critical source to provide important ecological services and economic values for locals. Its ecological water level to maintain the optimum salinity threshold was first calculated by applying a statistical analysis of relationships between the phytoplankton biomass, salinity and water level of the lake. Potential measures to preserve the ecological water level of the lake were subsequently evaluated based on a hydrological process analysis of the watershed. The results indicated that the optimum salinity threshold was 5.7 g/L. This value should be also valid for other endorheic salt lakes in this region. According to a function between the water storage and the mean water depth of this lake, the ecological water level was determined to be 10.28 m with an ecological water deficit of 2.5 × 108 m3. A basin water balance analysis using the results proposed measures to maintain a sustainable ecological water level, including controlling local water consumption and infusing ecological water. The results of this study could be extrapolated to other similar conditions to provide guidance for policy-makers, so that better decisions could be hopefully forged to protect eco-hydrological processes of endorheic salt lakes in the Mongolian Plateau, as well as other comparable scenarios.  相似文献   

16.
郑丙辉  曹晶  王坤  储昭升  姜霞 《湖泊科学》2022,34(3):699-710
目前,我国湖泊富营养化及蓝藻水华问题十分突出,国家高度重视湖泊的生态环境保护.自“九五”以来,国家就投入太湖、巢湖、滇池“老三湖”等重污染湖泊的治理,但成本巨大,且历经近30年才初见成效.按照湖泊污染程度,湖泊治理与保护可分为“污染治理型”“防治结合型”“生态保育型”3大类.“老三湖”的治理是典型的“先污染、后治理”的模式,水质较好湖泊主要属于生态保育型湖泊,因此,“老三湖”治理模式不适用于水质较好湖泊的保护.本文系统总结了我国水质较好湖泊优先保护理念的形成和水质较好湖泊专项实施的历程.根据水质较好湖泊的特点,及其生态系统退化与修复的一般过程,提出了水质较好湖泊保护的基本思路.从热力学角度,阐明了氮磷营养盐输入湖泊生态系统中是熵增过程,也是湖泊生态系统退化的根本原因,湖泊氮磷污染负荷源头控制是关键.湖泊流域生态安全格局是确保湖泊生态系统健康的基础,从景观生态学角度,阐明了优化湖泊流域水土资源利用、优化发展模式是减轻湖泊环境压力的重要途径.在浅水湖泊生态系统,以沉水植物占优势的“清水态”和以浮游植物占优势的“浊水态”转换过程不是沿着同一条途径,存在上临界阈值和下临界阈值,水生态修复过程表现出一种迟滞的现象.从湖泊水生态系统稳态转换理论角度,阐明了湖泊生态修复工程应在湖泊生态系统发生退化转变之前实施,才能获得较高的环境效益.通过国家财政专项对81个水质较好湖泊的支持,既能促进湖泊流域经济社会发展,又能确保湖泊水环境质量变好,湖泊水生态系统逐步改善.建议加强不同类型湖泊保护模式的总结,深入对水质较好湖泊生态系统演替理论和保护技术研究,支撑国家系统开展水质较好湖泊保护.  相似文献   

17.
武汉典型湖泊沉积物中重金属累积特征及其环境风险   总被引:20,自引:1,他引:19  
采集武汉市8个典型湖泊的表层沉积物,分析11种重金属的含量及其不同形态组成,研究了不同湖泊金属元素的富集与污染程度,探讨了沉积物中重金属的污染来源及其潜在生态风险,结果表明,沉积物中重金属Cd累积最严重,Zn和Hg也发生明显累积,龙阳湖污染较重,南太子湖和墨水湖污染中等,其它湖泊污染总体较轻.沉积物性质对重金属累积的影响不显著,城市工业活动强烈影响着重金属的分布,不同重金属的形态分布差异较大,Cd生物可利用态含量最高,其次为Mn、Zn、Co、Cu和Pb;而Sb和Hg以残留态占绝对优势,生态风险较小,相关分析和主成分分析表明,化石燃料燃烧、金属冶炼等是武汉市湖泊沉积物中重金属来源的主要贡献者,同时岩石风化等地球化学过程也影响着重金属的污染.  相似文献   

18.
人类活动对江汉湖群沼泽化的影响   总被引:3,自引:0,他引:3  
邹尚辉 《湖泊科学》1992,4(4):71-76
从破坏植被加速湖泊淤积速度、围湖造田使湖泊日渐萎缩、江湖隔绝促进水生高等植物生长、垸湖沼同体而互相转化等方面论述了人类活动加速了江汉湖群湖泊沼泽化的进程,并提出缓解湖泊沼泽化的措施;人类活动既具有加速湖泊沼泽化进程的作用亦具有延缓甚至逆转沼泽化进程的双向作用。  相似文献   

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