IPCC AR6报告解读：气候系统对二氧化碳移除响应

IPCC AR6报告中控温1.5℃和2℃的低排放情景需要在21世纪中叶以后实现净负CO₂排放,这需要在很大程度上依赖CO₂移除措施。AR6对CO₂移除的主要评估结论如下：CO₂移除有潜力从大气中去除CO₂（高信度);如果CO₂移除量超过CO₂排放量,将实现净负CO₂排放,降低大气CO₂浓度,减缓海洋酸化（高信度);通过CO₂移除方法从大气中去除的CO₂会部分被海洋和陆地释放的CO₂抵消（非常高信度);如果净负CO₂排放可以实现并且持续,CO₂引起的全球升温趋势将会逐渐扭转,但是气候系统的其他变化（例如海平面升高）仍会在未来的几十年到千年尺度上持续（高信度);不同CO₂移除方法会对生物化学循环和气候产生广泛的影响,这些影响会加强或减弱CO₂移除的降温潜力,并且影响水资源、食物生产和生物多样性（高信度）。     

Atmospheric response to deep-sea injections of fossil-fuel carbon dioxide

The possibility of controlling atmospheric carbon dioxide accumulation and attendant climatic effects from fossil-fuel burning by diverting a fraction of the combustion product and injecting it into the deep-ocean, as proposed by Marchetti, is analyzed using an atmosphere/mixed layer/diffusive deep-ocean model for the carbon cycle. The model includes the nonlinear buffering of CO₂ at the air/sea interface, and considers the long term trends associated with consuming an assumed fossil-fuel reserve equivalent to 7.09 × 10¹⁵ kg carbon as a logistic function of time as in the projections of Siegenthaler and Oeschger, except that atmospheric carbon dioxide levels are computed for five alternate strategies: (a) 100% injected into atmosphere, (b) 50% injected at oceanic depth of 1500 m and 50% into atmosphere, (c) 50% injected at sea floor (4000 m) and 50% into atmosphere, (d) 100% at 1500 m depth and (e) 100% at sea floor. Since no carbon leaves the system, all runs approached the same post-fossil fuel equilibrium after several thousand years, C _a - 1150 ppm, almost four times the pre-fossil fuel value (- 300 ppm). But the transient response of these cases showed a marked variation ranging from a peak overshoot value of 2800 ppm in the year 2130 for 100% atmospheric injection to a slight decrease to the pre-fossil fuel 300 ppm lasting till 2300 with a subsequent slow approach to equilibrium for the 100% deep-ocean injection. The implications of these results for an oceanic injection strategy to mitigate the climatic impact of fossil-fuel CO₂ is discussed, as are the ingredients of a second generation carbon cycle model for carrying out such forecasts on an engineering design basis.     

The atmospheric carbon dioxide response to oceanic primary productivity fluctuations

Data on the rate of primary production, the rate of sinking and oxidation of organic detritus, the rate of regeneration of calcium carbonate, the average rate of vertical mixing, and the vertical profile of dissolved carbon are consistent with a model of the ocean in which the downward transport of carbon by the sinking and oxidation of organic particulate matter is balanced by upward hydrodynamic mixing of dissolved inorganic carbon. A time dependent version of this model is used to make rough estimates of the effect of periodic and impulsive changes in the rate of primary production on the atmospheric CO₂ concentration. The computations suggest that a 1% decrease in marine biospheric productivity could result in a steady state increase of the atmospheric CO₂ concentration of from 0.5 to 2.5% depending on the rate of vertical mixing. Large but short term fluctuations in productivity, such as a die-off of the marine biosphere followed by an exponential recovery period, are estimated to produce smaller perturbations.Work performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under contract No. W-7405-ENG-48.     

Soil temperature response in Korea to a changing climate using a land surface model

The land surface processes play an important role in weather and climate systems through its regulation of radiation, heat, water and momentum fluxes. Soil temperature (ST) is one of the most important parameters in the land surface processes; however, there are few extensive measurements of ST with a long time series in the world. According to the CLImatology of Parameters at the Surface (CLIPS) methodology, the output of a trusted Soil-Vegetation- Atmosphere Transfer (SVAT) scheme can be utilized instead of observations to investigate the regional climate of interest. In this study, ST in South Korea is estimated in a view of future climate using the output from a trusted SVAT scheme — the University of TOrino model of land Process Interaction with Atmosphere (UTOPIA), which is driven by a regional climate model. Here characteristic changes in ST are analyzed under the IPCC A2 future climate for 2046-2055 and 2091-2100, and are compared with those under the reference climate for 1996-2005. The UTOPIA results were validated using the observed ST in the reference climate, and the model proved to produce reasonable ST in South Korea. The UTOPIA simulations indicate that ST increases due to environmental change, especially in air temperature (AT), in the future climate. The increment of ST is proportional to that of AT except for winter. In wintertime, the ST variations are different from region to region mainly due to variations in snow cover, which keeps ST from significant changes by the climate change.     

Dynamic responses of atmospheric carbon dioxide concentration to global temperature changes between 1850 and 2010

Changes in Earth's temperature have significant impacts on the global carbon cycle that vary at different time scales, yet to quantify such impacts with a simple scheme is traditionally deemed difficult. Here, we show that, by incorporating a temperature sensitivity parameter(1.64 ppm yr~(-1) ?C~(-1)) into a simple linear carbon-cycle model, we can accurately characterize the dynamic responses of atmospheric carbon dioxide(CO_2) concentration to anthropogenic carbon emissions and global temperature changes between 1850 and 2010(r~2 0.96 and the root-mean-square error 1 ppm for the period from 1960onward). Analytical analysis also indicates that the multiplication of the parameter with the response time of the atmospheric carbon reservoir(～12 year) approximates the long-term temperature sensitivity of global atmospheric CO_2concentration(～15 ppm?C~(-1)), generally consistent with previous estimates based on reconstructed CO_2 and climate records over the Little Ice Age. Our results suggest that recent increases in global surface temperatures, which accelerate the release of carbon from the surface reservoirs into the atmosphere, have partially offset surface carbon uptakes enhanced by the elevated atmospheric CO_2 concentration and slowed the net rate of atmospheric CO_2 sequestration by global land and oceans by ～30%since the 1960 s. The linear modeling framework outlined in this paper thus provides a useful tool to diagnose the observed atmospheric CO_2 dynamics and monitor their future changes.     

Importance of the mixed-phase cloud distribution in the control climate for assessing the response of clouds to carbon dioxide increase: a multi-model study

We have conducted a multi-model intercomparison of cloud-water in five state-of-the-art AGCMs run for control and doubled carbon dioxide climates. The most notable feature of the differences between the control and doubled carbon dioxide climates is in the distribution of cloud-water in the mixed-phase temperature band. The difference is greatest at mid and high latitudes. We found that the amount of cloud ice in the mixed phase layer in the control climate largely determines how much the cloud-water distribution changes for the doubled carbon dioxide climate. Therefore evaluation of the cloud ice distribution by comparison with data is important for future climate sensitivity studies. Cloud ice and cloud liquid both decrease in the layer below the melting layer, but only cloud liquid increases in the mixed-phase layer. Although the decrease in cloud-water below the melting layer occurs at all latitudes, the increase in cloud liquid in the mixed-phase layer is restricted to those latitudes where there is a large amount of cloud ice in the mixed-phase layer. If the cloud ice in the mixed-phase layer is concentrated at high latitudes, doubling of carbon dioxide might shift the center of cloud water distribution poleward which could decrease solar reflection because solar insolation is less at higher latitude. The magnitude of this poleward shift of cloud water appears to be larger for the higher climate sensitivity models, and it is consistent with the associated changes in cloud albedo forcing. For the control climate there is a clear relationship between the differences in cloud-water and relative humidity between the different models, for both magnitude and distribution. On the other hand the ratio of cloud ice to cloud-water follows the threshold temperature which is determined in each model. Improved measurements of relative humidity could be used to constrain the modeled representation of cloud water. At the same time, comparative analysis in global cloud resolving model simulations is necessary for further understanding of the relationships suggested in this paper.     

Impacts of carbon dioxide warming on climate and man in the semi-arid tropics

Tropical semi-arid climates occur between 10 and 35 deg latitude and are characterised by highly variable summer rainfall of between 300 and 750 mm in a rainy season of at least 4 months, generally adequate for rainfed cropping but with considerable drought risk. They support a mesic savanna vegetation. They have a land extent of 4.5 million km², mainly occupied by Third World nations with rapidly increasing populations which in the main are predominantly rural and largely agricultural with low per capita incomes, consequently vulnerable to climate change. A doubling of atmospheric CO₂ by the year 2030 is predicted to cause a rise in equilibrium mean temperature of 1–3 °C; however there is continuing uncertainty regarding the consequences for rainfall amount, variability and intensity, length of rainy season or the frequency of extreme rainfall events. Two scenarios are considered, with reduction and increase in rainfall respectively, involving corresponding latitudinal shifts in present climatic boundaries of about 200 km. Because of their variability, a clear signal of the greenhouse effect on these climates may be delayed, whilst regional responses may differ. Vegetational and hydrological responses under the alternative scenarios are considered. The possible consequences for rainfed and irrigated agriculture, water and energy supplies and disease and pest ecology are discussed. Lands of the semi-arid tropics are already extensively desertified, with consequent lowered productivity and heightened vulnerability to drought, and the possible impacts of greenhouse warming on desertification processes and on measures for land rehabilition to the year 2030 are reviewed. Measures to conserve the biological diversity of savanna lands in face of greenhouse warming are discussed.     

The European and global potential of carbon dioxide sequestration in tackling climate change

Although, it has received relatively little attention as a potential method of combating climate change in comparison to energy reduction measures and development of carbon-free energy technologies, sequestration of carbon dioxide in geologic or biospheric sinks has enormous potential. This paper reviews the potential for sequestration using geological and ocean storage as a means of reducing carbon dioxide emissions.Considerable quantities of carbon dioxide separated from natural gas deposits and from hydrogen production from steam reforming of methane are already used in enhanced oil recovery and in extraction of coalbed methane, the carbon dioxide remaining sequestered at the end of the process. A number of barriers lie in the way of its implementation on a large scale. There are concerns about possible environmental effects of large-scale injection of carbon dioxide especially into the oceans. Available technologies, especially of separating and capturing the carbon dioxide from waste stream, have high costs at present, perhaps representing an additional 40–100% onto the costs of generating electricity. In most of the world there are no mechanisms to encourage firms to consider sequestration.Considerable R&D is required to bring down the costs of the process, to elucidate the environmental effects of storage and to ensure that carbon dioxide will not escape from stores in unacceptably short timescales. However, the potential of sequestration should not be underestimated as a contribution to global climate change mitigation measures.     

The Montsouris series of carbon dioxide concentration measurements, 1877–1910

The longest continuous record of measurements of atmospheric CO₂ concentration available to date, that was made between 1877 and 1910 at the Montsouris Observatory in the outskirts of Paris, is presented and the methods used and the site are described. Annual, seasonal and daily variations in the record were considerable, especially between 1877 and 1880 and possible reasons for this high variability are discussed. Although no direct proof of the reliability of the series is available an attempt has been made to estimate this by comparisons with contemporary series whose precision is better known and also through an analysis of the results from the point of view of the major sources of error. The results suggest a precision of measurement better than 2%; analysis of the daily and the mean seasonal variation shows no evidence of any significant urban contamination of the Montsouris record. Mean decadal values of the Montsouris series show a marked rise in concentration from 283 ppm in the first decade to 313 ppm in the second, with a small and nonsignificant drop to 309 ppm in the third decade of the series. The results of the measurements are thus compatible with the hypothesis that a major and variable non-fossil fuel source of atmospheric CO₂ was active during the last quarter of the nineteenth century. Contribution from the Agricultural Research Organization, The Volcani Center, Bet Dagan, Israel. No. 254-E, 1981 series.     

Transient responses of North-American grasslands to changes in climate

Our objective was to evaluate the transient responses of grasslands in the central grassland region of North America to changes in climate. We used an individual plant-based gap dynamics simulation model (STEPPE-GP) linked with a soil water model (SOILWAT) to evaluate the effects of changes in climate on the composition and structure of grassland vegetation. Five functional types of plants were simulated based upon lifeform, physiology, and rooting distribution with depth. C₃ and C₄ perennial grasses with either a shallow or deep rooting distribution, and deeply rooted C₃ shrubs were simulated under current climatic conditions and under a GFDL climate change scenario for nine sites representative of the temperature and precipitation regimes in the grassland region.Although vegetation at the sites responded differently to climate change, shifts in functional types occurred within 40 years of the start of the climate change. C₄ grasses increased in dominance or importance at all sites with a change in climate, primarily as a result of increases in temperature in all months at all sites. The coolest sites that arc currently dominated by C₃ grasses were predicted to shift to a dominance by C₄ grasses, whereas sites that are currently dominated by C₄ grasses had an increase in importance of this functional type with a change in climate. Current annual temperature was the best predictor of changes in C₃ biomass, and C₃ and C₄ biomass combined; current annual precipitation was the best predictor of changes in C₄ biomass. These predicted shifts in dominance and importance of C₃ versus C₄ grasses would have important implications for the management of natural grasslands as well as the cultivation of crops in the central grassland region.     

Responses of arid and semiarid watersheds to increasing carbon dioxide and climate change as shown by simulation studies

The atmospheric concentration of carbon dioxide is expected to double in the next century causing increased temperatures and decreasing precipitation in some regions of the U.S. The increase in CO₂ will also directly affect stomatal conductance of plants. At the first-order watershed scale, changes in evaporative demand, transpiration, and runoff will also occur. Previous modeling studies of the effect of increased CO₂ on the water budgets of watersheds have been single-factor exercises where a single parameter representing stomatal conductance was reduced and the results noted. After showing validation results of the hydrology module, we used a comprehensive ecosystem model to examine the consequences of changes in precipitation, temperature, and CO₂-induced plant-function characteristics on small-basin runoff. As a result of the complex interactions and of the compensatory mechanisms simulated by the model, we conclude that for arid and semiarid watersheds of the western United States, there will be little change or an actual decrease in surface runoff because of increased CO₂ and climate change. This is due to the decrease in precipitation imposed on the model simulations. Implementing stomatal closure in the model did not increase runoff from the watersheds when temperatures were increased and precipitation decreased.     

The carbon dioxide/climate controversy: Some personal comments on two recent publications

The pervasive opinion on the relationship between the state of the climate and the increasing concentration of CO₂ is that a general global warming will occur with social, economical and environmental corollaries that may be adverse. However, there exist a number of dissenting arguments that call for a much smaller increase in global temperature or even an induced global cooling. Furthermore, the positive biological effects of a greater atmospheric CO₂ loading are emphasized.The difference of opinion is highlighted in two recent publications: CO ₂, Friend or Foe by Sherwood Idso and Carbon Dioxide: A Second Assessment by the National Academy of Science CO₂/Climate Review Committee. Using the two publications as focal points, some personal remarks are made regarding the controversy and the relative merits of the scientific arguments.