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1.
In many atmospheric flows, a dispersed phase is actively suspended by turbulence, whose competition with gravitational settling ultimately dictates its vertical distribution. Examples of dispersed phases include snow, sea-spray droplets, dust, or sand, where individual elements of much larger density than the surrounding air are carried by turbulent motions after emission from the surface. In cases where the particle is assumed to deviate from local fluid motions only by its gravitational settling (i.e., they are inertialess), traditional flux balances predict a power-law dependence of particle concentration with height. It is unclear, however, how particle inertia influences this relationship, and this question is the focus of this work. Direct numerical simulations are conducted of turbulent open-channel flow, laden with Lagrangian particles of specified inertia; in this way the study focuses on the turbulent transport which occurs in the lowest few meters of the planetary boundary layer, in regions critical for connecting emission fluxes to the fluxes felt by the full-scale boundary layer. Simulations over a wide range of particle Stokes number, while holding the dimensionless settling velocity constant, are performed to understand the role of particle inertia on vertical dispersion. It is found that particles deviate from their inertialess behaviour in ways that are not easily captured by traditional theory; concentrations are reduced with increasing Stokes number. Furthermore, a similarity-based eddy diffusivity for particle concentration fails as particles experience inertial acceleration, precluding a closed-form solution for particle concentration as in the case of inertialess particles. The primary consequence of this result is that typical flux parametrizations connecting surface emission models (e.g., saltation models or sea-spray generation functions) to elevated boundary conditions may overestimate particle concentrations due to the reduced vertical transport caused by inertia in between; likewise particle emission may be underestimated if inferred from concentration measurements aloft.  相似文献   

2.
Higher-order moments, minima and maxima of turbulent temperature and water vapour mixing ratio probability density functions measured with an eddy-covariance system near the ground were related to each other and to vertical boundary-layer profiles of the same scalars obtained through airborne soundings. The dependence of kurtosis on squared skewness showed a kurtosis intercept below the Gaussian expectation, suggesting a compression of the probability density function by the presence of natural boundaries. This hypothesis was corroborated by comparing actual minima and maxima of turbulent fluctuations to estimates obtained from the first four sample moments by fitting a four-parameter beta distribution. The most sharply defined boundaries were found for the minima of temperature datasets during the day, indicating that negative temperature fluctuations at the sensor are limited by the availability of lower temperatures in the boundary layer. By comparison to vertical profiles, it could be verified that the turbulent minimum of temperature near the ground is close to the minimum of potential temperature in the boundary layer. The turbulent minimum of water vapour mixing ratio was found to be equal to the mixing ratio at a height above the minimum of the temperature profile. This height roughly agrees with the top of the non-local unstable domain according to bulk Richardson number profiles. We conclude that turbulence statistics measured near the surface cannot be solely explained by local effects, but contain information about the whole boundary layer including the entrainment zone.  相似文献   

3.
Large-eddy simulation of turbulent flow above and within a forest   总被引:10,自引:22,他引:10  
A large-eddy simulation has been performed of an atmospheric surface layer in which the lower third of the domain is occupied by a drag layer and heat sources to represent a forest. Subgridscale processes are treated using second-order closure techniques. Lateral boundaries are periodic, while the upper boundary is a frictionless fixed lid. Mean vertical profiles of wind velocity derived from the output are realistic in their shape and response to forest density. Similarly, vertical profiles of Reynolds stress, turbulent kinetic energy and velocity skewness match observations, at least in a qualitative sense. The limited vertical extent of the domain and the artificial upper boundary, however, cause some departures from measured turbulence profiles in real forests. Instantaneous turbulent velocity and scalar fields are presented which show some of the features obtained by tower instrumentation in the field and in wind tunnels, such as the vertical coherence of vertical velocity and the slope of structures revealed by temperature patterns.  相似文献   

4.
Using the new high-frequency measurement equipment of the research aircraft DO 128, which is described in detail, turbulent vertical fluxes of ozone and nitric oxide have been calculated from data sampled during the ESCOMPTE program in the south of France. Based on airborne turbulence measurements, radiosonde data and surface energy balance measurements, the convective boundary layer (CBL) is examined under two different aspects. The analysis covers boundary-layer convection with respect to (i) the control of CBL depth by surface heating and synoptic scale influences, and (ii) the structure of convective plumes and their vertical transport of ozone and nitric oxides. The orographic structure of the terrain causes significant differences between planetary boundary layer (PBL) heights, which are found to exceed those of terrain height variations on average. A comparison of boundary-layer flux profiles as well as mean quantities over flat and complex terrain and also under different pollution situations and weather conditions shows relationships between vertical gradients and corresponding turbulent fluxes. Generally, NOx transports are directed upward independent of the terrain, since primary emission sources are located near the ground. For ozone, negative fluxes are common in the lower CBL in accordance with the deposition of O3 at the surface.The detailed structure of thermals, which largely carry out vertical transports in the boundary layer, are examined with a conditional sampling technique. Updrafts mostly contain warm, moist and NOx loaded air, while the ozone transport by thermals alternates with the background ozone gradient. Evidence for handover processes of trace gases to the free atmosphere can be found in the case of existing gradients across the boundary-layer top. An analysis of the size of eddies suggests the possibility of some influence of the heterogeneous terrain in mountainous area on the length scales of eddies.  相似文献   

5.
Two airborne campaigns were carried out to measure the tropospheric concentrations and variability of CO2, CO and O3 over Siberia. In order to quantify the influence of remote and regional natural and anthropogenic sources, we analysed a total of 52 vertical profiles of these species collected in April and September 2006, every ∼200 km and up to 7 km altitude. CO2 and CO concentrations were high in April 2006 (respectively 385–390 ppm CO2 and 160–200 ppb CO) compared to background values. CO concentrations up to 220 ppb were recorded above 3.5 km over eastern Siberia, with enhancements in 500–1000 m thick layers. The presence of CO enriched air masses resulted from a quick frontal uplift of a polluted air mass exposed to northern China anthropogenic emissions and to fire emissions in northern Mongolia. A dominant Asian origin for CO above 4 km (71.0%) contrasted with a dominant European origin below this altitude (70.9%) was deduced both from a transport model analysis, and from the contrasted ΔCO/ΔCO2 ratio vertical distribution. In September 2006, a significant O3 depletion (∼–30 ppb) was repeatedly observed in the boundary layer, as diagnosed from virtual potential temperature profiles and CO2 gradients, compared to the free troposphere aloft, suggestive of a strong O3 deposition over Siberian forests.  相似文献   

6.
2010年春季北京地区强沙尘暴过程的微气象学特征   总被引:3,自引:1,他引:2  
利用北京大学校园地区PM10质量浓度观测资料、中国科学院大气物理研究所325m气象塔气象要素梯度和湍流观测资料,分析了北京地区2010年3月20~22日两次强沙尘暴过程微气象学要素和沙尘参量的时空演变以及湍流输送特征,为理解北京地区强沙尘暴天气沙尘输送规律和微气象学特征提供参考。结果表明:3月20~22日强沙尘暴过程前后不同高度温度先升后降,气压和相对湿度则相反。强沙尘暴来临时,高层风速先迅速增大,低层风速增加略有滞后,风切变明显加强,PM10浓度最大值和风速极大值出现时间较吻合。强沙尘暴过境时,不同高度向下的湍流动量输送、向上的湍流热量输送和湍流动能明显加强。与3月21日非沙尘暴日相比,强沙尘暴过程湍流动量通量增加,有利于沙尘粒子的水平和垂直输送过程;由于冷锋过境,水平热通量增大;垂直热通量因白天温度垂直梯度减小而减小,夜间因逆温层被破坏而增加;水平湍流动能对湍流动能占主要贡献,垂直湍流动能仅占水平湍流动能的10%~25%。  相似文献   

7.
We study the dynamics of sea-spray particles in the coastal region of La Reunion Island on the basis of numerical simulations using the transport aerosol model MACMod (Marine Aerosol Concentration Model) and a survey of the aerosol size distributions measured at four locations at two different heights in the north-west part of the island. This allows evaluation of the performance of our model in case of pure marine air masses with implementation of accurate boundary conditions. First of all, an estimate of the aerosol concentration at 10-m height at the upwind boundary of the calculation domain is obtained using a revisited version of the MEDEX (Mediterranean Extinction) model. Estimates of the vertical profile of aerosol concentrations are then provided using aerosol data obtained at two different heights at the upwind boundary of the calculation domain. A parametrization of the vertical profiles of aerosol concentrations for maritime environment is proposed. The results are then compared to the vertical profiles of 0.532 \(\upmu \)m aerosol particle extinction coefficient obtained from lidar data provided by the Cloud-Aerosol LIdar with Orthogonal Polarization (CALIOP) and also to the data provided by the Aerosol Robotic Network (AERONET). This allows validation of the complete vertical profiles in the mixed layer and shows the validity of satellite data for determination of the vertical profiles. Two kinds of simulation were made: one without a particle advection flux at the upwind boundary of the numerical domain, whereas the second simulation was made with a particle advection flux. In the first case, the influence of the distance to the shoreline on the local sea-spray dynamics is investigated. In the second set of simulation, the particles issued from the local production in the surf zone near the shoreline are mixed with aerosols advected from the remote ocean. A good agreement between the model calculations using our boundary conditions and the data was found. The present results then attest the ability of this kind of model, as a first approach to predicting the local transport of sea-spray particles in a pure marine environment.  相似文献   

8.
Numerical simulations of scalar transport in neutral flow over forested ridges are performed using both a 1.5-order mixing-length closure scheme and a large-eddy simulation. Such scalar transport (particularly of CO2) has been a significant motivation for dynamical studies of forest canopy–atmosphere interactions. Results from the 1.5-order mixing-length simulations show that hills for which there is significant mean flow into and out of the canopy are more efficient at transporting scalars from the canopy to the boundary layer above. For the case with a source in the canopy this leads to lower mean concentrations of tracer within the canopy, although they can be very large horizontal variations over the hill. These variations are closed linked to flow separation and recirculation in the canopy and can lead to maximum concentrations near the separation point that exceed those over flat ground. Simple scaling arguments building on the analytical model of Finnigan and Belcher (Q J Roy Meteorol Soc 130:1–29, 2004) successfully predict the variations in scalar concentration near the canopy top over a range of hills. Interestingly this analysis suggests that variations in the components of the turbulent transport term, rather than advection, give rise to the leading order variations in scalar concentration. The scaling arguments provide a quantitative measure of the role of advection, and suggest that for smaller/steeper hills and deeper/sparser canopies advection will be more important. This agrees well with results from the numerical simulations. A large-eddy simulation is used to support the results from the mixing-length closure model and to allow more detailed investigation of the turbulent transport of scalars within and above the canopy. Scalar concentration profiles are very similar in both models, despite the fact that there are significant differences in the turbulent transport, highlighted by the strong variations in the turbulent Schmidt number both in the vertical and across the hill in the large-eddy simulation that are not represented in the mixing-length model.  相似文献   

9.
An expression for the vertical equilibrium concentration profile of heavy particles, including the effects of canopy on the eddy diffusivity as well as corrections for atmospheric stability, is proposed. This expression is validated against measurements of vertical concentration profiles of corn pollen above a corn field. The fitted theoretical profiles show that particle settling is correctly accounted for. The sensitivity to variations in the turbulent Schmidt number, settling velocity and stability corrections are explicitly characterized. The importance of independent measurements of the surface flux of pollen in future experiments is noted.  相似文献   

10.
We utilize experimental data collected in 2002 over an open field in Hanford, Washington, USA, to investigate the turbulent kinetic energy (TKE) budget in the atmospheric surface layer. The von Kármán constant was determined from the near-neutral wind profiles to be 0.36 ± 0.02 rather than the classical value of 0.4. The TKE budget was normalized and all terms were parameterized as functions of a stability parameter z/L, where z is the distance from the ground and L is the Obukhov length. The shear production followed the Businger–Dyer relation for −2 < z/L < 1. Contrary to the traditional Monin–Obukhov similarity theory (MOST), the shear, buoyancy and dissipation terms were found to be imbalanced due to a non-zero vertical transport over all stabilities. Motivated by this local imbalance, modified parameterizations of the dissipation and the turbulent transport were attempted and generated good agreement with the experimental data. Assuming stationarity and horizontal homogeneity, the pressure transport was estimated from the residual of the TKE budget.  相似文献   

11.
This is the first of a series of three papers describing experiments on the dispersion of trace heat from elevated line and plane sources within a model plant canopy in a wind tunnel. Here we consider the wind field and turbulence structure. The model canopy consisted of bluff elements 60 mm high and 10 mm wide in a diamond array with frontal area index 0.23; streamwise and vertical velocity components were measured with a special three-hot-wire anemometer designed for optimum performance in flows of high turbulence intensity. We found that:
  1. The momentum flux due to spatial correlations between time-averaged streamwise and vertical velocity components (the dispersive flux) was negligible, at heights near and above the top of the canopy.
  2. In the turbulent energy budget, turbulent transport was a major loss (of about one-third of local production) near the top of the canopy, and was the principal gain mechanism lower down. Wake production was greater than shear production throughout the canopy. Pressure transport just above the canopy, inferred by difference, appeared to be a gain in approximate balance with the turbulent transport loss.
  3. In the shear stress budget, wake production was negligible. The role of turbulent transport was equivalent to that in the turbulent energy budget, though smaller.
  4. Velocity spectra above and within the canopy showed the dominance of large eddies occupying much of the boundary layer and moving downstream with a height-independent convection velocity. Within the canopy, much of the vertical but relatively little of the streamwise variance occurred at frequencies characteristic of wake turbulence.
  5. Quadrant analysis of the shear stress showed only a slight excess of sweeps over ejections near the top of the canopy, in contrast with previous studies. This is a result of improved measurement techniques; it suggests some reappraisal of inferences previously drawn from quadrant analysis.
  相似文献   

12.
Abstract

Arctic haze has been attributed to industrial pollution released at mid‐latitudes. Our current understanding has been pieced together from routine meteorological data, ground‐based air chemistry observations and limited aircraft measurements. This study investigates the relationship between synoptic boundary‐layer meteorology and the composition of the near‐surface atmosphere during the polar sunrise at Alert, N.W.T. A secondary objective is to characterize the influence of local activity on the atmospheric composition at a site for a new baseline monitoring station and at a location where aerosol chemistry and grab‐flask samples for CO2 have been made for many years. Detailed measurements of the vertical distribution of aerosols were obtained from an upward‐looking lidar to complement the ground‐based measurements. Meteorological profiles of the near‐surface boundary layer were obtained from both free‐flying and tethered balloons. Near‐surface measurements were made of aerosol physical and chemical properties, O3, NO2, NO/NOx, Peroxyacetylnitrate (PAN) and hydrocarbons.

The study period was characterized by prolonged periods with strong surface inversions, which were broken up occasionally by intrusions of cold air into the warmer air aloft. Lidar observations showed that ice crystals often accompanied aerosols and were responsible for reducing visibility below 30–40 km. There was a strong correlation between aerosol mass in the diameter size range 0.15 to 1.5 μm and total SO4 = . PAN found at concentrations of about 200 ppt(v) was the main carrier of atmospheric nitrogen. Aerosol trace elements were divisible into anthropogenic soil, mixed soil/anthropogenic sea salt and halogens. Vertical transport in the surface boundary layer, as regulated by the strength of the surface radiation inversion, may play an important role in influencing the chemical composition of the air at the ground. The location of the new baseline monitoring laboratory was found to be generally windier and warmer than the lower altitude weather station, and the influence of local activity was found to be minimal.  相似文献   

13.
This study analyzes and compares aerosol properties and meteorological conditions during two air pollution episodes in 19–22 (E1) and 25–26 (E2) December 2016 in Northeast China. The visibility, particulate matter (PM) mass concentration, and surface meteorological observations were examined, together with the planetary boundary layer (PBL) properties and vertical profiles of aerosol extinction coefficient and volume depolarization ratio that were measured by a ground-based lidar in Shenyang of Liaoning Province, China during December 2016–January 2017. Results suggest that the low PBL height led to poor pollution dilution in E1, while the high PBL accompanied by low visibility in E2 might have been due to cross-regional and vertical air transmission. The PM mass concentration decreased as the PBL height increased in E1 while these two variables were positively correlated in E2. The enhanced winds in E2 diffused the pollutants and contributed largely to the aerosol transport. Strong temperature inversion in E1 resulted in increased PM2.5 and PM10 concentrations, and the winds in E2 favoured the southwesterly transport of aerosols from the North China Plain into the region surrounding Shenyang. The large extinction coefficient was partially attributed to the local pollution under the low PBL with high ground-surface PM mass concentrations in E1, whereas the cross-regional transport of aerosols within a high PBL and the low PM mass concentration near the ground in E2 were associated with severe aerosol extinction at high altitudes. These results may facilitate better understanding of the vertical distribution of aerosol properties during winter pollution events in Northeast China.  相似文献   

14.
A laser radar (lidar) operating at the ruby line 0.6943 μm has been observing horizontal profiles of particulate concentration in the air some 30 m above the surface within the city of London over a period of one year. Anomalous features in these profiles are interpreted as natural thermal plumes carrying particles upwards from surfaces such as paved roadways, paved parking lots, treed parks, residential construction sites, open ploughed fields, and the river. Insolation of the ground is required for their formation, and neutral thermal stability aloft favours their incidence.  相似文献   

15.
Multiaxis differential absorption spectroscopy(MAX-DOAS) is a newly developed advanced vertical profile detection method, but the vertical nitrogen dioxide(NO_2) profiles measured by MAX-DOAS have not yet been fully verified. In this study, we perform MAX-DOAS and tower gradient observations to simultaneously acquire tropospheric NO_2 observations in the Beijing urban area from 1 April to 31 May 2019. The average values of the tropospheric NO_2 vertical column densities measured by MAX-DOAS and the tropospheric monitoring instrument are 15.8 × 10~(15) and 12.4 × 10~(15) molecules cm~(-2), respectively, and the correlation coefficient R reaches 0.87. The MAX-DOAS measurements are highly consistent with the tower-based in situ measurements, and the correlation coefficients R from the ground to the upper air are 0.89(60 m), 0.87(160 m), and 0.76(280 m). MAX-DOAS accurately measures the trend of NO_2 vertical profile changes,although a large underestimation occurs by a factor of two. By analyzing the NO_2 vertical profile, the NO_2 concentration reveals an exponential decrease with height. The NO_2 vertical profile also coincides with the evolution of the boundary layer height. The study shows that the NO_2 over Beijing mainly originates from local sources and occurs in the boundary layer, and its vertical evolution pattern has an important guiding significance to better understand nitrate production and ozone pollution.  相似文献   

16.
大气污染物的垂直梯度观测是识别区域输送和本地贡献的必要手段。基于此,2020年8月在拉萨市利用光学粒子计数器(the Printed Optical Particle Spectrometer,简称POPS)在地面和系留气艇分别对0.13~3.39 μm粒径范围的气溶胶数浓度进行了测定。结果表明:(1)拉萨近地面气溶胶数浓度在16 cm?3到870 cm?3范围之间,比华北和珠江三角洲地区小2~3个量级;(2)气溶胶数浓度呈现两峰两谷的日变化结构,峰值通常以0.13~0.4 μm的小粒径粒子为主,且对应北京时间早(10:00)、晚(21:00)高峰时段;(3)气溶胶数浓度垂直分布与边界层演变密切相关,稳定边界层中的气溶胶随高度递减,粒子数浓度为194±94 cm?3,对流边界层和残留层中的气溶胶分布均一,数浓度分别为165±99 cm?3和123±95 cm?3,且显著低于稳定边界层。以上研究结果表明,拉萨的污染源主要为局地机动车排放,机动车污染物减排是打造高原生态旅游城市的必由之路。  相似文献   

17.
This case study introduces measurements of turbulent fluxes in a nocturnal boundary layer in North Germany with the new helicopter-borne turbulence measurement system HELIPOD, a detailed data analysis and examination in regard of systematic errors of the instrument, and some comparison with local similarity theory and experiments of the past, in order to confirm the occurrence of small vertical turbulent fluxes. The examined nocturnal boundary layer offered excellent conditions to analyse the quality of the measurement system. In this connection, a detailed look at a strong ground-based inversion disclosed small turbulent fluxes with a spectral maximum at ten metres wavelength or less, embedded in intermittent turbulence. For verification of these fluxes, the measurements were compared with well established results from past experiments. Local similarity theory was applied to calculate dimensionless variances of the turbulent quantities, which were found in good agreement with other observations. Since shear and stratification varied significantly on the horizontal flight legs due to global intermittency, a method was developed to determine vertical gradients on a horizontal flight pattern, by use of small fluctuations of the measurement height. With these locally determined gradients, gradient transport theory became applicable and the turbulent diffusivities for heat and momentum, the Richardson number, and the flux Richardson number were estimated within isolated strong turbulent outbursts. Within these outbursts the flux Richardson number was found between 0.1 and 0.2. The functional relationship between the gradient Richardson number and the turbulent Prandtl number agreed well with observations in past experiments and large eddy simulation. The impact of the stratification on the vertical turbulent exchange, as already described for the surface layer using Monin–Obukhov similarity, was analogously observed in the very stably stratified bulk flow when local scaling was applied.  相似文献   

18.
Detailed measurements of profiles of mean and turbulent variablesthrough the nocturnal stable boundary layer over a valley arepresented. Two nights of data are analysed in detail, one with only aweakly stable boundary layer and one with a strongly stable boundarylayer. The weakly stratified night shows high levels of turbulence inwhich the flow remains attached to the valley and the boundary layeracts as a single coherent layer. On the strongly stratified night, twoflow regimes are identified: attached flow, as on the weaklystratified night, and decoupled flow in which the air in the valleybecomes so dynamically stable that there is no turbulent interactionwith the mean flow aloft. Because the valley is sloping, the decoupledlower stagnant air then forms a drainage current. We find that theFroude number evaluated at the hill height, FH = U(H)/N(H) H,diagnoses the flow regime: when FH = 2, the flow remainsattached and when FH 2 the flow in the valley becomesdecoupled from the flow aloft. The dynamics of the flow regimes areshown to be understandable in terms of the gradient Richardson number,which indicates the turbulent mixing. We show that the gradientRichardson number is a key parameter in diagnosing each flow regime.  相似文献   

19.
从湍流经典理论到大气湍流非平衡态热力学理论   总被引:2,自引:0,他引:2  
湍流是日常生活中一种普遍的自然现象,也是经典物理学仍未完全解决的难题。湍流更是大气运动的最基本特征。本文系统地回顾了大气湍流经典理论发展简史,进一步详细介绍了大气湍流非平衡态热力学理论。大气湍流非平衡态热力学理论在熵平衡方程中引入动力过程,进而统一推导出大气湍流输送的Fourier定律、Flick定律和Newton定律,证明了Dufour效应、Soret效应、可逆动力过程与热力不可逆湍流输送过程之间的交叉耦合效应,以及湍流强度定理。这些定律和定理中得到了观测的事实验证,同时它们的唯象系数也由观测资料所确定。湍流强度定理揭示,湍流发展的宏观原因是速度和温度的剪切效应,Reynolds湍流和Rayleigh-Bénard湍流共存于大气湍流中。热力过程和动力过程间耦合效应现象的发现突破了传统湍流输送理论,即Fourier定律、Flick定律和Newton定律的观点——一个宏观量的输送通量等价于这个宏观量的梯度湍流输送通量。热力和动力过程间的耦合原理认为,一个宏观量的输送通量包括这个量的梯度湍流输送通量和速度耦合输送通量两部分。因此,能量和物质的垂直输送通量除了相应物理量梯度造成的湍流输送外,还应包括垂直速度耦合效应,即辐散或辐合运动造成的耦合效应。在一个很宽的尺度范围内,地表面的空间特征是非均匀的。下垫面非均匀性造成的对流运动将引起大气的辐散或辐合运动。这可能是导致地表能量收支不平衡的重要原因之一。垂直速度对垂直湍流输送的交叉耦合效应为非均匀下垫面大气边界层理论的发展,并为克服地表能量收支不平衡问题及非均匀下垫面大气边界层参数化遇到的困难提供了可能的线索。  相似文献   

20.
Simultaneous surface-based remote sensing with optical (Ceilometer) and acoustic (Sodar) methods allows the diurnal variation of the structure of the atmospheric boundary layer to be deduced with high temporal resolution. Primarily the convective boundary layer, the nocturnal stable surface layer, and the residual layer can be identified from the measured vertical profiles of aerosol concentration and thermal fluctuations. The ability of the two remote sensing techniques is shown in different examples from two different locations and two seasons. The impact on urban air quality assessment is addressed.  相似文献   

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