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1.
The study has analyzed the variability and trends in monthly, seasonal and annual rainfall and rainy days of four locations over different agro-ecological zones of Bihar, namely Samastipur (zone-I), Madhepura (zone-II), Sabour (zone-IIIA) and Patna (zone-IIIB). The Mann–Kendall nonparametric test was employed for detection of statistical significance and slopes of the trend lines were determined using the method of least square linear fitting. The variability and trends of onset of effective monsoon and length of monsoon period were also analyzed using the same method. The mean annual rainfall varies from 1137 mm at Patna to 1219 mm at Sabour. July is the rainiest month in all the zones followed by August. Maximum increase in annual rainfall was found at Sabour (40.1% of mean/30 years at 95% confidence level) and minimum for Patna (10.1% of mean/30 years). Significant increasing trend of rainfall during July, August and September at rates of 41.9, 83.2, and 112.7% of the mean/30 years, respectively has been noticed at Madhepura. Analysis of rainy days indicates that rainy days increased during winter and annually for all the sites. The mean effective onset of monsoon varies from 18th June at Sabour to 28th June at Patna. The trends in the date of effective onset of monsoon indicate that the date tends to be early in all the sites except Madhepura. But a significant delayed trend in the onset at a rate of 2.8% of the mean/30 years has been observed for Madhepura. The early trend of the effective onset of monsoon and increasing trends of length of monsoon season have been observed for Samastipur, Sabour and Patna.  相似文献   

2.
We propose a semi-empirical model for the relation between global mean surface temperature and global sea-levels. In contradistinction to earlier approaches to this problem, the model allows for valid statistical inference and joint estimation of trend components and interaction term of temperature and sea-level. Estimation of the model on the data set used in Rahmstorf (2007) yields a proportionality coefficient of 4.6 mm/year per °C at a one-sided significance level of 7.6 percent or higher. Long-term simulations of the model result in a two-sided 90-percent confidence interval for the sea-level rise in the year 2100 of [15 cm, 150 cm] above the 1990 level. This is a wider margin of error than was reported in the previous literature, and it reflects the substantial uncertainty in relating two trending time series.  相似文献   

3.
A mooring equipped with 200 high-resolution temperature sensors between 6 and 404 m above the bottom was moored in 1890 m water depth above a steep, about 10° slope of Mount Josephine, NE-Atlantic. The sensors have a precision of less than 0.5 mK. They are synchronized via induction every 4 h so that the 400 m range is measured to within 0.02 s, every 1 s. Thin cables and elliptical buoyancy assured vertical mooring motions to be smaller than 0.1 m under maximum 0.2 m s−1 current speeds. The local bottom slope is supercritical for semidiurnal internal tides by a factor of two. Exploring a one-month record in detail, the observations show: 1/semidiurnal tidal dominance in variations of dissipation rate ε, eddy diffusivity Kz and temperature, but no significant correlation between the records of ε and total kinetic energy, 2/a variation with time over four orders of magnitude of 100-m vertically averaged ε, 3/a local minimum in density stratification between 50 and 100 m above the bottom, 4/a gradual decrease in daily or longer averaged ε and Kz by one order of magnitude over a vertical distance of 250 m, upwards from 150 m above the bottom, 5/monthly mean values of <[ε]> = 2 ± 0.5 × 10−7 m2 s−3, <[Kz]> = 8 ± 3 × 10−3 m2 s−1 averaged over the lower 150 m above the bottom.  相似文献   

4.
How individuals perceive climate change is linked to whether individuals support climate policies and whether they alter their own climate-related behaviors, yet climate perceptions may be influenced by many factors beyond local shifts in weather. Infrastructure designed to control or regulate natural resources may serve as an important lens through which people experience climate, and thus may influence perceptions. Likewise, perceptions may be influenced by personal beliefs about climate change and whether it is human-induced. Here we examine farmer perceptions of historical climate change, how perceptions are related to observed trends in regional climate, how perceptions are related to the presence of irrigation infrastructure, and how perceptions are related to beliefs and concerns about climate change. We focus on the regions of Marlborough and Hawke’s Bay in New Zealand, where irrigation is utilized on the majority of cropland. Data are obtained through analysis of historical climate records from local weather stations, interviews (n = 20), and a farmer survey (n = 490). Across both regions, no significant historical trends in annual precipitation and summer temperatures since 1980 are observed, but winter warming trends are significant at around 0.2–0.3 °C per decade. A large fraction of farmers perceived increases in annual rainfall despite instrumental records indicating no significant trends, a finding that may be related to greater perceived water availability associated with irrigation growth. A greater fraction of farmers perceived rainfall increases in Marlborough, where irrigation growth has been most substantial. We find those classes of farmers more likely to have irrigation were also significantly more likely to perceive an increase in annual rainfall. Furthermore, we demonstrate that perceptions of changing climate – regardless of their accuracy – are correlated with increased belief in climate change and an increased concern for future climate impacts. Those farmers that believe climate change is occurring and is human induced are more likely to perceive temperature increases than farmers who believe climate change is not occurring and is not human induced. These results suggest that perceptions are influenced by a variety of personal and environmental factors, including infrastructure, which may in turn alter decisions about climate adaptation.  相似文献   

5.
It has long been accepted that the relative affluence and technological efficiency of nations are important contributors to their rate of emissions. These associations have, in turn, driven questions about the feasibility of mitigating anthropogenic greenhouse gas emissions through incremental transition to “business as usual” policy structures in variant social contexts. Here, I explore the extent to which the historical context of colonial relations impacts the feasibility of a nation mitigating emissions per capita, emissions per dollar, and total emissions under current development logics. To do so I examine the structure of variation for 152 nations during the 1960–2018 period. Subsequently, I examine how being situated as an extractive colony in the past serves to moderate the association of GDP per capita with CO 2 emissions per capita, CO 2 emissions per dollar, and total CO 2 emissions in the present. I find that roughly 11% of cross-national variation in CO 2 emissions per capita and CO 2 emissions per dollar, as well as nearly 6% of variation in total CO 2 emissions between 1960 and 2018 is attributable to having been historically subjected to extractive colonial processes. These findings suggest that mitigation of emissions through transition of “business as usual” policy structures appears significantly less feasible for nations positioned as extractive colonies in the past, relative to all others.  相似文献   

6.
This paper evaluates the impacts of climate change to European economies under an increase in global mean temperature at +2 °C and +4 °C. It is based on a summary of conclusions from available studies of how climate change may affect various sectors of the economies in different countries. We apply a macroeconomic general equilibrium model, which integrates impacts of climate change on different activities of the economies. Agents adapt by responding to the changes in market conditions following the climatic changes, thus bringing consistency between economic behaviour and adaptation to climate change. Europe is divided into 85 sub-regions in order to capture climate variability and variations in vulnerabilities within countries. We find that the impacts in the +2 °C are moderate throughout Europe, with positive impacts on GDP in some sub-regions and negative impacts down to 0.1 per cent per year in others. At +4 °C, GDP is negatively affected throughout Europe, and most substantially in the southern parts, where it falls by up to 0.7 per cent per year in some sub-regions. We also find that climate change causes differentiations in wages across Europe, which may cause migration from southern parts of Europe to northern parts, especially to the Nordic countries.  相似文献   

7.
Rainfall characteristics of the Madden–Julian oscillation (MJO) are analyzed primarily using tropical rainfall measuring mission (TRMM) precipitation radar (PR), TRMM microwave imager (TMI) and lighting imaging sensor (LIS) data. Latent heating structure is also examined using latent heating data estimated with the spectral latent heating (SLH) algorithm.The zonal structure, time evolution, and characteristic stages of the MJO precipitation system are described. Stratiform rain fraction increases with the cloud activity, and the amplitude of stratiform rain variation associated with the MJO is larger than that of convective rain by a factor of 1.7. Maximum peaks of both convective rain and stratiform rain precede the minimum peak of the outgoing longwave radiation (OLR) anomaly which is often used as a proxy for the MJO convection. Stratiform rain remains longer than convective rain until ∼4000 km behind the peak of the mature phase. The stratiform rain contribution results in the top-heavy heating profile of the MJO.Associated with the MJO, there are tri-pole convective rain top heights (RTH) at 10–11, ∼7 and ∼3 km, corresponding to the dominance of afternoon showers, organized systems, and shallow convections, respectively. The stratiform rain is basically organized with convective rain, having similar but slightly lower RTH and slightly lags the convective rain maximum. It is notable that relatively moderate (∼7 km) RTH is dominant in the mature phase of the MJO, while very tall rainfall with RTH over 10 km and lightning frequency increase in the suppressed phase. The rain-yield-per flash (RPF) varies about 20–100% of the mean value of ∼2–10 × 109 kg fl−1 over the tropical warm ocean and that of ∼2–5 × 109 kg fl−1 over the equatorial Islands, between the convectively suppressed phase and the active phase of MJO, in the manner that RPF is smaller in the suppressed phase and larger in the active phase.  相似文献   

8.
The Water vapour Strong Lines at 183 GHz (183-WSL) fast retrieval method retrieves rain rates and classifies precipitation types for applications in nowcasting and weather monitoring. The retrieval scheme consists of two fast algorithms, over land and over ocean, that use the water vapour absorption lines at 183.31 GHz corresponding to the channels 3 (183.31 ± 1 GHz), 4 (183.31 ± 3 GHz) and 5 (183.31 ± 7 GHz) of the Advanced Microwave Sounding Unit module B (AMSU-B) and of the Microwave Humidity Sounder (MHS) flying on NOAA-15-18 and Metop-A satellite series, respectively.The method retrieves rain rates by exploiting the extinction of radiation due to rain drops following four subsequent steps. After ingesting the satellite data stream, the window channels at 89 and 150 GHz are used to compute scattering-based thresholds and the 183-WSLW module for rainfall area discrimination and precipitation type classification as stratiform or convective on the basis of the thresholds calculated for land/mixed and sea surfaces. The thresholds are based on the brightness temperature difference Δwin = TB89 ? TB150 and are different over land (L) and over sea (S): cloud droplets and water vapour (Δwin < 3 K L; Δwin < 0 K S), stratiform rain (3 K < Δwin < 10 K L; 0 K < Δwin < 10 K S), and convective rain (Δwin > 10 K L and S). The thresholds, initially empirically derived from observations, are corroborated by the simulations of the RTTOV radiative transfer model applied to 20000 ECMWF atmospheric profiles at midlatitudes and the use of data from the Nimrod radar network. A snow cover mask and a digital elevation model are used to eliminate false rain area attribution, especially over elevated terrain. A probability of detection logistic function is also applied in the transition region from no-rain to rain adjacent to the clouds to ensure continuity of the rainfall field. Finally, the last step is dedicated to the rain rate retrieval with the modules 183-WSLS (stratiform) and 183WSLC (convective), and the module 183-WSL for total rainfall intensity derivation.A comparison with rainfall retrievals from the Goddard Profiling (GPROF) TRMM 2A12 algorithm is done with good results on a stratiform and hurricane case studies. A comparison is also conducted with the MSG-based Precipitation Index (PI) and the Scattering Index (SI) for a convective-stratiform event showing good agreement with the 183-WSLC retrieval. A complete validation of the product is the subject of Part II of the paper.  相似文献   

9.
The chemical mass balance model was applied to atmospheric Polycyclic Aromatic Hydrocarbons (PAHs) in Istanbul, Turkey. A total of 326 airborne samples were collected and analyzed for 16 PAHs and Total Suspended Particles (TSP) in the September 2006–December 2007 period at three monitoring stations: Yildiz, DMO (urban sites) and Kilyos (rural site). The total average PAH concentrations were 100.66 ± 61.26, 84.63 ± 46.66 and 25.12 ± 13.34 ng m?3 and the TSP concentrations were 101.16 ± 53.22, 152.31 ± 99.12, 49.84 ± 18.58 μg m?3 for Yildiz, DMO and Kilyos stations respectively. At all the sites, the lighter compounds were the most abundant, notably Nap, AcPy and PA. The average correlation values between TSP and total heavier PAH were greater than 0.5 for Yildiz and DMO stations. The patterns of PAH and TSP concentrations showed spatial and temporal variations. PAH concentrations were evaluated for the PAH contribution from four sources (diesel engines, gasoline engines, natural gas combustion, and coal + wood burning). Vehicle emissions appear to be the major source with contributions of 61.2%, 63.3% and 54.1% for Yildiz, DMO and Kilyos stations respectively. Seasonal and yearly variations had different trends for all sites.  相似文献   

10.
The observed long-term trends in extreme temperatures in Hong Kong were studied based on the meteorological data recorded at the Hong Kong Observatory Headquarters from 1885-2008. Results show that, over the past 124 years, the extreme daily minimum and maximum temperatures, as well as the length of the warm spell in Hong Kong, exhibit statistically significant long-term rising trends, while the length of the cold spell shows a statistically significant decreasing trend. The time-dependent return period analysis also indicated that the return period for daily minimum temperature at 4°C or lower lengthened considerably from 6 years in 1900 to over 150 years in 2000, while the return periods for daily maximum temperature reaching 35°C or above shortened drastically from 32 years in 1900 to 4.5 years in 2000. Past trends in extreme temperatures from selected weather stations in southern China from 1951-2004 were also assessed. Over 70% of the stations studied yielded a statistically significant rising trend in extreme daily minimum temperature, while the trend for extreme maximum temperatures was found to vary, with no significant trend established for the majority of stations.  相似文献   

11.
The upper layer, wind-driven circulation of the South China Sea (SCS), its through-flow (SCSTF) and the Indonesian through flow (ITF) are simulated using a high resolution model, FVCOM (finite volume coastal ocean model) in a regional domain comprising the Maritime Continent. The regional model is embedded in the MIT global ocean general circulation model (ogcm) which provides surface forcing and boundary conditions of all the oceanographic variables at the lateral open boundaries in the Pacific and Indian oceans. A five decade long simulation is available from the MITgcm and we choose to investigate and compare the climatologies of two decades, 1960–1969 and 1990–1999.The seasonal variability of the wind-driven circulation produced by the monsoon system is realistically simulated. In the SCS the dominant driving force is the monsoon wind and the surface circulation reverses accordingly, with a net cyclonic tendency in winter and anticyclonic in summer. The SCS circulation in the 90s is weaker than in the 60s because of the weaker monsoon system in the 90s. In the upper 50 m the interaction between the SCSTF and ITF is very important. The southward ITF can be blocked by the SCSTF at the Makassar Strait during winter. In summer, part of the ITF feeds the SCSTF flowing into the SCS through the Karimata Strait. Differently from the SCS, the ITF is primarily controlled by the sea level difference between the western Pacific and eastern Indian Ocean. The ITF flow, consistently southwestward below the surface layer, is stronger in the 90s.The volume transports for winter, summer and yearly are estimated from the simulation through all the interocean straits. On the annual average, there is a ∼5.6 Sv of western Pacific water entering the SCS through the Luzon Strait and ∼1.4 Sv exiting through the Karimata Strait into the Java Sea. Also, ∼2 Sv of SCS water enters the Sulu Sea through the Mindoro Strait, while ∼2.9 Sv flow southwards through the Sibutu Strait merging into the ITF. The ITF inflow occurs through the Makassar Strait (up to ∼62%) and the Lifamatola Strait (∼38%). The annual average volume transport of the ITF inflow from the simulation is ∼15 Sv in the 60s and ∼16.6 Sv in the 90s, very close to the long term observations. The ITF outflow through the Lombok, Ombai and Timor straits is ∼16.8 Sv in the 60s and 18.9 Sv in the 90s, with the outflow greater by 1.7 Sv and 2.3 Sv respectively. The transport estimates of the simulation at all the straits are in rather good agreement with the observational estimates.We analyze the thermal structure of the domain in the 60s and 90s and assess the simulated temperature patterns against the SODA reanalysis product, with special focus on the shallow region of the SCS. The SODA dataset clearly shows that the yearly averaged temperatures of the 90s are overall warmer than those of the 60s in the surface, intermediate and some of the deep layers and the decadal differences (90s  60s) indicate that the overall warming of the SCS interior is a local effect. In the simulation the warm trend from the 60s to the 90s in well reproduced in the surface layer. In particular, the simulated temperature profiles at two shallow sites at midway in the SCSTF agree rather well with the SODA profiles. However, the warming trend in the intermediate (deep) layers is not reproduced in the simulation. We find that this deficiency is mostly due to a deficiency in the initial temperature fields provide by the MITgcm.  相似文献   

12.
Conventional surface data and quantitative estimations of precipitation are used to document the occurrence and spatial distribution of severe weather phenomena associated with deep moist convection over southeastern South America.Data used in this paper are 24-hour rainfall, maximum hourly gusts and present weather reports from the surface station network for Argentina to the north of 40°S and cover the period 2000–2005. Hourly rainfall estimated with the CMORPH technique (CPC MORPHing technique, R. J. Joyce et al., 2004) is included in the analysis in order to increase the density of the precipitation database from January 2003 to December 2005. Extreme events are detected by means of a 95th-percentile analysis of the 24-hour rainfall and wind; values greater than 30 mm and 25 m s?1 respectively are considered extreme in the study area. These results are related to the presence of deep convection by considering the 235 K and 218 K cloud shield evolution in Geostationary Operational Environmental Satellite-12 Infrared (GOES-IR) imagery evaluated by the Forecasting and Tracking of Cloud Cluster (FORTRACC) technique. Rainfall above 30 mm day?1 and present convection-related weather events tend to occur in the northeast of the country.Finally, an analysis is made of the relationship between severe phenomena and the location and lifecycle of Mesoscale Convective Systems (MCSs) defined by the 218 K or 235 K levels. According to the reports, favorable locations for severe weather concentrate to the northeast of the cloud shield anvil centroid although most of the cases are found in the northwest. This feature can be seen in systems with anvil areas larger than 250,000 km2 in association to the predominant mid-level wind shear direction from the northwest over the area. Moreover, systems with centers located north of 30°S present a more circular shape while those to the south are more elongated with a NW–SE main axis clearly related to the presence and interaction with frontal zones over the area. Most of the events occur previous to the moment when the systems reach their maximum extension, between 2 and 10 h after the initiation of the system depending on the size of the MCSs.  相似文献   

13.
The short-term rainfall climatology regime over Saudi Arabia is obtained from the Tropical Rainfall Measuring Mission (TRMM) data for the period 1998–2009. The TRMM rainfall amounts are calibrated with respect to the rain-gauge data recorded at 29 stations across the country. Day-to-day rainfall comparisons show that the TRMM rainfall trends are very similar to the observed data trends, even if a general overestimation in the satellite products must be highlighted. Besides, especially during the wet season, some of the TRMM algorithm runs tend to underestimate the retrieved rainfalls. The TRMM rainfall data also closely follow the observed annual cycle on a monthly scale. The correlation coefficient for rainfall between the TRMM and the rain-gauge data is about 0.90, with a 99% level of significance on the monthly scale.The spatio-temporal distributions of rainfall over Saudi Arabia are analyzed. Besides the four conventional seasons, this analysis consider the wet (November–April) and dry (June–September) seasons, based on the rainfall amounts recorded. Spring is the highest and winter is the second highest rainfall-occurring season, resulting in large amounts of rainfall during the wet season over most of the country. Regional variations in the rainfall climatology over Saudi Arabia are studied through defining four regions. The false alarm ratio, probability of detection, threat score, and skill score are calculated to evaluate the TRMM performance. The country's average annual rainfall measured by the TRMM is 89.42 mm, whereas the observed data is 82.29 mm. Thus, the rainfall in Saudi Arabia is suggested as being the TRMM value multiplied by 0.93 plus 0.04. After this calibration, the TRMM-measured rainfall is almost 100% of the observed data, thereby confirming that TRMM data may be used in a variety of water-related applications in Saudi Arabia.  相似文献   

14.
Climate output from the UK Hadley Centre's HadCM2 and HadCM3 experiments for the period 1860 to 2100, with IS92a greenhouse gas forcing, together with predicted patterns of N deposition and increasing CO2, were input (offline) to the dynamic vegetation model, Hybrid v4.1 (Friend et al., 1997; Friend and White, 1999). This model represents biogeochemical, biophysical and biogeographical processes, coupling the carbon, nitrogen and water cycles on a sub-daily timestep, simulating potential vegetation and transient changes in annual growth and competition between eight generalized plant types in response to climate.Global vegetation carbon was predicted to rise from about 600 to 800 PgC (or to 650 PgC for HadCM3) while the soil carbon pool of about 1100 PgC decreased by about 8%. By the 2080s, climate change caused a partial loss of Amazonian rainforest, C4 grasslands and temperate forest in areas of southern Europe and eastern USA, but an expansion in the boreal forest area. These changes were accompanied by a decrease in net primary productivity (NPP) of vegetation in many tropical areas, southern Europe and eastern USA (in response to warming and a decrease in rainfall), but an increase in NPP of boreal forests. Global NPP increased from 45 to 50 PgC y−1 in the 1990s to about 65 PgC y−1 in the 2080s (about 58 PgC y−1 for HadCM3). Global net ecosystem productivity (NEP) increased from about 1.3 PgC y−1 in the 1990s to about 3.6 PgC y−1 in the 2030s and then declined to zero by 2100 owing to a loss of carbon from declining forests in the tropics and at warm temperate latitudes — despite strengthening of the carbon sink at northern high latitudes. HadCM3 gave a more erratic temporal evolution of NEP than HadCM2, with a dramatic collapse in NEP in the 2050s.  相似文献   

15.
Mixing states of cloud interstitial particles between water-soluble and insoluble materials apparently differ under various cloud-forming conditions. To study the mixing states of cloud interstitial particles, we made observations at Mt. Tateyama, Japan (2300 m a.s.l.) during June 2007 using fog (> 10 μm)-cut inlets. Number concentrations of dried particles (0.3–0.5 μm diameter) selected for less-grown (LG) particles (particles smaller than 0.56 μm diameter at 88% relative humidity) were used to quantify tendencies of the growth characteristics of cloud interstitial particles. Size-segregated soot mass concentrations (< 0.4 and < 1.1 μm) were also measured for cloud interstitial particles. Three samples of cloud interstitial LG particles at 88% RH were investigated for water-soluble and insoluble components using dialysis (extraction) of water-soluble materials with transmission electron microscopy (TEM). For one TEM sample with high fractions of the LG particles and high soot mass concentrations under high precipitation (2–6 mm/h), most particles (0.1–0.5 μm) were found to be water insoluble. More than half of the water-insoluble particles were considered to be soot particles showing chain aggregations of electron-opaque spherules. Regarding the other two TEM samples with low fractions of the LG particles under less intense precipitation (ca. 1 mm/h), most particles were partly water soluble. The scavenging process in the precipitating cloud can change the population of particles left behind, preferentially leaving insoluble particles according to cloud formation conditions.  相似文献   

16.
《Atmospheric Research》2009,91(2-4):195-202
We present results of direct aerosol radiative forcing over a French Mediterranean coastal zone based on one year of continuous observations of aerosol optical properties during 2005–2006. Monthly-mean aerosol optical depth at 440 nm ranged between 0.1 and 0.34, with high Angstrom coefficient (α > 1.2). The single scattering albedo (at 525 nm) estimated at the surface ranged between 0.7 and 0.8, indicating significant absorption. The presence of aerosols over the Mediterranean zone during summer decreases the shortwave radiation reaching the surface by as much as 26 ± 3.9 W m 2, and increases the top of the atmosphere reflected radiation by as much as 5.2 ± 1.0 W m 2. The shortwave atmospheric absorption translates to an atmospheric heating of 2.5 to 4.6 K day 1. Concerted efforts are needed for investigating the possible impact of the increase in heating rate on the maintenance of heat-waves frequently occurring over this coastal region during summer time.  相似文献   

17.
The character of turbulent overturns in a weakly stratified deep-sea is investigated in some detail using 144 high-resolution temperature sensors at 0.7 m intervals, starting 5 m above the bottom. A 9-day, 1 Hz sampled record from the 912 m depth flat-bottom (<0.5% bottom-slope) mooring site in the central-north Alboran Sea (W-Mediterranean) demonstrates an overall conservative temperature range of only 0.05 °C, a typical mean buoyancy period as large as 3 h and a 1 Hz-profile-vertically-averaged turbulence dissipation rate maximum of only 10−8 m2 s−3. Nonetheless, this ‘boundary layer’ varies in height between <6 and >104 m above the bottom and is thus not homogeneous throughout; the temperature variations are seldom quiescent and are generally turbulent in appearance, well exceeding noise levels. The turbulence character is associated with small-scale internal waves; examples are found of both shear- and convection-driven turbulence; particular association, although not phase-locked, is found between turbulence variations and tidal rather than with inertial motions; the mean buoyancy frequency of a few times the inertial frequency implies the importance of ‘slantwise convection’ in the direction of the earth rotational vector rather than in the direction of gravity. Such convection is observed both in near-homogeneous and weakly stratified form.  相似文献   

18.
Identifying the sources of reactive nitrogen (N) and quantifying their contributions to groundwater nitrate concentrations are critical to understanding the dynamics of groundwater nitrate contamination. Here we assessed groundwater nitrate contamination in China using literature analysis and N balance calculation in coupled human and natural systems. The source appointment via N balance was well validated by field data via literature analysis. Nitrate was detected in 96% of groundwater samples based on a common detection threshold of 0.2 mg N L?1, and 28% of groundwater samples exceeded WHO's maximum contaminant level (10 mg N L?1). Groundwater nitrate concentrations were the highest beneath industrial land (median: 34.6 mg N L?1), followed by urban land (10.2 mg N L?1), cropland (4.8 mg N L?1), and rural human settlement (4.0 mg N L?1), with the lowest found beneath natural land (0.8 mg N L?1). During the period 1980–2008, total reactive N leakage to groundwater increased about 1.5 times, from 2.0 to 5.0 Tg N year?1, in China. Despite that the contribution of cropland to the total amount of reactive N leakage to groundwater was reduced from 50 to 40% during the past three decades, cropland still was the single largest source, while the contribution from landfill rapidly increased from 10 to 34%. High reactive N leakage mainly occurred in relatively developed agricultural or urbanized regions with a large population. The amount of reactive N leakage to groundwater was mainly driven by anthropogenic factors (population, gross domestic product, urbanization rate and land use type). We constructed a high resolution map of reactive N source appointment and this could be the basis for future modeling of groundwater nitrate dynamics and for policy development on mitigation of groundwater contamination.  相似文献   

19.
Concentrations and flux densities of methane were determined during a Lagrangian study of an advective filament in the permanent upwelling region off western Mauritania. Newly upwelled waters were dominated by the presence of North Atlantic Central Water and surface CH4 concentrations of 2.2 ± 0.3 nmol L−1 were largely in equilibrium with atmospheric values, with surface saturations of 101.7 ± 14%. As the upwelling filament aged and was advected offshore, CH4 enriched South Atlantic Central Water from intermediate depths of 100–350 m was entrained into the surface mixed layer of the filament following intense mixing associated with the shelf break. Surface saturations increased to 198.9 ± 15% and flux densities increased from a mean value over the shelf of 2.0 ± 1.1 μmol m−2 d−1 to a maximum of 22.6 μmol m−2 d−1. Annual CH4 emissions for this persistent filament were estimated at 0.77 ± 0.64 Gg which equates to a maximum of 0.35% of the global oceanic budget. This raises the known outgassing intensity of this area and highlights the importance of advecting filaments from upwelling waters as efficient vehicles for air-sea exchange.  相似文献   

20.
We analyzed a 20-year time series (January 1st, 1993 through December 31st, 2012) of Loop Current (LC) surface area derived from satellite altimetry in the eastern Gulf of Mexico to estimate kinematical metrics of this potent flow. On average the LC intrudes to its maximum northward position about 216 ± 126 days after the previous eddy separation; and ∼30 ± 31 days later sheds a large anticyclonic eddy. When the northern extent of the LC intrusion following the previous eddy separation is greater than 27°N, the current retreats very quickly until it sheds another eddy with the entire separation process occurring on the order of 30 days. To first order the change in areal extent of the LC during intrusion into the Gulf occurs at an average rate of 225 km2 day−1, which corresponds to an intrusion velocity of 1.7 cm s−1 of the LC front, and adds Caribbean water to the Gulf at a rate of 2.6 ± 0.7 Sv.  相似文献   

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