Turbulent Dispersion of Non-uniformly Emitted Passive Tracers in the Convective Boundary Layer

The impact of spatially non-uniform emissions on the turbulence dispersion of passive tracers in the convective boundary layer is studied by means of large-eddy simulation. We explicitly calculated the different terms of the budget equations for the concentrations, fluxes and variances, and used sub-domain averaging where each sub-domain is the typical size of a large-scale model grid cell. We found that the concentration profiles in the sub-domain where the emission takes place are lightly affected by the size of the emission release. This effect becomes more relevant in the downwind sub-domain. Although sub-domain averaged fluxes are not affected by the emission source size, concentration variances are dramatically increased when the emission shrinks. This increase originates from the mixing of highly concentrated air parcels with those of low concentrations. We also found that the concentration variance at the surface is driven neither by the position of the emission source nor the strength of the shear forcing but solely by the emission variance.     

Lagrangian Stochastic Models For Turbulent Dispersion In The Atmospheric Boundary Layer

A one-particle three-dimensional stochastic Lagrangian model fortransport of particles in a horizontally-homogeneous atmosphericsurface layer with arbitrary one-point probability density functionof Eulerian velocity fluctuations is suggested. A uniquely definedLagrangian stochastic model in the class of well-mixed models isconstructed from physically plausible assumptions. These assumptionsare: (i) in the neutrally stratified horizontally homogeneous surface layer, the vertical motion is mainly controlled by eddies whose size is of order of the current height; and (ii), the streamwise drift term is independent of the crosswind velocity. Numerical simulations for neutral stratification have shown a good agreement of our model with the well-known Thomson's model, with Flesch and Wilson's model, and with experimental measurements as well. However there is a discrepancy of these results with the results obtained by Reynolds' model.     

Wave-Modified Flux and Plume Dispersion in the Stable Boundary Layer

The effects of a pressure jump and a following internal gravity wave on turbulence and plume diffusion in the stable planetary boundary layer are examined. The pressure jump was accompanied by a sudden increase in turbulence and plume dispersion. The effects of wave perturbations on turbulence statistics are analysed by calculating fluxes and variances with and without the wave signal for averaging times ranging from 1 to 30 min. The wave signals are obtained using a band-pass filter. It is shown that second-order turbulence quantities calculated without first subtracting the wave perturbations from the time are greater than those calculated when the wave signal is separated from the turbulence. Estimates of the vertical dispersion of an elevated tracer plume in the stable boundary layer are made using an elastic backscatter lidar. Plume dispersion observed 25 m downwind of the source increases rapidly with the arrival of the flow disturbances. Measured plume dispersion and plume centreline height correlate with the standard deviation of the vertical velocity but not with the wave signal.     

Modelling Fractal Turbulent Velocity Spectra: Application to a Dispersion Model of Contaminants in Particular Cases of the Planetary Boundary Layer

Boundary-Layer Meteorology - The present work develops a model for the turbulent velocity spectra that considers the anomalous behaviour of the turbulent flow. The $$\beta $$ -model assumes that...     

Large-eddy Simulation of the Dispersion of Solid Particles in a Turbulent Boundary Layer

A large-eddy simulation (LES) with the dynamic Smagorinsky-Germano subgrid-scale (SGS) model is used to study the dispersion of solid particles in a turbulent boundary layer. Solid particles are tracked in a Lagrangian way. The instantaneous velocity of the surrounding fluid is considered to have a large-scale part (directly computed by the LES) and a small-scale part. The SGS velocity of the surrounding fluid is given by a three-dimensional Langevin model written in terms of SGS statistics at a mesh level. An appropriate Lagrangian correlation time scale is considered in order to include the influences of gravity and inertia of the solid particle. Inter-particle collisions and the influence of particles on the mean flow are also taken into account. The results of the LES are compared with the wind-tunnel experiments of Nalpanis et al. (1993 J Fluid Mech 251: 661–685) and of Tanière et al. (1997 Exp in Fluids 23:463–471) on sand particles in saltation and in modified saltation, respectively.     

Lagrangian Stochastic Modeling of Dispersion in the Stable Boundary Layer

Lagrangian stochastic models are well-suited for modeling dispersion in the stable boundary layer, especially in complex terrain. This note briefly describes the formulations and application of a Lagrangian stochastic model to predict dispersion of tracers released within nocturnal drainage flows.     

Pollutant Plume Dispersion in the Atmospheric Boundary Layer over Idealized Urban Roughness

The Gaussian model of plume dispersion is commonly used for pollutant concentration estimates. However, its major parameters, dispersion coefficients, barely account for terrain configuration and surface roughness. Large-scale roughness elements (e.g. buildings in urban areas) can substantially modify the ground features together with the pollutant transport in the atmospheric boundary layer over urban roughness (also known as the urban boundary layer, UBL). This study is thus conceived to investigate how urban roughness affects the flow structure and vertical dispersion coefficient in the UBL. Large-eddy simulation (LES) is carried out to examine the plume dispersion from a ground-level pollutant (area) source over idealized street canyons for cross flows in neutral stratification. A range of building-height-to-street-width (aspect) ratios, covering the regimes of skimming flow, wake interference, and isolated roughness, is employed to control the surface roughness. Apart from the widely used aerodynamic resistance or roughness function, the friction factor is another suitable parameter that measures the drag imposed by urban roughness quantitatively. Previous results from laboratory experiments and mathematical modelling also support the aforementioned approach for both two- and three-dimensional roughness elements. Comparing the UBL plume behaviour, the LES results show that the pollutant dispersion strongly depends on the friction factor. Empirical studies reveal that the vertical dispersion coefficient increases with increasing friction factor in the skimming flow regime (lower resistance) but is more uniform in the regimes of wake interference and isolated roughness (higher resistance). Hence, it is proposed that the friction factor and flow regimes could be adopted concurrently for pollutant concentration estimate in the UBL over urban street canyons of different roughness.     

Scaling of the Vertical Spreading of a Plume of a Passive Tracer in a Rough-Wall Neutral Boundary Layer

The influence of surface roughness on the dispersion of a passive scalar in a rough wall turbulent boundary layer has been studied using wind-tunnel experiments. The surface roughness was varied using different sizes of roughness elements, and different spacings between the elements. Vertical profiles of average concentration were measured at different distances downwind of the source, and the vertical spread of the plume was computed by fitting a double Gaussian profile to the data. An estimate of the integral length scale is derived from the turbulence characteristics of the boundary layer and is then used to scale the measured values of plume spread. This scaling reduces the variability in the data, confirming the validity of the model for the Lagrangian integral time scale, but does not remove it entirely. The scaled plume spreading shows significant differences from predictions of theoretical models both in the near and in the far field. In the region immediately downwind of the source this is due to the influence of the wake of the injector for which we have developed a simple model. In the far field we explain that the differences are mainly due to the absence of large-scale motions. Finally, further downwind of the source the scaled values of plume spread fall into two distinct groups. It is suggested that the difference between the two groups may be related to the lack of dynamical similarity between the boundary-layer flows for varying surface roughness or to biased estimates of the plume spread.     

Marine Boundary Layer And Turbulent Fluxes Over The Baltic Sea: Measurements And Modelling

Two weeks of measurements of the boundary-layer height over a small island (Christiansø) in the Baltic Sea are discussed. The meteorological conditions are characterised by positive heat flux over the sea. The boundary-layer height was simulated with two models, a simple applied high-resolution (2 km × 2 km) model, and the operational numerical weather prediction model HIRLAM (grid resolution of 22.5 km × 22.5 km). For southwesterly winds it was foundthat a relatively large island (Bornholm) lying 20-km upwind of the measuring site influences the boundary-layer height. In this situation the high-resolution simple applied model reproduces the characteristics of the boundary-layer height over the measuring site. Richardson-number based methods using data from simulations with the HIRLAM model fail, most likely because the island and the water fetch to the measuring site are about the size of the grid resolution of the HIRLAM model and therefore poorly resolved. For northerly winds, the water fetch to the measuring site is about 100 km. Both models reproduce the characteristics of the height of the marine boundary layer. This suggests that the HIRLAM model adequately resolves a water fetch of 100 km with respect to predictions of the height of the marine boundary layer.     

Flux Footprints in the Convective Boundary Layer: Large-Eddy Simulation and Lagrangian Stochastic Modelling

We investigated the flux footprints of receptors at different heights in the convective boundary layer (CBL). The footprints were derived using a forward Lagrangian stochastic (LS) method coupled with the turbulent fields from a large-eddy simulation model. Crosswind-integrated flux footprints shown as a function of upstream distances and sensor heights in the CBL were derived and compared using two LS particle simulation methods: an instantaneous area release and a crosswind linear continuous release. We found that for almost all sensor heights in the CBL, a major positive flux footprint zone was located close to the sensor upstream, while a weak negative footprint zone was located further upstream, with the transition band in non-dimensional upwind distances −X between approximately 1.5 and 2.0. Two-dimensional (2D) flux footprints for a point sensor were also simulated. For a sensor height of 0.158 z _i, where z _i is the CBL depth, we found that a major positive flux footprint zone followed a weak negative zone in the upstream direction. Two even weaker positive zones were also present on either side of the footprint axis, where the latter was rotated slightly from the geostrophic wind direction. Using CBL scaling, the 2D footprint result was normalized to show the source areas and was applied to real parameters obtained using aircraft-based measurements. With a mean wind speed in the CBL of U = 5.1 m s⁻¹, convective velocity of w _* = 1.37 m s⁻¹, CBL depth of z _i = 1,000 m, and flight track height of 159 m above the surface, the total flux footprint contribution zone was estimated to range from about 0.1 to 4.5 km upstream, in the case where the wind was perpendicular to the flight track. When the wind was parallel to the flight track, the total footprint contribution zone covered approximately 0.5 km on one side and 0.8 km on the other side of the flight track.     

Wind-Tunnel Experiments for Gas Dispersion in an Atmospheric Boundary Layer with Large-Scale Turbulent Motion

Large-scale turbulent motions enhancing horizontal gas spread in an atmospheric boundary layer are simulated in a wind-tunnel experiment. The large-scale turbulent motions can be generated using an active grid installed at the front of the test section in the wind tunnel, when appropriate parameters for the angular deflection and the rotation speed are chosen. The power spectra of vertical velocity fluctuations are unchanged with and without the active grid because they are strongly affected by the surface. The power spectra of both streamwise and lateral velocity fluctuations with the active grid increase in the low frequency region, and are closer to the empirical relations inferred from field observations. The large-scale turbulent motions do not affect the Reynolds shear stress, but change the balance of the processes involved. The relative contributions of ejections to sweeps are suppressed by large-scale turbulent motions, indicating that the motions behave as sweep events. The lateral gas spread is enhanced by the lateral large-scale turbulent motions generated by the active grid. The large-scale motions, however, do not affect the vertical velocity fluctuations near the surface, resulting in their having a minimal effect on the vertical gas spread. The peak concentration normalized using the root-mean-squared value of concentration fluctuation is remarkably constant over most regions of the plume irrespective of the operation of the active grid.     

Statistics of Scalar Fields in the Atmospheric Boundary Layer Based on Large-eddy Simulations. Part 1: Free Convection

Convection in a quasi-steady, cloud-free, shear-free atmospheric boundary layer is investigated based on a large-eddy simulation model. The performed tests indicate that the characteristic (peak) values of statistical moments at the top of the mixed layer are proportional to the interfacial scales (from gradients of scalars in the interfacial layer). Based on this finding a parameterization is proposed for profiles of scalar variances. The parameterization employs two, semi-empirical similarity functions F_m(z/z_i) andF_i(z/z_i), multiplied by a combination of the mixed-layer scales and the interfacial scales.     

Statistics of Scalar Fields in the Atmospheric Boundary Layer Based on Large-Eddy Simulations. Part II: Forced Convection

Forced convection in a quasi-steady atmospheric boundary layer is investigated based on a large-eddy simulation (LES) model. The performed simulations show that in the upper portion of the mixed layer the dimensionless (in terms of mixed layer scales) vertical gradients of temperature, humidity, and wind velocity depend on the dimensionless height z/z _i and the Reech number Rn. The peak values of variances and covariances at the top of the mixed layer, scaled in terms of the interfacial scales, are functions of the interfacial Richardson number Ri. As a result expressions for the entrainment rates, in the case when the interfacial layer has a finite depth, and a condition for the presence of moistening or drying regimes in the mixed layer, are derived. Profiles of dimensionless scalar moments in the mixed layer are proposed to be expressed in terms of two empirical similarity functions F _m and F _i , dependent on dimensionless height z/z _i , and the interfacial Richardson number Ri. The obtained similarity expressions adequately approximate the LES profiles of scalar statistics, and properly represent the impact of stability, shear, and entrainment. They are also consistent with the parameterization proposed for free convection in the first part of this paper.     

A Lagrangian Stochastic Model for Heavy Particle Dispersion in the Atmospheric Marine Boundary Layer

The dispersion of heavy particles and pollutants is often simulated with Lagrangian stochastic (LS) models. Although these models have been employed successfully over land, the free surface at the air-sea interface complicates the implementation of traditional LS models. We present an adaptation of traditional LS models to the atmospheric marine boundary layer (MBL), where the bottom boundary is represented by a realistic wavy surface that moves and deforms. In addition, the correlation function for the turbulent flow following a particle is extended to the anisotropic, unsteady case. Our new model reproduces behaviour for Lagrangian turbulence in a stratified air flow that departs only slightly from the expected behaviour in isotropic turbulence. When solving for the trajectory of a heavy particle in the air flow, the modelled turbulent forcing on the particle also behaves remarkably well. For example, the spectrum of the turbulence at the particle location follows that of a massless particle for time scales approximately larger than the Stokes’ particle response time. We anticipate that this model will prove especially useful in the context of sea-spray dispersion and its associated momentum, sensible and latent heat, and gas fluxes between spray droplets and the atmosphere.     

Wind-tunnel Modelling of Dispersion from a Scalar Area Source in Urban-Like Roughness

A wind-tunnel study was conducted to investigate ventilation of scalars from urban-like geometries at neighbourhood scale by exploring two different geometries a uniform height roughness and a non-uniform height roughness, both with an equal plan and frontal density of λ _p = λ _f = 25%. In both configurations a sub-unit of the idealized urban surface was coated with a thin layer of naphthalene to represent area sources. The naphthalene sublimation method was used to measure directly total area-averaged transport of scalars out of the complex geometries. At the same time, naphthalene vapour concentrations controlled by the turbulent fluxes were detected using a fast Flame Ionisation Detection (FID) technique. This paper describes the novel use of a naphthalene coated surface as an area source in dispersion studies. Particular emphasis was also given to testing whether the concentration measurements were independent of Reynolds number. For low wind speeds, transfer from the naphthalene surface is determined by a combination of forced and natural convection. Compared with a propane point source release, a 25% higher free stream velocity was needed for the naphthalene area source to yield Reynolds-number-independent concentration fields. Ventilation transfer coefficients w _T /U derived from the naphthalene sublimation method showed that, whilst there was enhanced vertical momentum exchange due to obstacle height variability, advection was reduced and dispersion from the source area was not enhanced. Thus, the height variability of a canopy is an important parameter when generalising urban dispersion. Fine resolution concentration measurements in the canopy showed the effect of height variability on dispersion at street scale. Rapid vertical transport in the wake of individual high-rise obstacles was found to generate elevated point-like sources. A Gaussian plume model was used to analyse differences in the downstream plumes. Intensified lateral and vertical plume spread and plume dilution with height was found for the non-uniform height roughness.     

Numerical Study of Dual-Plume Interference in a Turbulent Boundary Layer

Direct numerical simulation is used to investigate the interference arising from the dispersion of passive scalar plumes released from a pair of point sources in a fully-developed wall-bounded shear flow. Four different lateral separations of the two sources for both near ground-level and elevated releases are considered. The downwind evolution of the correlation between the plume concentrations along the centreline between the two sources and the behaviour of the lateral profiles of the correlation at various locations downwind of the two sources are examined in detail. Differences in the exceedance probability over a high concentration level for a single plume and the total plume are highlighted and studied, and the effects of destructive and constructive interferences on the exceedance probabilities for the total plume are used to explain these differences. One significant result is that all higher-order (third-order and above) moments of the total concentration can be inferred from the application of a clipped-gamma distribution using the information embodied in only the first- and second-order concentration moments of each single plume, and in the cross-correlation coefficient of the instantaneous concentration of the two plumes.     

Dispersion of a Passive Scalar Within and Above an Urban Street Network

The transport of a passive scalar from a continuous point-source release in an urban street network is studied using direct numerical simulation (DNS). Dispersion through the network is characterized by evaluating horizontal fluxes of scalar within and above the urban canopy and vertical exchange fluxes through the canopy top. The relative magnitude and balance of these fluxes are used to distinguish three different regions relative to the source location: a near-field region, a transition region and a far-field region. The partitioning of each of these fluxes into mean and turbulent parts is computed. It is shown that within the canopy the horizontal turbulent flux in the street network is small, whereas above the canopy it comprises a significant fraction of the total flux. Vertical fluxes through the canopy top are predominantly turbulent. The mean and turbulent fluxes are respectively parametrized in terms of an advection velocity and a detrainment velocity and the parametrization incorporated into a simple box-network model. The model treats the coupled dispersion problem within and above the street network in a unified way and predictions of mean concentrations compare well with the DNS data. This demonstrates the usefulness of the box-network approach for process studies and interpretation of results from more detailed numerical simulations.