Analysis of Radionuclide Releases from the Fukushima Dai-Ichi Nuclear Power Plant Accident Part I

Part I of this publication deals with the analysis of fission product releases consecutive to the Fukushima Dai-ichi accident. Reactor core damages are assessed relying on radionuclide detections performed by the CTBTO radionuclide network, especially at the particulate station located at Takasaki, 210 km away from the nuclear power plant. On the basis of a comparison between the reactor core inventory at the time of reactor shutdowns and the fission product activities measured in air at Takasaki, especially ⁹⁵Nb and ¹⁰³Ru, it was possible to show that the reactor cores were exposed to high temperature for a prolonged time. This diagnosis was confirmed by the presence of ¹¹³Sn in air at Takasaki. The ¹³³Xe assessed release at the time of reactor shutdown (8 × 10¹⁸ Bq) turned out to be in the order of 80 % of the amount deduced from the reactor core inventories. This strongly suggests a broad meltdown of reactor cores.     

Cancer risk estimation from dietary arsenic,a new approach from longitudinal cohort study

Inorganic arsenic is a carcinogen and consumption in low dose may lead to cancer. We estimated the cancer risk of the participants from arsenic endemic regions of West Bengal, India. The probable cancer risk was estimated following the assessment of daily inorganic arsenic intake through drinking water and diets of 20 participants for three consecutive years who had been using low arsenic water in the Indian context (median arsenic concentration in the study Years-I, II and III were 22, 16, 13 µg/l respectively). Probable cancer risk of the population was 2.80 × 10^?4, 2.94 × 10^?4, 3.12 × 10^?4 in the three respective study years (Year-I, II and III); just higher than the US EPA risk level of concern. The arsenic species content of the paired raw, cooked rice and urine was estimated in the as is taken basis. The major diet component, rice contained 72–86% inorganic arsenic whereas urine contains 70% organic arsenic on an average. The cancer risk assessment has been proposed to be modified by inclusion of urine arsenic release, considering the fact of arsenic release through urine. The risk became 1.28 × 10^?5, 1.13 × 10^?5, 1.01 × 10^?5 in the study Year-I, II and III respectively, considering urinary arsenic release, attributed the consideration of urine arsenic release into probable cancer risk estimation.     

Estimation of Explosion Energy Yield at Chernobyl NPP Accident

The value of the ¹³³Xe/^133mXe isometric activity ratio for the stationary regime of reactor work is about 35, and that for an instant fission (explosion) is about 11, which allowed estimation of the nuclear component of the instant (explosion) energy release during the NPP accident. Atmospheric xenon samples were taken at the trajectory of accident product transfers (in the Cherepovetz area); these samples were measured by a gamma spectrometer, and the ¹³³Xe/^133mXe ratio was determined as an average value of 22.4. For estimations a mathematic model was elaborated considering both the value of instant released energy and the schedule of reactor power change before the accident, as well as different fractionation conditions on the isobaric chain. Comparison of estimated results with the experimental data showed the value of the instant specific energy release in the Chernobyl NPP accident to be 2·10⁵–2·10⁶ J/Wt or 6·10¹⁴–6·10¹⁵ J (100–1,000 kt). This result is matched up to a total reactor power of 3,200 MWt. However this estimate is not comparable with the actual explosion scale estimated as 10t TNT. This suggests a local character of the instant nuclear energy release and makes it possible to estimate the mass of fuel involved in this explosion process to be from 0.01 to 0.1% of total quantity.     

The application of caesium‐137 measurements to investigate floodplain deposition in a large semi‐arid catchment in Queensland,Australia: a low‐fallout environment

Floodplains comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of large dryland floodplains is not well understood. Processes occurring on such floodplains are often difficult to observe, and techniques used to investigate smaller perennial floodplains are often not practical in these environments. This study assesses the utility of ¹³⁷Cs inventory and depth‐profile techniques for determining relative amounts of floodplain sedimentation in the Fitzroy River, northeastern Australia; a 143 000 km² semi‐arid river system. Caesium‐137 inventories were calculated for floodplain and reference location bulk soil cores collected from four sites. Depth profiles of ¹³⁷Cs concentration from each floodplain site and a reference location were recorded. The areal density of ¹³⁷Cs at reference locations ranged from 13 to 978 Bq m^–2 (0–1367 Bq m^–2 at the 95% confidence interval), and the mean value ± 2 (standard error of the mean) was 436 ± 264 Bq m^–2, similar to published data from other Southern Hemisphere locations. Floodplain inventories ranged from 68 to 1142 Bq m^–2 (0–1692 Bq m^–2 at the 95% confidence interval), essentially falling within the range of reference inventory values, thus preventing calculation of erosion or deposition. Depth‐profiles of ¹³⁷Cs concentration indicate erosion at one site and over 66 cm of deposition at another since 1954. Analysis of ^239+240Pu concentrations in a depositional core substantiated the interpretation made from ¹³⁷Cs data, and depict a more tightly constrained peak in concentration. Average annual deposition rates range from 0 to 15 mm. The similarity between floodplain and reference bulk inventories does not necessarily indicate a lack of erosion or deposition, due to low ¹³⁷Cs fallout in the region and associated high measurement uncertainties, and a likely influence of gully and bank eroded sediments with no or limited adsorbed ¹³⁷Cs. In this low‐fallout environment, detailed depth‐profile data are necessary for investigating sedimentation using ¹³⁷Cs. Copyright © 2009 John Wiley & Sons, Ltd.     

Assessment of sediment yield in a small karst catchment by using 137Cs tracer technique

There is very thin soil layer in karst rocky desertification areas in Southwest China,sediment deposition and sediment yield in the karst area affects the development of vegetation greatly.In the present study,the ¹³⁷Cs technique was used to assess the rate of sediment deposition and sediment yield in a small karst catchment.The ¹³⁷Cs inventory within the depression varied between 800 m^-2 and 2,200 Bq m^-2,with the mean value of 1,500.1 Bq m^-2.The ¹³⁷Cs reference inventory at a nearby reference site was 805.9 Bq m^-2.It could be inferred to that sediment deposition had occurred in the catchment.The mean depth of sediments deposition in the depression was 6 cm and the deposition rate was approximately 0.13 cm yr^-1.The analysis of the topographic characteristics of the catchment revealed that the sediment deposition occurred mainly at the lower part of the small catchment.Although,there was a sinkhole in the depression,little sediment had drained out with runoff through the sinkhole,because the local people built ridges around the sinkholes for storing water.According to this,sediment yield rate in the small catchment was estimated to be approximately 19.25 to 27.5 t km^-2 yr^-1,and the extremely low sediment yield was maybe the main obstacle to vegetation restoration in karst rocky desertification areas.     

Carbon sinks/sources in the Yellow and East China Seas—Air-sea interface exchange,dissolution in seawater,and burial in sediments

The sinks/sources of carbon in the Yellow Sea(YS) and East China Sea(ECS), which are important continental shelf seas in China, could exert a great influence on coastal ecosystem dynamics and the regional climate change process. The CO_2 exchange process across the seawater-air interface, dissolved and particulate carbon in seawater, and carbon burial in sediments were studied to understand the sinks/sources of carbon in the continental shelf seas of China. The YS and the ECS generally have different patterns of seasonal air-sea CO_2 exchange. In the YS, regions west of 124°E can absorb CO_2 from the atmosphere during spring and winter, and release CO_2 to the atmosphere during summer and autumn. The entire YS is considered as a CO_2 source throughout the year with respect to the atmosphere, but there are still uncertainties regarding the exact air-sea CO_2 exchange flux. Surface temperature and phytoplankton production were the key controlling factors of the air-sea CO_2 exchange flux in the offshore region and nearshore region of the YS, respectively. The ECS can absorb CO_2 during spring, summer, and winter and release CO_2 to the atmosphere during autumn. The annual average exchange rate in the ECS was-4.2±3.2 mmol m~(-2) d~(-1) and it served as an obvious sink for atmospheric CO_2 with an air-sea exchange flux of 13.7×10~6 t. The controlling factors of the air-sea CO_2 exchange in the ECS varied significantly seasonally. Storage of dissolved inorganic carbon(DIC) and dissolved organic carbon(DOC) in the YS and the ECS were 425×10~6 t and 1364×10~6 t, and 28.2×10~6 t and 54.1×10~6 t,respectively. Long-term observation showed that the DOC content in the YS had a decreasing trend, indicating that the "practical carbon sink" in the YS was decreasing. The total amount of particulate organic carbon(POC) stored in the YS and ECS was10.6×10~6 t, which was comparable to the air-sea CO_2 flux in these two continental shelf seas. The amounts of carbon sequestered by phytoplankton in the YS and the ECS were 60.42×10~6 t and 153.41×10~6 t, respectively. Artificial breeding of macroalgae could effectively enhance blue carbon sequestration, which could fix 0.36×10~6–0.45×10~6 t of carbon annually. Organic carbon(OC) buried in the sediments of the YS was estimated to be 4.75×10~6 t, and OC of marine origin was 3.03×10~6 t, accounting for5.0% of the TOC fixed by phytoplankton primary production. In the ECS, the corresponding depositional flux of OC in the sediment was estimated to be 7.4×10~6 t yr~(-1), and the marine-origin OC was 5.5×10~6 t, accounting for 5.4% of the phytoplankton primary production. Due to the relatively high average depositional flux of OC in the sediment, the YS and ECS have considerable potential to store a vast amount of "blue carbon."     

Magnetic susceptibility and Cs-137 inventory variability as influenced by land use change and slope positions in a hilly,semiarid region of west-central Iran

The objective of this study was to explore the slope position and land use change effects on the variability in magnetic susceptibility and ¹³⁷Cs inventory as the soil redistribution indicators in a hilly semiarid calcareous area in Iran. The selected study area is located in a hilly region with pasture and cultivation land use of Fereydunshahr, Isfahan Province in west-central Iran. In the two mentioned dominant ecosystems, four slope positions including summit, shoulder, backslope and footslope were identified and in each land use and slope position, three cores were selected to collect 72 soil samples from three depths (0–10, 10–20, 20–30 cm) in an area of 15 × 15 cm. Additional 28 soil samples were collected from the reference site for soil loss and deposition calculations by using the Cs-137 measurement. The results of the study with the use of the Cs-137 technique showed that the average soil loss in the pasture land (46.4 t ha^− 1 yr^− 1) was significantly (p < 0.05) lower than the average soil loss in the cultivated land (80.4 t ha^− 1 yr^− 1). The highest soil loss in both land uses was obtained in the shoulder position, 60.1 and 84.4 t ha^− 1 yr^− 1, respectively, for the pasture and cultivated lands. Moreover, the highest rates of soil deposition was observed in a footslope position in both land uses and they were 34 and 32.4 t ha^− 1 yr^− 1 for the pasture and cultivated lands, respectively. Magnetic susceptibility was significantly (p < 0.05) greater in pasture (χ_lf = 41.51 × 10^− 8 m³/kg) than in the cultivated land (χ_lf = 34.90 × 10^− 8 m³/kg). The pasture land with a lower soil loss rate, indicated significantly higher magnetic susceptibility in all landform positions as compared to that in the cultivated land. The results of the correlation analysis showed that among the studied soil physico-chemical properties, χ_lf (r = 0.83, p < 0.01) in the pasture land had the highest correlation with the Cs-137 inventory. Throughout the non-linear regression analysis, χ_lf was introduced for relating soil parameters and the cesium inventory explained 68% and 79% of the total variability of ¹³⁷Cs in the pasture and cultivated lands, respectively. The results implied that the variability in the magnetic susceptibility within the hillslope is consistent with the variation of the Cs-inventory; and the results thus demonstrate the slope and land use effects on soil redistribution.     

Bayesian network-based risk assessment for hazmat transportation on the Middle Route of the South-to-North Water Transfer Project in China

A Bayesian network-based risk assessment (BN-RA) model was developed to assess the risk of hazmat transportation by identifying, modeling, and quantitatively calculating the risk on the Middle Route of the South-to-North Water Transfer Project (MRSNWTP) in China. First, we selected seven parameters from five categories of impact factors (i.e., human, vehicle, tank, weather, and road environment) as quintessential risk factors for accidents. Second, we used the developed BN-RA model to predict the probability of accidents. Third, using bidirectional inference in the BN approach, we analyzed and ranked the importance of the effects of these factors. The developed model was subsequently applied to assess the risks of major bridges crossing canals with different pavement grades and traffic flow levels both at present and in the future for the Beijing-Shijiazhuang Section of the MRSNWTP. The results indicated the following: (1) Although the overall potential risk of hazmat transportation accidents on all bridges in the Beijing-Shijiazhuang Section was fairly low (e.g., 0.08 %), the impacts cannot be ignored because of the potential for huge losses. (2) According to the analysis of many factors that may affect accidents, the driving patterns of drivers exerted the strongest influence on the probability of an accident, followed by vehicle conditions and lighting conditions. (3) If a vehicle were to fail, the highest probability (0.17 %) of an accident would arise if it were traveling on a road with no street lighting and poor road conditions at night. (4) Assuming that a vehicle was in good condition, the highest probability (0.12 %) of an accident arised when the vehicle suddenly encountered poor road conditions with no lights on a foggy night. (5) The predicted probabilities of accidents on Bridge TCWRR (short for the Tang County West Ring Road Bridge) in the short (i.e., the year 2017), medium (i.e., the year 2022) and long terms (i.e., the year 2027) were 3.25 × 10^?4, 5.37 × 10^?4, and 8.89 × 10^?4, respectively. For Bridge DNR (short for the Dian Bridge on the North Road), these values were 8.64 × 10^?6, 1.02 × 10^?5, and 1.21 × 10^?5, respectively. Based on the risk assessment results, to lower the accident probability and avoid the serious consequences resulting from hazmat transportation accidents, we developed an appropriate emergency response program to reduce potential hazards. This research resolved the problems of randomness and uncertainty associated with hazmat transportation in the MRSNWTP and can provide a reference for the effective prevention of hazmat transportation accidents and scientific decision-making in risk management.     

Optical depth,size distribution and flux of dust from Owens Lake,California

A joint United States/Russian/French collaborative experiment was undertaken in March 1993 and March 1996. Projects LODE I and II (Lake Owens Dust Experiments) took place on the anthropogenically desertified playa (dry lakebed) and surrounding regions of Owens Lake, in east-central California. One of the five parts of Project LODE was to determine relationships between optical depth and flux of dust emitted from the dry lake. Project LODE II included subsequent dust plume measurements and size distributions obtained through April 1996, to further refine the flux measurements for distinct mineral aerosol source regions at Owens Lake. Size distributions of dust aerosol were determined and aerosol optical depths were calculated from sunphotometer solar extinction measurements taken downwind in plumes coming from the emissive areas of Owens Lake. This source was visually observed for 10 measured dust storms. The plume mass was calculated to be 1·5 × 10⁹ g using ground-based measurements and ≥1·6 × 10⁹ g from satellite data. Project LODE II results were found to be consistent with LODE I results for the south end of the playa, but flux values were found to be reduced for the northeastern portion of the playa by comparison. Vertical flux values estimated by sunphotometry were found to be consistent with values estimated via a micrometeorological method. Copyright © 1999 John Wiley & Sons, Ltd.     

Caesium-137 soil sampling and inventory variability in reference locations: A literature survey

Soil sampling design, the number of samples collected and the lateral variation of caesium-137 (¹³⁷Cs) in uneroded reference locations were extracted from previously published work. The focus was on published work which used ¹³⁷Cs reference inventory (Bq m⁻²) for qualitative or quantitative estimation of sediment redistribution (SRD) within the landscape. The objective of this study was to address one of the methodological concerns facing the ¹³⁷Cs technique—that is, the lack of a rigorous statistical treatment of reference locations. The limited attention paid to the reference location is not justified as ‘true’ estimates of SRD are based on the assumption of an unbiased, independent, random probability sample estimate, commonly the arithmetic mean. Results from the literature survey indicated that only 11% of the reference locations sampled for ¹³⁷Cs expressly stated that a probability sampling design was used (transect or systematic-aligned grid). The remaining locations were generally sampled using a non-probability based design, more commonly known as haphazard sampling. Of the 75 reference study areas identified only 40 provided enough information to determine the dispersion around the mean, and from this the coefficient of variation (CV) was calculated for all available data. The median CV was 19·3%, with 95% confidence limits of 13·0–23.4%, indicating that approximately 11 random, independent samples would generally be necessary to adequately quantify the reference ¹³⁷Cs area activity with an allowable error of 10% at 90% confidence. Further analysis indicated that only one-third of the studies sampled a sufficient number of ¹³⁷Cs reference locations. This value would actually be lower as sampling frameworks were based on non-probability sampling procedures. For ¹³⁷Cs reference locations it is recommended that a probability sampling design be utilized, preferably the systematic-aligned grid method, and as a minimum first-order estimate about 11 samples should be collected for inventory estimates.     

Potassium Permanganate Doped Geopolymers for Remedial Applications

This study investigates the use of KMnO₄ doped geopolymers as controlled‐release materials for remedial applications. The geopolymers were prepared by mixing alkali activated Na‐silicate solutions, metakaolin, and various amounts of granular KMnO₄. Samples were heat treated at 75 °C for 48 h. Concentrations of KMnO₄ in samples 1, 2, and 3 were 1.40 × 10^?1, 4.63 × 10^?1, and 6.07 × 10^?1 g/cm³, respectively. 1D column experiments showed that a high MnO₄^? release rate lasted for the first few hours, followed by a gradual decrease of MnO₄^? release. Neither cracks nor surface erosion of the geopolymers were observed throughout the experiments. Sample 1 approached exhaustion at the end of the Day 7. It took about 18 d for exhaustion of KMnO₄ releases in samples 2 and 3. Modeling of the observed KMnO₄ releases suggested diffusion and dissolution‐related fast transport as the most important mechanisms. This latter mechanism involves the creation of a connected secondary porosity in the geopolymers by dissolution of KMnO₄ granules. The contribution of Fickian diffusion to the total release decreased as the KMnO₄ content of the samples increased, and the dissolution mechanism became increasingly important.     

Spatial and Temporal Dependence of Temperature Variations Induced by Atmospheric Pressure Variations in Shallow Underground Cavities

Pressure-induced temperature (PIT) variations are systematically observed in the atmosphere of underground cavities. Such PIT variations are due to the compressibility of the air, damped by heat exchange with the rock surface. It is important to characterize such processes for numerous applications, such as the preservation of painted caves or the assessment of the long-term stability of underground laboratories and underground waste repositories. In this paper we thoroughly study the spatiotemporal dependence of the PIT response versus frequency using vertical and horizontal profiles of temperature installed in an abandoned underground quarry located in Vincennes, near Paris. The PIT response varies from about 20 × 10^?3°C hPa^?1 at a frequency of 2 × 10^?4 Hz to 2–3 × 10^?3°C hPa^?1 at a frequency of one cycle per day. An analytical expression based on a simple heat exchange model accounts for the observed features of the PIT response and allows for correcting the measured time series, having standard deviations of about 10^?2°C, to residual variations with a standard deviation of about 2 × 10^?3°C. However, a frequency-dependent attenuation of the response, corresponding to a reduction in amplitude with a factor varying from 2 to 3, is observed near the walls. This effect is not included in the simple analytical expression, but it can be accounted for by a one-dimensional differential equation, solved numerically, where temperature variations in the atmosphere are damped by an effective radiative coupling with the rock surface, complemented by a diffusive coupling near the walls. The TIP response is observed to remain stable over several years, but a large transient enhancement of about a factor of two is observed near the roof at one location from July to October 2005. In a cavity located below the Paris Observatory, an additional contribution is identified in the PIT response function versus frequency for frequencies smaller than 2 × 10^?5 Hz. This contribution can be described using a modified analytical expression that includes the effect of heat diffusion into the surrounding rock. Using this expression, in this case also, the temperature time series can then be corrected, giving a residual standard deviation smaller than 1.6 × 10^?3°C. Transient temporal variations of the PIT response are observed in all sites, with possible nonlinear components in the PIT. Such effects are not properly understood at this stage, and limit the reduction of time series to standard deviations of the order of 2 × 10^?3°C, and consequently limit the search for new transient or seasonal temperature signals, for example due to the presence of tiny heat sources in the cavity or to geodynamical effects.     

Major ion chemistry of two cratonic rivers in the tropics: Weathering rates and their controlling factors

Continental weathering plays a dominant role in regulating the global carbon cycle, soil chemistry and nutrient supply to oceans. The CO₂-mediated silicate weathering acts as a major CO₂ sink, whereas sulphuric acid-mediated carbonate dissolution releases CO₂ to the atmosphere–ocean system. In this study, dissolved major ions and silica concentrations of two tropical (Damodar and Subarnarekha) river systems from India have been measured to constrain the type and rate of chemical weathering for these basins. The total dissolved solids (TDS) of these rivers, a measure of total solute supply from all possible sources, are about 2–3 times higher than that of the global average for rivers. Mass balance calculations involving inverse modelling estimate that 63 ± 11% of total cations are derived from rock weathering, of which 27 ± 7% of cations are supplied through silicate weathering. The sulphide-S concentrations are estimated by comparing the water chemistry of these two rivers with that of a nearby river (Brahmani) with similar lithology but no signatures of sulphide oxidation. The outflows of Damodar and Subarnarekha rivers receive 17% and 55% of SO₄ through sulphide oxidation, respectively. The sulphide oxidation fluxes from the ore mining areas, such as upper Damodar (0.52 × 10⁹ mol/yr) and lower Subarnarekha (0.66 × 10⁹ mol/yr) basins, are disproportionally (~9 times) higher compared to their fractional areal coverage to the global drainage area. The corresponding CO₂ release rate (2.84 × 10⁴ mol/km²/yr) for the Damodar basin is lower by five times than its CO₂ uptake rate (1.38 × 10⁵ mol/km²/yr). The outcomes of this study underscore the dominance of sulphide oxidation in controlling the dissolved chemical (cationic and sulphur) fluxes.     

Backtracking of Noble Gas Measurements Taken in the Aftermath of the Announced October 2006 Event in North Korea by Means of PTS Methods in Nuclear Source Estimation and Reconstruction

The announced October 2006 nuclear test explosion in the Democratic People’s Republic of Korea (DPRK) has been the first real test regarding the technical capabilities of the verification system built up by the Vienna-based Provisional Technical Secretariat (PTS) of the Comprehensive Nuclear-Test-Ban Treaty Organization (CTBTO) to detect and locate a nuclear test event. This paper enhances the resolution of the DPRK events’ xenon source reconstruction published by Saey et al. (2007, “A long distance measurement of radioxenon in Yellowknife, Canada, in late October 2006”, GRL, Vol. 34, L20802) that was based solely on radio-xenon measurements taken at the remote radionuclide station in Yellowknife, Canada by involving additional measurements taken by a mobile noble gas system deployed quite close to the event location in the Republic of Korea (ROK). Moreover the horizontal resolution of the forward and backward atmospheric transport modelling methods applied for the source scenario reconstruction has been enhanced appropriately to reflect the considerably shorter source-receptor distances examined in comparison to the previously published source reconstruction. It is shown that the ¹³³Xe measurements in Yellowknife could register ¹³³Xe traces from the nuclear explosion during the first 3 days after the event, while the mobile measurements were rather sensitive to releases during days 2–4 after the explosion. According to the analysis, the most likely source scenario would consist of an initial (possibly up to 21 h delayed) venting of 1 × 10^?15 Bq ¹³³Xe during the first 24 h, followed by a two orders of magnitude weaker seepage during the following 3 days. Both measurements corroborate the scenario of a rather rapid venting and soil diffusion of the ¹³³Xe yielded during the explosion. While the Swedish mobile measurements were crucial to enhancement of the reconstruction of the source scenario, given the installation status of the IMS xenon network at the time of the event, a sensitivity analysis revealed that the fully developed network would have been able to detect ¹³³Xe traces from the Korean explosion at a number of stations and allowed for an even better constraint on the release function. The station Ussuriysk, Russia, being in operation in 2006, would have registered ¹³³Xe within 1 day and with a three orders of magnitudes stronger signal compared to the detection at Yellowknife.     

ASSESSMENT OF SOIL LOSS ON UNCULTIVATED SLOPE LAND BY USING 137CS TECHNIQUE IN THE UPPER YANGTZE RIVER BASIN OF CHINA

Radionuclides are used as tracers of sediments in areas where no plot data or field monitoring data are not available. Caesium-137 can provide important information on both soil loss rates and sediment sources. The 137Cs technique is employed to assess soil erosion rates in forest and grass lands in the Upper Yangtze River Basin, China. The study area includes 6 forestlands and 4 grasslands in 8 counties and cities over the eastern part of the basin. The ^137Cs reference inventories ranged from 620.9 Bq m-2 to 2560.3 Bq m^-2. For the 6 forestlands, the average 137Cs inventory over a field ranges from 960.8 Bq m^-2 to 2560.3 Bq m^-2. The average erosion rate is estimated from the ^137Cs measurements between 0 to 588 t km^-2yr^-1. For the 4 grasslands, the average ^137Cs inventory ranges from 119.0 Bq m2 to 869.7 Bq m^-2. The average rate of erosion from grassland varies from 0 to 4435 t km^-2 yrl. Where the erosion was more severe, the ^137Cs inventory was lower. The results showed that there is no clear relationship between ^137Cs inventory, slope length and slope gradient on uncultivated land. The erosion rates for uncultivated land and cultivated land is compared. The result indicates that the erosion rates on uncultivated land is much lower than those on cultivated slopes and the severity of the soil erosion is closely related to vegetation cover.     

14C content of ten meteorites measured by tandem accelerator mass spectrometry

¹⁴C has been measured in three North American and seven Antarctic meteorites with the Chalk River MP tandem accelerator. In most cases cosmogenic¹⁴C, which is tightly bound, was separated from absorbed atmospheric radiocarbon by stepwise heating extractions. Terrestrial ages obtained by comparing cosmogenic¹⁴C in the meteorite to that in Bruderheim are (7.2 ± 0.6) × 10³ years for Yamato 7304, (11.6 ± 0.4) × 10³ years for Estacado, and range from (32.7 ± 0.5) × 10³ to (41.0 ± 0.8) × 10³ years for six meteorites recovered at Allan Hills and its vicinity. The present upper limit to age determination by the accelerator method varies from 50 × 10³ to 70 × 10³ years depending upon mass and carbon content of the sample. The natural limit caused by cosmic ray production of¹⁴C in silicate rocks at 2000 m elevation is estimated to be (55 ± 5) × 10³ years. “Weathering ages” were estimated for the Antarctic meteorites from the specific activity of loosely-bound CO₂ considered to be absorbed from the terrestrial atmosphere on weathering. The accelerator measurements are in accordance with previous low-level counting measurements but have higher precision and sensitivity.     

Constraining tephra dispersion and deposition from three subplinian explosions in 2011 at Shinmoedake volcano,Kyushu, Japan

Constraining physical parameters of tephra dispersion and deposition from explosive volcanic eruptions is a significant challenge, because of both the complexity of the relationship between tephra distribution and distance from the vent and the difficulties associated with direct and comprehensive real-time observations. Three andesitic subplinian explosions in January 2011 at Shinmoedake volcano, Japan, are used as a case study to validate selected empirical and theoretical models using observations and field data. Tephra volumes are estimated using relationships between dispersal area and tephra thickness or mass/area. A new cubic B-spline interpolation method is also examined. Magma discharge rate is estimated using theoretical plume models incorporating the effect of wind. Results are consistent with observed plume heights (6.4–7.3 km above the vent) and eruption durations. Estimated tephra volumes were 15–34?×?10⁶ m³ for explosions on the afternoon of 26 January and morning of 27 January, and 5.0–7.6?×?10⁶ m³ for the afternoon of 27 January; magma discharge rates were in the range 1–2?×?10⁶ kg/s for all three explosions. Clast dispersal models estimated plume height at 7.1?±?1 km above the vent for each explosion. The three subplinian explosions occurred with approximately 12-h reposes and had similar mass discharge rates and plume heights but decreasing erupted magma volumes and durations.     

The mass estimation of volatile emission during 1199–1200 AD eruption of Baitoushan volcano and its significance

On the basis of the study of volcanic products during 1199–1200AD eruption of Baitou Mountain (Baitoushan), the released volatile content was estimated by comparing Cl, F, S, H₂O concentrations of undegassed glass inclusions with those of degassed matrix glasses. The calculations show that volatile yields, released from the melt, are 109.88 × 10⁶ ton of HCl, 196.80 × 10⁶ ton of HF, 1477.84 × 10⁶ ton of H₂O, 23.14 × 10⁶ ton of SO₂, which could have formed 35.43 x10⁶ ton of H²SO₄ aerosol in the atmosphere. They could have substantial effect on paleoclimate and paleo-environment.     

Chernobyl reactor accident consequences on small atmospheric ions concentration above Athens

In the present study the variation in small ion concentration (SIC), positive and negative, above Athens (=37°58.3N, =23°43E,h=107 m) after Chernobyl reactor accident is examined.SIC started to increase importantly at the National Observatory of Athens (N.O.A) since 3 May 1986 and reached its highest mean daily values on Monday, 5 May. These maximum values were 4 times the normal for positive ions and 5 times the normal for negative ions. Correlation coefficients were calculated between SIC and radionuclides I-131, Cs-137, Ru-103 and outdoor exposure rate.     

Understanding flow dynamics and density currents in a river-reservoir system under upstream reservoir releases

ABSTRACT

A three-dimensional flow and temperature model was applied for a 124 km river-reservoir system from Lewis Smith Dam tailrace to Bankhead Lock & Dam, Alabama. The model was calibrated against measured water levels, temperatures, velocities and flow rates from 4 May to 3 September 2011 under small constant release (2.83 m³/s) and large intermittent releases (~140 m³/s) from an upstream reservoir. Distributions of simulated flow and temperatures and particle tracking at various locations were analyzed which revealed the complex interactions of density currents, dynamic surface waves and solar heating. Flows in the surface and bottom layers moved in both upstream and downstream directions. If there was small constant release only from Smith Dam, simulated bottom temperatures at Cordova were on average 4.8°C higher than temperatures under actual releases. The momentum generated from large releases pushed bottom density currents downstream, but the released water took several days to reach Cordova.

Editor D. Koutsoyiannis; Associate editor B. Dewals