Do Cloud Properties in a Puerto Rican Tropical Montane Cloud Forest Depend on Occurrence of Long-Range Transported African Dust?

We investigated cloud properties of warm clouds in a tropical montane cloud forest at Pico del Este (1,051 m a.s.l.) in the northeastern part of Puerto Rico to address the question of whether cloud properties in the Caribbean could potentially be affected by African dust transported across the Atlantic Ocean. We analyzed data collected during 12 days in July 2011. Cloud droplet size spectra were measured using the FM-100 fog droplet spectrometer that measured droplet size distributions in the range from 2 to 49 µm, primarily during fog events. The droplet size spectra revealed a bimodal structure, with the first peak (D < 6 µm) being more pronounced in terms of droplet number concentrations, whereas the second peak (10 µm < D < 20 µm) was found to be the one relevant for total liquid water content (LWC) of the cloud. We identified three major clusters of characteristic droplet size spectra by means of hierarchical clustering. All clusters differed significantly from each other in droplet number concentration ( \(N_{\rm tot}\) ), effective diameter (ED), and median volume diameter (MVD). For the cluster comprising the largest droplets and the lowest droplet number concentrations, we found evidence of inhomogeneous mixing in the cloud. Contrastingly, the other two clusters revealed microphysical behavior, which could be expected under homogeneous mixing conditions. For those conditions, an increase in cloud condensation nuclei—e.g., from processed African dust transported to the site—is supposed to lead to an increased droplet concentration. In fact, one of these two clusters showed a clear shift of cloud droplet size spectra towards smaller droplet diameters. Since this cluster occurred during periods with strong evidence for the presence of long-range transported African dust, we hypothesize a link between the observed dust episodes and cloud characteristics in the Caribbean at our site, which is similar to the anthropogenic aerosol indirect effect.     

A comparative study on the growth of cloud drops by condensation using an air parcel model with and without entrainment

During a study of the growth of cloud drops by condensation the evolution of cloud drop size spectra with height above cloud base was determined for maritime aerosols, and for continental aerosols containing aerosol particles of mixed composition. Air parcel models were used in which the parcel was either completely closed to mass and heat transfer (strictly adiabatic models), or open to heat transfer and to partial or complete mass transfer (entrainment models). It was found that adiabatic models and models which consider the entraining of air devoid of aerosol particles predict drop size distributions which are considerably narrower than those observed in non-precipitating cumulus clouds, and have only a single maximum. On the other hand, relative broad drop size distributions and distributions with a double maximum — as they are observed in atmospheric clouds — are predicted if the entrainment of both air and aerosol particles are considered in the condensation model. Our results support the findings ofWarner (1973) which were obtained for a purely maritime aerosol.     

中国东部层积云发展过程中云微物理特征的演变

基于2007—2010年的CloudSat卫星观测数据,以云层液态水路径为指标将层积云的发展过程划分为五个阶段,对比研究了中国东部降水与非降水层积云发展过程中云微物理特征和云微物理机制的演变,并分析了其海陆差异.研究表明：非降水层积云中,云滴增长主要通过凝结过程完成,但云滴的凝结增长有限,难以形成降水,在非降水层积云发展的旺盛阶段,云层中上部云滴发生较弱的碰并过程.降水层积云中云滴碰并增长活跃,当云层液态水路径小于500 g·m^-2时,云滴在从云顶下落至云底的过程中持续碰并,并在云底附近出现云水向雨水的转化;当降水层积云液态水路径超过500 g·m^-2时,云滴碰并增长主要发生在云层上部,在云层中部,云液态水含量、液态粒子数浓度和液态粒子有效半径达到最大,云水向雨水的转化最为活跃.层积云微物理特征的海陆差异主要是由海陆上空气溶胶浓度和云中上升气流强度不同导致的.在非降水层积云中下部,陆地丰富的气溶胶为云滴凝结增长提供了充足的云凝结核,因而云微物理量的量值在陆地上空更大,而在云层中上部,云滴凝结增长达到极限,海洋充足的水汽输送使云微物理量的量值在海洋上空更大.当降水层积云液态水路径大于500 g·m^-2时,陆地层积云中更强的上升气流使大量云滴在云层中上部累积滞留,云滴碰并增长活跃,云层中上部云微物理量的量值在陆地上空更大.

     

The physics of precipitation in cumulus clouds

Summary Over the past several years, the University of Chicago has conducted a program of research into the physics and chemistry of cumulus cloud precipitation. From these measurements it has been possible to isolate the sublimation-coalescence mechanism (Bergeron process) from the condensation-coalescence mechanism and to estimate the relative role of each process in the formation of rain n cumulus clouds. It is found that size of cloud capable of raining is a strong function of geography, that the environment of the cloud is very important in determining the probability of rain and that liquid water content is one of the most important within-cloud parameters.An essential part of the research concerned cloud treatment. Definite, positive treatment effects were demonstrated for rain initiation through coalescence using water spray. No effects were detectable from dry ice seeding of subcooled clouds, although any such effects may have been obscured by sample size (27 cloud pairs).Text of paper presented before Physical Society and Royal Meteorological Society Joint Conference on Cloud Physics, London, England, Jan. 4–5, 1956. The research reported in this paper has been sponsored by the Geophysics Research. Directorate of the Air Force Cambridge Research Center, Air Research and Development Command under Contract Nos. AF 19 (604)-618 and AF 19 (604)-1388.     

The influence of cloud structure and droplet concentration on the reflectance of shortwave radiation

The effects of cloud shadowing, channelling, cloud side illumination and droplet concentration are investigated with regard to the reflection of shortwave solar radiation. Using simple geometric clouds, coupled with a Monte Carlo model the transmission properties of idealized cloud layers are found. The clouds are illuminated with direct solar radiation from above. The main conclusion reached is that the distribution of the cloud has a very large influence on the reflectivity of a cloud layer. In particular, if the cloud contains vertical gaps through the cloud layer in which the liquid water content is zero, then, smaller more numerous gaps are more influential on the radiation than fewer, larger gaps with equal cloud fraction. At very low solar zenith angles channelling of the radiation reduces the reflection expected on the basis of the percentage cloud cover. At high solar zenith angles the illumination of the cloud edges significantly increases the reflection despite the shadowing of one cloud by another when the width of the gaps is small. The impact of droplet concentration upon the reflection of cloud layers is also investigated. It is found that at low solar zenith angles where channelling is important, the lower concentrations increase the transmission. Conversely, when cloud edge illumination is dominant the cloud distribution is found to be more important for the higher concentrations.     

The impact of cloud inhomogeneities on the Earth radiation budget: the 14 October 1989 I.C.E. convective cloud case study

Through their multiple interactions with radiation, clouds have an important impact on the climate. Nonetheless, the simulation of clouds in climate models is still coarse. The present evolution of modeling tends to a more realistic representation of the liquid water content; thus the problem of its subgrid scale distribution is crucial. For a convective cloud field observed during ICE 89, Landsat TM data (resolution: 30m) have been analyzed in order to quantify the respective influences of both the horizontal distribution of liquid water content and cloud shape on the Earth radiation budget. The cloud field was found to be rather well-represented by a stochastic distribution of hemi-ellipsoidal clouds whose horizontal aspect ratio is close to 2 and whose vertical aspect ratio decreases as the cloud cell area increases. For that particular cloud field, neglecting the influence of the cloud shape leads to an over-estimate of the outgoing longwave flux; in the shortwave, it leads to an over-estimate of the reflected flux for high solar elevations but strongly depends on cloud cell orientations for low elevations. On the other hand, neglecting the influence of cloud size distribution leads to systematic over-estimate of their impact on the shortwave radiation whereas the effect is close to zero in the thermal range. The overall effect of the heterogeneities is estimated to be of the order of 10 W m⁻² for the conditions of that Landsat picture (solar zenith angle 65○, cloud cover 70%); it might reach 40 W m⁻² for an overhead sun and overcast cloud conditions.     

Characteristics of Cloud Drop Spectra at Different Levels and with Respect to Cloud Thickness

--Measurements on drop size spectra were made in cumulus clouds over Pune (inland) region on many days during the summer monsoon seasons. In this paper, the measurements in non-raining cumulus clouds made in the years 1984, 1985 and 1986 at different levels and for different cloud thickness have been studied. In general, the drop size spectra broadened with height and the concentration of drops with diameter > 50 wm (N_L), mean volume diameter (MVD), liquid water content (LWC) and dispersion increased with height while the concentration of drops with diameter < 20 wm (N_S) and the total concentration of drops (N_T) decreased with height. The average drop size distributions were unimodal at the lower levels while they were bimodal at the higher levels. High water contents were confined to drops in the size range 5-25 wm at both higher and lower levels. The average drop size spectra were broader and N_L, LWC, MVD and dispersion greater while N_T and N_S smaller for thicker clouds (range of vertical extent 1.1-2.1 km) as compared to those for thinner clouds (range of vertical extent 0.3-1.1 km). Water contents for the drops > 28 wm were higher while those for the drops > 28 wm lower in thicker clouds than in thinner clouds. The average drop size distributions were bimodal in the former case, while they were unimodal in the other case.     

A new aspect of condensation theory

This paper examines the effects of the mixing of dry air into a cloud top from the point of view of the droplet spectra. It is shown theoretically that the resulting cycling of the air up and down in the cloud, as seems to be the essential mechanism by which cumuli have been diluted to their observed liquid water mixing ratio, can double the largest drop radius and generate cloud parcels containing drops of all sizes up to this maximum. These changes in the droplet distribution with size occur by a process which is not greatly influenced by the cloud condensation nuclei or the details of droplet growth since maritime like spectra can develop in continental type cumuli. It shows that large numbers of cloud condensation nuclei should not have much effect in inhibiting the rainforming process by reducing coalescence growth. On the contrary, the controlling parameters which determine precipitation efficiency and times seem to be those which control the mixing.     

Size distribution models of fog and cloud droplets and their volume extinction coefficients at visible and infrared wavelengths

Based on the average variability of the skewness with respect to the droplet mode radius, a wide set of mean size-distribution models is presented in terms of the modified gamma function for fog and stratified cloud droplets. These models appear appropriate for giving reliable size-distribution curves relative to the various formation stages of the droplet population both in fogs and in stratus and stratocumulus clouds.The corresponding volume extinction coefficient has been computed at various wavelengths from 0.4 to 17 m using Van de Hulst's (1957) approximation multiplied by Deirmendjian's (1960) correction factors. This set of theoretical extinction data has been compared with experimental extinction measurements performed in atmospheres characterized by a marked thermal inversion for describing the evolutionary features of the water droplet size distribution within the whole ground layer.     

On the application of the classic Kessler and Berry schemes in Large Eddy Simulation models with a particular emphasis on cloud autoconversion, the onset time of precipitation and droplet evaporation

Many Large Eddy Simulation (LES) models use the classic Kessler parameterisation either as it is or in a modified form to model the process of cloud water autoconversion into precipitation. The Kessler scheme, being linear, is particularly useful and is computationally straightforward to implement. However, a major limitation with this scheme lies in its inability to predict different autoconversion rates for maritime and continental clouds. In contrast, the Berry formulation overcomes this difficulty, although it is cubic. Due to their different forms, it is difficult to match the two solutions to each other. In this paper we single out the processes of cloud conversion and accretion operating in a deep model cloud and neglect the advection terms for simplicity. This facilitates exact analytical integration and we are able to derive new expressions for the time of onset of precipitation using both the Kessler and Berry formulations. We then discuss the conditions when the two schemes are equivalent. Finally, we also critically examine the process of droplet evaporation within the framework of the classic Kessler scheme. We improve the existing parameterisation with an accurate estimation of the diffusional mass transport of water vapour. We then demonstrate the overall robustness of our calculations by comparing our results with the experimental observations of Beard and Pruppacher, and find excellent agreement.     

The Clouds of the Middle Troposphere: Composition, Radiative Impact, and Global Distribution

The clouds of the middle troposphere span the temperature range where both ice and liquid water in a supercooled state can exist. However, because one phase tends to dominate, of the two midlevel cloud types, altostratus are deep ice-dominated, while altocumulus are shallow water-dominated, mixed-phase clouds with ice crystal virga typically trailing below. Multiple remote sensor examples of these cloud types are given to illustrate their main features, and the radiative consequences of the different cloud microphysical compositions are discussed. Spaceborne radar and lidar measurements using the CloudSat and CALIPSO satellites are analyzed to determine the global distributions of cloud frequencies and heights of these clouds. It is found that together these little-studied clouds cover ~25% of the Earth’s surface, which is about one-third of the total cloud cover, and thus represent a significant contribution to the planet’s energy balance.     

Effect of remote clouds on surface UV irradiance

Clouds affect local surface UV irradiance, even if the horizontal distance from the radiation observation site amounts to several kilometers. In order to investigate this effect, which we call remote clouds effect, a 3-dimensional radiative transfer model is applied. Assuming the atmosphere is subdivided into a quadratic based sector and its surrounding, we quantify the influence of changing cloud coverage within this surrounding from 0% to 100% on surface UV irradiance at the sector center. To work out this remote clouds influence as a function of sector base size, we made some calculations for different sizes between 10 km × 10 km and 100 km × 100 km. It appears that in the case of small sectors (base size 20 km × 20 km) the remote clouds effect is highly variable: Depending on cloud structure, solar zenith angle and wavelength, the surface UV irradiance may be enhanced up to 15% as well as reduced by more than 50%. In contrast, for larger sectors it is always the case that enhancements become smaller by 5% if sector base size exceeds 60 km × 60 km. However, these values are upper estimates of the remote cloud effects and they are found only for special cloud structures. Since these structures might occur but cannot be regarded as typical, different satellite observed cloud formations (horizontal resolution about 1 km × 1 km) have also been investigated. For these more common cloud distributions we find remote cloud effects to be distinctly smaller than the corresponding upper estimates, e.g., for a sector with base size of 25 km × 25 km the surface UV irradiance error due to ignoring the actual remote clouds and replacing their influence with periodic horizontal boundary conditions is less than 3%, whereas the upper estimate of remote clouds effect would suggest an error close to 10%.     

Noctilucent clouds seen at 60°N: origin and development

A noctilucent cloud is seen at a particular time from a specified place. The journey of the cloud particles from nucleation to observation can be calculated by using a simple model of growth and taking account of the fall speed of the cloud particles. Cloud particles can be backtracked by bringing together growth and fall speed equations and a model of mesospheric winds to find where the particles of a cloud seen at a particular time and place have originated. The wind model that is used here suggests that there is a distinct outer edge to the summertime polar circulation pattern in which water vapour is being carried up from the lower mesosphere to the mesopause. The change in latitude of this outer edge during the summer season may well account for the observed seasonal change in occurrence of mesospheric clouds. Polar mesospheric clouds cause a drying of the upper mesosphere. It is suggested here that diffusion of water vapour dumped at the level of polar mesospheric clouds will take an appreciable time to carry water vapour back up to the mesopause. In consequence, there will be a significant separation between the observed location of a noctilucent cloud and its precursor polar mesospheric cloud.     

Preliminary laboratory studies of the optical scattering properties of the crystal clouds

Ice crystal clouds have an influence on the radiative budget of the earth; however, the exact size and nature of this influence has yet to be determined. A laboratory cloud chamber experiment has been set up to provide data on the optical scattering behaviour of ice crystals at a visible wavelength in order to gain information which can be used in climate models concerning the radiative characteristics of cirrus clouds. A PMS grey-scale probe is used to monitor simultaneously the cloud microphysical properties in order to correlate these closely with the observed radiative properties. Preliminary results show that ice crystals scatter considerably more at 90° than do water droplets, and that the halo effects are visible in a laboratorygenerated cloud when the ice crystal concentration is sufficiently small to prevent masking from multiple scattering.     

Characteristics of cloud drop spectra in tropical warm clouds

Characteristics of cloud drop spectra were studied using 400 samples obtained from 120 warm cumulus clouds formed during the summer monsoon season.The total concentration of cloud drops (N _T) varied from 384 to 884 cm^–3 and the maximum concentration was observed in the layer below the cloud-top. The width of the drop spectrum was broader in the cloud-base region and in the region below the cloud-top. The spectrum was multimodal at all levels except in the cloud-top region where it was unimodal. The concentration of drops with diameter greater than 50 m (N _L) varied from 0.0 to 0.674 cm^–3.N _L was larger in the cloud-base region.N _L decreased with height up to the middle level and thereafter showed an increase. In the cloud-top region no large drops were present. The computed values of the liquid water varied between 0.132 and 0.536 g m^–3 and the mean volume diameter (MVD) varied between 8.1 and 12.0 m. The LWC and MVD showed a decrease with height except in the middle region of the cloud where the values were higher than the adjacent levels. The dispersion of the cloud drops was lower (0.65) in the cloud-top region and higher (1.01) in the cloud-base region.The observed cloud microphysical characteristics were attributed to vertical mixing in clouds induced by the cloud-top gravity oscillations (buoyancy oscillations) generated by the intensification of turbulent eddies due to the buoyant production of energy by the microscale-fractional-condensation (MFC) in turbulent eddies.     

Observations of condensation growth determined by entity type mixing

It has been speculated for many years that the development of the droplet spectra in cloud is probably influenced by mixing processes. Various theoretical attempts to broaden the droplet spectra by mixing parcels with different velocity histories has shown that that particular effect is small. Similarly, very simpleuniform entrainment procedures did not lead to cloud drop size spectra which were broad enough, although by producing cloud drop size distributions with a double mode these models did substantially improve the drop size spectra of earlier adiabatic models which only exhibited a single mode.Recently a model based on entraining entities representing moving parcels of cloud air within the cloud was detailed byTelford andChai (1980). This study showed that the mixing in of dry air at cumulus turrets could lead to vertical cycling of diluted parcels, and that this cycling, with continual entrainment across the parcel boundaries, will produce much larger drops, as well as smaller drops of all sizes, in the droplet spectra. The entity entrainment concept studied there appears to apply to the observations of stratus cloud discussed in this paper.This paper presents data taken in marine stratus off the California coast which give a particularly clear example of how such droplet spectra modification occurs in practice. Both large drops, and the spread of the spectra to smaller sizes, occur in relation to other variables in such a way as to be consistent with an entity entrainment explanation, with no other obvious possibility.In a marine stratus cloud just over 200 m thick and many tens of miles in extent we find clear evidence that dry air is mixing in at cloud tops. Strong vertical motion is to be found in the cloud, large sized drops are found in cloud parcels where the mixing gives lower droplet concentrations, and there is evidence that newly formed cloud parcels are warmer and contain many more smaller droplets.The observations show that immediately following entrainment of dry air drop diameters are not reduced appreciably, but, in the same parcels, drop concentrations have been reduced by a factor of ten or more. Further down in the cloud big drops, able to start growth by coalescence, are found associated with low total droplet concentrations.Overall, it seems likely from the consideration of these observations that the formation of the large drops which lead to precipitation processes in clouds depends critically on the mixing in of dry air at cloud tops, and very little on the size of the small drops resulting from the condensation nucleus counts. As a conclusion it appears reasonable to state that if entrainment occurs at cloud tops, then big drops will be formed!     

Radiative properties of cirrus clouds in NOAA 4 VTPR channels: Some explorations of cloud scenes from satellites

A one-dimensional spectral infrared radiative transfer model has been developed for atmospheres containing cirrus clouds and absorbing gases above, below and within the cloud. The transfer model takes into consideration the inhomogeneity of the cloudy atmosphere, the gaseous absorption in scattering cloud layers and the wavenumber dependence of radiative transfer. In addition, the cirrus cloud is further divided into a number of sub-layers to account for the non-isothermal and inhomogeneous cloud characteristics. Single-scattering properties for ice crystals are calculated assuming ice cylinders 200 and 60 m in lenght and width, respectively, randomly oriented in a horizontal plane. The spectral infrared transfer program is applied to VTPR channels of the NOAA 4 satellite to simulate upward radiances in cirrus cloud conditions.Comparisons between satellite observed and theoretically simulated upward radiances are carried out for selected cirrus cloud cases. Incorporating atmospheric profiles obtained from radiosonde and the observed cloud information into the spectral transfer program, we show a systematic agreement between observed and computed upward radiances. Systematic reduction patterns of the upward radiance caused by the increase of the cloud ice content are clearly demonstrated for VTPR channels employing tropical and midlatitude atmospheric profiles. Having the quantitative relationships between upward radiances and ice contents, procedures are described for the inference of the cloud ice content and cloud amount. The proposed method has been successfully applied to the three cirrus cloud cases.     

Short-term ground ozone fluctuations at Poona

Short-term fluctuations superimposed on the diurnal variations of surface ozone recorded at Poona during 1969–1970 are discussed.While there is a net production of ozone during electrical discharges in a thunder cloud, the surface ozone recorder often registered a decrease in surface ozone concentration. This decrease coincided with updraughts generated during the formation of a thunderstorm. Similar sharp increases in ozone were observed with downdraughts. In cases of lightning without the development of a thunderstorm over the station, an increase in ozone density was observed just after the first lightning discharge.Apart from the fluctuations associated with thunderstorms in summer, sharp fluctuations in density were also noticed during winter, in the mornings. Abrupt falls in ozone occur with the formation of a stable layer near the ground at night and a sudden surge after the breaking up of the layers in the morning. The changes in ozone are, however, much more pronounced than those in temperature and wind and this striking correlation between surface ozone, surface air temperature and wind provides a unique tool for the study of low-level temperature inversions, their establishment and destruction.     

Evidence for global circuit current flow through water droplet layers

Foggy air and clear air have appreciably different electrical conductivities. The conductivity gradient at horizontal droplet boundaries causes droplet charging, as a result of vertical current flow in the global atmospheric electrical circuit. The charging is poorly known, as both the current flow through atmospheric water droplet layers and the air conductivity are poorly characterised experimentally. Surface measurements during three days of continuous fog using new instrument techniques show that a shallow (of order 100 m deep) fog layer still permits the vertical conduction current to pass. Further, the conductivity in the fog is estimated to be approximately 20% lower than in clear air. Assuming a fog transition thickness of one metre, this implies a vertical conductivity gradient of order 10 fS m^?2 at the boundary. The actual vertical conductivity gradient at a cloud boundary would probably be greater, due to the presence of larger droplets in clouds compared to fog, and cleaner, more conductive clear air aloft.     

Generation of available buoyant energy by cloud glaciation

The available buoyant energy (ABE, energy from the environment which becomes available to a parcel for buoyant accelerations) arising from glaciation is computed by integrating upward the differences in temperature between a parcel that undergoes instantaneous and isenthalpic freezing followed by an ice-saturation ascent, and one that experiences only a water-saturation ascent from the same initial cloud base conditions. This quantity is computed for three initial cloud base conditions representative of tropical, High Plains summertime, and Great Lakes wintertime cumuli. Substantial increases in parcel updraft speed are realized for all clouds if the ABE arising from glaciation is completely converted to parcel kinetic energy. Variations of the three components of parcel heating involved in the glaciation process (i.e., (1) release of latent heat of fusion from freezing of liquid water, (2) cooling or warming from sublimation or deposition as vapor pressure adjusts from water saturation to ice saturation at the post glaciation temperature, and (3) the additional warming or cooling relative to the intial water-saturation adiabat as the parcel follows an icesaturation ascent to a specified upper reference level) are also determined as functions of glaciation temperature. It is found that sublimation substantially counteracts the parcel warming arising from the freezing of liquid water in the case of warm moist cumuli. In addition, it is found that in some instances ice-saturation ascent following glaciation can produce cooling relative to the initial departure from the water saturation adiabat. This was indicated for Great Lakes wintertime cumuli and also for warm moist cumuli with glaciations at very cold temperatures. The effect upon the buoyancy force, of the change in the mass of condensate during glaciation, is small and can usually be neglected.