Trace contaminant concentrations in the Kara Sea and its adjacent rivers, Russia.

Trace organic (chlorinated pesticides, PCBs, PAHs and dioxins/furans) and trace metal concentrations were measured in surficial sediment and biological tissues (i.e., worms, crustaceans, bivalve molluscs, and fish livers) collected from the Russian Arctic. Total DDT, chlordane, PCB and PAH concentrations ranged from ND to 1.2, ND to <0.1, ND to 1.5 and <20-810 ng g(-1), respectively, in a suite of 40 surficial sediment samples from the Kara Sea and the adjacent Ob and Yenisey Rivers. High sedimentary concentrations of contaminants were found in the lower part of the Yenisey River below the salt wedge. Total dioxins/furans were analysed in a subset of 20 sediment samples and ranged from 1.4 to 410 pg g(-1). The highest trace organic contaminant concentrations were found in organisms, particularly fish livers. Concentrations as high as 89 ng g(-1) chlordane; 1010 ng g(-1) total DDTs; 460 ng g(-1) total PCBs; and 1110 ng g(-1) total PAH, were detected. A subset of 11 tissue samples was analysed for dioxins and furans with total concentrations ranging from 12 to 61 pg g(-1). Concentrations of many trace organic and metal contaminants in the Kara Sea appear to originate from riverine sources and atmospheric transport from more temperate areas. Most organic contaminant concentrations in sediments were low; however, contaminants are being concentrated in organisms and may pose a health hazard for inhabitants of coastal villages.     

Sorption of radioactive contaminants by sediment from the Kara Sea

The purpose of this study is to quantify some of the parameters needed to perform near-field modelling of sites in the Kara Sea that were impacted by the disposal of radioactive waste. The parameters of interest are: the distribution coefficients (Kd) for several important radionuclides, the mineralogy of the sediment, and the relationship of Kd to liquid-to-solid ratio. Sediment from the Kara Sea (location: 73 degrees 00'N, 58 degrees 00'E) was sampled from a depth of 287 m on August 23/24, 1992. Analysis of the material included mineralogy, grain size and total organic carbon (TOC). Uptake kinetics were determined for 85Sr, 137Cs, 241Am, 99Tc, 1251, 232U and 210Pb and distribution coefficients (Kd) were determined for these radionuclides using batch type experiments. Sorption isotherms, developed for 137Cs, 85Sr and 99Tc, were linear in each case. Increasing the liquid-to-solid ratio strongly increased uptake of 137Cs and moderately increased uptake of 99Tc. Analysis for anthropogenic radionuclides indicated the presence only of 239/240Pu in the sediment with the highest activity (at the top section of the core) being 0.420 Bq kg(-1). Other anthropogenic radionuclides were below detection limits.     

Pu, Cs and excess Pb in Russian Arctic sediments

The activity ratios of Pu and radiocesium isotopes have been used to delineate the major sources (such as global and close-in (debris) fallout, nuclear fuel reprocessing and fabrication plant effluents) in the environment. We have measured ²³⁸Pu, ^239,240Pu, ¹³⁷Cs, and excess ²¹⁰Pb concentrations in 107 surficial sediments as well as in 5 sediment cores collected in the summer months of 1993 and 1994 from the Ob and Yenisey Rivers (Russia) and the Kara sea. A comparison of the sediment core inventories of ^239,240Pu and ¹³⁷Cs, along with the ²³⁸Pu/^239,240Pu activity ratios, with those expected from global fallout allows us to estimate the relative amounts, if any, of reactor-derived ²³⁸Pu and ^239,240Pu from the dumped reactor sites in the study area.

In surficial sediment samples collected in 1993 and 1994, the ^239,240Pu concentrations varied between 4.2 and 856 mBq kg⁻¹, with a mean of 239 mBq kg⁻¹. In samples with a measurable ²³⁸Pu, the ²³⁸Pu/^239,240Pu activity ratios varied between 0.010 and 0.069, with an average value of 0.035 ± 0.014. This range can be compared to the average ²³⁸Pu/^239,240Pu activity ratio of 0.030 for the year 1993 from nuclear weapons testing and SNAP fallout obtained from soil studies, indicating very little (≤ 5%) additional sources of ²³⁸Pu to the sediments in the study area. The inventories of Pu in the 5 sediment cores from the study area varied between 2.67 ± 0.67 and 24.5 ± 2.2 Bq m⁻² with a mean value of 8.83 Bq m⁻². The ¹³⁷Cs concentrations in the upper 3 cm of the sediments varied between below detection limit to 71.4 Bq kg⁻¹, with a mean of 14.9 Bq kg⁻¹. The ¹³⁷Cs inventories in the 5 sediment cores varied between 156.7 ± 28.3 and 1600 ± 153.3 Bq m⁻², with a mean value of 583.3 Bq m⁻². The mean ratio of inventories of Pu to that of ¹³⁷Cs, 0.015, is comparable to the values in other places in the Arctic region. There is a significant correlation between total organic carbon and concentrations of ¹³⁷Cs, ^239,240Pu and ²¹⁰Pb, suggesting that organic matter-enriched fine particles are a likely carrier phase for these nuclides. The ratio of ¹³⁷Cs/^239,240Pu also suggests that most of these nuclides are derived from global fallout.     

Assessment of potential transport of pollutants into the Barents Sea via sea ice--an observational approach

The present estimates of ice drift in the Arctic include utilization of satellite imagery data (special sensor microwave/imager) and a reconstruction of air pressure for the period 1899-1998. A significant part of the sea ice in the Arctic Ocean has its origin in the Kara Sea and melts in the Greenland and the Barents Sea (BS). Consequently there may be a particular risk of pollutants in the Kara Sea entering the food webs of the Greenland and BS. The ice export from the Kara Sea between 1988 and 1994 was about 208,000 km2 (154 km3) per year. The import of ice into the BS was during the same period 161,000 km2 (183 km3) per year while the ice drift through the Fram Strait into the Greenland Sea was 583,000 km2 (1859 km3) per year. Ice which formed adjacent to the Ob and Yenisey rivers in early January, drifted into the BS within two years (with a probability of about 50%.     

Distribution of 137Cs in the Lena River estuary-Laptev Sea system.

Surface sediment samples in the Laptev Sea have average 137Cs content of 7.1 Bq kg(-1), a value intermediate between that of the western Kara Sea (23 Bq kg(-1) and the East Siberian Sea (4.2 Bq kg-'). Both surface sediment content and sediment inventory of 137Cs in the Laptev Sea sediments show significant variability, and the influence of a variety of environmental factors.137Cs concentrations in the Laptev Sea surface sediments range from 0.8 to 16 Bq kg(-1). There is a marked increase in 137Cs content of surface sediment samples collected near the Lena River delta, and a local enrichment in the 137Cs inventories at these sites is also evident. Fine-grained mixed-layer illite/ smectite rich sediments in the estuary provide effective adsorption sites to fix 137Cs, in spite of desorption processes associated with low salinities in estuarine mixing. The Lena River-Laptev Sea mixing zone is a major site of sea-ice production. River and shelf sediments are incorporated into sea-ice formed in this region (Holmes and Creager, 1974). The irregular 137Cs activity profiles of the Lena River estuary cores indicate disturbance or removal of 137Cs-laden sediments via sea-ice related processes. Lena River and Estuary sediments may have served as a secondary source (i.e. other than direct fallout) of 137Cs in sea-ice. North-east of the Lena River estuary, sediment contains a thin layer of 137Cs-bearing material over an erosion surface. The 137Cs-laden surface layer may be the result of transient deposition of estuarine sediments being delivered by sea-ice or spring floods.     

Particulate matter fluxes in the southern and central Kara Sea compared to sediments: Bulk fluxes, amino acids, stable carbon and nitrogen isotopes, sterols and fatty acids

The Kara Sea is one of the arctic marginal seas strongly influenced by fresh water and river suspension. The highly seasonal discharge by the two major rivers Yenisei and Ob induces seasonal changes in hydrography, sea surface temperature, ice cover, primary production and sedimentation. In order to obtain a seasonal pattern of sedimentation in the Kara Sea, sediment traps were deployed near the river mouth of the Yenisei (Yen) as well as in the central Kara Sea (Kara) within the framework of the German–Russian project “Siberian River run-off; SIRRO”. Two and a half years of time-series flux data were obtained between September 2000 and April 2003 and were analyzed for bulk components, amino acids, stable carbon and nitrogen isotopes as well as sterols and fatty acids.Sediment trap data show that much of the annual deposition occurred under ice cover, possibly enhanced by zooplanktonic activity and sediment resuspension. An early bloom of ice-associated algae in April/May occurred in the polynya area and may have been very important to sustain the life cycles of higher organisms after the light limitation of the winter months due to no/low insolation and ice cover. The strong river input dominated the months June–August in the southern part of the Kara Sea. The central Kara Sea had a much shorter productive period starting in August and was less affected by the river plumes. Despite different time-scales of sampling and trapping biases, total annual fluxes from traps were in the same order of magnitude as accumulation rates in surface sediments. Terrestrial organic carbon accumulation decreased from 10.7 to 0.3 g C m⁻² a⁻¹ from the riverine source to the central Kara Sea. Parallel to this, preservation of marine organic matter decreased from 10% to 2% of primary productivity which was probably related to decreasing rates of sedimentation.     

Radiocaesium distribution in the bottom sediments of the Kara Sea

The article presents the results of radiogeochemical studies carried out by the Institute of Geology of Ore Deposits, Petrography, Mineralogy, and Geochemistry, RAS (IGEM RAS), in the Kara Sea and the estuaries of the Ob and Yenisei rivers in 1995–2003. The studies were carried out onboard the Akademik Boris Petrov research vessel, belonging to the Institute of Geochemistry, RAS. Based on studies of circa 1500 samples of bottom sediments, taken from 172 marine and river stations, a map of ¹³⁷Cs distribution in the surface sediments has been compiled. Four zones of radiocesium overactivity (>15 Bk/kg) have been identified: Novaya Zemlya Zone, Vaigach Zone, Ob Zone, and Yenisei Zone. The zones have different radiocesium concentration levels, as well as different input sources, but all of them have formed under the influence of complex geochemical barriers. Data from 47 sectioned cores of bottom sediments, sampled in Ob and Yenisei overactivity zones, demonstrate distinct differences in the vertical radiocesium distribution. These differences have been shown to be due to many-year oscillations of suspended silt discharge, which are main transfer agents of solvable and poorly solvable radiocesium forms and to be independent of sedimentation conditions and the geochemical characteristics of the deposition environment.     

239+240Pu and 137Cs concentrations for zooplankton and nekton in the Northwest Pacific and Antarctic Oceans (1993-1996)

The concentrations of 239+240Pu and 137Cs in zooplankton and nekton in the Northwest Pacific and Southern Oceans were measured during the period 1993-1996. The object of the sampling was to assess the potential impacts of existing submerged anthropogenic-radioactive materials in the western North Pacific as well as the East China Sea. Samples from the Bransfield Strait of the Antarctic Ocean provided a control source impacted by only atmospheric bomb fallout. No particularly elevated levels of 239+240Pu were found in zooplankton samples from the Northwest Pacific, although significantly lower levels of 239+240Pu were found in three mixed zooplankton samples from the Bransfield Strait. The body burden of 239+240Pu in zooplankton appears to reflect concentrations in ambient seawater with some variation. Some additional measurements of 137Cs in fish are also reported here to complement existing databases and for future reference in the regional marine environmental radioactivity monitoring effort.     

Radiocesium reaction with illite and organic matter in marine sediment

The mineralogical effect on the (137)Cs reaction with marine sediment has not been systematically studied yet, even though illite has been known to adsorb Cs preferentially on its frayed edge sites in a low Cs concentration. Ninety-three marine sediment samples were collected near Yangnam, Korea for quantitative X-ray-diffraction (XRD), gamma-ray, and total organic carbon (TOC) analysis. Illite content was in the range of 0-23 wt.% and those of (137)Cs and TOC were minimum detectable activity (MDA) approximately 7.19 Bq/kg-dry and approximately 3.32%, respectively. The illite content in the marine sediment showed a good relationship with the (137)Cs content (R(2)=0.69), but with an increase in the illite content, the relationship became less linear. This trend can be clearly shown in two groups of samples with different size fractions (< and >5Mdvarphi). For the samples of larger particle sizes (low contents of illite), the relationship is linear, but for the samples of the smaller particle sizes (high illite content) it is less linear with a decreased slope, indicating that increase in illite content does not significantly contribute to the fixation of (137)Cs in marine sediment. Rather, the TOC has a more linear relationship with (137)Cs content with no slope change in all particle size ranges. This may indicate that humic materials in marine sediment block the access of (137)Cs to the frayed edge site and reduces the adsorption of (137)Cs on illite and that the organic materials in marine sediment play more important roles in adsorbing Cs than illite.     

Radionuclide ratios in wet and dry deposition samples from June 1976 through December 1977

²³⁸Pu,²³⁹Pu and¹³⁷Cs in rain and dry fallout and⁹⁰Sr in rain samples were measured at Woods Hole, Massachusetts, from June 1976 through December 1977. The dry fallout was estimated to be about 7.8% of the total deposition of²³⁹Pu and¹³⁷Cs.²³⁹Pu/¹³⁷Cs ratios, almost constant at about 0.011 in rain or dry fallout, February through December 1977, suggested that fractionation between the refractory and volatile radionuclides is insignificant in stratospheric fallout. This supports the idea of regional homogeneity of radionuclide ratios in fallout.     

Allochthonous subsidies of organic matter across a lake–river–fjord landscape in the Chilean Patagonia: Implications for marine zooplankton in inner fjord areas

Ecosystems can act as both sources and sinks of allochthonous nutrients and organic matter. In this sense, fjord ecosystems are a typical interface and buffer zone between freshwater systems, glaciated continents, and the coastal ocean. In order to evaluate the potential sources and composition of organic matter across fjord ecosystems, we characterized particulate organic matter along a lake–river–fjord corridor in the Chilean Patagonia using stable isotope (δ¹³C) and lipid (fatty acid composition) biomarker analyses. Furthermore, estimates of zooplankton carbon ingestion rates and measurements of δ¹³C and δ¹⁵N in zooplankton (copepods) were used to evaluate the implications of allochthonous subsidies for copepods inhabiting inner fjord areas. Our results showed that riverine freshwater flows contributed an important amount of dissolved silicon but, scarce nitrate and phosphate to the brackish surface layer of the fjord ecosystem. Isotopic signatures of particulate organic matter from lakes and rivers were distinct from their counterparts in oceanic influenced stations. Terrestrial allochthonous sources could support around 68–86% of the particulate organic carbon in the river plume and glacier melting areas, whereas fatty acid concentrations were maximal in the surface waters of the Pascua and Baker river plumes. Estimates of carbon ingestion rates and δ¹³C in copepods from the river plume areas indicated that terrestrial carbon could account for a significant percentage of the copepod body carbon (20–50%) during periods of food limitation. Particulate organic matter from the Pascua River showed a greater allochthonous contribution of terrigenous/vascular plant sources. Rivers may provide fjord ecosystems with allochthonous contributions from different sources because of the distinct vegetation coverage and land use along each river’s watershed. These observations have significant implications for the management of local riverine areas in the context of any human project that may modify terrestrial habitats as well as the productivity, food webs, and community structure of rivers, lakes, fjords, and the coastal ocean in the Chilean Patagonia.     

Pu and137Cs in coastal sediments

Analyses are presented of¹³⁷Cs,²³⁸Pu, and^239,240Pu, in relation to depth in sediment, in 21 gravity cores. These cores span the ranges of times 1964–1975, and of water depths 12–2000 m; they come from three distinct sedimentation areas off the northeast coast of the United States. Although the ranges of total sediment inventories of^239,240Pu and of¹³⁷Cs from the various areas hardly overlap, the range of ratios of the inventories of these two nuclides is probably the same in all the areas. In the shallow-water cores the^239,240Pu/¹³⁷Cs ratio regularly diminishes with depth in the core, and a tendency is seen for curves of this function to have similar slopes in each area; ratios of²³⁸Pu/^239,240Pu show no change with depth in these shallow-water cores. In the deeper-water cores, the^239,240Pu/¹³⁷Cs ratio shows no systematic change with depth, but sometimes the²³⁸Pu/^239,240Pu ratio shows a minimum at the sediment surface, and is much higher deeper in the cores. We believe that these phenomena can be explained in terms of a complicated bioturbational process moving the nuclides, together, down into the sediments, of chemical resolubilization, at depth, of plutonium only, and of its subsequent upward translocation in the interstitial solution. Some re-immobilization of plutonium near the sediment surface is implied, and a mechanism is suggested for this, based on displacement of plutonium from organic complexes by the increasing concentrations, in upper layers of the sediment, of re-oxidized dissolved iron.     

2.5ka来新疆吉力湖湖泊沉积记录的气候环境变化

选择位于西风区的吉力湖为研究对象,利用~(210)Pb、~(137)Cs和AMS~(14)C测年手段,建立了吉力湖沉积岩芯2.5ka以来的时间序列。对湖泊沉积物的粒度、总有机碳、总氮以及有机碳同位素等多环境指标的综合分析,重建了吉力湖2.5ka以来的气候环境演化特征。2.5ka以来吉力湖气候环境变化大致经历了5个阶段:500BC-50BC,暖干;50BC-650AD,冷湿,气候不稳定,冷暖波动较大;650-1350AD,暖干,对应于中世纪暖期(MWP),1350-1850AD,冷干,对应于小冰期(LIA);1850AD以来,温干,其中20世纪20年代后,尤其是70年代以来,气候变暖。吉力湖多环境指标记录的气候环境变化与其它地质记录以及历史文献记录均具有较好的一致性。     

137Cs湖泊沉积年代学方法应用的局限——以Crawford湖为例

＾１３７Ｃｓ湖泊沉积年代学方法是测定现代湖泊沉积物沉积年代和沉积速率的重要同位素年代学方法之一。对加拿大Ｃｒａｗｆｏｒｄ湖采集的沉积孔柱内＾１３７Ｃｓ垂直分布的研究发现,该方法给出时的标有明显偏差。比较＾２１０Ｐｂ和纹层等年代方法的结果,其１９６３年时标蓄积峰值所在位置明显移向表层,而作为１９５４年时标的该核素出现蓄积的层位则远早于该年沉积物蓄积层位。研究还表明,孔柱中较高的间隙水含量、缺少足以吸     

Anthropogenic Radionuclides in the Caspian Sea

Analysis and interpretation of the distribution of anthropogenic radionuclides ⁹⁰Sr, ¹³⁷Cs, and ^239,240Pu in the Caspian Sea water are presented. These radionuclides are shown to be of environmental importance and to be useful for studying water mass dynamics.     

The accumulation of radiocesium in coarse marine sediment: effects of mineralogy and organic matter

The controlling factors affecting the accumulation of (137)Cs in marine sediment have not been investigated in detail, especially in coarse grained sediment. Eighty eight coarse marine sediment samples near Wuljin, Korea, were characterized by quantitative X-ray-diffraction (XRD), gamma-ray, and total organic carbon (TOC) analysis. Those factors were then compared. The grain size was in the range of -0.48 to 3.6Mdphi corresponding to sand grains. TOC content was in the range of 0.06-1.75%, and the concentration of (137)Cs was 相似文献   

Variability of natural and bomb-produced radionuclide distributions in abyssal red clay sediments

The nature of sedimentation and mixing are examined in abyssal red clay sediments from the North Central Pacific using three types of indicators: ²³⁰Th/²³²Th, organic¹⁴C, and¹³⁷Cs and ^239.240Pu.²³⁰Th/²³²Th analysed revealed that the clay sedimentation rate in three box cores collected within a 50 km radius was less than 1.0 mm/10³ yr. However, analyses of the organic carbon in thin layers of sediment revealed that radiocarbon was present much deeper in the cores (down to 20 cm) than was expected from the ²³⁰Th/²³²Th distribution. In addition, both the stratigraphy and inventory of radiocarbon was significantly different between box cores. The distributions and inventories of¹³⁷Cs and^239.240Pu were similar to that found for radiocarbon, further illustrating the spatial variability of radionuclides in oligotrophic North Pacific red clays. These data suggest that bioturbational processes are important for transporting organic carbon down into the sediment column.     

Distribution and content of different artifical radio nuclides in the water of the North Sea during the years 1977 to 1981 (complemented with some results from 1982 to 1984)

Summary The measured concentrations of¹³⁷Cs in the water of the North Sea gained during the years 1977 to 1982 largely confirm the results found in the preceding years (Fig. 1). After a distinct maximum in 1978 — brought about by a particularly strong influx during 1977 — the total quantity of¹³⁷Cs present in the North Sea has reced, to around half of these peak values by the year 1982 (Table 1).On the way from the Sellafield Works near the Irish Sea as far as into the North Sea, a strong shift of the¹³⁷Cs:⁹⁰Sr ratio in favour of the⁹⁰Sr can be observed.By following the temporal course of that ratio at different measurement points, a transport time can be deduced of around 3 years between the Sellafield Works and the Pentland Firth; a further year would be needed to reach into the southeastern North Sea.The ratio Cs:Sr furthermore permits, in the southeastern North Sea, a good distinction between the watermasses comming from the north into the North Sea with respect to those that come through the Channel from the South. These masses practically flow side by side until about the entrance to the Skagerrak.The vertical distribution of the¹³⁷Cs shows, as is to be expected, seasonally conditioned differences. However, effects also occur, which — on the basis of the data available to date — do not yet permit a clear explanation.The⁹⁰Sr, as well as the^239+240Pu, present in the North Sea show an analogous distribution scheme compared with that of the¹³⁷Cs. Their concentrations lie far below that of the¹³⁷Cs (⁹⁰Sr 17.5%;^239+240Pu 0.03%).Tritium, on the other hand — with essentially higher concentrations — shows a completely different distribution, because it is principly introduced via the freshwater flowing in from the land.

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Verteilung und Gehalt verschiedener künstlicher Radionuklide im Wasser der Nordsee in den Jahren 1977 bis 1981 (ergänzt durch einige Ergebnisse von 1982 bis 1984)

Zusammenfassung Die in den Jahren 1977 bis 1982 gewonnenen Meßdaten der Aktivitätskonzentrationen von¹³⁷Cs im Wasser der Nordsee bestätigen weitgehend die in den vorhergehenden Jahren gefundenen Ergebnisse (Fig. 1) Nach einem deutlichen Maximum im Jahre 1978 — hervorgerufen durch eine besonders starke Zufuhr im Jahre 1977 —ist die in der Nordsee insgesamt vorhandene Menge an¹³⁷Cs bis zum Jahre 1982 wieder auf rund die Hälfte zurückgegangen (Tab. 1).Auf dem Weg von den Sellafield Works an der Irischen See bis in die Nordsee ist eine starke Verschiebung des¹³⁷Cs:⁹⁰Sr Verhältnisses zugunsten des⁹⁰Sr zu beobachten.Aus dem zeitlichen Verlauf dieses Verhältnisses an verschiedenen Meßpunkten ergeben sich Transportzeiten zwischen den Sellafield Works und dem Pentland Firth von rund 3 Jahren; bis in die südöstliche Nordsee wird ein weiteres Jahr benötigt.Das Verhältnis Cs:Sr erlaubt außerdem in der südöstlichen Nordsee eine gute Unterscheidung der aus der Nordsee bzw. durch den Kanal von Süden kommenden Wassermassen, die praktisch nebeneinander her bis etwa zum Beginn des Skagerraks fließen.Die Vertikalverteilung des¹³⁷Cs zeigt, wie zu erwarten ist, jahreszeitlich bedingte Unterschiede. Es treten aber auch Effekte auf, die sich anhand der bisher vorliegenden Daten noch nicht eindeutig erklären lassen.Das in der Nordsee vorhandene⁹⁰Sr sowie das^239+240Pu zeigen ein analoges Verteilungsschema verglichen mit dem des¹³⁷Cs. Ihre Konzentrationen liegen weit unter der des¹³⁷Cs (⁹⁰Sr 17,5%,^239+240Pu 0,03%).Das Tritium zeigt bei wesentlich höheren Konzentrationen dagegen eine völlig andere Verteilung, da seine Hauptzufuhr im wesentlichen über das von Land her zufließende Süßwasser erfolgt.

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Distribution et teneur de differents radionucleides artificiels, dans les eaux de la Mer du Nord entre les années 1977 et 1981 (completes par quelques résultats de 1982 à 1984)

Résumé Les mesures de concentration du Césium 137 dans les eaux de la Mer du Nord, acquises entre les années 1977 et 1982, confirment largement les résultats obtenus au cours des années précédentes. Après un net maximum en 1978 — occassionné par un apport particulièrement fort en 1977 — la quantité totale de Césium 137 présent en Mer du Nord a régressé,jusqu'en 1982, aux alentours de la moitié de ces valeurs maximales.Il a pu être observé une modification importante du rapport Césium 137/Strontium 90, en faveur du Strontium 90, sur le trajet de Sellafield Works prés de la Mer d'Irlande jusqu'à la Mer du Nord.En suivant l'évolution temporelle de la valuer de ce rapport en différents points de mesure, on peut en déduire une durée de transport d'environ 3 ans entre Sellafield Works et Pentland Firth; une année supplémentaire est ensuite nécessaire pour pénétrer en Mer du Nord Sud-orientale.En Mer du Nord Sud-orientale, le rapport Césium/Strontium permet en outre d'effectuer une nette distinction entre les masses d'eau pénétrant respectivement par le Nord dans la Mer du Nord et celles pénétrant par le Sud et venant de la Manche. Ces masses d'eau s'écoulent pratiquement côte à côte jusqu'à l'entrée du Skagerrak.Comme l'on pouvait s'y attendre, la distribution verticale du Césium est différente suivant les saisons. Cependant il apparaît également des effects qui, sur la base des données disponibles à ce jour, ne s'expliquent pas encore clairement.Le Strontium 90 aussi bien que le Plutonium 239+240 présent dans la Mer du Nord, montrent une distribution comparable, analogue à celle du Césium 137. Leurs concentrations sont bien inférieures à celle du Césium 137 (Strontium 90 17,5%; Plutonium 239+240 0,03%).Le tritium d'autre part, — avec des concentrations significativement plus fortes —montre une distribution complètement différente, due principalement au fait qu'il est introduit par l'intermédiaire de l'écoulement d'eau douce provenant de la terre.

     

Plutonium,radiocesium and radiocobalt in sediments of the Hudson River estuary

Anthropogenic radionuclides have reached the Hudson estuary as global fallout from nuclear weapons testing and through local releases from commercial nuclear reactors. Significant activities of²³⁸Pu and^239,240Pu (fallout-derived),¹³⁴Cs and⁶⁰Co (reactor-released), and¹³⁷Cs (derived from both sources), have accumulated in the sediments throughout the estuary, with the primary zone of accumulation near the downstream end of the system in New York harbor. The estuary appears to have trapped nearly all of the^239,240Pu delivered as fallout, and consequently, ocean dumping of dredged harbor sediment is currently the primary means for the net transport of these nuclides to coastal waters. In contrast, only 10–30% of the¹³⁷Cs,¹³⁴Cs and⁶⁰Co delivered to the estuary have been retained on the fine particles which accumulate at a rapid rate in the harbor.The primary factors which have governed the distribution of anthropogenic radionuclides in Hudson sediments are: (1) spread of fine particles labeled with both fallout and reactor nuclides throughout the axis of the estuary, (2) differences in timing of the peak fallout years (1962–1964) and years of maximum reactor releases (1971–1972), (3) large variations in sediment accumulation rates, ranging from a few millimeters per year or less to many tens of centimeters per year, (4) appreciable desorption of¹³⁷Cs and¹³⁴Cs from particles at higher salinities, and (5) possible enhanced desorption of⁶⁰Co at higher salinities (relative to¹³⁴Cs and¹³⁷Cs) which may be associated with the release of reduced manganese from the harbor sediments.