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1.
This paper presents samples of Saharan dust outbreak affecting the Mediterranean Tunisian coasts and its impact on PM10 (Particles with an aerodynamic diameter below 10 µm) surface concentrations measured at seven monitoring stations during summer 2006. During the events, the daily PM10 levels at all stations exceeded EU and Tunisian air quality standard limits which are equal to 50 µg/m3. The maximum values ranged from 200 µg/m3 to 300 µg/m3 depending on the monitoring station. The impact is even more dramatic on PM10 hourly concentrations leading to maximum hourly peaks ranging from 400 µg/m3 to 850 µg/m3 again depending on the monitoring station (industrial or residential, traffic and commercial). Comparison between backward air masses trajectories reaching Tunisian coasts and satellite imageries vis-à-vis the PM10 hourly concentrations measured at the monitoring stations during 2006 evidenced the influence of the Saharan dust outbreaks on surface concentrations. The origin of the air masses is found to be from South-West direction under the influence of air masses from the Algerian Saharan desert.  相似文献   

2.
The average composition and seasonal variations of atmospheric organic particulates with respect to n-alkanes, n-alkanoic acid, polycyclic aromatic hydrocarbon (PAHs), and nitrated polycyclic aromatic hydrocarbons (N-PAHs) were determined at the biggest municipal waste landfill in Algeria located in Oued Smar, 13 km east of downtown Algiers. Samplings were carried out from August 2002 to February 2003, and organic compounds adsorbed in air particles having an aerodynamic diameter lower than 10 μm (PM10) were characterized using gas chromatography coupled with mass spectrometric detection (GC/MSD). Total concentrations ranged from 828 to 11,068 ng per cubic meter of air for n-alkanes, from 1714 to 21,710 ng per cubic meter of air for n-alkanoic acids, from 13 to 212 ng per cubic meter of air for PAHs and from 93 to 205 pg per cubic meter of air for N-PAHs. n-Alkanoic acids accounted for 85 and 56% of the total organic composition of the aerosol measured in summer and winter, respectively, were the biggest fraction. The distribution profiles and the diagnostic ratios of some marker compounds allowed to identify the combustion and microbial activity as the major sources of particulate organic pollutants associated with direct emission. The year-time dependence of organic fraction content of aerosol in Oued Smar appeared to be related to average meteorological conditions as well as variability of rate and nature of materials wasted into the landfill.  相似文献   

3.
GPS-synchronized measurements of electric (E) field changes induced by lightning flashes were recorded at six stations in the northeastern verge of the Tibetan Plateau. The height and magnitude of charge neutralized by 65 return strokes, including 16 negative cloud-to-ground (CG) flashes and 2 positive CG flashes, have been fitted with the nonlinear least-square method based on the E field changes of CG flashes observed in a typical thunderstorm with larger-than-usual lower positive charge center (LPCC). Results show that the height of the charge region neutralized by negative CG flashes ranges from 3 km to 5 km above the ground, corresponding to an ambient temperature between − 2 °C and − 15 °C. For the two positive CG flashes, the neutralized charge regions are located at a height of about 5.5 km and the ambient temperature is about − 18 °C, indicating the existence of upper positive charge in the thunderstorm.  相似文献   

4.
Observational study of surface ozone at an urban site in East China   总被引:4,自引:1,他引:3  
In this study, we present the observational data of near surface ozone and some meteorological parameters during 2004, at an urban site (36°42′ N, 117°08′ E, 34.5 m a.s.l.) of Jinan, China. Hourly ozone concentrations exceeding the standard value of China, 100 ppbv, were observed for 65 h (in 23 days) from April to October, and values exceeding US NAAQS (National Ambient Air Quality Standard) for 1 h ozone, 120 ppbv, were observed for 15 h (in 7 days) from late May to early July. Ozone formation presented the phenomenon of “weekend effect”, especially in summer. Monthly variation of ozone coincided with temperature except for July and August. The low ozone levels in July and August may be due to the short sunshine duration and much rainfall during this period. Among these meteorological parameters, daily averaged ozone shows a significant correlation with temperature (r = 0.66) in the year and with relative humidity (r = − 0.75) in summer. Throughout the year, high ozone concentrations were mainly associated with the wind from 180 to 247.5°, while high ozone concentration seemed to have no obvious correlation with a given wind direction in summer. An anomalous nocturnal high ozone episode during 23–25 May 2004 was investigated. Growth fractions of ozone during the nighttime episode were 62.2% and 71.1% for 23 and 24 May, respectively. Synoptic analysis shows that favorable synoptic condition had presumably elevated the background ozone level in this region. Backward trajectory analysis shows that the increase of ozone concentration and the relatively constant high ozone concentrations during the night of May 23 might originate from the transport of ozone rich air mass above boundary layer. Transport of ozone from Yangtze Delta and East Central China might be a significant process for the high ozone level during night May 24 at Jinan.  相似文献   

5.
Data from the Antarctic winter at Halley Base have been used in order to evaluate qualitatively and quantitatively how the stratification in the low atmosphere (evaluated with the gradient Richardson number, Ri) influences the eddy transfers of heat and momentum. Vertical profiles of wind and temperature up to 32 m, and turbulent fluxes ( , and ) measured from three ultrasonic thermo-anemometers installed at 5, 17 and 32 m are employed to calculate Ri, the friction velocity (u *) and the eddy diffusivities for heat (K h ) and momentum (K m ). The results show a big dependence of stability onK m ,K h andu *, with a sharp decrease of these turbulent parameters with increasing stability. The ratio of eddy diffusivities (K h /K m ) is also analyzed and presents a decreasing tendency as Ri increases, reaching values even less than 1, i.e., there were situations where the turbulent transfer of momentum was greater than that of heat. Possible mechanisms of turbulent mixing are discussed.  相似文献   

6.
Automobile exhaust emissions are becoming increasingly serious with the drastic increase of the number of vehicles in Beijing. In order to investigate the air pollution level and characteristics in the areas near the main traffic lines in Beijing and to identify the contributions from traffic and other sources, gaseous pollutants including NOx, CO, O3, SO2, and meteorological parameters have been monitored at a monitoring site and a contrasting site in winter and summer in 2006. The volumes of vehicles on Beiyuan Road were recorded. The average concentrations of NO, NO2, NOx, CO, O3, and SO2 at the monitoring site were 0.148 mg/m3, 0.107 mg/m3, 0.333 mg/m3, 5.110 mg/m3, 0.006 mg/m3, and 0.157 mg/m3, respectively during the sampling period in winter and 0.021 mg/m3, 0.068 mg/m3, 0.101 mg/m3, 4.170 mg/m3, 0.083 mg/m3, and 0.056 mg/m3, respectively in summer. The high concentrations of CO and O3 reflect the influence of vehicles emission near the traffic lines evidently. The higher concentrations of CO, NO and O3 in summer may indicate that the characteristics of traffic pollution were more pronounced in summer. Results of regression analysis showed that in winter the concentrations of SO2 and CO were significantly positively correlated with the emission of heating boilers at night and negatively correlated with wind speed in daytime. The concentrations of NO and NOx were negatively correlated with wind speed, positively correlated with emission of heating boilers in daytime and positively correlated with traffic density at nighttime. The concentrations of NO2 were positively correlated with the emission of heating boilers in daytime and traffic density at nighttime. In summer, the air quality at the monitoring site and the contrasting site was mainly influenced by the traffic emissions.  相似文献   

7.
In the Atacama Desert, the narrow littoral plain and the adjacent mountain range have a unique climate. This area is locally called the “coastal desert with abundant cloudiness”, and extends from the coastline up to an elevation of 1000 m. The climate is designated as being BWn according to Köppen's Climate Classification as adapted for Chile. In the original classification the acronym (Bn) is used for foggy environments. Toward the east a “normal desert” climate (BW) is found. This is known as one of the most extreme deserts of the world. In the BWn areas there are meteorological differences between low and high elevation zones. The climate of the coastal plains and the mountains is described in this paper in order to show that there is an area where the climate differs from those classified as BWn and BW in the Chilean Climate Classification. This area is located between 650 and 1200 m a.s.l. and contains several fog oases or lomas vegetation, rich in biodiversity and endemism.The weather is warmer near sea level, with an annual average temperature of 18 °C. At high elevation sites like Alto Patache, the temperature decreases at a rate of 0.7 °C for every 100-m increase in altitude. The average annual minimum temperature often approaches 1 °C in winter, while the mean annual temperature range is significant (8.3 °C in Los Cóndores). The mean monthly relative humidity in Alto Patache is over 80%, except during the summer months. During autumn, winter and spring high elevation fog is present in the study area at altitudes ranging from 650 m up to 1060 m, giving annual water yields of 0.8 to 7 L m− 2 day− 1. If vegetation is used as an indicator, the foggy zone lies between 650 m a.s.l. and 1200 m a.s.l. About 70% of the mountain range experiences the foggy climate, as opposed to the coastal plains that are characterized by a cloudy climate.  相似文献   

8.
Influence of drizzle on ZM relationships in warm clouds   总被引:1,自引:0,他引:1  
This paper addresses the sensitivity of the relationships between radar reflectivity (Z) and liquid water content (M) for liquid water clouds to microphysical drizzle parameters by means of simulated radar observation at a frequency of 3 GHz of modeled cumulus clouds. A power law relationship for non drizzling clouds with water content as high as 3 gm− 3: Zc = 0.026 Mc1.61 is numerically derived and agreed with previous empirical relationships relative to cumulus and stratocumulus. This relationship is then used to explore the influence of drizzle on the correlation between radar reflectively and water content. Due to their large diameters with respect to cloud droplets, drizzle sized drops dominate radar reflectivity but do not carry the cloud water content so that reflectivity and liquid water content are expected to be not correlated in clouds containing drizzle. It is shown that for congestus or extreme congestus cumuli, microphysical conditions for which the ZcMc relationship can be used with a tolerance of 5 and 10% are provided whereas for humilis or mediocris cumuli, the presence of drizzle breaks down the ZcMc relationship whatever the situations.  相似文献   

9.
To project potential habitat changes of 57 fish species under global warming, their suitable thermal habitat at 764 stream gaging stations in the contiguous United States was studied. Global warming was specified by air temperature increases projected by the Canadian Centre of Climate Modelling General Circulation Model for a doubling of atmospheric CO2. The aquatic thermal regime at each gaging station was related to air temperature using a nonlinear stream temperature/air temperature relationship.Suitable fish thermal habitat was assumed to be constrained by both maximum temperature and minimum temperature tolerances. For cold water fishes with a 0 °C lower temperature constraint, the number of stations with suitable thermal habitat under a 2×CO2 climate scenario is projected to decrease by 36%, and for cool water fishes by 15%. These changes are associated with a northward shift of the range. For warm water fishes with a 2 °C lower temperature constraint, the potential number of stations with suitable thermal habitat is projected to increase by 31%.  相似文献   

10.
Heterogeneous nucleation of supersaturated n-nonane vapour on seed particles of different size and composition has been investigated using a fast expansion chamber. Monodisperse seed particle sizes were ranging from about 4 nm up to about 24 nm in diameter. By using different types of particle generators WOx, Ag and (NH4)2SO4 particles were generated. For direct comparison between different particle compositions overlapping sizes have been generated for WOx and Ag at about 7 nm particle diameter as well as for Ag and (NH4)2SO4 at about 15 nm. Nucleation temperature was kept constant at about 278 K. Experimental data were compared to Kelvin equation and Fletcher theory including the effect of line tension. It was found that heterogeneous nucleation of n-nonane seems to be independent of seed particle composition and starts well below the Kelvin curve. Good agreement was achieved with Fletcher theory including the effect of line tension.  相似文献   

11.
The forest water balance has never been studied in Reunion Island (Indian Ocean). This study focuses on the interception of fog water by Sophora denudata, an endemic tree, which provides an important water input into the hydrologic budget of the upper-montane forest. Canopy throughfall, rainfall and fog have been compared. The first data were obtained in 2001 in Nez de Bœuf, 2040 m asl, from manual rain gauges. The measurements were made during the day only. The aim was to propose a typology of events, to understand the spatial pattern of canopy throughfall, especially fogdrip, and their relation to the trade-wind direction. A second series of experiments, carried out in 2004 in Piton de Tangues, 2150 m asl, investigated how throughfall and atmospheric water varied with time, using automatic instruments such as the shielded Grunow-type fog collector. Here measurements were made continuously and night data were not excluded. Over a period of 8 months, the throughfall gauges, which were placed under the trees, indicated 1180 mm whereas the total amount of rainfall had reached only 948 mm. The difference (232 mm) is attributed to fog. Of 278 events, 234 showed fog contribution; fog occurred alone in 167 cases. The observations confirm what was found in Nez de Bœuf, namely that fog or rain can occur separately or together. The role of fog contribution to the forest water budget is significant: the spatial variation of canopy throughfall does not only depend on the type of event, but also on wind direction.  相似文献   

12.
The measurements of the photosynthetic photon flux density (Qp) and other solar components have been in Beijing for 2-year period. The Qp, broadband solar radiation (Rs) and the PAR fraction (Qp / Rs) showed similar seasonal features that peaked in value during the Summer and reached their lowest value during the Winter. The PAR fraction ranged from 1.68 E M J− 1 (Winter) to 1.98 E M J− 1 (Summer) with an annual mean value of 1.83 E M J− 1. The analysis of the hourly values also revealed a diurnal pattern, with higher values of Qp and Rs being observed around noon. The PAR fraction increased from 1.78 to 1.89 μE J− 1 (hourly values), as the sky conditions changed from clear to cloudy. The monthly mean hourly PAR fraction also revealed a diurnal variation, however, with lower values being observed around noon during most months. In November, the diurnal variations showed an opposite feature in comparison with other months. This is mainly attributed to the diurnal variations in the water vapor concentration.Two models were developed to estimate Qp from Rs. The models consisted of atmospheric parameters that were found to cause substantial changes to the PAR fraction, such as sky clearness, brightness and path length. The estimated Qp obtained via different equations was much closer to the observed values, with relative errors below 20% in Beijing. The Qp and Rs data collected at three stations with featuring different climate types from within Beijing were used for verifying the transferability of the models. The correlation coefficients between the measured and estimated Qp values decreased at these stations, and the relative error increased. This indicates that the estimation models need to be modified accordingly for the local climatic conditions.  相似文献   

13.
Turbulent dispersion of spores was studied near a source located inside a wheat canopy. Two colors of Lycopodium spores were released simultaneously at a steady rate from line sources at two heights (0.4–0.5 m and 0.7–0.8 m) in a 0.8 to 1.0 m tall crop. The number of spores of each color released was estimated by weighing the sources before and after each release. Aerial spore concentrations were measured at 2 and 4 m downwind of the sources using rotorods placed at four heights above the canopy and small suction traps at two heights inside the canopy. Concentrations near the ground were estimated from deposits on sticky glass microscope slides placed on the ground. Experiments were conducted on six different days. Friction velocities ranged from about 0.3 to 0.5 m s–1. The average horizontal fluxes of spores were calculated as the product of the observed concentrations and average wind speeds. At a distance of 2 m downwind from the sources, more than 16 to 44% of the flux of spores released from the lower source and more than 41 to 50% of the flux of spores released from the upper source were estimated to be above the canopy. These fluxes were compared with fluxes calculated using both a K-theory model and a random-flight-fluid-parcel-trajectory simulation model. The fluxes predicted by the models were generally considerably less than the values determined experimentally.  相似文献   

14.
Measuring of charged nanometer particles in atmospheric air is a routine task in research on atmospheric electricity, where these particles are called the atmospheric ions. An aspiration condenser is the most popular instrument for measuring atmospheric ions. Continuous scanning of a mobility distribution is possible when the aspiration condenser is connected as an arm of a balanced bridge. Transfer function of an aspiration condenser is calculated according to the measurements of geometric dimensions, air flow rate, driving voltage, and electric current. The most complicated phase of the calibration is the estimation of the inlet loss of ions due to the Brownian deposition. The available models of ion deposition on the protective inlet screen and the inlet control electrofilter have the uncertainty of about 20%. To keep the uncertainty of measurements low the adsorption should not exceed a few tens of percent. The online conversion of the mobility distribution to the size distribution and a correct reduction of inlet losses are possible when air temperature and pressure are measured simultaneously with the mobility distribution. Two instruments called the Balanced Scanning Mobility Analyzers (BSMA) were manufactured and tested in routine atmospheric measurements. The concentration of atmospheric ions of the size of about a few nanometers is very low and a high air flow rate is required to collect enough of ion current. The air flow of 52 l/s exceeds the air flow in usual aerosol instruments by 2–3 orders of magnitude. The high flow rate reduces the time of ion passage to 60 ms and the heating of air in an analyzer to 0.2 K, which suppresses a possible transformation of ions inside the instrument. The mobility range of the BSMA of 0.032–3.2 cm2 V− 1 s− 1 is logarithmically uniformly divided into 16 fractions. The size distribution is presented by 12 fractions in the diameter range of 0.4–7.5 nm. The measurement noise of a fraction concentration is typically about 5 cm− 3 and the time resolution is about 10 min when measuring simultaneously both positive and negative ions in atmospheric air.  相似文献   

15.
Correlation methods in fingerprint detection studies   总被引:2,自引:0,他引:2  
This investigation addresses two general issues regarding the role of pattern similarity statistics in greenhouse warming detection studies: normalization, and the relative merits of centered versus uncentered statistics. A pattern correlation statistic is used to search for the greenhouse warming signals predicted by five different models in the observed records of land and ocean surface temperature changes. Two forms of this statistic were computed: R (t), which makes use of nonnormalized data, and (t), which employs point-wise normalized data in order to focus the search on regions where the signal-to-noise ratio is large. While there are no trends in the R (t) time series, the time series of (t) show large positive trends. However, it is not possible to infer from the (t) results that the observed pattern of temperature change is, in fact, becoming increasingly similar to the model-predicted signal. This is because point-wise normalization of the observed and simulated mean change fields by a single common field introduces a common factor effect, which means that the quantities being compared should show some similarity a priori. This does not necessarily make normalization inapplicable, because the detection test involves seeking a trend in the similarity statistic. We show, however, that trends in (t) must arise almost completely from the observed data, and cannot be an indicator of increasing observed data/signal similarity. We also compare the information provided by centered statistics such as R(t) and the uncentered C(t) statistic introduced by Barnett. We show that C(t) may be expressed as the weighted sum of two terms, one proportional to R(t) and the other proportional to the observed spatial mean. For near-surface temperatures, the spatial average term dominates over the R(t) term. In this case the use of C(t) is equivalent to the use of spatial-mean temperature. We conclude that at present, the most informative pattern correlation statistic for detection purposes is R(t), the standard product-moment correlation coefficient between the observed and model fields. Our failure to find meaningful trends in R(t) may be due to the fact that the signal is being obscured by the background noise of natural variability, and/or because of incorrect model signals or sensitivities.  相似文献   

16.
杨舵  王淑民  桑修诚 《气象》2000,26(4):29-32
根据乌鲁木齐市1994~1997年SO2浓度和气象监测资料,分析了SO2浓度的时空分布特征及其可能原因,并对各监测点SO2 污染等级作出了评价。  相似文献   

17.
本文利用2014年全年北京市12个空气质量监测站的逐小时PM_(2.5)地面观测资料,以及Terra卫星和Aqua卫星的MODIS 3 km气溶胶光学厚度(AOD)产品,分析了地面PM_(2.5)和两颗卫星AOD的时空分布特征,并在时空匹配的基础上,建立了AOD与PM_(2.5)浓度之间的回归模型。结果表明:PM_(2.5)浓度在城区高、郊区低,最低值位于定陵站,城区站和郊区站的逐时PM_(2.5)浓度的日变化分别呈"双峰型"和"单峰型";两颗卫星AOD数值也均是城区高、郊区低,沿山区的边界有明显的AOD梯度,且城区上午Terra卫星的AOD高于下午Aqua卫星的AOD,而郊区上、下午的AOD基本相同;Aqua卫星AOD与PM_(2.5)的确定系数(R2)较Terra卫星AOD与PM_(2.5)的确定系数平均高0.11,且城区站点两颗卫星AOD与PM_(2.5)相关性均较郊区站点AOD与PM_(2.5)相关性偏高;综合来看,Aqua卫星的AOD与城区的PM_(2.5)相关系数最高,即Aqua卫星的AOD更适于监测和反演城区地面的PM_(2.5)。  相似文献   

18.
The study of fog dynamics in the island of Tenerife began in 1993 at six sites. The analysis of the relationship between fog and several meteorological parameters was conducted at the site located at Anaga. Anaga is located at the summit of a mountain range, at an altitude of 842 m and 3.5 km away from the north-western coastline of the island. The study uses hourly data of the three summer months (June, July and August) that were collected over a period of nine years — from 1996 to 2005. The mean summer (June–August) rainfall was found to be 21.2 mm whilst the total volume of fog water collected was 879.9 l m− 2; the daily average fog water collection was 9.5 l m− 2 day− 1, and the hourly average about 0.4 l m− 2 h− 1. Although these amounts were recorded with wind speeds of between 8 and 12 m s− 1, the correlation between water collected and wind speed is not statistically significant. In spite of this, the volume of fog water collected and wind speed showed a very distinct daily behavioural pattern, their frequency and speed reaching their minimum at 12 a.m. and their maximum from 7 p.m. to 8 a.m. GMT. The importance of this research is that it shows that the fog in the Canary Islands occurs more frequently and makes a more significant contribution to the growth of vegetation in the summer (the dry season) than in the winter, when fog accompanies rainfall.  相似文献   

19.
Ion mobility spectrometry offers a robust and effective technique to study ion clusters in ambient conditions. Here, we have experimentally studied the influence of temperature on the positive ion cluster formation of 2-propanol vapor in air, along with parallel measurements for n-butyl acetate vapor in air. For both of these low proton affinity compounds in the ppm concentration range, temperatures below 0 °C tend to favor formation of dimers and trimers. The measurements indicate that approximate estimations for the fractions of these n-mers (n > 1) in the ion spectra, can be obtained by classical theory for ion induced nucleation. Presence of natural background vapors however slightly blurs the data, especially for the fraction of monomers, so that accurate prediction of the fractions of n-mers in the spectra would require more accurate information on the gas composition. The findings concerning thermal behavior of ions help to understand better ion phenomena also in field conditions.  相似文献   

20.
Esmaiel Malek   《Atmospheric Research》2008,88(3-4):367-380
An automated-ventilated radiation station has been set up in a mountainous valley at the Logan Airport in northern Utah, USA, since mid-1995, to evaluate the daily and annual radiation budget components, and develop an algorithm to study cloudiness and its contribution to the daily and annual radiation. This radiation station (composed of pyranometers, pyrgeometers and a net radiometer) provides continuous measurements of downward and upward shortwave, longwave and net radiation throughout the year. The surface temperature and pressure, the 2-m air temperature and humidity, precipitation, and wind at this station were also measured. A heated rain gauge provided precipitation information. Using air temperature and moisture and measured downward longwave (atmospheric) radiation, appropriate formula (among four approaches) was chosen for computation of cloudless-skies atmospheric emissivity. Considering the additional longwave radiation during the cloudy skies coming from the cloud in the waveband which the gaseous emission lacks (from 8–13 μm), an algorithm was developed which provides continuous 20-min cloud information (cloud base height, cloud base temperature, percent of skies covered by cloud, and cloud contribution to the radiation budget) over the area during day and night. On the partly-cloudy day of 3 February, 2003, for instance, cloud contributed 1.34 MJ m− 2 d− 1 out of 26.92 MJ m− 2 d− 1 to the daily atmospheric radiation. On the overcast day of 18 December, 2003, this contribution was 5.77 MJ m− 2 d− 1 out of 29.38 MJ m− 2 d− 1. The same contribution for the year 2003 amounted to 402.85 MJ m− 2 y− 1 out of 9976.08 MJ m− 2 y− 1. Observations (fog which yielded a zero cloud base height and satellite cloud imaging data) throughout the year confirmed the validity of the computed data. The nearby Bowen ratio station provided the downward radiation and net radiation data. If necessary, these data could be substituted for the missing data at the radiation station. While the automated surface observing systems (ASOS) ceilometer at the Logan airport provides only the overhead cloud information, the proposed algorithm provides this information over the valley. The proposed algorithm is a promising approach for evaluation of the cloud base temperature, cloud base height, percent of skies covered by cloud, and cloud contribution to the daily and annual radiation budget at local and regional scales.  相似文献   

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