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1.
This paper presents the results of a 6-year (1998–2003) survey of trace toxics in the intertidal mussel Perna viridis conducted by the Hong Kong Environmental Protection Department. Concentrations of heavy metals and trace organics were measured in the soft bodies of P. viridis collected from five sites in Hong Kong waters, i.e. Wu Kai Sha (Tolo Harbour), Ma Wan (Northwest), Tsim Sha Tsui (Victoria Harbour), Tai Tam (Hong Kong South) and Lamma Island (Southern Waters) in order to establish the spatial patterns of contaminants in mussels. Among the metals analysed, Cd showed a significant concentration gradient in Hong Kong waters. The levels of Cd in P. viridis were significantly higher at Ma Wan as compared to the other sites studied. Ma Wan also had relatively higher concentrations of Pb. Mn concentrations were particularly prominent at Wu Kai Sha. Significantly higher concentrations of Hg and Cu were recorded at Tai Tam and Tsim Sha Tsui. Tai Tam and Wu Kai Sha had higher levels of V; whereas higher Ni concentrations were recorded at Lamma Island and Tai Tam. No clear spatial patterns for Al, As, Cr, Fe and Zn were observed.Higher concentrations of PAHs in P. viridis were observed around urban centres impacted by sewage discharges (e.g. Tsim Sha Tsui); whereas higher PCB levels were found not only in Tsim Sha Tsui but also in less urbanised areas such as Lamma Island and Tai Tam, suggesting that these may be due to non-sewage related inputs. The study also shows that Northwest and Southern waters are subject to a higher degree of DDT pollution compared with other sites. Of the 17 dioxin compounds analysed, positive data were mostly recorded for two compounds which are of low toxicity (i.e. OCDD and 1,2,3,4,6,7,8-HpCDD) whereas the most toxic congeners (i.e. 2,3,7,8-TCDD and 1,2,3,7,8-PeCDD) were not detected in the 6 years of monitoring. In general, the levels of OCDD in P. viridis were found to be higher in Tai Tam and Lamma Island in Southern Waters of Hong Kong.This study found that the levels of some highly toxic heavy metals (i.e. Cd, Hg and Pb) in the mussel P. viridis did not exceed the recommended limits for shellfish as food in Hong Kong (i.e. Cd: 2.0 ppm; Hg: 0.5 ppm; Pb: 6.0 ppm wet weight). The levels of As and Ni in P. viridis were also well below the action limits set by the US FDA (i.e. As: 86 ppm; Ni: 80 ppm wet weight). DDT and PCB contaminations in P. viridis were below the concentrations of concern. Compared with data obtained in the 1980s, the current levels of DDTs in P. viridis were 4–16 times lower; whereas Pb concentrations recorded in Tsim Sha Tsui have also been lowered significantly. This is mainly related to reduction in local and regional pollution sources in the past 20 years.  相似文献   

2.
The Western Scheldt river and estuary is known to be highly polluted as it receives industrial, agricultural and domestic effluents from one of the most populated and industrialised zones in Europe. Aquatic organisms are exposed to pollutants, specifically metals that are present in different environmental phases, e.g. dissolved, suspended material or sediment phases. The objective of this study was to study the relationship that exists between environmental metal levels, the degree of metal uptake by aquatic organisms with the concomitant biological responses. For this purpose the bivalve mollusk, Mytilus edulis, was selected as bioaccumulation indicator organism. Environmental (water and sediment) and mussel samples were collected during the late winter (March 2000) from sampling sites in the Scheldt estuary. Sites were selected to represent a salinity gradient from the mouth of the estuary to the furthest distribution area of mussels upstream in the system. Together with standard water quality parameters (e.g. salinity, dissolved oxygen, dissolved organic carbon, etc.) concentrations of twelve metals were analysed in the water (dissolved and suspended matter) and sediments. Levels of these metals were also measured in the soft tissue of M. edulis, together with concomitant biomarker responses in resident mussel populations at each site. The biomarkers that were included in this study were condition index, scope for growth, survival in air, cell membrane stability, DNA damage, and metallothioneins. Data were subjected to multivariate statistical analysis. The physico-chemical parameters and metals in the environmental samples clustered the sites to reflect the distribution based on the salinity gradient. Bioaccumulation results revealed increased metal uptake along a pollution gradient with the highest metal bioaccumulation occurring at the upstream most sites and therefore closest to the in the industrial activities. However, the biomarker responses clustered the sites in a manner that reflected the influence of combination of internal exposure (bioaccumulation) and external exposure (physico-chemical conditions). These differences in biomarker responses clearly demonstrated were attributed to abiotic factors other than metal pollution alone e.g. localized short-term increases in increased suspended sediment concentrations and decreased dissolved oxygen concentrations.  相似文献   

3.
Elevated concentrations of trace metals in surficial sediments off Palos Verdes Peninsula, site of the Los Angeles County outfall system, clearly reflect the submarine discharge of treated municipal (domestic and industrial) wastewater. The following contamination factors (median outfall/median baseline) were obtained for the eight metals measured in a 45 km2 region of the outfall monitoring zone: Ag-27; Cd-36; Cr-12; Cu-20; Hg-23; Ni-5.4; Pb-17; Zn-7.7.  相似文献   

4.
Solar radiation-controlled microclimatic variation has been considered a major force on hillslope evolution via feedback among geomorphology, vegetation, soil and hydrology. In this study, we investigate the influence of solar radiation on hillslope dynamics on Santa Catalina Island, CA by comparing hillslope morphology and frequency–magnitude relationships of shallow landslides, rills and gullies on slopes receiving low annual solar radiation (LSR) and high annual solar radiation (HSR), which were found equivalent to north- and south-facing slopes, respectively. LSR slopes on Santa Catalina Island were found more vegetated compared to HSR slopes. LiDAR elevation-derived hillslope morphology showed LSR slopes steeper, rougher and more concave than HSR slopes. Similarly, frequency–magnitude plots showed larger relative frequency of high-magnitude shallow landslides, rills and gullies on LSR slopes, and low-magnitude shallow landslides, rills and gullies on HSR slopes. We argue that the morphology, mass movement and erosion characteristics of LSR and HSR slopes reflect the process–response of microclimate-controlled variation in type and density of vegetation cover, soil physical properties – including moisture, texture, structure, infiltration and erodibility – and surface and subsurface hydrology. © 2019 John Wiley & Sons, Ltd. © 2019 John Wiley & Sons, Ltd.  相似文献   

5.
Topsoil (0–20 cm) samples were collected from the edge of roads to the locations about 200 m off the roads along the four roads with different transportation periods in October 2005. Total concentrations of As, Cd, Cr, Cu, Ni, Pb and Zn were determined using the inductively coupled plasma atomic absorption spectrometry in order to assess and compare road transportation pollution. Results showed that with the exception of As, Cu and Pb, the average concentrations of heavy metals were generally, higher than the regional elemental background values. Most soil samples were moderately or highly polluted by Cd or Ni, but the contamination index (P i ) values for As, Pb and Zn were lower than other heavy metals in all sites. Among the four roads, heavy metal pollution was heavier for Dali Road due to longer transportation periods, while low or no contamination could be observed for the other roads. However, the integrated contamination index (P c ) values showed a generally low contamination or no contamination level for all soil samples in this region, followed by the order of Dali Road > Dabao Highway > Road 320 > Sixiao Highway. The same pollution source of these heavy metals was found using factor analysis.  相似文献   

6.
The use of bivalves such as the brown mussel (Perna perna) and the black mussel (Choromytilus meridionalis) is common in the study of marine pollution and the effect of these pollutants on ecosystems and are important in both economic and ecological roles. Namibian marine ecosystems are threatened by pollution from mining, commercial fishing and population growth. The aims of this study were to determine baseline metal concentrations, spatial variation and variation between species. Metal levels in C. meridionalis from Guano Platform (GP) are the lowest of all the sites. The most polluted sites are Rocky Point (RP), Halifax Island (HIL) and between Walvis Bay and Swakopmund (WS). The bioaccumulation of metals between P. perna and C. meridionalis were not uniform for all metals. Overall the study indicates the condition of the coastline to be mostly normal, with Cd and Pb levels being of concern.  相似文献   

7.
将人工繁育的"标准化"背角无齿蚌(Anodonta woodiana)移殖至太湖五里湖,并以仍养殖在未受污染的中国水产科学研究院淡水渔业研究中心南泉基地的同批蚌作为对照,进行为期9个月的主动监测研究.每3个月回收一次蚌样,应用电感耦合等离子质谱仪(ICP-MS)测定15种重金属(Al、Cr、Mn、Fe、Co、Ni、Cu、Zn、As、Mo、Ag、Cd、Ba、Tl和Pb)的含量.结果表明,南泉基地对照组和五里湖移殖组的蚌样对重金属均产生了明显的生物积累.培养3个月的五里湖移殖组蚌样中As的含量显著高于同期南泉基地对照组,而前者Mn、Fe、Zn和Ba含量显著低于后者;培养6个月的五里湖移殖组蚌样中Al和Pb的含量显著低于同期南泉基地对照组;培养9个月的五里湖移殖组蚌样中Pb含量显著低于同期南泉基地对照组.然而,南泉基地对照组和五里湖移殖组蚌样中重金属(Cr、Cu、As、Cd和Pb)含量均低于我国及国际上的相关标准.培养3、6和9个月的南泉基地对照组及五里湖移殖组蚌样的重金属污染指数分别为1.8、1.8,2.4、2.1和8.3、16.8,均值综合污染指数分别为0.0218、0.0289,0.0337、0.0218和0.0560、0.0732,属于正常背景水平,并且两水体蚌样的重金属污染指数和均值综合污染指数无显著差异,提示五里湖和南泉基地均未受到明显的重金属污染.  相似文献   

8.
白洋淀沉积物-沉水植物-水系统重金属污染分布特征   总被引:5,自引:1,他引:5  
通过对白洋淀沉水植物及对应沉积物和水中Cd、Pb、As含量测定,以期揭示白洋淀沉积物-沉水植物-水系统中重金属污染状况及分布规律,明确不同沉水植物对重金属的富集能力.结果表明,地表水Cd、Pb、As浓度均符合我国地表水I类水质标准,不同采样区重金属浓度差异不显著.上覆水Pb浓度显著高于地表水和间隙水,间隙水As浓度显著高于地表水和上覆水;地积累指数法和潜在生态危害指数法评价结果表明,沉积物中重金属污染程度表现为Cd > Pb > As,Cd污染最严重,达到"轻度-偏重度"污染程度,"中等-极强"生态危害级别,As为清洁水平,不同采样区重金属污染程度表现为生活水产养殖区 > 纳污区 > 淀边缘区;沉水植物重金属富集能力表现为金鱼藻(Ceratophyllum demersum L.) > 菹草(Potamogeton crispus L.)和穗状狐尾藻(Myriophyllum spicatum L.) > 篦齿眼子菜(Potamogeton pectinatus L.).植物体内重金属含量与体内氮、磷含量呈显著正相关,氮、磷营养盐影响沉水植物对重金属的富集.  相似文献   

9.
A combination of retention pond and reed bed was tested for its effectiveness in reducing non-point source runoff pollution from an urban area. This paper presents data on the development of reed plants (Phragmites australis Cav. Trin.), on the effectiveness of runoff purification and on the accumulation of contaminants in the pond sediment and the reed bed for the years 1993–1995. P. australis was well established and grew according to normal development. The measured length and biomass values of P. australis were larger on sand than on gravel and coarse materials. Toxic levels of heavy metals in the plants were not reached. Harvested plants can be composted. The purification system is effective within the following ranges: The rate of retention of suspended solids and heavy metals varies between 16% and 91%. For chemical oxygen demand the average values is 25%. Poor retention rates usually occur along with very low input concentrations. Generally retention within the reed bed is higher than in the pond. Between 1993 and 1995 the concentration of contaminants within the organic layer of the reed bed increased by 50% for lead and by 90% for poly aromatic hydrocarbons. Until 1994 the concentrations of mineral oil hydrocarbons also increased by 60%. Between 1994 and 1995 however the concentration of mineral oil hydrocarbons in the reed bed decreased rapidly by more than 50%: Mineral oil hydrocarbons underlie biological degradation within the reed bed. In the pond sediment a significant accumulation of heavy metals, poly aromatic hydrocarbons and mineral oil hydrocarbons has also been found. The concentrations of these contaminants are still far from inhibiting the function of the system.  相似文献   

10.
Mixed heavy metals tolerance and radial oxygen loss in mangrove seedlings   总被引:2,自引:0,他引:2  
The effects of a mixture of heavy metals (Pb, Zn and Cu) on growth, radial oxygen loss (ROL) and the spatial pattern of ROL were investigated in mangrove seedlings of three species: Aegiceras corniculatum, Avicennia marina and Bruguiera gymnorrhiza. Heavy metals inhibited the growth of seedlings and led to decreased ROL and changes in the “tight” barrier spatial pattern of ROL. There was a significant positive correlation between the amount of ROL from the roots of seedlings and metal tolerance. The species with the highest ROL amount, B. gymnorrhiza, were also the most tolerant to heavy metals. The “tight” barrier spatial ROL pattern was also related to metal tolerance in the seedlings. Therefore, we conclude that both ROL amount and “tight” barrier spatial ROL pattern in the roots of the mangrove seedlings play an important role in resistance to heavy metal toxicity.  相似文献   

11.
Through source control, total DDT annual emissions from the Los Angeles County Sanitation Districts' submarine outfalls decreased by a factor of 30 between 1971 and 1977 Here we report persistent elevated levels of DDT residues measured in three species of marine fishes with distinctly different feeding habits. Over the study interval, median levels of DDT residues have decreased 3-fold (8-fold and 4-fold from peak medians) in flesh of black perch and kelp bass. However, there was no apparent decrease in Dover sole. The sediment reservoir is the likely source of persistent contamination of fishes in the discharge area.  相似文献   

12.
The effects from two winter rain storms on the coastal ocean of the Southern California Bight were examined as part of the Bight ‘03 program during February 2004 and February–March 2005. The impacts of stormwater from fecal indicator bacteria, water column toxicity, and nutrients were evaluated for five major river discharges: the Santa Clara River, Ballona Creek, the San Pedro Shelf (including the Los Angeles, San Gabriel, and Santa Ana Rivers), the San Diego River, and the Tijuana River. Exceedances of bacterial standards were observed in most of the systems. However, the areas of impact were generally spatially limited, and contaminant concentrations decreased below California Ocean Plan standards typically within 2–3 days. The largest bacterial concentrations occurred in the Tijuana River system where exceedances of fecal indicator bacteria were noted well away from the river mouth. Maximum nitrate concentrations (~40 μM) occurred in the San Pedro Shelf region near the mouth of the Los Angeles River. Based on the results of general linear models, individual sources of stormwater differ in both nutrient concentrations and the concentration and composition of fecal indicator bacteria. While nutrients appeared to decrease in plume waters due to simple mixing and dilution, the concentration of fecal indicator bacteria in plumes depends on more than loading and dilution rates. The relationships between contaminants (nutrients and fecal indicator bacteria) and plume indicators (salinity and total suspended solids) were not strong indicating the presence of other potentially important sources and/or sinks of both nutrients and fecal indicator bacteria. California Ocean Plan standards were often exceeded in waters containing greater than 10% stormwater (<28–30 salinity range). The median concentration dropped below the standard in the 32–33 salinity range (1–4% stormwater) for total coliforms and Enterococcus spp. and in the 28–30 salinity range (10–16% stormwater) for fecal coliforms. Nutrients showed a similar pattern with the highest median concentrations in water with greater than 10% stormwater. Relationships between colored dissolved organic matter (CDOM) and salinity and between total suspended solids and beam attenuation indicate that readily measurable, optically active variables can be used as proxies to provide at least a qualitative, if not quantitative, evaluation of the distribution of the dissolved, as well as the particulate, components of stormwater plumes. In this context, both CDOM absorption and the beam attenuation coefficient can be derived from satellite ocean color measurements of inherent optical properties suggesting that remote sensing of ocean color should be useful in mapping the spatial areas and durations of impacts from these contaminants.  相似文献   

13.
The occurrence and concentration of the fuel additive methyl-tert-butyl ether (MTBE) were measured in dry weather runoff, municipal wastewater and industrial effluents, and coastal receiving waters in southern California. Combined, refineries and sewage treatment plants release approximately 214 kg day(-1) of MTBE into the marine environment, with Santa Monica Bay receiving most (98%) of this discharge. Dry weather urban runoff was analysed for samples collected from 25 streams and rivers, and accounted for less than 0.5% of the mass of MTBE discharged to coastal waters. Receiving water samples were collected from 23 stations in Santa Monica Bay, Los Angeles Harbour and Mission Bay or San Diego Bay. MTBE was detected at low concentrations near effluent discharges, however there was no evidence of baywide MTBE contamination related to these outfalls. Marinas and areas used intensively for recreational boating had the highest average MTBE concentration (8.8 microg l(-1)). Surface water contamination was most widespread in San Diego Bay and Mission Bay, areas with no refinery or sewage treatment plant inputs.  相似文献   

14.
Using X-ray Energy Spectroscopy trace metal concentrations (Ti, V, Mn, Fe, Ni, Cu, Zn, As, Pb) were measured in specimens of Eudistylia vancouveri (feather duster tube worms) collected from floating wharves near and far from a storm water outfall in a metropolitan area. As for the well-studied bio-accumulator Mytilus edulis (mussels), higher metal concentrations were noted in specimens near the pollution source. In particular the worms accumulated certain metals, namely vanadium and titanium, not picked up by the mussels, signaling that a new sentinel organism could be available.  相似文献   

15.
With the existence of eight substantial islands in the Southern California Bight, the oceanic circulation is significantly affected by island wakes. In this paper a high-resolution numerical model (on a 1 km grid), forced by a high-resolution wind (2 km), is used to study the wakes. Island wakes arise due both to currents moving past islands and to wind wakes that force lee currents in response. A comparison between simulations with and without islands shows the surface enstrophy (i.e., area-integrated square of the vertical component of vorticity at the surface) decreases substantially when the islands in the oceanic model are removed, and the enstrophy decrease mainly takes place in the areas around the islands. Three cases of wake formation and evolution are analyzed for the Channel Islands, San Nicolas Island, and Santa Catalina Island. When flows squeeze through gaps between the Channel Islands, current shears arise, and the bottom drag makes a significant contribution to the vorticity generation. Downstream the vorticity rolls up into submesoscale eddies. When the California Current passes San Nicolas Island from the northwest, a relatively strong flow forms over the shelf break on the northeastern coast and gives rise to a locally large bottom stress that generates anticyclonic vorticity, while on the southwestern side, with an adverse flow pushing the main wake current away from the island, positive vorticity has been generated and a cyclonic eddy detaches into the wake. When the northward Southern California Countercurrent passes the irregular shape of Santa Catalina Island, cyclonic eddies form on the southeastern coast of the island, due primarily to lateral stress rather than bottom stress; they remain coherent as they detach and propagate downstream, and thus they are plausible candidates for the submesoscale “spirals on the sea” seen in many satellite images. Finally, the oceanic response to wind wakes is analyzed in a spin-up experiment with a time-invariant wind that exhibits strips of both positive and negative curl in the island lee. Corresponding vorticity strips in the ocean develop through the mechanism of Ekman pumping.  相似文献   

16.
章萍  曾宪哲  王亲媛  王伟  吴代赦 《湖泊科学》2019,31(6):1592-1600
基于鄱阳湖南矶山湿地土壤及藜蒿Cd、As污染风险评价,利用盆栽实验研究水分条件对区域土壤理化性质、砷镉形态及其上生长的藜蒿(Artemisia selengensis)重金属富集能力的影响.结果表明:土壤Cd含量超标,存在生态风险,藜蒿茎中As含量达食品污染限量标准,存在食用风险;藜蒿对Cd、As的富集能力受土壤水分环境影响,水分增加会造成土壤pH与有机质含量上升,抑制藜蒿富集Cd的同时促进富集As.线性回归计算显示土壤有效态As含量与藜蒿As富集量呈显著正相关,可以用来评价藜蒿As富集情况,而土壤有效态Cd含量与藜蒿Cd富集量间无显著相关性.结合区域土壤Cd、As污染情况,适宜控制水分为缺水或旱湿交替条件,可以降低藜蒿等湿地植物中Cd的富集量;适宜控制水分为淹水条件,可以减少土壤Cd、As有效态含量.  相似文献   

17.
洞庭湖流域对湘江湖南段6个城市江段铜锈环棱螺(Bellamya aeruginosa)腹足和内脏团的As、Cd、Pb、Cu、Zn、Cr富集量进行分析,运用单因子污染指数法评价其受污染程度,并分别采用平均每周/每月摄入量法和目标危害系数法对其膳食风险进行评估,旨在为湘江流域居民铜锈环棱螺的消费安全提供参考.结果显示,铜锈环棱螺腹足As、Cd、Pb、Cu和Zn的富集量均值分别为0.92、1.65、0.90、13.01和67.62 mg/kg,Cr未检出,As、Cd、Pb和Cu的超标率分别为87.06%、27.06%、24.72%和2.35%.内脏团As、Cd、Pb、Cu、Zn和Cr的富集量均值分别为9.61、3.21、3.75、33.58、169.05和1.23 mg/kg,As、Cd、Pb、Cu和Cr超标率分别为100%、71.76%、65.88%、14.12%和75.8%.所有江段成人As、Cu和Zn的每周摄入量均值和最高值均低于FAO/WHO食品添加剂联合专家委员会(JECFA)提出的暂定每周耐受摄入量参考值(PTWI),但株洲成人Cd的每月摄入量均值超过其每月耐受摄入量参考值,且最大值是其参考值的3.44倍,永州、湘潭地区成人Cd的每月摄入量最大值也分别是其参考值的1.16和1.68倍.所有江段铜锈环棱螺摄入的单一重金属健康风险值除As外均小于1,但多种重金属复合暴露健康风险值均接近或大于1.结果表明,湘江湖南段6个城市江段铜锈环棱螺均受到一定程度的污染,其中衡阳、湘潭和株洲江段较为严重,且各江段铜锈环棱螺内脏团重金属富集量整体上均高于腹足,故当地居民长期食用后存在潜在的健康风险.  相似文献   

18.
Preferred characteristics of biological indicators for heavy metal monitoring in marine ecosystems were documented 30 years ago. Heavy metal data from Raine Island on the outer-northern Great Barrier Reef are presented to introduce additional attributes for consideration, including a widened choice of biological tissues due to advances in trace heavy metal analysis. Kidney tissues, visceral mass and adductor muscle from the giant clam (Tridacna maxima), muscle tissue from trochus (Trochus niloticus) and axial muscle from four species of fish were targeted. The kidneys of giant clams had concentrations of heavy metals from 2 (Zn) to 2780 (Ni) times higher than corresponding concentrations in adductor muscles. Also, tissues of giant clam and the muscle of trochus gave different signals with respect to bio-available heavy metals. Linear correlations for heavy metals within and between tissues of giant clam and within muscle tissue of trochus, offer opportunities for the use of surrogates as well as a possible mathematical basis for assessing trends in heavy metal pollution.  相似文献   

19.
The suitability of using four bivalve molluscs (Sanguinolaria acuminata, Anadara granosa, Meretrix meretrix, and Pelecyora trigona) in biomonitoring of heavy metals (Cu, Pb, Cd, Zn, and Hg) collected from intertidal regions of the Sunderban mangrove wetland, northeastern part of the Bay of Bengal, were evaluated. Both speciesdependent variability and temporal variations were pronounced. A high degree of organ specificity was evident in the bivalves where gill and mantle exhibited higher metal accumulation due to ion exchange property of the mucous layer covering these organs while shells represent very poor accumulation. Elevated values of Zn and Cu reflect high potential for biomagnification through marine food chain. Metal concentrations in different body size groups of the bivalves do not follow uniform trend. Correlation coefficient between different metal couplings as tested statistically revealed significant coupling for Pb–Zn, Pb–Cu, Zn–Cu, and Hg–Cu. Concentrations of all the metals in specific organs (visceral mass, mantle and gill) of the bivalves exceeded the safe levels according to the international standards for metals compiled by Food and Agricultural Organization of the United Nations and would be of great risk for human consumption. It is concluded that the mussel and clam are suitable biomonitors to employ in programs designed to assess changes in metal pollution in the Sunderban mangrove wetland.  相似文献   

20.
It is important to determine trace metal concentrations in marine sediments because these could be important sources of contamination of marine organisms that reside there. In this study we measured the concentrations of thirteen metals in sediments obtained from Long Island Sound. We found great variations in metal levels for various geographic areas in the Sound; but, generally the highest concentrations found were in the extreme western end of the Sound. Comparison is made between metal levels in sediments from the Sound to seven other areas located in the U.S. and U.K.  相似文献   

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